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href="https://www.academia.edu/124421207/Nanoscale_mineral_contaminant_redox_reaction_processes_impact_on_oxyanion_contaminant_fate_in_oscillating_anoxic_environments"><img alt="Research paper thumbnail of Nanoscale mineral/contaminant redox reaction processes: impact on oxyanion contaminant fate in oscillating anoxic environments" class="work-thumbnail" src="https://attachments.academia-assets.com/118649809/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421207/Nanoscale_mineral_contaminant_redox_reaction_processes_impact_on_oxyanion_contaminant_fate_in_oscillating_anoxic_environments">Nanoscale mineral/contaminant redox reaction processes: impact on oxyanion contaminant fate in oscillating anoxic environments</a></div><div class="wp-workCard_item wp-workCard--actions"><span 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href="https://www.academia.edu/124421206/Gentamicin_Montmorillonite_Intercalation_Compounds_as_an_Active_Component_of_Hydroxypropylmethylcellulose_Bionanocomposite_Films_with_Antimicrobial_Properties"><img alt="Research paper thumbnail of Gentamicin-Montmorillonite Intercalation Compounds as an Active Component of Hydroxypropylmethylcellulose Bionanocomposite Films with Antimicrobial Properties" class="work-thumbnail" src="https://attachments.academia-assets.com/118649806/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421206/Gentamicin_Montmorillonite_Intercalation_Compounds_as_an_Active_Component_of_Hydroxypropylmethylcellulose_Bionanocomposite_Films_with_Antimicrobial_Properties">Gentamicin-Montmorillonite Intercalation Compounds as an Active Component of Hydroxypropylmethylcellulose Bionanocomposite Films with Antimicrobial Properties</a></div><div class="wp-workCard_item"><span>Clays and Clay Minerals</span><span>, Oct 1, 2021</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="5fdb954344170f218042e3a840c7e5cd" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649806,"asset_id":124421206,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649806/download_file?st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421206"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421206"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421206; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421206]").text(description); $(".js-view-count[data-work-id=124421206]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421206; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421206']"); 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$('.js-work-strip[data-work-id=124421206]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421206,"title":"Gentamicin-Montmorillonite Intercalation Compounds as an Active Component of Hydroxypropylmethylcellulose Bionanocomposite Films with Antimicrobial Properties","translated_title":"","metadata":{"publisher":"Springer Science+Business Media","grobid_abstract":"The present study introduces an overview of gentamicin-clay mineral systems for applications in biomedicine and then focuses on the development of a series of gentamicin/clay hybrid materials to be used as the bioactive phase of hydroxypropylmethylcellulose (HPMC) to produce bionanocomposite membranes possessing antimicrobial activity of interest in wound-dressing applications. Gentamicin (Gt) was adsorbed from aqueous solutions into a montmorillonite (Cloisite®-Na +) to produce intercalation compounds with tunable content of the antibiotic. The hybrids were characterized by CHN chemical analysis, energy-dispersive X-ray analysis, X-ray diffraction, Fouriertransform infrared spectroscopy, and thermogravimetric analysis, confirming the intercalation of Gt by an ion-exchange mechanism. The release of Gt from the hybrids was tested in water and in buffer solution to check their stability. Hybrids with various amounts of Gt were incorporated into a HPMC matrix at various loadings and processed as films by the casting method. The resulting Gt-clay/HPMC bionanocomposites were characterized by means of field-emission scanning electron microscopy, and were also evaluated for their wateradsorption and mechanical properties to confirm their suitability for wound-dressing applications. 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Dynamics Control on Amorphous Calcium Carbonate Crystallization: Precise Control of Calcite Crystal Sizes" class="work-thumbnail" src="https://attachments.academia-assets.com/118649832/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421202/Nanoscale_Ion_Dynamics_Control_on_Amorphous_Calcium_Carbonate_Crystallization_Precise_Control_of_Calcite_Crystal_Sizes">Nanoscale Ion Dynamics Control on Amorphous Calcium Carbonate Crystallization: Precise Control of Calcite Crystal Sizes</a></div><div class="wp-workCard_item"><span>Journal of Physical Chemistry C</span><span>, Nov 4, 2020</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="acff5206ade6ae87e437049b8b988769" class="wp-workCard--action" rel="nofollow" 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Here, we performed X-ray photon correlation spectroscopy experiments on ACC which show that the amount of adsorbed water has a strong control over its diffusive dynamics. Results of crystallization experiments under conditions of controlled humidity indicate that the adsorbed water is enough to spark crystallization of calcite. A direct proportionality is found between the relative humidity of the environment and the final size of the calcite crystals. Different hypotheses are made to explain this result, with the confinement within the amorphous matrix being the main suspect of controlling the size of the crystallites. Control of water activity and water content is, therefore, a possible way to regulate biomineral crystallinity both in nature and for the design of functional biomimetic materials.","publication_date":{"day":4,"month":11,"year":2020,"errors":{}},"publication_name":"Journal of Physical Chemistry C","grobid_abstract_attachment_id":118649832},"translated_abstract":null,"internal_url":"https://www.academia.edu/124421202/Nanoscale_Ion_Dynamics_Control_on_Amorphous_Calcium_Carbonate_Crystallization_Precise_Control_of_Calcite_Crystal_Sizes","translated_internal_url":"","created_at":"2024-10-04T08:33:35.724-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[{"id":118649832,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649832/thumbnails/1.jpg","file_name":"acs.jpcc.pdf","download_url":"https://www.academia.edu/attachments/118649832/download_file?st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Nanoscale_Ion_Dynamics_Control_on_Amorph.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649832/acs.jpcc-libre.pdf?1728057726=\u0026response-content-disposition=attachment%3B+filename%3DNanoscale_Ion_Dynamics_Control_on_Amorph.pdf\u0026Expires=1733244890\u0026Signature=S990tf4JuWuXGsZRkYTWahaMN0h3C~aJxiBZdWy7OpJaGRinbWDfThEDNFiMoZ9lWwmDCqiPF~GG2rkMLITmQ52KFcyeOW1etHFvNNYPIdzlXWhPzxCzQtcltEZD46ZwJBAB1fVppYqQvCi3wghtK4KF8lt5t3rkgr952QbmY8Li6Gt7WkDXfapdITs6YG9eCg1gxdLxf~G5joSlF4ULzjpYJT7Ya-rosUyg8INBn3ER3-nN6lxk4mCpFLnozFNKFiSXdi96FYEO7U1i~O5q~rRoNOT-V~-OEo66dcpzdcd6Us0x7ne97lAKoq56A0Wz1v-~2FBCa9bB~VyXO30IQQ__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"slug":"Nanoscale_Ion_Dynamics_Control_on_Amorphous_Calcium_Carbonate_Crystallization_Precise_Control_of_Calcite_Crystal_Sizes","translated_slug":"","page_count":12,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[{"id":118649832,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649832/thumbnails/1.jpg","file_name":"acs.jpcc.pdf","download_url":"https://www.academia.edu/attachments/118649832/download_file?st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Nanoscale_Ion_Dynamics_Control_on_Amorph.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649832/acs.jpcc-libre.pdf?1728057726=\u0026response-content-disposition=attachment%3B+filename%3DNanoscale_Ion_Dynamics_Control_on_Amorph.pdf\u0026Expires=1733244890\u0026Signature=S990tf4JuWuXGsZRkYTWahaMN0h3C~aJxiBZdWy7OpJaGRinbWDfThEDNFiMoZ9lWwmDCqiPF~GG2rkMLITmQ52KFcyeOW1etHFvNNYPIdzlXWhPzxCzQtcltEZD46ZwJBAB1fVppYqQvCi3wghtK4KF8lt5t3rkgr952QbmY8Li6Gt7WkDXfapdITs6YG9eCg1gxdLxf~G5joSlF4ULzjpYJT7Ya-rosUyg8INBn3ER3-nN6lxk4mCpFLnozFNKFiSXdi96FYEO7U1i~O5q~rRoNOT-V~-OEo66dcpzdcd6Us0x7ne97lAKoq56A0Wz1v-~2FBCa9bB~VyXO30IQQ__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"research_interests":[{"id":48,"name":"Engineering","url":"https://www.academia.edu/Documents/in/Engineering"},{"id":511,"name":"Materials Science","url":"https://www.academia.edu/Documents/in/Materials_Science"},{"id":923,"name":"Technology","url":"https://www.academia.edu/Documents/in/Technology"},{"id":12597,"name":"Crystallization","url":"https://www.academia.edu/Documents/in/Crystallization"},{"id":91258,"name":"Carbonate","url":"https://www.academia.edu/Documents/in/Carbonate"},{"id":156638,"name":"Amorphous Calcium Carbonate","url":"https://www.academia.edu/Documents/in/Amorphous_Calcium_Carbonate"},{"id":205543,"name":"Calcite","url":"https://www.academia.edu/Documents/in/Calcite"},{"id":260118,"name":"CHEMICAL SCIENCES","url":"https://www.academia.edu/Documents/in/CHEMICAL_SCIENCES"},{"id":348756,"name":"Ion","url":"https://www.academia.edu/Documents/in/Ion"},{"id":630941,"name":"Calcium Carbonate","url":"https://www.academia.edu/Documents/in/Calcium_Carbonate"}],"urls":[{"id":44976103,"url":"https://doi.org/10.1021/acs.jpcc.0c08670"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421201"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421201/In_Vitro_Preparation_of_Actively_Maturing_Bovine_Articular_Cartilage_Explants_for_X_Ray_Phase_Contrast_Imaging"><img alt="Research paper thumbnail of In Vitro Preparation of Actively Maturing Bovine Articular Cartilage Explants for X-Ray Phase Contrast Imaging" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421201/In_Vitro_Preparation_of_Actively_Maturing_Bovine_Articular_Cartilage_Explants_for_X_Ray_Phase_Contrast_Imaging">In Vitro Preparation of Actively Maturing Bovine Articular Cartilage Explants for X-Ray Phase Contrast Imaging</a></div><div class="wp-workCard_item"><span>Journal of Visualized Experiments</span><span>, Jan 31, 2022</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">Understanding the mechanisms that underpin post-natal maturation of articular cartilage is of cru...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">Understanding the mechanisms that underpin post-natal maturation of articular cartilage is of crucial importance for designing the next generation of tissue engineering strategies and potentially repairing diseased or damaged cartilage. In general, postnatal maturation of the articular cartilage, which is a wholesale change in collagen structure and function of the tissue to accommodate growth of the organism, occurs over a timescale ranging from months to years. Conversely dissolution of the structural organization of the cartilage that also occurs over long timescales is the hallmark of tissue degeneration. Our ability to study these biological processes in detail have been enhanced by the findings that growth factors can induce precocious in vitro maturation of immature articular cartilage. The developmental and disease related changes that occur in the joint involve bone and cartilage and an ability to co-image these tissues would significantly increase our understanding of their intertwined roles. The simultaneous visualization of soft tissue, cartilage and bone changes is nowadays a challenge to overcome for conventional preclinical imaging modalities used for the joint disease follow-up. Three-dimensional X-ray Phase-Contrast Imaging methods (PCI) have been under perpetual developments for 20 years due to high performance for imaging low density objects and their ability to provide additional information compared to conventional X-ray imaging. In this protocol we detail the procedure used in our experiments from biopsy of the cartilage, generation of in vitro matured cartilage to data analysis of image collected using X-ray phase contrast imaging.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421201"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421201"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421201; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421201]").text(description); $(".js-view-count[data-work-id=124421201]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421201; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421201']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421201, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=124421201]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421201,"title":"In Vitro Preparation of Actively Maturing Bovine Articular Cartilage Explants for X-Ray Phase Contrast Imaging","translated_title":"","metadata":{"abstract":"Understanding the mechanisms that underpin post-natal maturation of articular cartilage is of crucial importance for designing the next generation of tissue engineering strategies and potentially repairing diseased or damaged cartilage. In general, postnatal maturation of the articular cartilage, which is a wholesale change in collagen structure and function of the tissue to accommodate growth of the organism, occurs over a timescale ranging from months to years. Conversely dissolution of the structural organization of the cartilage that also occurs over long timescales is the hallmark of tissue degeneration. Our ability to study these biological processes in detail have been enhanced by the findings that growth factors can induce precocious in vitro maturation of immature articular cartilage. The developmental and disease related changes that occur in the joint involve bone and cartilage and an ability to co-image these tissues would significantly increase our understanding of their intertwined roles. The simultaneous visualization of soft tissue, cartilage and bone changes is nowadays a challenge to overcome for conventional preclinical imaging modalities used for the joint disease follow-up. Three-dimensional X-ray Phase-Contrast Imaging methods (PCI) have been under perpetual developments for 20 years due to high performance for imaging low density objects and their ability to provide additional information compared to conventional X-ray imaging. In this protocol we detail the procedure used in our experiments from biopsy of the cartilage, generation of in vitro matured cartilage to data analysis of image collected using X-ray phase contrast imaging.","publisher":"MyJOVE","publication_date":{"day":31,"month":1,"year":2022,"errors":{}},"publication_name":"Journal of Visualized Experiments"},"translated_abstract":"Understanding the mechanisms that underpin post-natal maturation of articular cartilage is of crucial importance for designing the next generation of tissue engineering strategies and potentially repairing diseased or damaged cartilage. 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$a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421199"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421199/Exploring_carbonate_rock_wettability_across_scales_Role_of_bio_minerals"><img alt="Research paper thumbnail of Exploring carbonate rock wettability across scales: Role of (bio)minerals" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421199/Exploring_carbonate_rock_wettability_across_scales_Role_of_bio_minerals">Exploring carbonate rock wettability across scales: Role of (bio)minerals</a></div><div class="wp-workCard_item"><span>Journal of Colloid and Interface Science</span><span>, Jul 1, 2023</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421199"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421199"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421199; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) 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data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421197/Selenium_Nanowire_Formation_by_Reacting_Selenate_with_Magnetite">Selenium Nanowire Formation by Reacting Selenate with Magnetite</a></div><div class="wp-workCard_item"><span>Environmental Science & Technology</span><span>, Oct 3, 2022</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421197"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421197"><i class="fa 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nanoscale: Insights into the iron sulfide formation in low-temperature aqueous solution</a></div><div class="wp-workCard_item"><span>Geochimica et Cosmochimica Acta</span><span>, Dec 1, 2022</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421196"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421196"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421196; window.Academia.workViewCountsFetcher.queue(workId, 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require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=124421196]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421196,"title":"Thermodynamic stability reversal of iron sulfides at the nanoscale: Insights into the iron sulfide formation in low-temperature aqueous solution","translated_title":"","metadata":{"publisher":"Elsevier 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href="https://www.academia.edu/124421195/Water_Trapping_Dynamics_in_Carbohydrate_Populated_Smectite_Interlayer_Nanopores">Water Trapping Dynamics in Carbohydrate-Populated Smectite Interlayer Nanopores</a></div><div class="wp-workCard_item"><span>Journal of Physical Chemistry C</span><span>, Nov 4, 2019</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="6ff4e66584043509bc8647a219a04fe5" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649829,"asset_id":124421195,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649829/download_file?st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span 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The hydrodynamics of cationsaturated smectite nanopores are well documented. However, little is known about the influence of small organic compounds. Here we investigate the effects of carbohydrates (glucose and cellobiose), representing an important class of organic compounds, on the hydration and nanopore structures of montmorillonite, a prototypical smectite. To achieve the same amount of adsorbed water, higher relative humidity was required in the presence of the adsorbed carbohydrates than with the clay alone. The decrease in the characteristic micropore water adsorption with the clay−carbohydrate aggregates implied that water adsorption was constrained within the clay nanopore regions. The presence of carbohydrates promoted water retention as a function of gradual decrease in moisture content. Moisture-dependent X-ray diffraction patterns determined that, relative to the mineral alone, greater nanopore sizes were preserved in the presence of the carbohydrates, despite severe dehydration that is expected to induce clay nanopore collapse. Fourier-transform infrared spectroscopy captured disruption in the population of exchangeable waters within the carbohydrate-populated clay nanopores, with some agreement with the measured water-desorption profiling. These new findings demonstrate that carbohydrates can restructure smectite interlayer nanopores and water trapping dynamics.","publication_date":{"day":4,"month":11,"year":2019,"errors":{}},"publication_name":"Journal of Physical Chemistry C","grobid_abstract_attachment_id":118649829},"translated_abstract":null,"internal_url":"https://www.academia.edu/124421195/Water_Trapping_Dynamics_in_Carbohydrate_Populated_Smectite_Interlayer_Nanopores","translated_internal_url":"","created_at":"2024-10-04T08:33:29.781-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[{"id":118649829,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649829/thumbnails/1.jpg","file_name":"acs.jpcc.9b0924620241004-1-t42xja.pdf","download_url":"https://www.academia.edu/attachments/118649829/download_file?st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Water_Trapping_Dynamics_in_Carbohydrate.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649829/acs.jpcc.9b0924620241004-1-t42xja-libre.pdf?1728057724=\u0026response-content-disposition=attachment%3B+filename%3DWater_Trapping_Dynamics_in_Carbohydrate.pdf\u0026Expires=1733244890\u0026Signature=YYB2smYgTv6zrra3brUYV8qAGo3a~6EUrtz0CEfERMx~Umtj9URjqCZlwXRms1I~Ic~nvAikuEN08Wkaw7WFsm-7Omj1hoUTVoPAZl9DVyr1jMv-5tvRL1pgWPHJGpDV229NuIslOfebowyToCvHZEBOzgt0eUmCpsbwofHfxytMdhyAzBS4OPXbold-v2-FOPtyrqJeZVM7Y6exM-aOQ9yoRe7TIVLbcx7j3n~Cxm81r2OZ9d2dWDoul7RM3wRYVwL6ui7U4rBVgldNloo2PvMuPjumOBSOVkWFlHp0nN2H5f~fXqrXovRnrXib98hPH9HnWDfWQeqFsLtEjGZp-g__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"slug":"Water_Trapping_Dynamics_in_Carbohydrate_Populated_Smectite_Interlayer_Nanopores","translated_slug":"","page_count":12,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[{"id":118649829,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649829/thumbnails/1.jpg","file_name":"acs.jpcc.9b0924620241004-1-t42xja.pdf","download_url":"https://www.academia.edu/attachments/118649829/download_file?st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Water_Trapping_Dynamics_in_Carbohydrate.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649829/acs.jpcc.9b0924620241004-1-t42xja-libre.pdf?1728057724=\u0026response-content-disposition=attachment%3B+filename%3DWater_Trapping_Dynamics_in_Carbohydrate.pdf\u0026Expires=1733244890\u0026Signature=YYB2smYgTv6zrra3brUYV8qAGo3a~6EUrtz0CEfERMx~Umtj9URjqCZlwXRms1I~Ic~nvAikuEN08Wkaw7WFsm-7Omj1hoUTVoPAZl9DVyr1jMv-5tvRL1pgWPHJGpDV229NuIslOfebowyToCvHZEBOzgt0eUmCpsbwofHfxytMdhyAzBS4OPXbold-v2-FOPtyrqJeZVM7Y6exM-aOQ9yoRe7TIVLbcx7j3n~Cxm81r2OZ9d2dWDoul7RM3wRYVwL6ui7U4rBVgldNloo2PvMuPjumOBSOVkWFlHp0nN2H5f~fXqrXovRnrXib98hPH9HnWDfWQeqFsLtEjGZp-g__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"research_interests":[{"id":48,"name":"Engineering","url":"https://www.academia.edu/Documents/in/Engineering"},{"id":72,"name":"Chemical Engineering","url":"https://www.academia.edu/Documents/in/Chemical_Engineering"},{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":923,"name":"Technology","url":"https://www.academia.edu/Documents/in/Technology"},{"id":21728,"name":"Clay Minerals","url":"https://www.academia.edu/Documents/in/Clay_Minerals"},{"id":22300,"name":"Chemical Physics","url":"https://www.academia.edu/Documents/in/Chemical_Physics"},{"id":39752,"name":"Adsorption","url":"https://www.academia.edu/Documents/in/Adsorption"},{"id":260118,"name":"CHEMICAL SCIENCES","url":"https://www.academia.edu/Documents/in/CHEMICAL_SCIENCES"},{"id":334138,"name":"Montmorillonite","url":"https://www.academia.edu/Documents/in/Montmorillonite"},{"id":456380,"name":"Trapping","url":"https://www.academia.edu/Documents/in/Trapping"},{"id":3478741,"name":"Nanopore","url":"https://www.academia.edu/Documents/in/Nanopore"}],"urls":[{"id":44976096,"url":"https://doi.org/10.1021/acs.jpcc.9b09246"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421194"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421194/Acid_volatile_sulfides_and_simultaneously_extracted_metals_A_new_miniaturized_purge_and_trap_system_for_laboratory_and_field_measurements"><img alt="Research paper thumbnail of Acid volatile sulfides and simultaneously extracted metals: A new miniaturized ‘purge and trap’ system for laboratory and field measurements" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421194/Acid_volatile_sulfides_and_simultaneously_extracted_metals_A_new_miniaturized_purge_and_trap_system_for_laboratory_and_field_measurements">Acid volatile sulfides and simultaneously extracted metals: A new miniaturized ‘purge and trap’ system for laboratory and field measurements</a></div><div class="wp-workCard_item"><span>Talanta</span><span>, Oct 1, 2021</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">In natural environments, Acid Volatile Sulfides (AVS) contained in anoxic waters or sediments, ar...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">In natural environments, Acid Volatile Sulfides (AVS) contained in anoxic waters or sediments, are composed of dissolved sulfides and neo-formed sulfides colloids or particles. Under acidic addition, AVS emit hydrogen sulfide gas and release the so-called simultaneously extracted metals (SEM). The measurement of AVS coupled with that of the SEM enables to evaluate the metal trapping capacity of sulfides in the environment. Because AVS are extremely reactive to oxidation, the most accurate methodology to quantify AVS and SEM requires to be able to process the samples extraction on-site, directly after sampling and avoiding oxygen exposure. However, most of available systems are based on glassware &#39;purge and trap&#39; techniques developed for the laboratory and are not often adapted to field studies. In these systems, AVS extraction time can range from 30 min to 3 h with relative standard deviation from 7 to 44%. In this study, we developed a new &#39;purge and trap&#39; system designed for both laboratory use and field AVS/SEM extractions. The system is optimized with a shortened extraction time, miniaturized, unbreakable, easy and reproducible to develop parallel extraction benches. Analytical yields, precision and stability have been improved, allowing to reduce the extraction time to 1 h with an absolute quantification limit of 0.12 μmol S(-II) with a relative standard deviation between 7 and 11% and under a complete extraction efficiency.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421194"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421194"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421194; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421194]").text(description); $(".js-view-count[data-work-id=124421194]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421194; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421194']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421194, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=124421194]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421194,"title":"Acid volatile sulfides and simultaneously extracted metals: A new miniaturized ‘purge and trap’ system for laboratory and field measurements","translated_title":"","metadata":{"abstract":"In natural environments, Acid Volatile Sulfides (AVS) contained in anoxic waters or sediments, are composed of dissolved sulfides and neo-formed sulfides colloids or particles. Under acidic addition, AVS emit hydrogen sulfide gas and release the so-called simultaneously extracted metals (SEM). The measurement of AVS coupled with that of the SEM enables to evaluate the metal trapping capacity of sulfides in the environment. Because AVS are extremely reactive to oxidation, the most accurate methodology to quantify AVS and SEM requires to be able to process the samples extraction on-site, directly after sampling and avoiding oxygen exposure. However, most of available systems are based on glassware \u0026#39;purge and trap\u0026#39; techniques developed for the laboratory and are not often adapted to field studies. In these systems, AVS extraction time can range from 30 min to 3 h with relative standard deviation from 7 to 44%. In this study, we developed a new \u0026#39;purge and trap\u0026#39; system designed for both laboratory use and field AVS/SEM extractions. The system is optimized with a shortened extraction time, miniaturized, unbreakable, easy and reproducible to develop parallel extraction benches. Analytical yields, precision and stability have been improved, allowing to reduce the extraction time to 1 h with an absolute quantification limit of 0.12 μmol S(-II) with a relative standard deviation between 7 and 11% and under a complete extraction efficiency.","publisher":"Elsevier BV","publication_date":{"day":1,"month":10,"year":2021,"errors":{}},"publication_name":"Talanta"},"translated_abstract":"In natural environments, Acid Volatile Sulfides (AVS) contained in anoxic waters or sediments, are composed of dissolved sulfides and neo-formed sulfides colloids or particles. Under acidic addition, AVS emit hydrogen sulfide gas and release the so-called simultaneously extracted metals (SEM). The measurement of AVS coupled with that of the SEM enables to evaluate the metal trapping capacity of sulfides in the environment. Because AVS are extremely reactive to oxidation, the most accurate methodology to quantify AVS and SEM requires to be able to process the samples extraction on-site, directly after sampling and avoiding oxygen exposure. However, most of available systems are based on glassware \u0026#39;purge and trap\u0026#39; techniques developed for the laboratory and are not often adapted to field studies. In these systems, AVS extraction time can range from 30 min to 3 h with relative standard deviation from 7 to 44%. In this study, we developed a new \u0026#39;purge and trap\u0026#39; system designed for both laboratory use and field AVS/SEM extractions. The system is optimized with a shortened extraction time, miniaturized, unbreakable, easy and reproducible to develop parallel extraction benches. Analytical yields, precision and stability have been improved, allowing to reduce the extraction time to 1 h with an absolute quantification limit of 0.12 μmol S(-II) with a relative standard deviation between 7 and 11% and under a complete extraction efficiency.","internal_url":"https://www.academia.edu/124421194/Acid_volatile_sulfides_and_simultaneously_extracted_metals_A_new_miniaturized_purge_and_trap_system_for_laboratory_and_field_measurements","translated_internal_url":"","created_at":"2024-10-04T08:33:28.847-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"Acid_volatile_sulfides_and_simultaneously_extracted_metals_A_new_miniaturized_purge_and_trap_system_for_laboratory_and_field_measurements","translated_slug":"","page_count":null,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":524,"name":"Analytical Chemistry","url":"https://www.academia.edu/Documents/in/Analytical_Chemistry"},{"id":26327,"name":"Medicine","url":"https://www.academia.edu/Documents/in/Medicine"},{"id":139317,"name":"Purge","url":"https://www.academia.edu/Documents/in/Purge"},{"id":476869,"name":"Hydrogen Sulfide","url":"https://www.academia.edu/Documents/in/Hydrogen_Sulfide"}],"urls":[{"id":44976095,"url":"https://doi.org/10.1016/j.talanta.2021.122490"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421191"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421191/Interplay_of_S_and_As_in_Mekong_Delta_sediments_during_redox_oscillations"><img alt="Research paper thumbnail of Interplay of S and As in Mekong Delta sediments during redox oscillations" class="work-thumbnail" src="https://attachments.academia-assets.com/118649828/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421191/Interplay_of_S_and_As_in_Mekong_Delta_sediments_during_redox_oscillations">Interplay of S and As in Mekong Delta sediments during redox oscillations</a></div><div class="wp-workCard_item"><span>Geoscience frontiers</span><span>, Sep 1, 2019</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="b289616a965d9666438d51c8ab401a45" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649828,"asset_id":124421191,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649828/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421191"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421191"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421191; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421191]").text(description); $(".js-view-count[data-work-id=124421191]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421191; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421191']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421191, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (true){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "b289616a965d9666438d51c8ab401a45" } } $('.js-work-strip[data-work-id=124421191]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421191,"title":"Interplay of S and As in Mekong Delta sediments during redox oscillations","translated_title":"","metadata":{"publisher":"Elsevier BV","grobid_abstract":"The cumulative effects of periodic redox cycling on the mobility of As, Fe, and S from alluvial sediment to groundwater were investigated in bioreactor experiments. Two particular sediments from the alluvial floodplain of the Mekong Delta River were investigated: Matrix A (14 m deep) had a higher pyrite concentration than matrix B (7 m deep) sediments. Gypsum was present in matrix B but absent in matrix A. In the reactors, the sediment suspensions were supplemented with As(III) and SO 4 2À , and were subjected to three full-redox cycles entailing phases of nitrogen/CO 2 , compressed air sparging, and cellobiose addition. Major differences in As concentration and speciation were observed upon redox cycling. Evidences support the fact that initial sediment composition is the main factor controlling arsenic release and its speciation during the redox cycles. Indeed, a high pyrite content associated with a low SO 4 2À content resulted in an increase in dissolved As concentrations, mainly in the form of As(III), after anoxic half-cycles; whereas a decrease in As concentrations mainly in the form of As(V), was instead observed after oxic half-cycles. In addition, oxic conditions were found to be responsible for pyrite and arsenian pyrite oxidation, increasing the As pool available for mobilization. The same processes seem to occur in sediment with the presence of gypsum, but, in this case, dissolved As were sequestered by biotic or abiotic redox reactions occurring in the FeeS system, and by specific physico-chemical condition (e.g. pH). The contrasting results obtained for two sediments sampled from the same core show that many complexes and entangled factors are at work, and further refinement is needed to explain the spatial and temporal variability of As release to groundwater of the Mekong River Delta (Vietnam).","publication_date":{"day":1,"month":9,"year":2019,"errors":{}},"publication_name":"Geoscience frontiers","grobid_abstract_attachment_id":118649828},"translated_abstract":null,"internal_url":"https://www.academia.edu/124421191/Interplay_of_S_and_As_in_Mekong_Delta_sediments_during_redox_oscillations","translated_internal_url":"","created_at":"2024-10-04T08:33:28.144-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[{"id":118649828,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649828/thumbnails/1.jpg","file_name":"1-s2.0-S1674987118300872-main.pdf","download_url":"https://www.academia.edu/attachments/118649828/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Interplay_of_S_and_As_in_Mekong_Delta_se.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649828/1-s2.0-S1674987118300872-main-libre.pdf?1728057720=\u0026response-content-disposition=attachment%3B+filename%3DInterplay_of_S_and_As_in_Mekong_Delta_se.pdf\u0026Expires=1733244891\u0026Signature=RjpcUGy~fF5ZPmlAZjPYCJ15llPWN~HgS1hEQmdZPKuDmvSunbB0uvefBAoz0nZEXs5bKNZ6MZjgkOQD9P~9Eb6w0s9WJEldAYmF~D0HGmJpKM8gp411u-7eGc6BamTlGf06TYlMtjWpq94BM839Sd-gz9qWlXXejAsDJik7ZhrR5YhtBsMaFVq36qSEqz2VmS~3CzbsznBrQiiGsHbSopNTMQf15whtQgFAUHaidI9-EDFGoIhXqsCHq~Hkl43~HYIvE4K88dUR6eT33nhw1ld-Z~wdL5c7Oc7kWtWcBsSt9ZiUeYK5mpWHyquQBzUaHvokSkYWD-m9waDCwXB33g__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"slug":"Interplay_of_S_and_As_in_Mekong_Delta_sediments_during_redox_oscillations","translated_slug":"","page_count":16,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[{"id":118649828,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649828/thumbnails/1.jpg","file_name":"1-s2.0-S1674987118300872-main.pdf","download_url":"https://www.academia.edu/attachments/118649828/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Interplay_of_S_and_As_in_Mekong_Delta_se.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649828/1-s2.0-S1674987118300872-main-libre.pdf?1728057720=\u0026response-content-disposition=attachment%3B+filename%3DInterplay_of_S_and_As_in_Mekong_Delta_se.pdf\u0026Expires=1733244891\u0026Signature=RjpcUGy~fF5ZPmlAZjPYCJ15llPWN~HgS1hEQmdZPKuDmvSunbB0uvefBAoz0nZEXs5bKNZ6MZjgkOQD9P~9Eb6w0s9WJEldAYmF~D0HGmJpKM8gp411u-7eGc6BamTlGf06TYlMtjWpq94BM839Sd-gz9qWlXXejAsDJik7ZhrR5YhtBsMaFVq36qSEqz2VmS~3CzbsznBrQiiGsHbSopNTMQf15whtQgFAUHaidI9-EDFGoIhXqsCHq~Hkl43~HYIvE4K88dUR6eT33nhw1ld-Z~wdL5c7Oc7kWtWcBsSt9ZiUeYK5mpWHyquQBzUaHvokSkYWD-m9waDCwXB33g__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"research_interests":[{"id":406,"name":"Geology","url":"https://www.academia.edu/Documents/in/Geology"},{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":15836,"name":"Environmental Chemistry","url":"https://www.academia.edu/Documents/in/Environmental_Chemistry"},{"id":142977,"name":"Delta","url":"https://www.academia.edu/Documents/in/Delta"},{"id":156636,"name":"Pyrite","url":"https://www.academia.edu/Documents/in/Pyrite"},{"id":192294,"name":"Sediment","url":"https://www.academia.edu/Documents/in/Sediment"},{"id":859634,"name":"Mekong Delta","url":"https://www.academia.edu/Documents/in/Mekong_Delta"},{"id":1009236,"name":"Redox","url":"https://www.academia.edu/Documents/in/Redox"},{"id":1216203,"name":"Earth Science","url":"https://www.academia.edu/Documents/in/Earth_Science"}],"urls":[{"id":44976093,"url":"https://doi.org/10.1016/j.gsf.2018.03.008"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421189"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421189/Effects_of_redox_oscillations_on_the_phosphogypsum_waste_in_an_estuarine_salt_marsh_system"><img alt="Research paper thumbnail of Effects of redox oscillations on the phosphogypsum waste in an estuarine salt-marsh system" class="work-thumbnail" src="https://attachments.academia-assets.com/118649802/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421189/Effects_of_redox_oscillations_on_the_phosphogypsum_waste_in_an_estuarine_salt_marsh_system">Effects of redox oscillations on the phosphogypsum waste in an estuarine salt-marsh system</a></div><div class="wp-workCard_item"><span>Chemosphere</span><span>, Mar 1, 2020</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="791959471469dbb0120dd141a86e6625" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649802,"asset_id":124421189,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649802/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421189"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421189"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421189; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421189]").text(description); $(".js-view-count[data-work-id=124421189]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421189; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421189']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421189, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (true){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); 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In the present study, we focus on the effects of variable redox conditions imposed to a highly-polluted phosphogypsum stack that is directly piled over the salt marsh soil in the Tinto River estuary (Huelva, Spain). The behaviour of contaminants is evaluated in the phosphogypsum waste and in the marsh basement, separately, in controlled, experimentally-induced oscillating redox conditions. The results revealed that Fe, and to a lesser extent S, control most precipitation/dissolution processes. Ferric iron precipitates in the form of phosphates and oxyhydroxides, while metal sulphide precipitation is insignificant and appears to be prevented by the abundant formation of Fe phosphates. An antagonistic evolution with changing redox conditions was observed for the remaining contaminants such as Zn, As, Cd and U, which remained mobile in solution during most of experimental run. Therefore, these findings revealed that high concentrations of phosphates inhibit the typical processes of immobilization of pollutants in salt-marshes which highlights the elevated contaminant potential of phosphogypsum wastes on coastal environments.","publication_date":{"day":1,"month":3,"year":2020,"errors":{}},"publication_name":"Chemosphere","grobid_abstract_attachment_id":118649802},"translated_abstract":null,"internal_url":"https://www.academia.edu/124421189/Effects_of_redox_oscillations_on_the_phosphogypsum_waste_in_an_estuarine_salt_marsh_system","translated_internal_url":"","created_at":"2024-10-04T08:33:27.796-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[{"id":118649802,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649802/thumbnails/1.jpg","file_name":"document.pdf","download_url":"https://www.academia.edu/attachments/118649802/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Effects_of_redox_oscillations_on_the_pho.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649802/document-libre.pdf?1728057748=\u0026response-content-disposition=attachment%3B+filename%3DEffects_of_redox_oscillations_on_the_pho.pdf\u0026Expires=1733244891\u0026Signature=GKK2w52utd6LMeflx3pAuTmv1jB8zG86QVxdUfl4PneTPTR9TNhdorGCiVJ3PFuFNavaXpPFyYh8ZOsOR--f8lUjWqy~f~gvvbimasjWhGr92lQSETYe0CrMEQixlaCIdreWo-FW5LdVQQHx17hVJYm-4m3e5AofBsuxJMkmB4CDKNLBbkEb9MjWS0FqloeJMxFmeyHq0zSTZvzxLley9h~W3dFA7A~1coRhI~aQyYnDSq0YvhYBU5C5~kno3W5-h~41H2lyh3ORTDGyFF0KtmthS8bbcS8ioVNxIwAedBh97JbCeo7hgZY26qVOm4pJNUrF0Ki5gmJjiN5E1td0SQ__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"slug":"Effects_of_redox_oscillations_on_the_phosphogypsum_waste_in_an_estuarine_salt_marsh_system","translated_slug":"","page_count":39,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[{"id":118649802,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649802/thumbnails/1.jpg","file_name":"document.pdf","download_url":"https://www.academia.edu/attachments/118649802/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Effects_of_redox_oscillations_on_the_pho.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649802/document-libre.pdf?1728057748=\u0026response-content-disposition=attachment%3B+filename%3DEffects_of_redox_oscillations_on_the_pho.pdf\u0026Expires=1733244891\u0026Signature=GKK2w52utd6LMeflx3pAuTmv1jB8zG86QVxdUfl4PneTPTR9TNhdorGCiVJ3PFuFNavaXpPFyYh8ZOsOR--f8lUjWqy~f~gvvbimasjWhGr92lQSETYe0CrMEQixlaCIdreWo-FW5LdVQQHx17hVJYm-4m3e5AofBsuxJMkmB4CDKNLBbkEb9MjWS0FqloeJMxFmeyHq0zSTZvzxLley9h~W3dFA7A~1coRhI~aQyYnDSq0YvhYBU5C5~kno3W5-h~41H2lyh3ORTDGyFF0KtmthS8bbcS8ioVNxIwAedBh97JbCeo7hgZY26qVOm4pJNUrF0Ki5gmJjiN5E1td0SQ__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":15836,"name":"Environmental Chemistry","url":"https://www.academia.edu/Documents/in/Environmental_Chemistry"},{"id":26327,"name":"Medicine","url":"https://www.academia.edu/Documents/in/Medicine"},{"id":28235,"name":"Multidisciplinary","url":"https://www.academia.edu/Documents/in/Multidisciplinary"},{"id":291658,"name":"Precipitation","url":"https://www.academia.edu/Documents/in/Precipitation"},{"id":576179,"name":"Salt marsh","url":"https://www.academia.edu/Documents/in/Salt_marsh"},{"id":1009236,"name":"Redox","url":"https://www.academia.edu/Documents/in/Redox"},{"id":1129780,"name":"Phosphogypsum","url":"https://www.academia.edu/Documents/in/Phosphogypsum"}],"urls":[{"id":44976090,"url":"https://hal.science/hal-03043993/document"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421179"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421179/The_influence_of_pH_and_reaction_time_on_the_formation_of_FeSe_sub_2_sub_upon_selenite_reduction_by_nano_sized_pyrite_greigite"><img alt="Research paper thumbnail of The influence of pH and reaction time on the formation of FeSe<sub>2</sub> upon selenite reduction by nano-sized pyrite-greigite" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421179/The_influence_of_pH_and_reaction_time_on_the_formation_of_FeSe_sub_2_sub_upon_selenite_reduction_by_nano_sized_pyrite_greigite">The influence of pH and reaction time on the formation of FeSe<sub>2</sub> upon selenite reduction by nano-sized pyrite-greigite</a></div><div class="wp-workCard_item"><span>Radiochimica Acta</span><span>, Jun 8, 2016</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The influence of pH and reaction time on the formation of FeSe2 by reductive precipitation of Se(...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The influence of pH and reaction time on the formation of FeSe2 by reductive precipitation of Se(IV) with nano-sized pyrite-greigite was investigated. Reductive precipitation is an effective method of attenuating the mobility of 79Se, which is foreseen to be a dangerous radioisotope for the geological disposal of high-level radioactive waste (HLW). The results indicated that Se(0)was formed at pH &amp;lt;4.05, whereas, at pH &amp;gt; 6.07, considerable amount of FeSe2 was formed along with Se(0). These observations are in agreement with the thermodynamic predictions reported in this work. Furthermore, the formation of FeSe2 was found to continue by increasing the reaction time, indicating that the Se(0) formed in the early reaction stage is gradually transformed to FeSe2 upon the depletion of aqueous Se(IV). Since FeSe2 has a stronger reactivity than pyrite, it was proposed that greigite, rather than pyrite, was responsible for the formation of FeSe2. The findings in this study are of interest for key geochemical processes governing the mobility of toxic 79Se in the environment in presence of iron sulfides.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421179"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421179"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421179; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421179]").text(description); $(".js-view-count[data-work-id=124421179]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421179; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421179']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421179, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=124421179]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421179,"title":"The influence of pH and reaction time on the formation of FeSe\u003csub\u003e2\u003c/sub\u003e upon selenite reduction by nano-sized pyrite-greigite","translated_title":"","metadata":{"abstract":"The influence of pH and reaction time on the formation of FeSe2 by reductive precipitation of Se(IV) with nano-sized pyrite-greigite was investigated. Reductive precipitation is an effective method of attenuating the mobility of 79Se, which is foreseen to be a dangerous radioisotope for the geological disposal of high-level radioactive waste (HLW). The results indicated that Se(0)was formed at pH \u0026amp;lt;4.05, whereas, at pH \u0026amp;gt; 6.07, considerable amount of FeSe2 was formed along with Se(0). These observations are in agreement with the thermodynamic predictions reported in this work. Furthermore, the formation of FeSe2 was found to continue by increasing the reaction time, indicating that the Se(0) formed in the early reaction stage is gradually transformed to FeSe2 upon the depletion of aqueous Se(IV). Since FeSe2 has a stronger reactivity than pyrite, it was proposed that greigite, rather than pyrite, was responsible for the formation of FeSe2. The findings in this study are of interest for key geochemical processes governing the mobility of toxic 79Se in the environment in presence of iron sulfides.","publisher":"R. Oldenbourg Verlag","publication_date":{"day":8,"month":6,"year":2016,"errors":{}},"publication_name":"Radiochimica Acta"},"translated_abstract":"The influence of pH and reaction time on the formation of FeSe2 by reductive precipitation of Se(IV) with nano-sized pyrite-greigite was investigated. Reductive precipitation is an effective method of attenuating the mobility of 79Se, which is foreseen to be a dangerous radioisotope for the geological disposal of high-level radioactive waste (HLW). The results indicated that Se(0)was formed at pH \u0026amp;lt;4.05, whereas, at pH \u0026amp;gt; 6.07, considerable amount of FeSe2 was formed along with Se(0). These observations are in agreement with the thermodynamic predictions reported in this work. Furthermore, the formation of FeSe2 was found to continue by increasing the reaction time, indicating that the Se(0) formed in the early reaction stage is gradually transformed to FeSe2 upon the depletion of aqueous Se(IV). Since FeSe2 has a stronger reactivity than pyrite, it was proposed that greigite, rather than pyrite, was responsible for the formation of FeSe2. The findings in this study are of interest for key geochemical processes governing the mobility of toxic 79Se in the environment in presence of iron sulfides.","internal_url":"https://www.academia.edu/124421179/The_influence_of_pH_and_reaction_time_on_the_formation_of_FeSe_sub_2_sub_upon_selenite_reduction_by_nano_sized_pyrite_greigite","translated_internal_url":"","created_at":"2024-10-04T08:33:23.547-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"The_influence_of_pH_and_reaction_time_on_the_formation_of_FeSe_sub_2_sub_upon_selenite_reduction_by_nano_sized_pyrite_greigite","translated_slug":"","page_count":null,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":156636,"name":"Pyrite","url":"https://www.academia.edu/Documents/in/Pyrite"},{"id":214346,"name":"Greigite","url":"https://www.academia.edu/Documents/in/Greigite"},{"id":291658,"name":"Precipitation","url":"https://www.academia.edu/Documents/in/Precipitation"}],"urls":[{"id":44976088,"url":"https://doi.org/10.1515/ract-2015-2496"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421178"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421178/Copper_Isotopes_and_Copper_to_Zinc_Ratio_as_Possible_Biomarkers_for_Thyroid_Cancer"><img alt="Research paper thumbnail of Copper Isotopes and Copper to Zinc Ratio as Possible Biomarkers for Thyroid Cancer" class="work-thumbnail" src="https://attachments.academia-assets.com/118649789/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421178/Copper_Isotopes_and_Copper_to_Zinc_Ratio_as_Possible_Biomarkers_for_Thyroid_Cancer">Copper Isotopes and Copper to Zinc Ratio as Possible Biomarkers for Thyroid Cancer</a></div><div class="wp-workCard_item"><span>Frontiers in Medicine</span><span>, Sep 8, 2021</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="426a9efaab89544b4bd1632a25d367c6" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649789,"asset_id":124421178,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649789/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421178"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421178"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421178; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421178]").text(description); $(".js-view-count[data-work-id=124421178]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421178; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421178']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421178, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (true){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); 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There is no systematic screening for such cancer, and the current challenge is to find potential biomarkers to facilitate an early diagnosis. Copper (Cu) and zinc (Zn) are essential micronutrients involved in the proper functioning of the thyroid gland, and changes in their concentrations have been observed in the development of cancer. Previous studies have highlighted the potential 65 Cu/ 63 Cu ratio (δ 65 Cu) to be a cancer biomarker. This study tests its sensitivity on plasma samples (n = 46) of Algerian patients with papillary thyroid carcinoma and a set of corresponding biopsies (n = 11). The δ 65 Cu ratio in blood and tumor samples was determined using multi collector inductively coupled plasma-mass spectrometry (MC-ICP-MS), and their corresponding Cu and Zn plasma total concentrations using total reflection X-ray fluorescence (TXRF). Plasma concentrations of Cu were significantly higher (1346.1 ± 328.3 vs. 1060.5 ± 216.1 µg/L, p \u003c 0.0001), and Zn significantly lower (942.1 ± 205.2 vs. 1027.9 ± 151.4 µg/L, p \u003c 0.05) in thyroid cancer patients as compared to healthy controls (n = 50). Accordingly, the Cu/Zn ratio was significantly different between patients and controls (1.5 ± 0.4 vs. 1.0 ± 0.3, p \u003c 0.0001). Furthermore, the δ 65 Cu plasma levels of patients were significantly lower than healthy controls (p \u003c 0.0001), whereas thyroid tumor tissues presented high δ 65 Cu values. These results support the hypothesis that Cu isotopes and plasma trace elements may serve as suitable biomarkers of thyroid cancer diagnosis.","publication_date":{"day":8,"month":9,"year":2021,"errors":{}},"publication_name":"Frontiers in Medicine","grobid_abstract_attachment_id":118649789},"translated_abstract":null,"internal_url":"https://www.academia.edu/124421178/Copper_Isotopes_and_Copper_to_Zinc_Ratio_as_Possible_Biomarkers_for_Thyroid_Cancer","translated_internal_url":"","created_at":"2024-10-04T08:33:23.285-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[{"id":118649789,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649789/thumbnails/1.jpg","file_name":"pdf.pdf","download_url":"https://www.academia.edu/attachments/118649789/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Copper_Isotopes_and_Copper_to_Zinc_Ratio.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649789/pdf-libre.pdf?1728057726=\u0026response-content-disposition=attachment%3B+filename%3DCopper_Isotopes_and_Copper_to_Zinc_Ratio.pdf\u0026Expires=1733244891\u0026Signature=DKO1iU~05rPm0oAiCfMvEAiFM2nzxcKXmwfS~rB4cDQx95Ljyqk-2-Bcob6Iw7J6nffGUs7hHjxL01Vl--4mxvW63ZHbuu~OAH2zSxAdDtPqFFJUropgMl~diTAdeDGtP5UzlPc1zrX8oaCGkGThhNDxpb0k3TJNmZO0bh1~nonnjbdT1rKvOyqHF0nU8Z7IyE2G00fGLxFVsSa4-~KMSg14sv~OKLrN2Qi0COr9uKzlL5lSxMhIWPvm3hvZyAE9IOnJNDKXk2zddnahZF178VXQdj8emvSnbMXyisNDn9g2PgY-vfoxlYgU0-I2zFa4BgGOKtL1Xnw3Ozq8m1XsSg__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"slug":"Copper_Isotopes_and_Copper_to_Zinc_Ratio_as_Possible_Biomarkers_for_Thyroid_Cancer","translated_slug":"","page_count":9,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent 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Cancer","url":"https://www.academia.edu/Documents/in/Thyroid_Cancer"},{"id":65390,"name":"Internal Medicine","url":"https://www.academia.edu/Documents/in/Internal_Medicine"},{"id":80692,"name":"Copper","url":"https://www.academia.edu/Documents/in/Copper"},{"id":158165,"name":"Zinc","url":"https://www.academia.edu/Documents/in/Zinc"},{"id":338534,"name":"Biomarker","url":"https://www.academia.edu/Documents/in/Biomarker"},{"id":864424,"name":"Micronutrient","url":"https://www.academia.edu/Documents/in/Micronutrient"}],"urls":[{"id":44976079,"url":"https://www.frontiersin.org/articles/10.3389/fmed.2021.698167/pdf"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421177"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421177/Hydration_of_Hg_sup_2_sup_in_Aqueous_Solution_Studied_by_Neutron_Diffraction_with_Isotopic_Substitution"><img alt="Research paper thumbnail of Hydration of Hg<sup>2+</sup> in Aqueous Solution Studied by Neutron Diffraction with Isotopic Substitution" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421177/Hydration_of_Hg_sup_2_sup_in_Aqueous_Solution_Studied_by_Neutron_Diffraction_with_Isotopic_Substitution">Hydration of Hg<sup>2+</sup> in Aqueous Solution Studied by Neutron Diffraction with Isotopic Substitution</a></div><div class="wp-workCard_item"><span>Journal of Physical Chemistry A</span><span>, May 31, 2007</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The structural parameters of Hg2+ hydration were studied in 0.225 mol/L solutions of Hg2+ in DNO3...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The structural parameters of Hg2+ hydration were studied in 0.225 mol/L solutions of Hg2+ in DNO3/D2O by means of neutron diffraction with isotopic substitution of 199Hg for natHg. It was found that Hg2+ is hydrated by a first solvation shell of six water molecules. The observed Hg-O and Hg-H distances are equal to 2.48+/-0.05 and 3.08+/-0.05 A, respectively. The angle phi between the plane of the water molecule and the cation-water oxygen axis is approximately 35 degrees . The solvation of Hg2+ therefore mimics very closely that of Ca2+ (the Ca-O and Ca-H distances are 2.40 and 3.03 A, respectively) and helps to account for the extreme toxicity of mercury(II). We note also that the Hg-O distance obtained in the neutron diffraction experiment is larger by approximately 0.1 A than that obtained by X-ray diffraction. This difference is consistent with a shift of the oxygen electron density toward the mercury cation due to the covalency of the Hg-O interaction.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421177"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421177"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421177; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421177]").text(description); $(".js-view-count[data-work-id=124421177]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421177; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421177']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421177, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=124421177]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421177,"title":"Hydration of Hg\u003csup\u003e2+\u003c/sup\u003e in Aqueous Solution Studied by Neutron Diffraction with Isotopic Substitution","translated_title":"","metadata":{"abstract":"The structural parameters of Hg2+ hydration were studied in 0.225 mol/L solutions of Hg2+ in DNO3/D2O by means of neutron diffraction with isotopic substitution of 199Hg for natHg. It was found that Hg2+ is hydrated by a first solvation shell of six water molecules. The observed Hg-O and Hg-H distances are equal to 2.48+/-0.05 and 3.08+/-0.05 A, respectively. The angle phi between the plane of the water molecule and the cation-water oxygen axis is approximately 35 degrees . The solvation of Hg2+ therefore mimics very closely that of Ca2+ (the Ca-O and Ca-H distances are 2.40 and 3.03 A, respectively) and helps to account for the extreme toxicity of mercury(II). We note also that the Hg-O distance obtained in the neutron diffraction experiment is larger by approximately 0.1 A than that obtained by X-ray diffraction. This difference is consistent with a shift of the oxygen electron density toward the mercury cation due to the covalency of the Hg-O interaction.","publisher":"American Chemical Society","publication_date":{"day":31,"month":5,"year":2007,"errors":{}},"publication_name":"Journal of Physical Chemistry A"},"translated_abstract":"The structural parameters of Hg2+ hydration were studied in 0.225 mol/L solutions of Hg2+ in DNO3/D2O by means of neutron diffraction with isotopic substitution of 199Hg for natHg. It was found that Hg2+ is hydrated by a first solvation shell of six water molecules. The observed Hg-O and Hg-H distances are equal to 2.48+/-0.05 and 3.08+/-0.05 A, respectively. The angle phi between the plane of the water molecule and the cation-water oxygen axis is approximately 35 degrees . The solvation of Hg2+ therefore mimics very closely that of Ca2+ (the Ca-O and Ca-H distances are 2.40 and 3.03 A, respectively) and helps to account for the extreme toxicity of mercury(II). We note also that the Hg-O distance obtained in the neutron diffraction experiment is larger by approximately 0.1 A than that obtained by X-ray diffraction. 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href="https://www.academia.edu/124421206/Gentamicin_Montmorillonite_Intercalation_Compounds_as_an_Active_Component_of_Hydroxypropylmethylcellulose_Bionanocomposite_Films_with_Antimicrobial_Properties"><img alt="Research paper thumbnail of Gentamicin-Montmorillonite Intercalation Compounds as an Active Component of Hydroxypropylmethylcellulose Bionanocomposite Films with Antimicrobial Properties" class="work-thumbnail" src="https://attachments.academia-assets.com/118649806/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421206/Gentamicin_Montmorillonite_Intercalation_Compounds_as_an_Active_Component_of_Hydroxypropylmethylcellulose_Bionanocomposite_Films_with_Antimicrobial_Properties">Gentamicin-Montmorillonite Intercalation Compounds as an Active Component of Hydroxypropylmethylcellulose Bionanocomposite Films with Antimicrobial Properties</a></div><div class="wp-workCard_item"><span>Clays and Clay Minerals</span><span>, Oct 1, 2021</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="5fdb954344170f218042e3a840c7e5cd" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649806,"asset_id":124421206,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649806/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421206"><a 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"5fdb954344170f218042e3a840c7e5cd" } } $('.js-work-strip[data-work-id=124421206]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421206,"title":"Gentamicin-Montmorillonite Intercalation Compounds as an Active Component of Hydroxypropylmethylcellulose Bionanocomposite Films with Antimicrobial Properties","translated_title":"","metadata":{"publisher":"Springer Science+Business Media","grobid_abstract":"The present study introduces an overview of gentamicin-clay mineral systems for applications in biomedicine and then focuses on the development of a series of gentamicin/clay hybrid materials to be used as the bioactive phase of hydroxypropylmethylcellulose (HPMC) to produce bionanocomposite membranes possessing antimicrobial activity of interest in wound-dressing applications. Gentamicin (Gt) was adsorbed from aqueous solutions into a montmorillonite (Cloisite®-Na +) to produce intercalation compounds with tunable content of the antibiotic. The hybrids were characterized by CHN chemical analysis, energy-dispersive X-ray analysis, X-ray diffraction, Fouriertransform infrared spectroscopy, and thermogravimetric analysis, confirming the intercalation of Gt by an ion-exchange mechanism. The release of Gt from the hybrids was tested in water and in buffer solution to check their stability. Hybrids with various amounts of Gt were incorporated into a HPMC matrix at various loadings and processed as films by the casting method. The resulting Gt-clay/HPMC bionanocomposites were characterized by means of field-emission scanning electron microscopy, and were also evaluated for their wateradsorption and mechanical properties to confirm their suitability for wound-dressing applications. The antimicrobial activity of the bionanocomposite films was tested in vitro toward various microorganisms (Escherichia coli, Pseudomonas aeruginosa, Staphylococcus aureus, methicillin-resistant Staphylococcus aureus (MRSA), vancomycin-resistant Enterococcus faecium, Acinetobacter baumannii, and Klebsiella pneumonia), showing a complete bacterial reduction even in films with small Gt contents.","publication_date":{"day":1,"month":10,"year":2021,"errors":{}},"publication_name":"Clays and Clay 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});</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (true){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "acff5206ade6ae87e437049b8b988769" } } $('.js-work-strip[data-work-id=124421202]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421202,"title":"Nanoscale Ion Dynamics Control on Amorphous Calcium Carbonate Crystallization: Precise Control of Calcite Crystal 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Here, we performed X-ray photon correlation spectroscopy experiments on ACC which show that the amount of adsorbed water has a strong control over its diffusive dynamics. Results of crystallization experiments under conditions of controlled humidity indicate that the adsorbed water is enough to spark crystallization of calcite. A direct proportionality is found between the relative humidity of the environment and the final size of the calcite crystals. Different hypotheses are made to explain this result, with the confinement within the amorphous matrix being the main suspect of controlling the size of the crystallites. Control of water activity and water content is, therefore, a possible way to regulate biomineral crystallinity both in nature and for the design of functional biomimetic materials.","publication_date":{"day":4,"month":11,"year":2020,"errors":{}},"publication_name":"Journal of Physical Chemistry C","grobid_abstract_attachment_id":118649832},"translated_abstract":null,"internal_url":"https://www.academia.edu/124421202/Nanoscale_Ion_Dynamics_Control_on_Amorphous_Calcium_Carbonate_Crystallization_Precise_Control_of_Calcite_Crystal_Sizes","translated_internal_url":"","created_at":"2024-10-04T08:33:35.724-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[{"id":118649832,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649832/thumbnails/1.jpg","file_name":"acs.jpcc.pdf","download_url":"https://www.academia.edu/attachments/118649832/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Nanoscale_Ion_Dynamics_Control_on_Amorph.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649832/acs.jpcc-libre.pdf?1728057726=\u0026response-content-disposition=attachment%3B+filename%3DNanoscale_Ion_Dynamics_Control_on_Amorph.pdf\u0026Expires=1733244890\u0026Signature=S990tf4JuWuXGsZRkYTWahaMN0h3C~aJxiBZdWy7OpJaGRinbWDfThEDNFiMoZ9lWwmDCqiPF~GG2rkMLITmQ52KFcyeOW1etHFvNNYPIdzlXWhPzxCzQtcltEZD46ZwJBAB1fVppYqQvCi3wghtK4KF8lt5t3rkgr952QbmY8Li6Gt7WkDXfapdITs6YG9eCg1gxdLxf~G5joSlF4ULzjpYJT7Ya-rosUyg8INBn3ER3-nN6lxk4mCpFLnozFNKFiSXdi96FYEO7U1i~O5q~rRoNOT-V~-OEo66dcpzdcd6Us0x7ne97lAKoq56A0Wz1v-~2FBCa9bB~VyXO30IQQ__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"slug":"Nanoscale_Ion_Dynamics_Control_on_Amorphous_Calcium_Carbonate_Crystallization_Precise_Control_of_Calcite_Crystal_Sizes","translated_slug":"","page_count":12,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[{"id":118649832,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649832/thumbnails/1.jpg","file_name":"acs.jpcc.pdf","download_url":"https://www.academia.edu/attachments/118649832/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Nanoscale_Ion_Dynamics_Control_on_Amorph.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649832/acs.jpcc-libre.pdf?1728057726=\u0026response-content-disposition=attachment%3B+filename%3DNanoscale_Ion_Dynamics_Control_on_Amorph.pdf\u0026Expires=1733244890\u0026Signature=S990tf4JuWuXGsZRkYTWahaMN0h3C~aJxiBZdWy7OpJaGRinbWDfThEDNFiMoZ9lWwmDCqiPF~GG2rkMLITmQ52KFcyeOW1etHFvNNYPIdzlXWhPzxCzQtcltEZD46ZwJBAB1fVppYqQvCi3wghtK4KF8lt5t3rkgr952QbmY8Li6Gt7WkDXfapdITs6YG9eCg1gxdLxf~G5joSlF4ULzjpYJT7Ya-rosUyg8INBn3ER3-nN6lxk4mCpFLnozFNKFiSXdi96FYEO7U1i~O5q~rRoNOT-V~-OEo66dcpzdcd6Us0x7ne97lAKoq56A0Wz1v-~2FBCa9bB~VyXO30IQQ__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"research_interests":[{"id":48,"name":"Engineering","url":"https://www.academia.edu/Documents/in/Engineering"},{"id":511,"name":"Materials Science","url":"https://www.academia.edu/Documents/in/Materials_Science"},{"id":923,"name":"Technology","url":"https://www.academia.edu/Documents/in/Technology"},{"id":12597,"name":"Crystallization","url":"https://www.academia.edu/Documents/in/Crystallization"},{"id":91258,"name":"Carbonate","url":"https://www.academia.edu/Documents/in/Carbonate"},{"id":156638,"name":"Amorphous Calcium Carbonate","url":"https://www.academia.edu/Documents/in/Amorphous_Calcium_Carbonate"},{"id":205543,"name":"Calcite","url":"https://www.academia.edu/Documents/in/Calcite"},{"id":260118,"name":"CHEMICAL SCIENCES","url":"https://www.academia.edu/Documents/in/CHEMICAL_SCIENCES"},{"id":348756,"name":"Ion","url":"https://www.academia.edu/Documents/in/Ion"},{"id":630941,"name":"Calcium Carbonate","url":"https://www.academia.edu/Documents/in/Calcium_Carbonate"}],"urls":[{"id":44976103,"url":"https://doi.org/10.1021/acs.jpcc.0c08670"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421201"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421201/In_Vitro_Preparation_of_Actively_Maturing_Bovine_Articular_Cartilage_Explants_for_X_Ray_Phase_Contrast_Imaging"><img alt="Research paper thumbnail of In Vitro Preparation of Actively Maturing Bovine Articular Cartilage Explants for X-Ray Phase Contrast Imaging" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421201/In_Vitro_Preparation_of_Actively_Maturing_Bovine_Articular_Cartilage_Explants_for_X_Ray_Phase_Contrast_Imaging">In Vitro Preparation of Actively Maturing Bovine Articular Cartilage Explants for X-Ray Phase Contrast Imaging</a></div><div class="wp-workCard_item"><span>Journal of Visualized Experiments</span><span>, Jan 31, 2022</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">Understanding the mechanisms that underpin post-natal maturation of articular cartilage is of cru...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">Understanding the mechanisms that underpin post-natal maturation of articular cartilage is of crucial importance for designing the next generation of tissue engineering strategies and potentially repairing diseased or damaged cartilage. In general, postnatal maturation of the articular cartilage, which is a wholesale change in collagen structure and function of the tissue to accommodate growth of the organism, occurs over a timescale ranging from months to years. Conversely dissolution of the structural organization of the cartilage that also occurs over long timescales is the hallmark of tissue degeneration. Our ability to study these biological processes in detail have been enhanced by the findings that growth factors can induce precocious in vitro maturation of immature articular cartilage. The developmental and disease related changes that occur in the joint involve bone and cartilage and an ability to co-image these tissues would significantly increase our understanding of their intertwined roles. The simultaneous visualization of soft tissue, cartilage and bone changes is nowadays a challenge to overcome for conventional preclinical imaging modalities used for the joint disease follow-up. Three-dimensional X-ray Phase-Contrast Imaging methods (PCI) have been under perpetual developments for 20 years due to high performance for imaging low density objects and their ability to provide additional information compared to conventional X-ray imaging. In this protocol we detail the procedure used in our experiments from biopsy of the cartilage, generation of in vitro matured cartilage to data analysis of image collected using X-ray phase contrast imaging.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421201"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421201"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421201; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421201]").text(description); $(".js-view-count[data-work-id=124421201]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421201; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421201']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421201, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=124421201]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421201,"title":"In Vitro Preparation of Actively Maturing Bovine Articular Cartilage Explants for X-Ray Phase Contrast Imaging","translated_title":"","metadata":{"abstract":"Understanding the mechanisms that underpin post-natal maturation of articular cartilage is of crucial importance for designing the next generation of tissue engineering strategies and potentially repairing diseased or damaged cartilage. In general, postnatal maturation of the articular cartilage, which is a wholesale change in collagen structure and function of the tissue to accommodate growth of the organism, occurs over a timescale ranging from months to years. Conversely dissolution of the structural organization of the cartilage that also occurs over long timescales is the hallmark of tissue degeneration. Our ability to study these biological processes in detail have been enhanced by the findings that growth factors can induce precocious in vitro maturation of immature articular cartilage. The developmental and disease related changes that occur in the joint involve bone and cartilage and an ability to co-image these tissues would significantly increase our understanding of their intertwined roles. The simultaneous visualization of soft tissue, cartilage and bone changes is nowadays a challenge to overcome for conventional preclinical imaging modalities used for the joint disease follow-up. Three-dimensional X-ray Phase-Contrast Imaging methods (PCI) have been under perpetual developments for 20 years due to high performance for imaging low density objects and their ability to provide additional information compared to conventional X-ray imaging. In this protocol we detail the procedure used in our experiments from biopsy of the cartilage, generation of in vitro matured cartilage to data analysis of image collected using X-ray phase contrast imaging.","publisher":"MyJOVE","publication_date":{"day":31,"month":1,"year":2022,"errors":{}},"publication_name":"Journal of Visualized Experiments"},"translated_abstract":"Understanding the mechanisms that underpin post-natal maturation of articular cartilage is of crucial importance for designing the next generation of tissue engineering strategies and potentially repairing diseased or damaged cartilage. In general, postnatal maturation of the articular cartilage, which is a wholesale change in collagen structure and function of the tissue to accommodate growth of the organism, occurs over a timescale ranging from months to years. Conversely dissolution of the structural organization of the cartilage that also occurs over long timescales is the hallmark of tissue degeneration. Our ability to study these biological processes in detail have been enhanced by the findings that growth factors can induce precocious in vitro maturation of immature articular cartilage. The developmental and disease related changes that occur in the joint involve bone and cartilage and an ability to co-image these tissues would significantly increase our understanding of their intertwined roles. The simultaneous visualization of soft tissue, cartilage and bone changes is nowadays a challenge to overcome for conventional preclinical imaging modalities used for the joint disease follow-up. Three-dimensional X-ray Phase-Contrast Imaging methods (PCI) have been under perpetual developments for 20 years due to high performance for imaging low density objects and their ability to provide additional information compared to conventional X-ray imaging. In this protocol we detail the procedure used in our experiments from biopsy of the cartilage, generation of in vitro matured cartilage to data analysis of image collected using X-ray phase contrast imaging.","internal_url":"https://www.academia.edu/124421201/In_Vitro_Preparation_of_Actively_Maturing_Bovine_Articular_Cartilage_Explants_for_X_Ray_Phase_Contrast_Imaging","translated_internal_url":"","created_at":"2024-10-04T08:33:35.451-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"In_Vitro_Preparation_of_Actively_Maturing_Bovine_Articular_Cartilage_Explants_for_X_Ray_Phase_Contrast_Imaging","translated_slug":"","page_count":null,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[],"research_interests":[{"id":26327,"name":"Medicine","url":"https://www.academia.edu/Documents/in/Medicine"},{"id":78188,"name":"Cartilage","url":"https://www.academia.edu/Documents/in/Cartilage"},{"id":1146501,"name":"Articular Cartilage","url":"https://www.academia.edu/Documents/in/Articular_Cartilage"}],"urls":[{"id":44976102,"url":"https://doi.org/10.3791/61607"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421200"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421200/From_water_rock_interactions_to_the_DNA_a_review_of_selenium_issues"><img alt="Research paper thumbnail of From water-rock interactions to the DNA: a review of selenium issues" class="work-thumbnail" src="https://attachments.academia-assets.com/118649804/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421200/From_water_rock_interactions_to_the_DNA_a_review_of_selenium_issues">From water-rock interactions to the DNA: a review of selenium issues</a></div><div class="wp-workCard_item"><span>HAL (Le Centre pour la Communication Scientifique Directe)</span><span>, Oct 16, 2016</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="8d77db7193e466bb3246d1a48b2a8cc4" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649804,"asset_id":124421200,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649804/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421200"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421200"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421200; 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hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421196/Thermodynamic_stability_reversal_of_iron_sulfides_at_the_nanoscale_Insights_into_the_iron_sulfide_formation_in_low_temperature_aqueous_solution"><img alt="Research paper thumbnail of Thermodynamic stability reversal of iron sulfides at the nanoscale: Insights into the iron sulfide formation in low-temperature aqueous solution" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421196/Thermodynamic_stability_reversal_of_iron_sulfides_at_the_nanoscale_Insights_into_the_iron_sulfide_formation_in_low_temperature_aqueous_solution">Thermodynamic stability reversal of iron sulfides at the nanoscale: Insights into the iron sulfide formation in low-temperature aqueous solution</a></div><div class="wp-workCard_item"><span>Geochimica et Cosmochimica Acta</span><span>, Dec 1, 2022</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421196"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421196"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421196; window.Academia.workViewCountsFetcher.queue(workId, 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require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=124421196]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421196,"title":"Thermodynamic stability reversal of iron sulfides at the nanoscale: Insights into the iron sulfide formation in low-temperature aqueous solution","translated_title":"","metadata":{"publisher":"Elsevier BV","publication_date":{"day":1,"month":12,"year":2022,"errors":{}},"publication_name":"Geochimica et Cosmochimica 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Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[],"research_interests":[{"id":406,"name":"Geology","url":"https://www.academia.edu/Documents/in/Geology"},{"id":407,"name":"Geochemistry","url":"https://www.academia.edu/Documents/in/Geochemistry"},{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":125058,"name":"Nucleation","url":"https://www.academia.edu/Documents/in/Nucleation"},{"id":156578,"name":"Iron Sulfide","url":"https://www.academia.edu/Documents/in/Iron_Sulfide"},{"id":156636,"name":"Pyrite","url":"https://www.academia.edu/Documents/in/Pyrite"},{"id":494635,"name":"Mackinawite","url":"https://www.academia.edu/Documents/in/Mackinawite"},{"id":989646,"name":"Aqueous Solution","url":"https://www.academia.edu/Documents/in/Aqueous_Solution"},{"id":1235582,"name":"Sulfide","url":"https://www.academia.edu/Documents/in/Sulfide"}],"urls":[{"id":44976097,"url":"https://doi.org/10.1016/j.gca.2022.10.021"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421195"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421195/Water_Trapping_Dynamics_in_Carbohydrate_Populated_Smectite_Interlayer_Nanopores"><img alt="Research paper thumbnail of Water Trapping Dynamics in Carbohydrate-Populated Smectite Interlayer Nanopores" class="work-thumbnail" src="https://attachments.academia-assets.com/118649829/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421195/Water_Trapping_Dynamics_in_Carbohydrate_Populated_Smectite_Interlayer_Nanopores">Water Trapping Dynamics in Carbohydrate-Populated Smectite Interlayer Nanopores</a></div><div class="wp-workCard_item"><span>Journal of Physical Chemistry C</span><span>, Nov 4, 2019</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="6ff4e66584043509bc8647a219a04fe5" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649829,"asset_id":124421195,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649829/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span 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_.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "6ff4e66584043509bc8647a219a04fe5" } } $('.js-work-strip[data-work-id=124421195]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421195,"title":"Water Trapping Dynamics in Carbohydrate-Populated Smectite Interlayer Nanopores","translated_title":"","metadata":{"publisher":"American Chemical Society","ai_title_tag":"Carbohydrate Effects on Water Dynamics in Smectite Nanopores","grobid_abstract":"Smectite-type clays play a critical role in the trapping of fluids within soil and atmospheric nanoparticles. The hydrodynamics of cationsaturated smectite nanopores are well documented. However, little is known about the influence of small organic compounds. Here we investigate the effects of carbohydrates (glucose and cellobiose), representing an important class of organic compounds, on the hydration and nanopore structures of montmorillonite, a prototypical smectite. To achieve the same amount of adsorbed water, higher relative humidity was required in the presence of the adsorbed carbohydrates than with the clay alone. The decrease in the characteristic micropore water adsorption with the clay−carbohydrate aggregates implied that water adsorption was constrained within the clay nanopore regions. The presence of carbohydrates promoted water retention as a function of gradual decrease in moisture content. Moisture-dependent X-ray diffraction patterns determined that, relative to the mineral alone, greater nanopore sizes were preserved in the presence of the carbohydrates, despite severe dehydration that is expected to induce clay nanopore collapse. Fourier-transform infrared spectroscopy captured disruption in the population of exchangeable waters within the carbohydrate-populated clay nanopores, with some agreement with the measured water-desorption profiling. These new findings demonstrate that carbohydrates can restructure smectite interlayer nanopores and water trapping dynamics.","publication_date":{"day":4,"month":11,"year":2019,"errors":{}},"publication_name":"Journal of Physical Chemistry C","grobid_abstract_attachment_id":118649829},"translated_abstract":null,"internal_url":"https://www.academia.edu/124421195/Water_Trapping_Dynamics_in_Carbohydrate_Populated_Smectite_Interlayer_Nanopores","translated_internal_url":"","created_at":"2024-10-04T08:33:29.781-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[{"id":118649829,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649829/thumbnails/1.jpg","file_name":"acs.jpcc.9b0924620241004-1-t42xja.pdf","download_url":"https://www.academia.edu/attachments/118649829/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Water_Trapping_Dynamics_in_Carbohydrate.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649829/acs.jpcc.9b0924620241004-1-t42xja-libre.pdf?1728057724=\u0026response-content-disposition=attachment%3B+filename%3DWater_Trapping_Dynamics_in_Carbohydrate.pdf\u0026Expires=1733244890\u0026Signature=YYB2smYgTv6zrra3brUYV8qAGo3a~6EUrtz0CEfERMx~Umtj9URjqCZlwXRms1I~Ic~nvAikuEN08Wkaw7WFsm-7Omj1hoUTVoPAZl9DVyr1jMv-5tvRL1pgWPHJGpDV229NuIslOfebowyToCvHZEBOzgt0eUmCpsbwofHfxytMdhyAzBS4OPXbold-v2-FOPtyrqJeZVM7Y6exM-aOQ9yoRe7TIVLbcx7j3n~Cxm81r2OZ9d2dWDoul7RM3wRYVwL6ui7U4rBVgldNloo2PvMuPjumOBSOVkWFlHp0nN2H5f~fXqrXovRnrXib98hPH9HnWDfWQeqFsLtEjGZp-g__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"slug":"Water_Trapping_Dynamics_in_Carbohydrate_Populated_Smectite_Interlayer_Nanopores","translated_slug":"","page_count":12,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[{"id":118649829,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649829/thumbnails/1.jpg","file_name":"acs.jpcc.9b0924620241004-1-t42xja.pdf","download_url":"https://www.academia.edu/attachments/118649829/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MCw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Water_Trapping_Dynamics_in_Carbohydrate.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649829/acs.jpcc.9b0924620241004-1-t42xja-libre.pdf?1728057724=\u0026response-content-disposition=attachment%3B+filename%3DWater_Trapping_Dynamics_in_Carbohydrate.pdf\u0026Expires=1733244890\u0026Signature=YYB2smYgTv6zrra3brUYV8qAGo3a~6EUrtz0CEfERMx~Umtj9URjqCZlwXRms1I~Ic~nvAikuEN08Wkaw7WFsm-7Omj1hoUTVoPAZl9DVyr1jMv-5tvRL1pgWPHJGpDV229NuIslOfebowyToCvHZEBOzgt0eUmCpsbwofHfxytMdhyAzBS4OPXbold-v2-FOPtyrqJeZVM7Y6exM-aOQ9yoRe7TIVLbcx7j3n~Cxm81r2OZ9d2dWDoul7RM3wRYVwL6ui7U4rBVgldNloo2PvMuPjumOBSOVkWFlHp0nN2H5f~fXqrXovRnrXib98hPH9HnWDfWQeqFsLtEjGZp-g__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"research_interests":[{"id":48,"name":"Engineering","url":"https://www.academia.edu/Documents/in/Engineering"},{"id":72,"name":"Chemical Engineering","url":"https://www.academia.edu/Documents/in/Chemical_Engineering"},{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":923,"name":"Technology","url":"https://www.academia.edu/Documents/in/Technology"},{"id":21728,"name":"Clay Minerals","url":"https://www.academia.edu/Documents/in/Clay_Minerals"},{"id":22300,"name":"Chemical Physics","url":"https://www.academia.edu/Documents/in/Chemical_Physics"},{"id":39752,"name":"Adsorption","url":"https://www.academia.edu/Documents/in/Adsorption"},{"id":260118,"name":"CHEMICAL SCIENCES","url":"https://www.academia.edu/Documents/in/CHEMICAL_SCIENCES"},{"id":334138,"name":"Montmorillonite","url":"https://www.academia.edu/Documents/in/Montmorillonite"},{"id":456380,"name":"Trapping","url":"https://www.academia.edu/Documents/in/Trapping"},{"id":3478741,"name":"Nanopore","url":"https://www.academia.edu/Documents/in/Nanopore"}],"urls":[{"id":44976096,"url":"https://doi.org/10.1021/acs.jpcc.9b09246"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421194"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421194/Acid_volatile_sulfides_and_simultaneously_extracted_metals_A_new_miniaturized_purge_and_trap_system_for_laboratory_and_field_measurements"><img alt="Research paper thumbnail of Acid volatile sulfides and simultaneously extracted metals: A new miniaturized ‘purge and trap’ system for laboratory and field measurements" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421194/Acid_volatile_sulfides_and_simultaneously_extracted_metals_A_new_miniaturized_purge_and_trap_system_for_laboratory_and_field_measurements">Acid volatile sulfides and simultaneously extracted metals: A new miniaturized ‘purge and trap’ system for laboratory and field measurements</a></div><div class="wp-workCard_item"><span>Talanta</span><span>, Oct 1, 2021</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">In natural environments, Acid Volatile Sulfides (AVS) contained in anoxic waters or sediments, ar...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">In natural environments, Acid Volatile Sulfides (AVS) contained in anoxic waters or sediments, are composed of dissolved sulfides and neo-formed sulfides colloids or particles. Under acidic addition, AVS emit hydrogen sulfide gas and release the so-called simultaneously extracted metals (SEM). The measurement of AVS coupled with that of the SEM enables to evaluate the metal trapping capacity of sulfides in the environment. Because AVS are extremely reactive to oxidation, the most accurate methodology to quantify AVS and SEM requires to be able to process the samples extraction on-site, directly after sampling and avoiding oxygen exposure. However, most of available systems are based on glassware &#39;purge and trap&#39; techniques developed for the laboratory and are not often adapted to field studies. In these systems, AVS extraction time can range from 30 min to 3 h with relative standard deviation from 7 to 44%. In this study, we developed a new &#39;purge and trap&#39; system designed for both laboratory use and field AVS/SEM extractions. The system is optimized with a shortened extraction time, miniaturized, unbreakable, easy and reproducible to develop parallel extraction benches. Analytical yields, precision and stability have been improved, allowing to reduce the extraction time to 1 h with an absolute quantification limit of 0.12 μmol S(-II) with a relative standard deviation between 7 and 11% and under a complete extraction efficiency.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421194"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421194"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421194; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421194]").text(description); $(".js-view-count[data-work-id=124421194]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421194; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421194']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421194, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=124421194]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421194,"title":"Acid volatile sulfides and simultaneously extracted metals: A new miniaturized ‘purge and trap’ system for laboratory and field measurements","translated_title":"","metadata":{"abstract":"In natural environments, Acid Volatile Sulfides (AVS) contained in anoxic waters or sediments, are composed of dissolved sulfides and neo-formed sulfides colloids or particles. Under acidic addition, AVS emit hydrogen sulfide gas and release the so-called simultaneously extracted metals (SEM). The measurement of AVS coupled with that of the SEM enables to evaluate the metal trapping capacity of sulfides in the environment. Because AVS are extremely reactive to oxidation, the most accurate methodology to quantify AVS and SEM requires to be able to process the samples extraction on-site, directly after sampling and avoiding oxygen exposure. However, most of available systems are based on glassware \u0026#39;purge and trap\u0026#39; techniques developed for the laboratory and are not often adapted to field studies. In these systems, AVS extraction time can range from 30 min to 3 h with relative standard deviation from 7 to 44%. In this study, we developed a new \u0026#39;purge and trap\u0026#39; system designed for both laboratory use and field AVS/SEM extractions. The system is optimized with a shortened extraction time, miniaturized, unbreakable, easy and reproducible to develop parallel extraction benches. Analytical yields, precision and stability have been improved, allowing to reduce the extraction time to 1 h with an absolute quantification limit of 0.12 μmol S(-II) with a relative standard deviation between 7 and 11% and under a complete extraction efficiency.","publisher":"Elsevier BV","publication_date":{"day":1,"month":10,"year":2021,"errors":{}},"publication_name":"Talanta"},"translated_abstract":"In natural environments, Acid Volatile Sulfides (AVS) contained in anoxic waters or sediments, are composed of dissolved sulfides and neo-formed sulfides colloids or particles. Under acidic addition, AVS emit hydrogen sulfide gas and release the so-called simultaneously extracted metals (SEM). The measurement of AVS coupled with that of the SEM enables to evaluate the metal trapping capacity of sulfides in the environment. Because AVS are extremely reactive to oxidation, the most accurate methodology to quantify AVS and SEM requires to be able to process the samples extraction on-site, directly after sampling and avoiding oxygen exposure. However, most of available systems are based on glassware \u0026#39;purge and trap\u0026#39; techniques developed for the laboratory and are not often adapted to field studies. In these systems, AVS extraction time can range from 30 min to 3 h with relative standard deviation from 7 to 44%. In this study, we developed a new \u0026#39;purge and trap\u0026#39; system designed for both laboratory use and field AVS/SEM extractions. The system is optimized with a shortened extraction time, miniaturized, unbreakable, easy and reproducible to develop parallel extraction benches. Analytical yields, precision and stability have been improved, allowing to reduce the extraction time to 1 h with an absolute quantification limit of 0.12 μmol S(-II) with a relative standard deviation between 7 and 11% and under a complete extraction efficiency.","internal_url":"https://www.academia.edu/124421194/Acid_volatile_sulfides_and_simultaneously_extracted_metals_A_new_miniaturized_purge_and_trap_system_for_laboratory_and_field_measurements","translated_internal_url":"","created_at":"2024-10-04T08:33:28.847-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"Acid_volatile_sulfides_and_simultaneously_extracted_metals_A_new_miniaturized_purge_and_trap_system_for_laboratory_and_field_measurements","translated_slug":"","page_count":null,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":524,"name":"Analytical Chemistry","url":"https://www.academia.edu/Documents/in/Analytical_Chemistry"},{"id":26327,"name":"Medicine","url":"https://www.academia.edu/Documents/in/Medicine"},{"id":139317,"name":"Purge","url":"https://www.academia.edu/Documents/in/Purge"},{"id":476869,"name":"Hydrogen Sulfide","url":"https://www.academia.edu/Documents/in/Hydrogen_Sulfide"}],"urls":[{"id":44976095,"url":"https://doi.org/10.1016/j.talanta.2021.122490"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421191"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421191/Interplay_of_S_and_As_in_Mekong_Delta_sediments_during_redox_oscillations"><img alt="Research paper thumbnail of Interplay of S and As in Mekong Delta sediments during redox oscillations" class="work-thumbnail" src="https://attachments.academia-assets.com/118649828/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421191/Interplay_of_S_and_As_in_Mekong_Delta_sediments_during_redox_oscillations">Interplay of S and As in Mekong Delta sediments during redox oscillations</a></div><div class="wp-workCard_item"><span>Geoscience frontiers</span><span>, Sep 1, 2019</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="b289616a965d9666438d51c8ab401a45" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649828,"asset_id":124421191,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649828/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421191"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421191"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421191; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421191]").text(description); $(".js-view-count[data-work-id=124421191]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421191; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421191']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421191, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (true){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "b289616a965d9666438d51c8ab401a45" } } $('.js-work-strip[data-work-id=124421191]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421191,"title":"Interplay of S and As in Mekong Delta sediments during redox oscillations","translated_title":"","metadata":{"publisher":"Elsevier BV","grobid_abstract":"The cumulative effects of periodic redox cycling on the mobility of As, Fe, and S from alluvial sediment to groundwater were investigated in bioreactor experiments. Two particular sediments from the alluvial floodplain of the Mekong Delta River were investigated: Matrix A (14 m deep) had a higher pyrite concentration than matrix B (7 m deep) sediments. Gypsum was present in matrix B but absent in matrix A. In the reactors, the sediment suspensions were supplemented with As(III) and SO 4 2À , and were subjected to three full-redox cycles entailing phases of nitrogen/CO 2 , compressed air sparging, and cellobiose addition. Major differences in As concentration and speciation were observed upon redox cycling. Evidences support the fact that initial sediment composition is the main factor controlling arsenic release and its speciation during the redox cycles. Indeed, a high pyrite content associated with a low SO 4 2À content resulted in an increase in dissolved As concentrations, mainly in the form of As(III), after anoxic half-cycles; whereas a decrease in As concentrations mainly in the form of As(V), was instead observed after oxic half-cycles. In addition, oxic conditions were found to be responsible for pyrite and arsenian pyrite oxidation, increasing the As pool available for mobilization. The same processes seem to occur in sediment with the presence of gypsum, but, in this case, dissolved As were sequestered by biotic or abiotic redox reactions occurring in the FeeS system, and by specific physico-chemical condition (e.g. pH). The contrasting results obtained for two sediments sampled from the same core show that many complexes and entangled factors are at work, and further refinement is needed to explain the spatial and temporal variability of As release to groundwater of the Mekong River Delta (Vietnam).","publication_date":{"day":1,"month":9,"year":2019,"errors":{}},"publication_name":"Geoscience frontiers","grobid_abstract_attachment_id":118649828},"translated_abstract":null,"internal_url":"https://www.academia.edu/124421191/Interplay_of_S_and_As_in_Mekong_Delta_sediments_during_redox_oscillations","translated_internal_url":"","created_at":"2024-10-04T08:33:28.144-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[{"id":118649828,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649828/thumbnails/1.jpg","file_name":"1-s2.0-S1674987118300872-main.pdf","download_url":"https://www.academia.edu/attachments/118649828/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Interplay_of_S_and_As_in_Mekong_Delta_se.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649828/1-s2.0-S1674987118300872-main-libre.pdf?1728057720=\u0026response-content-disposition=attachment%3B+filename%3DInterplay_of_S_and_As_in_Mekong_Delta_se.pdf\u0026Expires=1733244891\u0026Signature=RjpcUGy~fF5ZPmlAZjPYCJ15llPWN~HgS1hEQmdZPKuDmvSunbB0uvefBAoz0nZEXs5bKNZ6MZjgkOQD9P~9Eb6w0s9WJEldAYmF~D0HGmJpKM8gp411u-7eGc6BamTlGf06TYlMtjWpq94BM839Sd-gz9qWlXXejAsDJik7ZhrR5YhtBsMaFVq36qSEqz2VmS~3CzbsznBrQiiGsHbSopNTMQf15whtQgFAUHaidI9-EDFGoIhXqsCHq~Hkl43~HYIvE4K88dUR6eT33nhw1ld-Z~wdL5c7Oc7kWtWcBsSt9ZiUeYK5mpWHyquQBzUaHvokSkYWD-m9waDCwXB33g__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"slug":"Interplay_of_S_and_As_in_Mekong_Delta_sediments_during_redox_oscillations","translated_slug":"","page_count":16,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[{"id":118649828,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649828/thumbnails/1.jpg","file_name":"1-s2.0-S1674987118300872-main.pdf","download_url":"https://www.academia.edu/attachments/118649828/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Interplay_of_S_and_As_in_Mekong_Delta_se.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649828/1-s2.0-S1674987118300872-main-libre.pdf?1728057720=\u0026response-content-disposition=attachment%3B+filename%3DInterplay_of_S_and_As_in_Mekong_Delta_se.pdf\u0026Expires=1733244891\u0026Signature=RjpcUGy~fF5ZPmlAZjPYCJ15llPWN~HgS1hEQmdZPKuDmvSunbB0uvefBAoz0nZEXs5bKNZ6MZjgkOQD9P~9Eb6w0s9WJEldAYmF~D0HGmJpKM8gp411u-7eGc6BamTlGf06TYlMtjWpq94BM839Sd-gz9qWlXXejAsDJik7ZhrR5YhtBsMaFVq36qSEqz2VmS~3CzbsznBrQiiGsHbSopNTMQf15whtQgFAUHaidI9-EDFGoIhXqsCHq~Hkl43~HYIvE4K88dUR6eT33nhw1ld-Z~wdL5c7Oc7kWtWcBsSt9ZiUeYK5mpWHyquQBzUaHvokSkYWD-m9waDCwXB33g__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"research_interests":[{"id":406,"name":"Geology","url":"https://www.academia.edu/Documents/in/Geology"},{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":15836,"name":"Environmental Chemistry","url":"https://www.academia.edu/Documents/in/Environmental_Chemistry"},{"id":142977,"name":"Delta","url":"https://www.academia.edu/Documents/in/Delta"},{"id":156636,"name":"Pyrite","url":"https://www.academia.edu/Documents/in/Pyrite"},{"id":192294,"name":"Sediment","url":"https://www.academia.edu/Documents/in/Sediment"},{"id":859634,"name":"Mekong Delta","url":"https://www.academia.edu/Documents/in/Mekong_Delta"},{"id":1009236,"name":"Redox","url":"https://www.academia.edu/Documents/in/Redox"},{"id":1216203,"name":"Earth Science","url":"https://www.academia.edu/Documents/in/Earth_Science"}],"urls":[{"id":44976093,"url":"https://doi.org/10.1016/j.gsf.2018.03.008"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421189"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421189/Effects_of_redox_oscillations_on_the_phosphogypsum_waste_in_an_estuarine_salt_marsh_system"><img alt="Research paper thumbnail of Effects of redox oscillations on the phosphogypsum waste in an estuarine salt-marsh system" class="work-thumbnail" src="https://attachments.academia-assets.com/118649802/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421189/Effects_of_redox_oscillations_on_the_phosphogypsum_waste_in_an_estuarine_salt_marsh_system">Effects of redox oscillations on the phosphogypsum waste in an estuarine salt-marsh system</a></div><div class="wp-workCard_item"><span>Chemosphere</span><span>, Mar 1, 2020</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="791959471469dbb0120dd141a86e6625" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649802,"asset_id":124421189,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649802/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421189"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421189"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421189; 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dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "791959471469dbb0120dd141a86e6625" } } $('.js-work-strip[data-work-id=124421189]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421189,"title":"Effects of redox oscillations on the phosphogypsum waste in an estuarine salt-marsh system","translated_title":"","metadata":{"publisher":"Elsevier BV","grobid_abstract":"Salt marshes are natural deposits of heavy metals in estuarine systems, where sulphide precipitation associated with redox changes often results in a natural attenuation of contamination. In the present study, we focus on the effects of variable redox conditions imposed to a highly-polluted phosphogypsum stack that is directly piled over the salt marsh soil in the Tinto River estuary (Huelva, Spain). The behaviour of contaminants is evaluated in the phosphogypsum waste and in the marsh basement, separately, in controlled, experimentally-induced oscillating redox conditions. The results revealed that Fe, and to a lesser extent S, control most precipitation/dissolution processes. Ferric iron precipitates in the form of phosphates and oxyhydroxides, while metal sulphide precipitation is insignificant and appears to be prevented by the abundant formation of Fe phosphates. An antagonistic evolution with changing redox conditions was observed for the remaining contaminants such as Zn, As, Cd and U, which remained mobile in solution during most of experimental run. Therefore, these findings revealed that high concentrations of phosphates inhibit the typical processes of immobilization of pollutants in salt-marshes which highlights the elevated contaminant potential of phosphogypsum wastes on coastal environments.","publication_date":{"day":1,"month":3,"year":2020,"errors":{}},"publication_name":"Chemosphere","grobid_abstract_attachment_id":118649802},"translated_abstract":null,"internal_url":"https://www.academia.edu/124421189/Effects_of_redox_oscillations_on_the_phosphogypsum_waste_in_an_estuarine_salt_marsh_system","translated_internal_url":"","created_at":"2024-10-04T08:33:27.796-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[{"id":118649802,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649802/thumbnails/1.jpg","file_name":"document.pdf","download_url":"https://www.academia.edu/attachments/118649802/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Effects_of_redox_oscillations_on_the_pho.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649802/document-libre.pdf?1728057748=\u0026response-content-disposition=attachment%3B+filename%3DEffects_of_redox_oscillations_on_the_pho.pdf\u0026Expires=1733244891\u0026Signature=GKK2w52utd6LMeflx3pAuTmv1jB8zG86QVxdUfl4PneTPTR9TNhdorGCiVJ3PFuFNavaXpPFyYh8ZOsOR--f8lUjWqy~f~gvvbimasjWhGr92lQSETYe0CrMEQixlaCIdreWo-FW5LdVQQHx17hVJYm-4m3e5AofBsuxJMkmB4CDKNLBbkEb9MjWS0FqloeJMxFmeyHq0zSTZvzxLley9h~W3dFA7A~1coRhI~aQyYnDSq0YvhYBU5C5~kno3W5-h~41H2lyh3ORTDGyFF0KtmthS8bbcS8ioVNxIwAedBh97JbCeo7hgZY26qVOm4pJNUrF0Ki5gmJjiN5E1td0SQ__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"slug":"Effects_of_redox_oscillations_on_the_phosphogypsum_waste_in_an_estuarine_salt_marsh_system","translated_slug":"","page_count":39,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[{"id":118649802,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/118649802/thumbnails/1.jpg","file_name":"document.pdf","download_url":"https://www.academia.edu/attachments/118649802/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Effects_of_redox_oscillations_on_the_pho.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/118649802/document-libre.pdf?1728057748=\u0026response-content-disposition=attachment%3B+filename%3DEffects_of_redox_oscillations_on_the_pho.pdf\u0026Expires=1733244891\u0026Signature=GKK2w52utd6LMeflx3pAuTmv1jB8zG86QVxdUfl4PneTPTR9TNhdorGCiVJ3PFuFNavaXpPFyYh8ZOsOR--f8lUjWqy~f~gvvbimasjWhGr92lQSETYe0CrMEQixlaCIdreWo-FW5LdVQQHx17hVJYm-4m3e5AofBsuxJMkmB4CDKNLBbkEb9MjWS0FqloeJMxFmeyHq0zSTZvzxLley9h~W3dFA7A~1coRhI~aQyYnDSq0YvhYBU5C5~kno3W5-h~41H2lyh3ORTDGyFF0KtmthS8bbcS8ioVNxIwAedBh97JbCeo7hgZY26qVOm4pJNUrF0Ki5gmJjiN5E1td0SQ__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":15836,"name":"Environmental Chemistry","url":"https://www.academia.edu/Documents/in/Environmental_Chemistry"},{"id":26327,"name":"Medicine","url":"https://www.academia.edu/Documents/in/Medicine"},{"id":28235,"name":"Multidisciplinary","url":"https://www.academia.edu/Documents/in/Multidisciplinary"},{"id":291658,"name":"Precipitation","url":"https://www.academia.edu/Documents/in/Precipitation"},{"id":576179,"name":"Salt marsh","url":"https://www.academia.edu/Documents/in/Salt_marsh"},{"id":1009236,"name":"Redox","url":"https://www.academia.edu/Documents/in/Redox"},{"id":1129780,"name":"Phosphogypsum","url":"https://www.academia.edu/Documents/in/Phosphogypsum"}],"urls":[{"id":44976090,"url":"https://hal.science/hal-03043993/document"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421179"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421179/The_influence_of_pH_and_reaction_time_on_the_formation_of_FeSe_sub_2_sub_upon_selenite_reduction_by_nano_sized_pyrite_greigite"><img alt="Research paper thumbnail of The influence of pH and reaction time on the formation of FeSe<sub>2</sub> upon selenite reduction by nano-sized pyrite-greigite" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421179/The_influence_of_pH_and_reaction_time_on_the_formation_of_FeSe_sub_2_sub_upon_selenite_reduction_by_nano_sized_pyrite_greigite">The influence of pH and reaction time on the formation of FeSe<sub>2</sub> upon selenite reduction by nano-sized pyrite-greigite</a></div><div class="wp-workCard_item"><span>Radiochimica Acta</span><span>, Jun 8, 2016</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The influence of pH and reaction time on the formation of FeSe2 by reductive precipitation of Se(...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The influence of pH and reaction time on the formation of FeSe2 by reductive precipitation of Se(IV) with nano-sized pyrite-greigite was investigated. Reductive precipitation is an effective method of attenuating the mobility of 79Se, which is foreseen to be a dangerous radioisotope for the geological disposal of high-level radioactive waste (HLW). The results indicated that Se(0)was formed at pH &amp;lt;4.05, whereas, at pH &amp;gt; 6.07, considerable amount of FeSe2 was formed along with Se(0). These observations are in agreement with the thermodynamic predictions reported in this work. Furthermore, the formation of FeSe2 was found to continue by increasing the reaction time, indicating that the Se(0) formed in the early reaction stage is gradually transformed to FeSe2 upon the depletion of aqueous Se(IV). Since FeSe2 has a stronger reactivity than pyrite, it was proposed that greigite, rather than pyrite, was responsible for the formation of FeSe2. The findings in this study are of interest for key geochemical processes governing the mobility of toxic 79Se in the environment in presence of iron sulfides.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421179"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421179"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421179; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421179]").text(description); $(".js-view-count[data-work-id=124421179]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421179; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421179']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421179, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=124421179]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421179,"title":"The influence of pH and reaction time on the formation of FeSe\u003csub\u003e2\u003c/sub\u003e upon selenite reduction by nano-sized pyrite-greigite","translated_title":"","metadata":{"abstract":"The influence of pH and reaction time on the formation of FeSe2 by reductive precipitation of Se(IV) with nano-sized pyrite-greigite was investigated. Reductive precipitation is an effective method of attenuating the mobility of 79Se, which is foreseen to be a dangerous radioisotope for the geological disposal of high-level radioactive waste (HLW). The results indicated that Se(0)was formed at pH \u0026amp;lt;4.05, whereas, at pH \u0026amp;gt; 6.07, considerable amount of FeSe2 was formed along with Se(0). These observations are in agreement with the thermodynamic predictions reported in this work. Furthermore, the formation of FeSe2 was found to continue by increasing the reaction time, indicating that the Se(0) formed in the early reaction stage is gradually transformed to FeSe2 upon the depletion of aqueous Se(IV). Since FeSe2 has a stronger reactivity than pyrite, it was proposed that greigite, rather than pyrite, was responsible for the formation of FeSe2. The findings in this study are of interest for key geochemical processes governing the mobility of toxic 79Se in the environment in presence of iron sulfides.","publisher":"R. Oldenbourg Verlag","publication_date":{"day":8,"month":6,"year":2016,"errors":{}},"publication_name":"Radiochimica Acta"},"translated_abstract":"The influence of pH and reaction time on the formation of FeSe2 by reductive precipitation of Se(IV) with nano-sized pyrite-greigite was investigated. Reductive precipitation is an effective method of attenuating the mobility of 79Se, which is foreseen to be a dangerous radioisotope for the geological disposal of high-level radioactive waste (HLW). The results indicated that Se(0)was formed at pH \u0026amp;lt;4.05, whereas, at pH \u0026amp;gt; 6.07, considerable amount of FeSe2 was formed along with Se(0). These observations are in agreement with the thermodynamic predictions reported in this work. Furthermore, the formation of FeSe2 was found to continue by increasing the reaction time, indicating that the Se(0) formed in the early reaction stage is gradually transformed to FeSe2 upon the depletion of aqueous Se(IV). Since FeSe2 has a stronger reactivity than pyrite, it was proposed that greigite, rather than pyrite, was responsible for the formation of FeSe2. The findings in this study are of interest for key geochemical processes governing the mobility of toxic 79Se in the environment in presence of iron sulfides.","internal_url":"https://www.academia.edu/124421179/The_influence_of_pH_and_reaction_time_on_the_formation_of_FeSe_sub_2_sub_upon_selenite_reduction_by_nano_sized_pyrite_greigite","translated_internal_url":"","created_at":"2024-10-04T08:33:23.547-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"The_influence_of_pH_and_reaction_time_on_the_formation_of_FeSe_sub_2_sub_upon_selenite_reduction_by_nano_sized_pyrite_greigite","translated_slug":"","page_count":null,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":156636,"name":"Pyrite","url":"https://www.academia.edu/Documents/in/Pyrite"},{"id":214346,"name":"Greigite","url":"https://www.academia.edu/Documents/in/Greigite"},{"id":291658,"name":"Precipitation","url":"https://www.academia.edu/Documents/in/Precipitation"}],"urls":[{"id":44976088,"url":"https://doi.org/10.1515/ract-2015-2496"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="124421178"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/124421178/Copper_Isotopes_and_Copper_to_Zinc_Ratio_as_Possible_Biomarkers_for_Thyroid_Cancer"><img alt="Research paper thumbnail of Copper Isotopes and Copper to Zinc Ratio as Possible Biomarkers for Thyroid Cancer" class="work-thumbnail" src="https://attachments.academia-assets.com/118649789/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421178/Copper_Isotopes_and_Copper_to_Zinc_Ratio_as_Possible_Biomarkers_for_Thyroid_Cancer">Copper Isotopes and Copper to Zinc Ratio as Possible Biomarkers for Thyroid Cancer</a></div><div class="wp-workCard_item"><span>Frontiers in Medicine</span><span>, Sep 8, 2021</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="426a9efaab89544b4bd1632a25d367c6" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":118649789,"asset_id":124421178,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/118649789/download_file?st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&st=MTczMzI0MTI5MSw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="124421178"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="124421178"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 124421178; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=124421178]").text(description); $(".js-view-count[data-work-id=124421178]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 124421178; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='124421178']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 124421178, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (true){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "426a9efaab89544b4bd1632a25d367c6" } } $('.js-work-strip[data-work-id=124421178]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":124421178,"title":"Copper Isotopes and Copper to Zinc Ratio as Possible Biomarkers for Thyroid Cancer","translated_title":"","metadata":{"publisher":"Frontiers Media","grobid_abstract":"Thyroid cancer is the most common endocrine cancer. There is no systematic screening for such cancer, and the current challenge is to find potential biomarkers to facilitate an early diagnosis. Copper (Cu) and zinc (Zn) are essential micronutrients involved in the proper functioning of the thyroid gland, and changes in their concentrations have been observed in the development of cancer. Previous studies have highlighted the potential 65 Cu/ 63 Cu ratio (δ 65 Cu) to be a cancer biomarker. This study tests its sensitivity on plasma samples (n = 46) of Algerian patients with papillary thyroid carcinoma and a set of corresponding biopsies (n = 11). The δ 65 Cu ratio in blood and tumor samples was determined using multi collector inductively coupled plasma-mass spectrometry (MC-ICP-MS), and their corresponding Cu and Zn plasma total concentrations using total reflection X-ray fluorescence (TXRF). Plasma concentrations of Cu were significantly higher (1346.1 ± 328.3 vs. 1060.5 ± 216.1 µg/L, p \u003c 0.0001), and Zn significantly lower (942.1 ± 205.2 vs. 1027.9 ± 151.4 µg/L, p \u003c 0.05) in thyroid cancer patients as compared to healthy controls (n = 50). Accordingly, the Cu/Zn ratio was significantly different between patients and controls (1.5 ± 0.4 vs. 1.0 ± 0.3, p \u003c 0.0001). Furthermore, the δ 65 Cu plasma levels of patients were significantly lower than healthy controls (p \u003c 0.0001), whereas thyroid tumor tissues presented high δ 65 Cu values. 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href="https://www.academia.edu/124421177/Hydration_of_Hg_sup_2_sup_in_Aqueous_Solution_Studied_by_Neutron_Diffraction_with_Isotopic_Substitution"><img alt="Research paper thumbnail of Hydration of Hg<sup>2+</sup> in Aqueous Solution Studied by Neutron Diffraction with Isotopic Substitution" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/124421177/Hydration_of_Hg_sup_2_sup_in_Aqueous_Solution_Studied_by_Neutron_Diffraction_with_Isotopic_Substitution">Hydration of Hg<sup>2+</sup> in Aqueous Solution Studied by Neutron Diffraction with Isotopic Substitution</a></div><div class="wp-workCard_item"><span>Journal of Physical Chemistry A</span><span>, May 31, 2007</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The structural parameters of Hg2+ hydration were studied in 0.225 mol/L solutions of Hg2+ in DNO3...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The structural parameters of Hg2+ hydration were studied in 0.225 mol/L solutions of Hg2+ in DNO3/D2O by means of neutron diffraction with isotopic substitution of 199Hg for natHg. It was found that Hg2+ is hydrated by a first solvation shell of six water molecules. The observed Hg-O and Hg-H distances are equal to 2.48+/-0.05 and 3.08+/-0.05 A, respectively. The angle phi between the plane of the water molecule and the cation-water oxygen axis is approximately 35 degrees . The solvation of Hg2+ therefore mimics very closely that of Ca2+ (the Ca-O and Ca-H distances are 2.40 and 3.03 A, respectively) and helps to account for the extreme toxicity of mercury(II). We note also that the Hg-O distance obtained in the neutron diffraction experiment is larger by approximately 0.1 A than that obtained by X-ray diffraction. 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This difference is consistent with a shift of the oxygen electron density toward the mercury cation due to the covalency of the Hg-O interaction.","internal_url":"https://www.academia.edu/124421177/Hydration_of_Hg_sup_2_sup_in_Aqueous_Solution_Studied_by_Neutron_Diffraction_with_Isotopic_Substitution","translated_internal_url":"","created_at":"2024-10-04T08:33:22.944-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":31565326,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"Hydration_of_Hg_sup_2_sup_in_Aqueous_Solution_Studied_by_Neutron_Diffraction_with_Isotopic_Substitution","translated_slug":"","page_count":null,"language":"en","content_type":"Work","owner":{"id":31565326,"first_name":"Laurent","middle_initials":null,"last_name":"Charlet","page_name":"LaurentCharlet","domain_name":"independent","created_at":"2015-05-26T13:21:10.202-07:00","display_name":"Laurent Charlet","url":"https://independent.academia.edu/LaurentCharlet"},"attachments":[],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":2215,"name":"Water","url":"https://www.academia.edu/Documents/in/Water"},{"id":21553,"name":"Neutron Diffraction","url":"https://www.academia.edu/Documents/in/Neutron_Diffraction"},{"id":26327,"name":"Medicine","url":"https://www.academia.edu/Documents/in/Medicine"},{"id":49735,"name":"Solvation","url":"https://www.academia.edu/Documents/in/Solvation"},{"id":90017,"name":"Mercury","url":"https://www.academia.edu/Documents/in/Mercury"},{"id":143483,"name":"Deuterium","url":"https://www.academia.edu/Documents/in/Deuterium"},{"id":380825,"name":"Oxygen","url":"https://www.academia.edu/Documents/in/Oxygen"},{"id":386527,"name":"X ray diffraction","url":"https://www.academia.edu/Documents/in/X_ray_diffraction"},{"id":390245,"name":"Particle Size","url":"https://www.academia.edu/Documents/in/Particle_Size"},{"id":414692,"name":"Solutions","url":"https://www.academia.edu/Documents/in/Solutions"},{"id":645605,"name":"THEORETICAL AND COMPUTATIONAL CHEMISTRY","url":"https://www.academia.edu/Documents/in/THEORETICAL_AND_COMPUTATIONAL_CHEMISTRY"},{"id":989646,"name":"Aqueous Solution","url":"https://www.academia.edu/Documents/in/Aqueous_Solution"},{"id":1029023,"name":"Molecule","url":"https://www.academia.edu/Documents/in/Molecule"},{"id":1257974,"name":"Ions","url":"https://www.academia.edu/Documents/in/Ions"}],"urls":[{"id":44976078,"url":"https://doi.org/10.1021/jp072650w"}]}, dispatcherData: dispatcherData }); 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