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is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> </div> <p class="title is-5 mathjax"> Kitaev physics in the two-dimensional magnet NiPSe$_3$ </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Peng%2C+C">Cheng Peng</a>, <a href="/search/cond-mat?searchtype=author&query=Mardanya%2C+S">Sougata Mardanya</a>, <a href="/search/cond-mat?searchtype=author&query=Petsch%2C+A+N">Alexander N. Petsch</a>, <a href="/search/cond-mat?searchtype=author&query=Sharma%2C+V+K">Vineet Kumar Sharma</a>, <a href="/search/cond-mat?searchtype=author&query=Li%2C+S">Shuyi Li</a>, <a href="/search/cond-mat?searchtype=author&query=Jia%2C+C">Chunjing Jia</a>, <a href="/search/cond-mat?searchtype=author&query=Bansil%2C+A">Arun Bansil</a>, <a href="/search/cond-mat?searchtype=author&query=Chowdhury%2C+S">Sugata Chowdhury</a>, <a href="/search/cond-mat?searchtype=author&query=Turner%2C+J+J">Joshua J. Turner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2403.09831v1-abstract-short" style="display: inline;"> The Kitaev interaction, found in candidate materials such as $伪$-RuCl$_3$, occurs through the metal ($M$)-ligand ($X$)-metal ($M$) paths of the edge-sharing octahedra because the large spin-orbit coupling (SOC) on the metal atoms activates directional spin interactions. Here, we show that even in $3d$ transition-metal compounds, where the SOC of the metal atom is negligible, heavy ligands can indu… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2403.09831v1-abstract-full').style.display = 'inline'; document.getElementById('2403.09831v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2403.09831v1-abstract-full" style="display: none;"> The Kitaev interaction, found in candidate materials such as $伪$-RuCl$_3$, occurs through the metal ($M$)-ligand ($X$)-metal ($M$) paths of the edge-sharing octahedra because the large spin-orbit coupling (SOC) on the metal atoms activates directional spin interactions. Here, we show that even in $3d$ transition-metal compounds, where the SOC of the metal atom is negligible, heavy ligands can induce bond-dependent Kitaev interactions. In this work, we take as an example the $3d$ transition-metal chalcogenophosphate NiPSe$_3$ and show that the key is found in the presence of a sizable SOC on the Se $p$ orbital, one which mediates the super-exchange between the nearest-neighbor Ni sites. Our study provides a pathway for engineering enhanced Kitaev interactions through the interplay of SOC strength, lattice distortions, and chemical substitutions. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2403.09831v1-abstract-full').style.display = 'none'; document.getElementById('2403.09831v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 14 March, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> March 2024. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">Supplementary material is included in the package</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2310.07948">arXiv:2310.07948</a> <span> [<a href="https://arxiv.org/pdf/2310.07948">pdf</a>, <a href="https://arxiv.org/format/2310.07948">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> </div> <p class="title is-5 mathjax"> 3D Heisenberg universality in the Van der Waals antiferromagnet NiPS$_3$ </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Plumley%2C+R">Rajan Plumley</a>, <a href="/search/cond-mat?searchtype=author&query=Mardanya%2C+S">Sougata Mardanya</a>, <a href="/search/cond-mat?searchtype=author&query=Peng%2C+C">Cheng Peng</a>, <a href="/search/cond-mat?searchtype=author&query=Nokelainen%2C+J">Johannes Nokelainen</a>, <a href="/search/cond-mat?searchtype=author&query=Assefa%2C+T">Tadesse Assefa</a>, <a href="/search/cond-mat?searchtype=author&query=Shen%2C+L">Lingjia Shen</a>, <a href="/search/cond-mat?searchtype=author&query=Burdet%2C+N">Nicholas Burdet</a>, <a href="/search/cond-mat?searchtype=author&query=Porter%2C+Z">Zach Porter</a>, <a href="/search/cond-mat?searchtype=author&query=Petsch%2C+A">Alexander Petsch</a>, <a href="/search/cond-mat?searchtype=author&query=Israelski%2C+A">Aidan Israelski</a>, <a href="/search/cond-mat?searchtype=author&query=Chen%2C+H">Hongwei Chen</a>, <a href="/search/cond-mat?searchtype=author&query=Lee%2C+J+S">Jun Sik Lee</a>, <a href="/search/cond-mat?searchtype=author&query=Morley%2C+S">Sophie Morley</a>, <a href="/search/cond-mat?searchtype=author&query=Roy%2C+S">Sujoy Roy</a>, <a href="/search/cond-mat?searchtype=author&query=Fabbris%2C+G">Gilberto Fabbris</a>, <a href="/search/cond-mat?searchtype=author&query=Blackburn%2C+E">Elizabeth Blackburn</a>, <a href="/search/cond-mat?searchtype=author&query=Feiguin%2C+A">Adrian Feiguin</a>, <a href="/search/cond-mat?searchtype=author&query=Bansil%2C+A">Arun Bansil</a>, <a href="/search/cond-mat?searchtype=author&query=Lee%2C+W">Wei-Sheng Lee</a>, <a href="/search/cond-mat?searchtype=author&query=Lindenberg%2C+A">Aaron Lindenberg</a>, <a href="/search/cond-mat?searchtype=author&query=Chowdhury%2C+S">Sugata Chowdhury</a>, <a href="/search/cond-mat?searchtype=author&query=Dunne%2C+M">Mike Dunne</a>, <a href="/search/cond-mat?searchtype=author&query=Turner%2C+J+J">Joshua J. Turner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2310.07948v4-abstract-short" style="display: inline;"> Van der Waals (vdW) magnetic materials are comprised of layers of atomically thin sheets, making them ideal platforms for studying magnetism at the two-dimensional (2D) limit. These materials are at the center of a host of novel types of experiments, however, there are notably few pathways to directly probe their magnetic structure. We report the magnetic order within a single crystal of NiPS$_3$… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2310.07948v4-abstract-full').style.display = 'inline'; document.getElementById('2310.07948v4-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2310.07948v4-abstract-full" style="display: none;"> Van der Waals (vdW) magnetic materials are comprised of layers of atomically thin sheets, making them ideal platforms for studying magnetism at the two-dimensional (2D) limit. These materials are at the center of a host of novel types of experiments, however, there are notably few pathways to directly probe their magnetic structure. We report the magnetic order within a single crystal of NiPS$_3$ and show it can be accessed with resonant elastic X-ray diffraction along the edge of the vdW planes in a carefully grown crystal by detecting structurally forbidden resonant magnetic X-ray scattering. We find the magnetic order parameter has a critical exponent of $尾\sim0.36$, indicating that the magnetism of these vdW crystals is more adequately characterized by the three-dimensional (3D) Heisenberg universality class. We verify these findings with first-principle density functional theory, Monte-Carlo simulations, and density matrix renormalization group calculations. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2310.07948v4-abstract-full').style.display = 'none'; document.getElementById('2310.07948v4-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 18 October, 2024; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 11 October, 2023; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> October 2023. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2306.02015">arXiv:2306.02015</a> <span> [<a href="https://arxiv.org/pdf/2306.02015">pdf</a>, <a href="https://arxiv.org/format/2306.02015">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Machine Learning">cs.LG</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Computational Physics">physics.comp-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Data Analysis, Statistics and Probability">physics.data-an</span> </div> </div> <p class="title is-5 mathjax"> Machine learning enabled experimental design and parameter estimation for ultrafast spin dynamics </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Chen%2C+Z">Zhantao Chen</a>, <a href="/search/cond-mat?searchtype=author&query=Peng%2C+C">Cheng Peng</a>, <a href="/search/cond-mat?searchtype=author&query=Petsch%2C+A+N">Alexander N. Petsch</a>, <a href="/search/cond-mat?searchtype=author&query=Chitturi%2C+S+R">Sathya R. Chitturi</a>, <a href="/search/cond-mat?searchtype=author&query=Okullo%2C+A">Alana Okullo</a>, <a href="/search/cond-mat?searchtype=author&query=Chowdhury%2C+S">Sugata Chowdhury</a>, <a href="/search/cond-mat?searchtype=author&query=Yoon%2C+C+H">Chun Hong Yoon</a>, <a href="/search/cond-mat?searchtype=author&query=Turner%2C+J+J">Joshua J. Turner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2306.02015v1-abstract-short" style="display: inline;"> Advanced experimental measurements are crucial for driving theoretical developments and unveiling novel phenomena in condensed matter and material physics, which often suffer from the scarcity of facility resources and increasing complexities. To address the limitations, we introduce a methodology that combines machine learning with Bayesian optimal experimental design (BOED), exemplified with x-r… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2306.02015v1-abstract-full').style.display = 'inline'; document.getElementById('2306.02015v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2306.02015v1-abstract-full" style="display: none;"> Advanced experimental measurements are crucial for driving theoretical developments and unveiling novel phenomena in condensed matter and material physics, which often suffer from the scarcity of facility resources and increasing complexities. To address the limitations, we introduce a methodology that combines machine learning with Bayesian optimal experimental design (BOED), exemplified with x-ray photon fluctuation spectroscopy (XPFS) measurements for spin fluctuations. Our method employs a neural network model for large-scale spin dynamics simulations for precise distribution and utility calculations in BOED. The capability of automatic differentiation from the neural network model is further leveraged for more robust and accurate parameter estimation. Our numerical benchmarks demonstrate the superior performance of our method in guiding XPFS experiments, predicting model parameters, and yielding more informative measurements within limited experimental time. Although focusing on XPFS and spin fluctuations, our method can be adapted to other experiments, facilitating more efficient data collection and accelerating scientific discoveries. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2306.02015v1-abstract-full').style.display = 'none'; document.getElementById('2306.02015v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 3 June, 2023; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> June 2023. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2304.12485">arXiv:2304.12485</a> <span> [<a href="https://arxiv.org/pdf/2304.12485">pdf</a>, <a href="https://arxiv.org/format/2304.12485">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Superconductivity">cond-mat.supr-con</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevB.108.L201111">10.1103/PhysRevB.108.L201111 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Interplay between atomic fluctuations and charge density waves in La$_{2-x}$Sr$_{x}$CuO$_{4}$ </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Shen%2C+L">L. Shen</a>, <a href="/search/cond-mat?searchtype=author&query=Esposito%2C+V">V. Esposito</a>, <a href="/search/cond-mat?searchtype=author&query=Burdet%2C+N+G">N. G. Burdet</a>, <a href="/search/cond-mat?searchtype=author&query=Zhu%2C+M">M. Zhu</a>, <a href="/search/cond-mat?searchtype=author&query=Petsch%2C+A+N">A. N. Petsch</a>, <a href="/search/cond-mat?searchtype=author&query=Croft%2C+T+P">T. P. Croft</a>, <a href="/search/cond-mat?searchtype=author&query=Collins%2C+S+P">S. P. Collins</a>, <a href="/search/cond-mat?searchtype=author&query=Ren%2C+Z">Z. Ren</a>, <a href="/search/cond-mat?searchtype=author&query=Westermeier%2C+F">F. Westermeier</a>, <a href="/search/cond-mat?searchtype=author&query=Sprung%2C+M">M. Sprung</a>, <a href="/search/cond-mat?searchtype=author&query=Hayden%2C+S+M">S. M. Hayden</a>, <a href="/search/cond-mat?searchtype=author&query=Turner%2C+J+J">J. J. Turner</a>, <a href="/search/cond-mat?searchtype=author&query=Blackburn%2C+E">E. Blackburn</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2304.12485v1-abstract-short" style="display: inline;"> In the cuprate superconductors, the spatial coherence of the charge density wave (CDW) state grows rapidly below a characteristic temperature $T_\mathrm{CDW}$, the nature of which is debated. We have combined a set of x-ray scattering techniques to study La$_{1.88}$Sr$_{0.12}$CuO$_{4}$ ($T_\mathrm{CDW}$~$\approx$~80\,K) to shed light on this discussion. We observe the emergence of a crystal struct… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2304.12485v1-abstract-full').style.display = 'inline'; document.getElementById('2304.12485v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2304.12485v1-abstract-full" style="display: none;"> In the cuprate superconductors, the spatial coherence of the charge density wave (CDW) state grows rapidly below a characteristic temperature $T_\mathrm{CDW}$, the nature of which is debated. We have combined a set of x-ray scattering techniques to study La$_{1.88}$Sr$_{0.12}$CuO$_{4}$ ($T_\mathrm{CDW}$~$\approx$~80\,K) to shed light on this discussion. We observe the emergence of a crystal structure, which is consistent with the CDW modulation in symmetry, well above $T_\mathrm{CDW}$. This global structural change also induces strong fluctuations of local atomic disorder in the intermediate temperature region. At $T_\mathrm{CDW}$, the temperature dependence of this structure develops a kink, while the atomic disorder is minimized. We find that the atomic relaxation dynamics cross over from a cooperative to an incoherent response at $T_\mathrm{CDW}$. These results reveal a rich interplay between the CDWs and atomic fluctuations of distinct spatio-temporal scales. For example, the CDW coherence is enhanced on quasi-elastic timescales by incoherent atomic relaxation. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2304.12485v1-abstract-full').style.display = 'none'; document.getElementById('2304.12485v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 24 April, 2023; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> April 2023. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2304.03949">arXiv:2304.03949</a> <span> [<a href="https://arxiv.org/pdf/2304.03949">pdf</a>, <a href="https://arxiv.org/format/2304.03949">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Artificial Intelligence">cs.AI</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Computer Vision and Pattern Recognition">cs.CV</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Data Analysis, Statistics and Probability">physics.data-an</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1038/s41467-023-41378-4">10.1038/s41467-023-41378-4 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Capturing dynamical correlations using implicit neural representations </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Chitturi%2C+S">Sathya Chitturi</a>, <a href="/search/cond-mat?searchtype=author&query=Ji%2C+Z">Zhurun Ji</a>, <a href="/search/cond-mat?searchtype=author&query=Petsch%2C+A">Alexander Petsch</a>, <a href="/search/cond-mat?searchtype=author&query=Peng%2C+C">Cheng Peng</a>, <a href="/search/cond-mat?searchtype=author&query=Chen%2C+Z">Zhantao Chen</a>, <a href="/search/cond-mat?searchtype=author&query=Plumley%2C+R">Rajan Plumley</a>, <a href="/search/cond-mat?searchtype=author&query=Dunne%2C+M">Mike Dunne</a>, <a href="/search/cond-mat?searchtype=author&query=Mardanya%2C+S">Sougata Mardanya</a>, <a href="/search/cond-mat?searchtype=author&query=Chowdhury%2C+S">Sugata Chowdhury</a>, <a href="/search/cond-mat?searchtype=author&query=Chen%2C+H">Hongwei Chen</a>, <a href="/search/cond-mat?searchtype=author&query=Bansil%2C+A">Arun Bansil</a>, <a href="/search/cond-mat?searchtype=author&query=Feiguin%2C+A">Adrian Feiguin</a>, <a href="/search/cond-mat?searchtype=author&query=Kolesnikov%2C+A">Alexander Kolesnikov</a>, <a href="/search/cond-mat?searchtype=author&query=Prabhakaran%2C+D">Dharmalingam Prabhakaran</a>, <a href="/search/cond-mat?searchtype=author&query=Hayden%2C+S">Stephen Hayden</a>, <a href="/search/cond-mat?searchtype=author&query=Ratner%2C+D">Daniel Ratner</a>, <a href="/search/cond-mat?searchtype=author&query=Jia%2C+C">Chunjing Jia</a>, <a href="/search/cond-mat?searchtype=author&query=Nashed%2C+Y">Youssef Nashed</a>, <a href="/search/cond-mat?searchtype=author&query=Turner%2C+J">Joshua Turner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2304.03949v1-abstract-short" style="display: inline;"> The observation and description of collective excitations in solids is a fundamental issue when seeking to understand the physics of a many-body system. Analysis of these excitations is usually carried out by measuring the dynamical structure factor, S(Q, $蠅$), with inelastic neutron or x-ray scattering techniques and comparing this against a calculated dynamical model. Here, we develop an artific… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2304.03949v1-abstract-full').style.display = 'inline'; document.getElementById('2304.03949v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2304.03949v1-abstract-full" style="display: none;"> The observation and description of collective excitations in solids is a fundamental issue when seeking to understand the physics of a many-body system. Analysis of these excitations is usually carried out by measuring the dynamical structure factor, S(Q, $蠅$), with inelastic neutron or x-ray scattering techniques and comparing this against a calculated dynamical model. Here, we develop an artificial intelligence framework which combines a neural network trained to mimic simulated data from a model Hamiltonian with automatic differentiation to recover unknown parameters from experimental data. We benchmark this approach on a Linear Spin Wave Theory (LSWT) simulator and advanced inelastic neutron scattering data from the square-lattice spin-1 antiferromagnet La$_2$NiO$_4$. We find that the model predicts the unknown parameters with excellent agreement relative to analytical fitting. In doing so, we illustrate the ability to build and train a differentiable model only once, which then can be applied in real-time to multi-dimensional scattering data, without the need for human-guided peak finding and fitting algorithms. This prototypical approach promises a new technology for this field to automatically detect and refine more advanced models for ordered quantum systems. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2304.03949v1-abstract-full').style.display = 'none'; document.getElementById('2304.03949v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 8 April, 2023; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> April 2023. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">12 pages, 7 figures</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2304.02546">arXiv:2304.02546</a> <span> [<a href="https://arxiv.org/pdf/2304.02546">pdf</a>, <a href="https://arxiv.org/format/2304.02546">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevResearch.5.033113">10.1103/PhysRevResearch.5.033113 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> High-energy spin waves in the spin-1 square-lattice antiferromagnet La$_2$NiO$_4$ </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Petsch%2C+A+N">A. N. Petsch</a>, <a href="/search/cond-mat?searchtype=author&query=Headings%2C+N+S">N. S. Headings</a>, <a href="/search/cond-mat?searchtype=author&query=Prabhakaran%2C+D">D. Prabhakaran</a>, <a href="/search/cond-mat?searchtype=author&query=Kolesnikov%2C+A+I">A. I. Kolesnikov</a>, <a href="/search/cond-mat?searchtype=author&query=Frost%2C+C+D">C. D. Frost</a>, <a href="/search/cond-mat?searchtype=author&query=Boothroyd%2C+A+T">A. T. Boothroyd</a>, <a href="/search/cond-mat?searchtype=author&query=Coldea%2C+R">R. Coldea</a>, <a href="/search/cond-mat?searchtype=author&query=Hayden%2C+S+M">S. M. Hayden</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2304.02546v2-abstract-short" style="display: inline;"> Inelastic neutron scattering is used to study the magnetic excitations of the $S=1$ square-lattice antiferromagnet La$_2$NiO$_4$. We find that the spin waves cannot be described by a simple classical (harmonic) Heisenberg model with only nearest-neighbor interactions. The spin-wave dispersion measured along the antiferromagnetic Brillouin-zone boundary shows a minimum energy at the $(1/2,0)$ posit… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2304.02546v2-abstract-full').style.display = 'inline'; document.getElementById('2304.02546v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2304.02546v2-abstract-full" style="display: none;"> Inelastic neutron scattering is used to study the magnetic excitations of the $S=1$ square-lattice antiferromagnet La$_2$NiO$_4$. We find that the spin waves cannot be described by a simple classical (harmonic) Heisenberg model with only nearest-neighbor interactions. The spin-wave dispersion measured along the antiferromagnetic Brillouin-zone boundary shows a minimum energy at the $(1/2,0)$ position as is observed in some $S=1/2$ square-lattice antiferromagnets. Thus, our results suggest that the quantum dispersion renormalization effects or longer-range exchange interactions observed in cuprates and other $S=1/2$ square-lattice antiferromagnets are also present in La$_2$NiO$_4$. We also find that the overall intensity of the spin-wave excitations is suppressed relative to linear spin-wave theory indicating that covalency is important. Two-magnon scattering is also observed. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2304.02546v2-abstract-full').style.display = 'none'; document.getElementById('2304.02546v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 22 August, 2023; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 5 April, 2023; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> April 2023. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">Final author version</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Research 5, 033113 (2023) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2007.07313">arXiv:2007.07313</a> <span> [<a href="https://arxiv.org/pdf/2007.07313">pdf</a>, <a href="https://arxiv.org/format/2007.07313">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Superconductivity">cond-mat.supr-con</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.125.257002">10.1103/PhysRevLett.125.257002 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Detection of Acoustic Plasmons in Hole-Doped Lanthanum and Bismuth Cuprate Superconductors Using Resonant Inelastic X-Ray Scattering </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Nag%2C+A">Abhishek Nag</a>, <a href="/search/cond-mat?searchtype=author&query=Zhu%2C+M">M. Zhu</a>, <a href="/search/cond-mat?searchtype=author&query=Bejas%2C+M">Matias Bejas</a>, <a href="/search/cond-mat?searchtype=author&query=Li%2C+J">J. Li</a>, <a href="/search/cond-mat?searchtype=author&query=Robarts%2C+H+C">H. C. Robarts</a>, <a href="/search/cond-mat?searchtype=author&query=Yamase%2C+H">Hiroyuki Yamase</a>, <a href="/search/cond-mat?searchtype=author&query=Petsch%2C+A+N">A. N. Petsch</a>, <a href="/search/cond-mat?searchtype=author&query=Song%2C+D">D. Song</a>, <a href="/search/cond-mat?searchtype=author&query=Eisaki%2C+H">H. Eisaki</a>, <a href="/search/cond-mat?searchtype=author&query=Walters%2C+A+C">A. C. Walters</a>, <a href="/search/cond-mat?searchtype=author&query=Garcia-Fernandez%2C+M">M. Garcia-Fernandez</a>, <a href="/search/cond-mat?searchtype=author&query=Greco%2C+A">Andres Greco</a>, <a href="/search/cond-mat?searchtype=author&query=Hayden%2C+S+M">S. M. Hayden</a>, <a href="/search/cond-mat?searchtype=author&query=Zhou%2C+K">Ke-Jin Zhou</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2007.07313v2-abstract-short" style="display: inline;"> High Tc superconductors show a rich variety of phases associated with their charge degrees of freedom. Valence charges can give rise to charge ordering or acoustic plasmons in these layered cuprate superconductors. While charge ordering has been observed for both hole- and electron-doped cuprates, acoustic plasmons have only been found in electron-doped materials. Here, we use resonant inelastic X… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2007.07313v2-abstract-full').style.display = 'inline'; document.getElementById('2007.07313v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2007.07313v2-abstract-full" style="display: none;"> High Tc superconductors show a rich variety of phases associated with their charge degrees of freedom. Valence charges can give rise to charge ordering or acoustic plasmons in these layered cuprate superconductors. While charge ordering has been observed for both hole- and electron-doped cuprates, acoustic plasmons have only been found in electron-doped materials. Here, we use resonant inelastic X-ray scattering (RIXS) to observe the presence of acoustic plasmons in two families of hole-doped cuprate superconductors [La2-xSrxCuO4 (LSCO) and Bi2Sr1.6La0.4CuO6+d (Bi2201)], crucially completing the picture. Interestingly, in contrast to the quasi-static charge ordering which manifests at both Cu and O sites, the observed acoustic plasmons are predominantly associated with the O sites, revealing a unique dichotomy in the behaviour of valence charges in hole-doped cuprates. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2007.07313v2-abstract-full').style.display = 'none'; document.getElementById('2007.07313v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 15 December, 2020; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 14 July, 2020; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> July 2020. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">11 pages, 7 figures + Supplementary Information</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 125, 257002 (2020) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2002.02856">arXiv:2002.02856</a> <span> [<a href="https://arxiv.org/pdf/2002.02856">pdf</a>, <a href="https://arxiv.org/format/2002.02856">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Superconductivity">cond-mat.supr-con</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.125.217004">10.1103/PhysRevLett.125.217004 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Reduction of the spin susceptibility in the superconducting state of Sr2RuO4 observed by polarized neutron scattering </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Petsch%2C+A+N">A. N. Petsch</a>, <a href="/search/cond-mat?searchtype=author&query=Zhu%2C+M">M. Zhu</a>, <a href="/search/cond-mat?searchtype=author&query=Enderle%2C+M">Mechthild Enderle</a>, <a href="/search/cond-mat?searchtype=author&query=Mao%2C+Z+Q">Z. Q. Mao</a>, <a href="/search/cond-mat?searchtype=author&query=Maeno%2C+Y">Y. Maeno</a>, <a href="/search/cond-mat?searchtype=author&query=Mazin%2C+I+I">I. I. Mazin</a>, <a href="/search/cond-mat?searchtype=author&query=Hayden%2C+S+M">S. M. Hayden</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2002.02856v2-abstract-short" style="display: inline;"> Recent observations [A.~Pustogow et al. Nature 574, 72 (2019)] of a drop of the $^{17}$O nuclear magnetic resonance (NMR) Knight shift in the superconducting state of Sr$_2$RuO$_4$ challenged the popular picture of a chiral odd-parity paired state in this compound. Here we use polarized neutron scattering to show that there is a $34 \pm 6$ % drop in the magnetic susceptibility at the ruthenium sit… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2002.02856v2-abstract-full').style.display = 'inline'; document.getElementById('2002.02856v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2002.02856v2-abstract-full" style="display: none;"> Recent observations [A.~Pustogow et al. Nature 574, 72 (2019)] of a drop of the $^{17}$O nuclear magnetic resonance (NMR) Knight shift in the superconducting state of Sr$_2$RuO$_4$ challenged the popular picture of a chiral odd-parity paired state in this compound. Here we use polarized neutron scattering to show that there is a $34 \pm 6$ % drop in the magnetic susceptibility at the ruthenium site below the superconducting transition temperature. Measurements are made at lower fields $H \sim \tfrac{1}{3} H_{c2}$ than a previous study allowing the suppression to be observed. Our results are consistent with the recent NMR observations and rule out the chiral odd-parity $\mathbf{d}=\hat{\mathbf{z}}(k_x\pm ik_y)$ state. The observed susceptibility is consistent with several recent proposals including even-parity $B_{1g}$ and odd-parity helical states. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2002.02856v2-abstract-full').style.display = 'none'; document.getElementById('2002.02856v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 26 August, 2020; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 7 February, 2020; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> February 2020. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">New version with Supplementary Material discussing orbital contributions to the susceptibility, Fermi liquid corrections and a two fluid model</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 125, 217004 (2020) </p> </li> </ol> <div class="is-hidden-tablet"> <!-- feedback for mobile only --> <span class="help" style="display: inline-block;"><a href="https://github.com/arXiv/arxiv-search/releases">Search v0.5.6 released 2020-02-24</a> </span> </div> </div> </main> <footer> <div class="columns is-desktop" role="navigation" aria-label="Secondary"> <!-- MetaColumn 1 --> <div class="column"> <div class="columns"> <div class="column"> <ul class="nav-spaced"> <li><a href="https://info.arxiv.org/about">About</a></li> <li><a href="https://info.arxiv.org/help">Help</a></li> </ul> </div> <div class="column"> <ul class="nav-spaced"> <li> <svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 512 512" class="icon filter-black" role="presentation"><title>contact arXiv</title><desc>Click here to contact arXiv</desc><path d="M502.3 190.8c3.9-3.1 9.7-.2 9.7 4.7V400c0 26.5-21.5 48-48 48H48c-26.5 0-48-21.5-48-48V195.6c0-5 5.7-7.8 9.7-4.7 22.4 17.4 52.1 39.5 154.1 113.6 21.1 15.4 56.7 47.8 92.2 47.6 35.7.3 72-32.8 92.3-47.6 102-74.1 131.6-96.3 154-113.7zM256 320c23.2.4 56.6-29.2 73.4-41.4 132.7-96.3 142.8-104.7 173.4-128.7 5.8-4.5 9.2-11.5 9.2-18.9v-19c0-26.5-21.5-48-48-48H48C21.5 64 0 85.5 0 112v19c0 7.4 3.4 14.3 9.2 18.9 30.6 23.9 40.7 32.4 173.4 128.7 16.8 12.2 50.2 41.8 73.4 41.4z"/></svg> <a href="https://info.arxiv.org/help/contact.html"> Contact</a> </li> <li> <svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 512 512" class="icon filter-black" role="presentation"><title>subscribe to arXiv mailings</title><desc>Click here to subscribe</desc><path d="M476 3.2L12.5 270.6c-18.1 10.4-15.8 35.6 2.2 43.2L121 358.4l287.3-253.2c5.5-4.9 13.3 2.6 8.6 8.3L176 407v80.5c0 23.6 28.5 32.9 42.5 15.8L282 426l124.6 52.2c14.2 6 30.4-2.9 33-18.2l72-432C515 7.8 493.3-6.8 476 3.2z"/></svg> <a href="https://info.arxiv.org/help/subscribe"> Subscribe</a> </li> </ul> </div> </div> </div> <!-- end MetaColumn 1 --> <!-- MetaColumn 2 --> <div class="column"> <div class="columns"> <div class="column"> <ul class="nav-spaced"> <li><a href="https://info.arxiv.org/help/license/index.html">Copyright</a></li> <li><a href="https://info.arxiv.org/help/policies/privacy_policy.html">Privacy Policy</a></li> </ul> </div> <div class="column sorry-app-links"> <ul class="nav-spaced"> <li><a href="https://info.arxiv.org/help/web_accessibility.html">Web Accessibility Assistance</a></li> <li> <p class="help"> <a class="a11y-main-link" href="https://status.arxiv.org" target="_blank">arXiv Operational Status <svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 256 512" class="icon filter-dark_grey" role="presentation"><path d="M224.3 273l-136 136c-9.4 9.4-24.6 9.4-33.9 0l-22.6-22.6c-9.4-9.4-9.4-24.6 0-33.9l96.4-96.4-96.4-96.4c-9.4-9.4-9.4-24.6 0-33.9L54.3 103c9.4-9.4 24.6-9.4 33.9 0l136 136c9.5 9.4 9.5 24.6.1 34z"/></svg></a><br> Get status notifications via <a class="is-link" href="https://subscribe.sorryapp.com/24846f03/email/new" target="_blank"><svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 512 512" class="icon filter-black" role="presentation"><path d="M502.3 190.8c3.9-3.1 9.7-.2 9.7 4.7V400c0 26.5-21.5 48-48 48H48c-26.5 0-48-21.5-48-48V195.6c0-5 5.7-7.8 9.7-4.7 22.4 17.4 52.1 39.5 154.1 113.6 21.1 15.4 56.7 47.8 92.2 47.6 35.7.3 72-32.8 92.3-47.6 102-74.1 131.6-96.3 154-113.7zM256 320c23.2.4 56.6-29.2 73.4-41.4 132.7-96.3 142.8-104.7 173.4-128.7 5.8-4.5 9.2-11.5 9.2-18.9v-19c0-26.5-21.5-48-48-48H48C21.5 64 0 85.5 0 112v19c0 7.4 3.4 14.3 9.2 18.9 30.6 23.9 40.7 32.4 173.4 128.7 16.8 12.2 50.2 41.8 73.4 41.4z"/></svg>email</a> or <a class="is-link" href="https://subscribe.sorryapp.com/24846f03/slack/new" target="_blank"><svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 448 512" class="icon filter-black" role="presentation"><path d="M94.12 315.1c0 25.9-21.16 47.06-47.06 47.06S0 341 0 315.1c0-25.9 21.16-47.06 47.06-47.06h47.06v47.06zm23.72 0c0-25.9 21.16-47.06 47.06-47.06s47.06 21.16 47.06 47.06v117.84c0 25.9-21.16 47.06-47.06 47.06s-47.06-21.16-47.06-47.06V315.1zm47.06-188.98c-25.9 0-47.06-21.16-47.06-47.06S139 32 164.9 32s47.06 21.16 47.06 47.06v47.06H164.9zm0 23.72c25.9 0 47.06 21.16 47.06 47.06s-21.16 47.06-47.06 47.06H47.06C21.16 243.96 0 222.8 0 196.9s21.16-47.06 47.06-47.06H164.9zm188.98 47.06c0-25.9 21.16-47.06 47.06-47.06 25.9 0 47.06 21.16 47.06 47.06s-21.16 47.06-47.06 47.06h-47.06V196.9zm-23.72 0c0 25.9-21.16 47.06-47.06 47.06-25.9 0-47.06-21.16-47.06-47.06V79.06c0-25.9 21.16-47.06 47.06-47.06 25.9 0 47.06 21.16 47.06 47.06V196.9zM283.1 385.88c25.9 0 47.06 21.16 47.06 47.06 0 25.9-21.16 47.06-47.06 47.06-25.9 0-47.06-21.16-47.06-47.06v-47.06h47.06zm0-23.72c-25.9 0-47.06-21.16-47.06-47.06 0-25.9 21.16-47.06 47.06-47.06h117.84c25.9 0 47.06 21.16 47.06 47.06 0 25.9-21.16 47.06-47.06 47.06H283.1z"/></svg>slack</a> </p> </li> </ul> </div> </div> </div> <!-- end MetaColumn 2 --> </div> </footer> <script src="https://static.arxiv.org/static/base/1.0.0a5/js/member_acknowledgement.js"></script> </body> </html>