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Critical slowing of the spin and charge density wave order in thin film Cr following photoexcitation </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Patel%2C+S+K+K">Sheena K. K. Patel</a>, <a href="/search/cond-mat?searchtype=author&query=Gorobtsov%2C+O+Y">Oleg Yu. Gorobtsov</a>, <a href="/search/cond-mat?searchtype=author&query=Cela%2C+D">Devin Cela</a>, <a href="/search/cond-mat?searchtype=author&query=Hrkac%2C+S+B">Stjepan B. Hrkac</a>, <a href="/search/cond-mat?searchtype=author&query=Hua%2C+N">Nelson Hua</a>, <a href="/search/cond-mat?searchtype=author&query=Medapalli%2C+R">Rajasekhar Medapalli</a>, <a href="/search/cond-mat?searchtype=author&query=Shabalin%2C+A+G">Anatoly G. Shabalin</a>, <a href="/search/cond-mat?searchtype=author&query=Wingert%2C+J">James Wingert</a>, <a href="/search/cond-mat?searchtype=author&query=Glownia%2C+J+M">James M. Glownia</a>, <a href="/search/cond-mat?searchtype=author&query=Zhu%2C+D">Diling Zhu</a>, <a href="/search/cond-mat?searchtype=author&query=Chollet%2C+M">Matthieu Chollet</a>, <a href="/search/cond-mat?searchtype=author&query=Shpyrko%2C+O+G">Oleg G. Shpyrko</a>, <a href="/search/cond-mat?searchtype=author&query=Singer%2C+A">Andrej Singer</a>, <a href="/search/cond-mat?searchtype=author&query=Fullerton%2C+E+E">Eric E. Fullerton</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2403.00267v2-abstract-short" style="display: inline;"> We report on the evolution of the charge density wave (CDW) and spin density wave (SDW) order of a chromium film following photoexcitation with an ultrafast optical laser pulse. The CDW is measured by ultrafast time-resolved x-ray diffraction of the CDW satellite that tracks the suppression and recovery of the CDW following photoexcitation. We find that as the temperature of the film approaches a… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2403.00267v2-abstract-full').style.display = 'inline'; document.getElementById('2403.00267v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2403.00267v2-abstract-full" style="display: none;"> We report on the evolution of the charge density wave (CDW) and spin density wave (SDW) order of a chromium film following photoexcitation with an ultrafast optical laser pulse. The CDW is measured by ultrafast time-resolved x-ray diffraction of the CDW satellite that tracks the suppression and recovery of the CDW following photoexcitation. We find that as the temperature of the film approaches a discontinuous phase transition in the CDW and SDW order, the time scales of recovery increase exponentially from the expected thermal time scales. We extend a Landau model for SDW systems to account for this critical slowing with the appropriate boundary conditions imposed by the geometry of the thin film system. This model allows us to assess the energy barrier between available CDW/SDW states with different spatial periodicities. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2403.00267v2-abstract-full').style.display = 'none'; document.getElementById('2403.00267v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 5 March, 2024; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 29 February, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> March 2024. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">Author typo fixed</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2201.06350">arXiv:2201.06350</a> <span> [<a href="https://arxiv.org/pdf/2201.06350">pdf</a>, <a href="https://arxiv.org/format/2201.06350">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Mesoscale and Nanoscale Physics">cond-mat.mes-hall</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Accelerator Physics">physics.acc-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Instrumentation and Detectors">physics.ins-det</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1107/S1600577522008414">10.1107/S1600577522008414 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Megahertz-rate Ultrafast X-ray Scattering and Holographic Imaging at the European XFEL </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Hagstr%C3%B6m%2C+N+Z">Nanna Zhou Hagstr枚m</a>, <a href="/search/cond-mat?searchtype=author&query=Schneider%2C+M">Michael Schneider</a>, <a href="/search/cond-mat?searchtype=author&query=Kerber%2C+N">Nico Kerber</a>, <a href="/search/cond-mat?searchtype=author&query=Yaroslavtsev%2C+A">Alexander Yaroslavtsev</a>, <a href="/search/cond-mat?searchtype=author&query=Parra%2C+E+B">Erick Burgos Parra</a>, <a href="/search/cond-mat?searchtype=author&query=Beg%2C+M">Marijan Beg</a>, <a href="/search/cond-mat?searchtype=author&query=Lang%2C+M">Martin Lang</a>, <a href="/search/cond-mat?searchtype=author&query=G%C3%BCnther%2C+C+M">Christian M. G眉nther</a>, <a href="/search/cond-mat?searchtype=author&query=Seng%2C+B">Boris Seng</a>, <a href="/search/cond-mat?searchtype=author&query=Kammerbauer%2C+F">Fabian Kammerbauer</a>, <a href="/search/cond-mat?searchtype=author&query=Popescu%2C+H">Horia Popescu</a>, <a href="/search/cond-mat?searchtype=author&query=Pancaldi%2C+M">Matteo Pancaldi</a>, <a href="/search/cond-mat?searchtype=author&query=Neeraj%2C+K">Kumar Neeraj</a>, <a href="/search/cond-mat?searchtype=author&query=Polley%2C+D">Debanjan Polley</a>, <a href="/search/cond-mat?searchtype=author&query=Jangid%2C+R">Rahul Jangid</a>, <a href="/search/cond-mat?searchtype=author&query=Hrkac%2C+S+B">Stjepan B. Hrkac</a>, <a href="/search/cond-mat?searchtype=author&query=Patel%2C+S+K+K">Sheena K. K. Patel</a>, <a href="/search/cond-mat?searchtype=author&query=Ovcharenko%2C+S">Sergei Ovcharenko</a>, <a href="/search/cond-mat?searchtype=author&query=Turenne%2C+D">Diego Turenne</a>, <a href="/search/cond-mat?searchtype=author&query=Ksenzov%2C+D">Dmitriy Ksenzov</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">Christine Boeglin</a>, <a href="/search/cond-mat?searchtype=author&query=Pronin%2C+I">Igor Pronin</a>, <a href="/search/cond-mat?searchtype=author&query=Baidakova%2C+M">Marina Baidakova</a>, <a href="/search/cond-mat?searchtype=author&query=Schmising%2C+C+v+K">Clemens von Korff Schmising</a>, <a href="/search/cond-mat?searchtype=author&query=Borchert%2C+M">Martin Borchert</a> , et al. (75 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2201.06350v2-abstract-short" style="display: inline;"> The advent of X-ray free-electron lasers (XFELs) has revolutionized fundamental science, from atomic to condensed matter physics, from chemistry to biology, giving researchers access to X-rays with unprecedented brightness, coherence, and pulse duration. All XFEL facilities built until recently provided X-ray pulses at a relatively low repetition rate, with limited data statistics. Here, we presen… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2201.06350v2-abstract-full').style.display = 'inline'; document.getElementById('2201.06350v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2201.06350v2-abstract-full" style="display: none;"> The advent of X-ray free-electron lasers (XFELs) has revolutionized fundamental science, from atomic to condensed matter physics, from chemistry to biology, giving researchers access to X-rays with unprecedented brightness, coherence, and pulse duration. All XFEL facilities built until recently provided X-ray pulses at a relatively low repetition rate, with limited data statistics. Here, we present the results from the first megahertz repetition rate X-ray scattering experiments at the Spectroscopy and Coherent Scattering (SCS) instrument of the European XFEL. We illustrate the experimental capabilities that the SCS instrument offers, resulting from the operation at MHz repetition rates and the availability of the novel DSSC 2D imaging detector. Time-resolved magnetic X-ray scattering and holographic imaging experiments in solid state samples were chosen as representative, providing an ideal test-bed for operation at megahertz rates. Our results are relevant and applicable to any other non-destructive XFEL experiments in the soft X-ray range. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2201.06350v2-abstract-full').style.display = 'none'; document.getElementById('2201.06350v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 20 January, 2022; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 17 January, 2022; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2022. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">13 pages, 5 figures. Supplementary Information as ancillary file</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> J. Synchrotron Rad. (2022), 29 </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2012.05353">arXiv:2012.05353</a> <span> [<a href="https://arxiv.org/pdf/2012.05353">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> </div> </div> <p class="title is-5 mathjax"> Phonon-assisted formation of an itinerant electronic density wave </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Li%2C+J">Jiaruo Li</a>, <a href="/search/cond-mat?searchtype=author&query=Gorobtsov%2C+O+Y">Oleg Yu. Gorobtsov</a>, <a href="/search/cond-mat?searchtype=author&query=Patel%2C+S+K+K">Sheena K. K. Patel</a>, <a href="/search/cond-mat?searchtype=author&query=Hua%2C+N">Nelson Hua</a>, <a href="/search/cond-mat?searchtype=author&query=Gregory%2C+B">Benjamin Gregory</a>, <a href="/search/cond-mat?searchtype=author&query=Shabalin%2C+A+G">Anatoly G. Shabalin</a>, <a href="/search/cond-mat?searchtype=author&query=Hrkac%2C+S">Stjepan Hrkac</a>, <a href="/search/cond-mat?searchtype=author&query=Wingert%2C+J">James Wingert</a>, <a href="/search/cond-mat?searchtype=author&query=Cela%2C+D">Devin Cela</a>, <a href="/search/cond-mat?searchtype=author&query=Glownia%2C+J+M">James M. Glownia</a>, <a href="/search/cond-mat?searchtype=author&query=Chollet%2C+M">Matthieu Chollet</a>, <a href="/search/cond-mat?searchtype=author&query=Zhu%2C+D">Diling Zhu</a>, <a href="/search/cond-mat?searchtype=author&query=Medapalli%2C+R">Rajasekhar Medapalli</a>, <a href="/search/cond-mat?searchtype=author&query=Fullerton%2C+E+E">Eric E. Fullerton</a>, <a href="/search/cond-mat?searchtype=author&query=Shpyrko%2C+O+G">Oleg G. Shpyrko</a>, <a href="/search/cond-mat?searchtype=author&query=Singer%2C+A">Andrej Singer</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2012.05353v1-abstract-short" style="display: inline;"> Electronic instabilities drive ordering transitions in condensed matter. Despite many advances in the microscopic understanding of the ordered states, a more nuanced and profound question often remains unanswered: how do the collective excitations influence the electronic order formation? Here, we experimentally show that a phonon affects the spin density wave (SDW) formation after an SDW-quench b… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2012.05353v1-abstract-full').style.display = 'inline'; document.getElementById('2012.05353v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2012.05353v1-abstract-full" style="display: none;"> Electronic instabilities drive ordering transitions in condensed matter. Despite many advances in the microscopic understanding of the ordered states, a more nuanced and profound question often remains unanswered: how do the collective excitations influence the electronic order formation? Here, we experimentally show that a phonon affects the spin density wave (SDW) formation after an SDW-quench by femtosecond laser pulses. In a thin film, the temperature-dependent SDW period is quantized, allowing us to track the out-of-equilibrium formation path of the SDW precisely. By exploiting its persistent coupling to the lattice, we probe the SDW through the transient lattice distortion, measured by femtosecond X-ray diffraction. We find that within 500 femtoseconds after a complete quench, the SDW forms with the low-temperature period, directly bypassing a thermal state with the high-temperature period. We argue that a momentum-matched phonon launched by the quench changes the formation path of the SDW through the dynamic pinning of the order parameter. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2012.05353v1-abstract-full').style.display = 'none'; document.getElementById('2012.05353v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 9 December, 2020; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> December 2020. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2001.11719">arXiv:2001.11719</a> <span> [<a href="https://arxiv.org/pdf/2001.11719">pdf</a>, <a href="https://arxiv.org/format/2001.11719">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Mesoscale and Nanoscale Physics">cond-mat.mes-hall</span> </div> </div> <p class="title is-5 mathjax"> Ultrafast perturbation of magnetic domains by optical pumping in a ferromagnetic multilayer </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Zusin%2C+D">Dmitriy Zusin</a>, <a href="/search/cond-mat?searchtype=author&query=Iacocca%2C+E">Ezio Iacocca</a>, <a href="/search/cond-mat?searchtype=author&query=Guyader%2C+L+L">Lo茂c Le Guyader</a>, <a href="/search/cond-mat?searchtype=author&query=Reid%2C+A+H">Alexander H. Reid</a>, <a href="/search/cond-mat?searchtype=author&query=Schlotter%2C+W+F">William F. Schlotter</a>, <a href="/search/cond-mat?searchtype=author&query=Liu%2C+T">Tian-Min Liu</a>, <a href="/search/cond-mat?searchtype=author&query=Higley%2C+D+J">Daniel J. Higley</a>, <a href="/search/cond-mat?searchtype=author&query=Coslovich%2C+G">Giacomo Coslovich</a>, <a href="/search/cond-mat?searchtype=author&query=Wandel%2C+S+F">Scott F. Wandel</a>, <a href="/search/cond-mat?searchtype=author&query=Tengdin%2C+P+M">Phoebe M. Tengdin</a>, <a href="/search/cond-mat?searchtype=author&query=Patel%2C+S+K+K">Sheena K. K. Patel</a>, <a href="/search/cond-mat?searchtype=author&query=Shabalin%2C+A">Anatoly Shabalin</a>, <a href="/search/cond-mat?searchtype=author&query=Hua%2C+N">Nelson Hua</a>, <a href="/search/cond-mat?searchtype=author&query=Hrkac%2C+S+B">Stjepan B. Hrkac</a>, <a href="/search/cond-mat?searchtype=author&query=Nembach%2C+H+T">Hans T. Nembach</a>, <a href="/search/cond-mat?searchtype=author&query=Shaw%2C+J+M">Justin M. Shaw</a>, <a href="/search/cond-mat?searchtype=author&query=Montoya%2C+S+A">Sergio A. Montoya</a>, <a href="/search/cond-mat?searchtype=author&query=Blonsky%2C+A">Adam Blonsky</a>, <a href="/search/cond-mat?searchtype=author&query=Gentry%2C+C">Christian Gentry</a>, <a href="/search/cond-mat?searchtype=author&query=Hoefer%2C+M+A">Mark A. Hoefer</a>, <a href="/search/cond-mat?searchtype=author&query=Murnane%2C+M+M">Margaret M. Murnane</a>, <a href="/search/cond-mat?searchtype=author&query=Kapteyn%2C+H+C">Henry C. Kapteyn</a>, <a href="/search/cond-mat?searchtype=author&query=Fullerton%2C+E+E">Eric E. Fullerton</a>, <a href="/search/cond-mat?searchtype=author&query=Shpyrko%2C+O">Oleg Shpyrko</a>, <a href="/search/cond-mat?searchtype=author&query=D%C3%BCrr%2C+H+A">Hermann A. D眉rr</a> , et al. (1 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2001.11719v4-abstract-short" style="display: inline;"> Ultrafast optical pumping of spatially nonuniform magnetic textures is known to induce far-from-equilibrium spin transport effects. Here, we use ultrafast x-ray diffraction with unprecedented dynamic range to study the laser-induced dynamics of labyrinth domain networks in ferromagnetic CoFe/Ni multilayers. We detected azimuthally isotropic, odd order, magnetic diffraction rings up to 5th order. T… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2001.11719v4-abstract-full').style.display = 'inline'; document.getElementById('2001.11719v4-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2001.11719v4-abstract-full" style="display: none;"> Ultrafast optical pumping of spatially nonuniform magnetic textures is known to induce far-from-equilibrium spin transport effects. Here, we use ultrafast x-ray diffraction with unprecedented dynamic range to study the laser-induced dynamics of labyrinth domain networks in ferromagnetic CoFe/Ni multilayers. We detected azimuthally isotropic, odd order, magnetic diffraction rings up to 5th order. The amplitudes of all three diffraction rings quench to different degrees within 1.6 ps. In addition, all three of the detected diffraction rings both broaden by 15% and radially contract by 6% during the quench process. We are able to rigorously quantify a 31% ultrafast broadening of the domain walls via Fourier analysis of the order-dependent quenching of the three detected diffraction rings. The broadening of the diffraction rings is interpreted as a reduction in the domain coherence length, but the shift in the ring radius, while unambiguous in its occurrence, remains unexplained. In particular, we demonstrate that a radial shift explained by domain wall broadening can be ruled out. With the unprecedented dynamic range of our data, our results provide convincing evidence that labyrinth domain structures are spatially perturbed at ultrafast speeds under far-from-equilibrium conditions, albeit the mechanism inducing the perturbations remains yet to be clarified. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2001.11719v4-abstract-full').style.display = 'none'; document.getElementById('2001.11719v4-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 9 June, 2022; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 31 January, 2020; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2020. </p> </li> </ol> <div class="is-hidden-tablet"> <!-- feedback for mobile only --> <span class="help" style="display: inline-block;"><a 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