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<button class="button is-small is-link">Go</button> </div> </div> </form> </div> </div> <ol class="breathe-horizontal" start="1"> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2403.11739">arXiv:2403.11739</a> <span> [<a href="https://arxiv.org/pdf/2403.11739">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> </div> <p class="title is-5 mathjax"> Tuning of the ultrafast demagnetization by ultrashort spin polarized currents in multi-sublattice ferrimagnets </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Gupta%2C+D">Deeksha Gupta</a>, <a href="/search/cond-mat?searchtype=author&query=Pankratova%2C+M">Maryna Pankratova</a>, <a href="/search/cond-mat?searchtype=author&query=Riepp%2C+M">Matthias Riepp</a>, <a href="/search/cond-mat?searchtype=author&query=Pereiro%2C+M">Manuel Pereiro</a>, <a href="/search/cond-mat?searchtype=author&query=Sanyal%2C+B">Biplab Sanyal</a>, <a href="/search/cond-mat?searchtype=author&query=Ershadrad%2C+S">Soheil Ershadrad</a>, <a href="/search/cond-mat?searchtype=author&query=Hehn%2C+M">Michel Hehn</a>, <a href="/search/cond-mat?searchtype=author&query=Pontius%2C+N">Niko Pontius</a>, <a href="/search/cond-mat?searchtype=author&query=Sch%C3%BC%C3%9Fler-Langeheine%2C+C">Christian Sch眉脽ler-Langeheine</a>, <a href="/search/cond-mat?searchtype=author&query=Abrudan%2C+R">Radu Abrudan</a>, <a href="/search/cond-mat?searchtype=author&query=Bergeard%2C+N">Nicolas Bergeard</a>, <a href="/search/cond-mat?searchtype=author&query=Bergman%2C+A">Anders Bergman</a>, <a href="/search/cond-mat?searchtype=author&query=Eriksson%2C+O">Olle Eriksson</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">Christine Boeglin</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2403.11739v3-abstract-short" style="display: inline;"> Femtosecond laser pulses can be used to induce ultrafast changes of the magnetization in magnetic materials. Several microscopic mechanisms have been proposed to explain the observations, including the transport of ultrashort spin-polarized hot-electrons (SPHE). Such ultrafast spin currents find growing interest because of the recent challenges in ultrafast spintronics however they are only poorly… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2403.11739v3-abstract-full').style.display = 'inline'; document.getElementById('2403.11739v3-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2403.11739v3-abstract-full" style="display: none;"> Femtosecond laser pulses can be used to induce ultrafast changes of the magnetization in magnetic materials. Several microscopic mechanisms have been proposed to explain the observations, including the transport of ultrashort spin-polarized hot-electrons (SPHE). Such ultrafast spin currents find growing interest because of the recent challenges in ultrafast spintronics however they are only poorly characterized. One of the key challenges is to characterize the spin-polarized ultrafast currents and the microscopic mechanisms behind SPHE induced manipulation of the magnetization, especially in the case of technologically relevant ferrimagnetic alloys. Here, we have used a combined approach using time- and element-resolved X-ray magnetic circular dichroism and theoretical calculations based on atomistic spin-dynamics simulations to address the ultrafast transfer of the angular momentum from spin-polarized currents into ferrimagnetic Fe74Gd26 films and the concomitant reduction of sub-lattice magnetization. Our study shows that using a Co/Pt multilayer as a polarizer in a spin-valve structure, the SPHE drives the demagnetization of the two sub-lattices of the Fe74Gd26 film. This behaviour is explained based on two physical mechanisms, i.e., spin transfer torque and thermal fluctuations induced by the SPHE. We provide a quantitative description of the heat transfer of the ultrashort SPHE pulse to the Fe74Gd26 films, as well as the degree of spin-polarization of the SPHE current density responsible for the observed magnetization dynamics. Our work finally characterizes the spin-polarization of the SPHEs revealing unexpected opposite spin polarization to the Co magnetization, explaining our experimental results. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2403.11739v3-abstract-full').style.display = 'none'; document.getElementById('2403.11739v3-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 30 April, 2024; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 18 March, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> March 2024. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">22 pages, 19 figures</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2401.05130">arXiv:2401.05130</a> <span> [<a href="https://arxiv.org/pdf/2401.05130">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> </div> <p class="title is-5 mathjax"> Laser induced ultrafast Gd 4f spin dynamics at the surface of amorphous CoxGd100-x ferrimagnetic alloys </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Pac%C3%A9%2C+M">Matthias Pac茅</a>, <a href="/search/cond-mat?searchtype=author&query=Gupta%2C+D">Deeksha Gupta</a>, <a href="/search/cond-mat?searchtype=author&query=Fert%C3%A9%2C+T">Tom Fert茅</a>, <a href="/search/cond-mat?searchtype=author&query=Riepp%2C+M">Matthias Riepp</a>, <a href="/search/cond-mat?searchtype=author&query=Malinowski%2C+G">Gregory Malinowski</a>, <a href="/search/cond-mat?searchtype=author&query=Hehn%2C+M">Michel Hehn</a>, <a href="/search/cond-mat?searchtype=author&query=Pressacco%2C+F">Federico Pressacco</a>, <a href="/search/cond-mat?searchtype=author&query=Silly%2C+M">Matthieu Silly</a>, <a href="/search/cond-mat?searchtype=author&query=Sirotti%2C+F">Fausto Sirotti</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">Christine Boeglin</a>, <a href="/search/cond-mat?searchtype=author&query=Bergeard%2C+N">Nicolas Bergeard</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2401.05130v3-abstract-short" style="display: inline;"> We have investigated the laser induced ultrafast dynamics of Gd 4f spins at the surface of CoxGd100-x alloys by means of surface-sensitive and time-resolved dichroic resonant Auger spectroscopy. We have observed that the laser induced quenching of Gd 4f magnetic order at the surface of the CoxGd100-x alloys occur on a much longer time scale than that previously reported in bulk sensitive time-reso… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2401.05130v3-abstract-full').style.display = 'inline'; document.getElementById('2401.05130v3-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2401.05130v3-abstract-full" style="display: none;"> We have investigated the laser induced ultrafast dynamics of Gd 4f spins at the surface of CoxGd100-x alloys by means of surface-sensitive and time-resolved dichroic resonant Auger spectroscopy. We have observed that the laser induced quenching of Gd 4f magnetic order at the surface of the CoxGd100-x alloys occur on a much longer time scale than that previously reported in bulk sensitive time-resolved experiments. In parallel, we have characterized the static structural and magnetic properties at the surface and in the bulk of these alloys by combining Physical Property Measurement System (PPMS) magnetometry with X-ray Magnetic Circular Dichroism in absorption spectroscopy (XMCD) and X-Ray Photoelectron spectroscopy (XPS). The PPMS and XMCD measurements give information regarding the composition in the bulk of the alloys. The XPS measurements show non-homogeneous composition at the surface of the alloys with a strongly increased Gd content within the first layers compared to the nominal bulk values. Such larger Gd concentration results in a reduced indirect Gd 4f spin-lattice coupling. It explains the slower Gd 4f demagnetization we have observed in our surface-sensitive and time-resolved measurements compared to that previously reported by bulk-sensitive measurements. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2401.05130v3-abstract-full').style.display = 'none'; document.getElementById('2401.05130v3-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 25 March, 2024; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 10 January, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2024. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">15 pages, 8 figures, 1 table</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2312.02654">arXiv:2312.02654</a> <span> [<a href="https://arxiv.org/pdf/2312.02654">pdf</a>, <a href="https://arxiv.org/format/2312.02654">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Optics">physics.optics</span> </div> </div> <p class="title is-5 mathjax"> THz-Driven Coherent Magnetization Dynamics in a Labyrinth Domain State </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Riepp%2C+M">M Riepp</a>, <a href="/search/cond-mat?searchtype=author&query=Philippi-Kobs%2C+A">A Philippi-Kobs</a>, <a href="/search/cond-mat?searchtype=author&query=Mueller%2C+L">L Mueller</a>, <a href="/search/cond-mat?searchtype=author&query=Froemter%2C+R">R Froemter</a>, <a href="/search/cond-mat?searchtype=author&query=Roseker%2C+W">W Roseker</a>, <a href="/search/cond-mat?searchtype=author&query=Rysov%2C+R">R Rysov</a>, <a href="/search/cond-mat?searchtype=author&query=Walther%2C+M">M Walther</a>, <a href="/search/cond-mat?searchtype=author&query=Bagschik%2C+K">K Bagschik</a>, <a href="/search/cond-mat?searchtype=author&query=Hennes%2C+M">M Hennes</a>, <a href="/search/cond-mat?searchtype=author&query=Gupta%2C+D">D Gupta</a>, <a href="/search/cond-mat?searchtype=author&query=Marotzke%2C+S">S Marotzke</a>, <a href="/search/cond-mat?searchtype=author&query=Bajt%2C+S">S Bajt</a>, <a href="/search/cond-mat?searchtype=author&query=Pan%2C+R">R Pan</a>, <a href="/search/cond-mat?searchtype=author&query=Golz%2C+T">T Golz</a>, <a href="/search/cond-mat?searchtype=author&query=Stojanovic%2C+N">N Stojanovic</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">C Boeglin</a>, <a href="/search/cond-mat?searchtype=author&query=Gruebel%2C+G">G Gruebel</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2312.02654v1-abstract-short" style="display: inline;"> Terahertz (THz) light pulses can be used for an ultrafast coherent manipulation of the magnetization. Driving the magnetization at THz frequencies is currently the fastest way of writing magnetic information in ferromagnets. Using time-resolved resonant magnetic scattering, we gain new insights to the THz-driven coherent magnetization dynamics on nanometer length scales. We observe ultrafast demag… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2312.02654v1-abstract-full').style.display = 'inline'; document.getElementById('2312.02654v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2312.02654v1-abstract-full" style="display: none;"> Terahertz (THz) light pulses can be used for an ultrafast coherent manipulation of the magnetization. Driving the magnetization at THz frequencies is currently the fastest way of writing magnetic information in ferromagnets. Using time-resolved resonant magnetic scattering, we gain new insights to the THz-driven coherent magnetization dynamics on nanometer length scales. We observe ultrafast demagnetization and coherent magnetization oscillations that are governed by a time-dependent damping. This damping is determined by the interplay of lattice heating and magnetic anisotropy reduction revealing an upper speed limit for THz-induced magnetization switching. We show that in the presence of nanometer-sized magnetic domains, the ultrafast magnetization oscillations are associated with a correlated beating of the domain walls. The overall domain structure thereby remains largely unaffected which highlights the applicability of THz-induced switching on the nanoscale. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2312.02654v1-abstract-full').style.display = 'none'; document.getElementById('2312.02654v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 5 December, 2023; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> December 2023. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">10 pages, 8 figures and 54 references</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2211.04265">arXiv:2211.04265</a> <span> [<a href="https://arxiv.org/pdf/2211.04265">pdf</a>, <a href="https://arxiv.org/format/2211.04265">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Instrumentation and Detectors">physics.ins-det</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1107/S1600577523000619">10.1107/S1600577523000619 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Photon shot-noise limited transient absorption soft X-ray spectroscopy at the European XFEL </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Guyader%2C+L+L">Lo茂c Le Guyader</a>, <a href="/search/cond-mat?searchtype=author&query=Eschenlohr%2C+A">Andrea Eschenlohr</a>, <a href="/search/cond-mat?searchtype=author&query=Beye%2C+M">Martin Beye</a>, <a href="/search/cond-mat?searchtype=author&query=Schlotter%2C+W">William Schlotter</a>, <a href="/search/cond-mat?searchtype=author&query=D%C3%B6ring%2C+F">Florian D枚ring</a>, <a href="/search/cond-mat?searchtype=author&query=Carinan%2C+C">Cammille Carinan</a>, <a href="/search/cond-mat?searchtype=author&query=Hickin%2C+D">David Hickin</a>, <a href="/search/cond-mat?searchtype=author&query=Agarwal%2C+N">Naman Agarwal</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">Christine Boeglin</a>, <a href="/search/cond-mat?searchtype=author&query=Bovensiepen%2C+U">Uwe Bovensiepen</a>, <a href="/search/cond-mat?searchtype=author&query=Buck%2C+J">Jens Buck</a>, <a href="/search/cond-mat?searchtype=author&query=Carley%2C+R">Robert Carley</a>, <a href="/search/cond-mat?searchtype=author&query=Castoldi%2C+A">Andrea Castoldi</a>, <a href="/search/cond-mat?searchtype=author&query=D%27Elia%2C+A">Alessandro D'Elia</a>, <a href="/search/cond-mat?searchtype=author&query=Delitz%2C+J">Jan-Torben Delitz</a>, <a href="/search/cond-mat?searchtype=author&query=Ehsan%2C+W">Wajid Ehsan</a>, <a href="/search/cond-mat?searchtype=author&query=Engel%2C+R">Robin Engel</a>, <a href="/search/cond-mat?searchtype=author&query=Erdinger%2C+F">Florian Erdinger</a>, <a href="/search/cond-mat?searchtype=author&query=Fangohr%2C+H">Hans Fangohr</a>, <a href="/search/cond-mat?searchtype=author&query=Fischer%2C+P">Peter Fischer</a>, <a href="/search/cond-mat?searchtype=author&query=Fiorini%2C+C">Carlo Fiorini</a>, <a href="/search/cond-mat?searchtype=author&query=F%C3%B6hlisch%2C+A">Alexander F枚hlisch</a>, <a href="/search/cond-mat?searchtype=author&query=Gelisio%2C+L">Luca Gelisio</a>, <a href="/search/cond-mat?searchtype=author&query=Gensch%2C+M">Michael Gensch</a>, <a href="/search/cond-mat?searchtype=author&query=Gerasimova%2C+N">Natalia Gerasimova</a> , et al. (39 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2211.04265v3-abstract-short" style="display: inline;"> Femtosecond transient soft X-ray Absorption Spectroscopy (XAS) is a very promising technique that can be employed at X-ray Free Electron Lasers (FELs) to investigate out-of-equilibrium dynamics for material and energy research. Here we present a dedicated setup for soft X-rays available at the Spectroscopy & Coherent Scattering (SCS) instrument at the European X-ray Free Electron Laser (EuXFEL). I… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2211.04265v3-abstract-full').style.display = 'inline'; document.getElementById('2211.04265v3-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2211.04265v3-abstract-full" style="display: none;"> Femtosecond transient soft X-ray Absorption Spectroscopy (XAS) is a very promising technique that can be employed at X-ray Free Electron Lasers (FELs) to investigate out-of-equilibrium dynamics for material and energy research. Here we present a dedicated setup for soft X-rays available at the Spectroscopy & Coherent Scattering (SCS) instrument at the European X-ray Free Electron Laser (EuXFEL). It consists of a beam-splitting off-axis zone plate (BOZ) used in transmission to create three copies of the incoming beam, which are used to measure the transmitted intensity through the excited and unexcited sample, as well as to monitor the incoming intensity. Since these three intensity signals are detected shot-by-shot and simultaneously, this setup allows normalized shot-by-shot analysis of the transmission. For photon detection, the DSSC imaging detector, which is capable of recording up to 800 images at 4.5 MHz frame rate during the FEL burst, is employed and allows approaching the photon shot-noise limit. We review the setup and its capabilities, as well as the online and offline analysis tools provided to users. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2211.04265v3-abstract-full').style.display = 'none'; document.getElementById('2211.04265v3-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 4 January, 2023; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 8 November, 2022; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> November 2022. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">11 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> J. Synchrotron Rad. (2023). 30, 284-300 </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2210.13162">arXiv:2210.13162</a> <span> [<a href="https://arxiv.org/pdf/2210.13162">pdf</a>, <a href="https://arxiv.org/format/2210.13162">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> </div> <p class="title is-5 mathjax"> The interplay of local electron correlations and ultrafast spin dynamics in fcc Ni </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Lojewski%2C+T">Tobias Lojewski</a>, <a href="/search/cond-mat?searchtype=author&query=Elhanoty%2C+M+F">Mohamed F. Elhanoty</a>, <a href="/search/cond-mat?searchtype=author&query=Guyader%2C+L+L">Lo茂c Le Guyader</a>, <a href="/search/cond-mat?searchtype=author&query=Gr%C3%A5n%C3%A4s%2C+O">Oscar Gr氓n盲s</a>, <a href="/search/cond-mat?searchtype=author&query=Agarwal%2C+N">Naman Agarwal</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">Christine Boeglin</a>, <a href="/search/cond-mat?searchtype=author&query=Carley%2C+R">Robert Carley</a>, <a href="/search/cond-mat?searchtype=author&query=Castoldi%2C+A">Andrea Castoldi</a>, <a href="/search/cond-mat?searchtype=author&query=David%2C+C">Christian David</a>, <a href="/search/cond-mat?searchtype=author&query=Deiter%2C+C">Carsten Deiter</a>, <a href="/search/cond-mat?searchtype=author&query=D%C3%B6ring%2C+F">Florian D枚ring</a>, <a href="/search/cond-mat?searchtype=author&query=Engel%2C+R+Y">Robin Y. Engel</a>, <a href="/search/cond-mat?searchtype=author&query=Erdinger%2C+F">Florian Erdinger</a>, <a href="/search/cond-mat?searchtype=author&query=Fangohr%2C+H">Hans Fangohr</a>, <a href="/search/cond-mat?searchtype=author&query=Fiorini%2C+C">Carlo Fiorini</a>, <a href="/search/cond-mat?searchtype=author&query=Fischer%2C+P">Peter Fischer</a>, <a href="/search/cond-mat?searchtype=author&query=Gerasimova%2C+N">Natalia Gerasimova</a>, <a href="/search/cond-mat?searchtype=author&query=Gort%2C+R">Rafael Gort</a>, <a href="/search/cond-mat?searchtype=author&query=de+Groot%2C+F">Frank de Groot</a>, <a href="/search/cond-mat?searchtype=author&query=Hansen%2C+K">Karsten Hansen</a>, <a href="/search/cond-mat?searchtype=author&query=Hauf%2C+S">Steffen Hauf</a>, <a href="/search/cond-mat?searchtype=author&query=Hickin%2C+D">David Hickin</a>, <a href="/search/cond-mat?searchtype=author&query=Izquierdo%2C+M">Manuel Izquierdo</a>, <a href="/search/cond-mat?searchtype=author&query=Van+Kuiken%2C+B+E">Benjamin E. Van Kuiken</a>, <a href="/search/cond-mat?searchtype=author&query=Kvashnin%2C+Y">Yaroslav Kvashnin</a> , et al. (26 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2210.13162v1-abstract-short" style="display: inline;"> The complex electronic structure of metallic ferromagnets is determined by a balance between exchange interaction, electron hopping leading to band formation, and local Coulomb repulsion. The interplay between the respective terms of the Hamiltonian is of fundamental interest, since it produces most, if not all, of the exotic phenomena observed in the solid state. By combining high energy and temp… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2210.13162v1-abstract-full').style.display = 'inline'; document.getElementById('2210.13162v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2210.13162v1-abstract-full" style="display: none;"> The complex electronic structure of metallic ferromagnets is determined by a balance between exchange interaction, electron hopping leading to band formation, and local Coulomb repulsion. The interplay between the respective terms of the Hamiltonian is of fundamental interest, since it produces most, if not all, of the exotic phenomena observed in the solid state. By combining high energy and temporal resolution in femtosecond time-resolved X-ray absorption spectroscopy with ab initio time-dependent density functional theory we analyze the electronic structure in fcc Ni on the time scale of these interactions in a pump-probe experiment. We distinguish transient broadening and energy shifts in the absorption spectra, which we demonstrate to be caused by electron repopulation and correlation-induced modifications of the electronic structure, respectively. Importantly, the theoretical description of this experimental result hence requires to take the local Coulomb interaction into account, revealing a temporal interplay between band formation, exchange interaction, and Coulomb repulsion. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2210.13162v1-abstract-full').style.display = 'none'; document.getElementById('2210.13162v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 24 October, 2022; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> October 2022. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2206.10422">arXiv:2206.10422</a> <span> [<a href="https://arxiv.org/pdf/2206.10422">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1140/epjs/s11734-023-00812-w">10.1140/epjs/s11734-023-00812-w <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Laser induced ultrafast Gd 4f spin dynamics in Co100-xGdx alloys by means of time-resolved XMCD </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Fert%C3%A9%2C+T">T. Fert茅</a>, <a href="/search/cond-mat?searchtype=author&query=Beens%2C+M">M. Beens</a>, <a href="/search/cond-mat?searchtype=author&query=Malinowski%2C+G">G. Malinowski</a>, <a href="/search/cond-mat?searchtype=author&query=Holldack%2C+K">K. Holldack</a>, <a href="/search/cond-mat?searchtype=author&query=Abrudan%2C+R">R. Abrudan</a>, <a href="/search/cond-mat?searchtype=author&query=Radu%2C+F">F. Radu</a>, <a href="/search/cond-mat?searchtype=author&query=Kachel%2C+T">T. Kachel</a>, <a href="/search/cond-mat?searchtype=author&query=Hehn%2C+M">M. Hehn</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">C. Boeglin</a>, <a href="/search/cond-mat?searchtype=author&query=Koopmans%2C+B">B. Koopmans</a>, <a href="/search/cond-mat?searchtype=author&query=Bergeard%2C+N">N. Bergeard</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2206.10422v1-abstract-short" style="display: inline;"> We have studied the laser induced ultrafast quenching of Gd 4f magnetic order in ferrimagnetic Co100-xGdx alloys to highlight the role of the inter-atomic exchange coupling. We have taken advantage of the ultrashort soft X-ray pulses deliver by the femtoslicing beamline at the BESSY II synchrotron radiation source at the Helmholtz-Zentrum Berlin to perform element- and time-resolved X-ray Magnetic… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2206.10422v1-abstract-full').style.display = 'inline'; document.getElementById('2206.10422v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2206.10422v1-abstract-full" style="display: none;"> We have studied the laser induced ultrafast quenching of Gd 4f magnetic order in ferrimagnetic Co100-xGdx alloys to highlight the role of the inter-atomic exchange coupling. We have taken advantage of the ultrashort soft X-ray pulses deliver by the femtoslicing beamline at the BESSY II synchrotron radiation source at the Helmholtz-Zentrum Berlin to perform element- and time-resolved X-ray Magnetic Circular Dichroism spectroscopy.Our results show that the laser induced quenching of Gd 4f magnetic order occurs on very different time-scales for the Co72Gd28, the Co77Gd23 and the Co79Gd21 alloys. Most of the magnetic moment losses occur within the first picosecond (ps) while the electron distribution is strongly out of equilibrium. After the equilibration of the electrons and lattice temperatures (t > 1 ps), the magnetic losses occur on slower rates that depend on the alloy composition: increasing the Co composition speeds up the demagnetization of Gd 4f sublattice. The strength of the inter-atomic exchange coupling which depends on composition, determines the efficiency of the angular momentum flow from the Gd 4f spin towards the lattice. Our results are in qualitative agreements with the predictions of the microscopic three temperatures model for ferrimagnetic alloys. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2206.10422v1-abstract-full').style.display = 'none'; document.getElementById('2206.10422v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 21 June, 2022; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> June 2022. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">8 pages, 6 figures</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2201.06350">arXiv:2201.06350</a> <span> [<a href="https://arxiv.org/pdf/2201.06350">pdf</a>, <a href="https://arxiv.org/format/2201.06350">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Mesoscale and Nanoscale Physics">cond-mat.mes-hall</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Accelerator Physics">physics.acc-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Instrumentation and Detectors">physics.ins-det</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1107/S1600577522008414">10.1107/S1600577522008414 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Megahertz-rate Ultrafast X-ray Scattering and Holographic Imaging at the European XFEL </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Hagstr%C3%B6m%2C+N+Z">Nanna Zhou Hagstr枚m</a>, <a href="/search/cond-mat?searchtype=author&query=Schneider%2C+M">Michael Schneider</a>, <a href="/search/cond-mat?searchtype=author&query=Kerber%2C+N">Nico Kerber</a>, <a href="/search/cond-mat?searchtype=author&query=Yaroslavtsev%2C+A">Alexander Yaroslavtsev</a>, <a href="/search/cond-mat?searchtype=author&query=Parra%2C+E+B">Erick Burgos Parra</a>, <a href="/search/cond-mat?searchtype=author&query=Beg%2C+M">Marijan Beg</a>, <a href="/search/cond-mat?searchtype=author&query=Lang%2C+M">Martin Lang</a>, <a href="/search/cond-mat?searchtype=author&query=G%C3%BCnther%2C+C+M">Christian M. G眉nther</a>, <a href="/search/cond-mat?searchtype=author&query=Seng%2C+B">Boris Seng</a>, <a href="/search/cond-mat?searchtype=author&query=Kammerbauer%2C+F">Fabian Kammerbauer</a>, <a href="/search/cond-mat?searchtype=author&query=Popescu%2C+H">Horia Popescu</a>, <a href="/search/cond-mat?searchtype=author&query=Pancaldi%2C+M">Matteo Pancaldi</a>, <a href="/search/cond-mat?searchtype=author&query=Neeraj%2C+K">Kumar Neeraj</a>, <a href="/search/cond-mat?searchtype=author&query=Polley%2C+D">Debanjan Polley</a>, <a href="/search/cond-mat?searchtype=author&query=Jangid%2C+R">Rahul Jangid</a>, <a href="/search/cond-mat?searchtype=author&query=Hrkac%2C+S+B">Stjepan B. Hrkac</a>, <a href="/search/cond-mat?searchtype=author&query=Patel%2C+S+K+K">Sheena K. K. Patel</a>, <a href="/search/cond-mat?searchtype=author&query=Ovcharenko%2C+S">Sergei Ovcharenko</a>, <a href="/search/cond-mat?searchtype=author&query=Turenne%2C+D">Diego Turenne</a>, <a href="/search/cond-mat?searchtype=author&query=Ksenzov%2C+D">Dmitriy Ksenzov</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">Christine Boeglin</a>, <a href="/search/cond-mat?searchtype=author&query=Pronin%2C+I">Igor Pronin</a>, <a href="/search/cond-mat?searchtype=author&query=Baidakova%2C+M">Marina Baidakova</a>, <a href="/search/cond-mat?searchtype=author&query=Schmising%2C+C+v+K">Clemens von Korff Schmising</a>, <a href="/search/cond-mat?searchtype=author&query=Borchert%2C+M">Martin Borchert</a> , et al. (75 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2201.06350v2-abstract-short" style="display: inline;"> The advent of X-ray free-electron lasers (XFELs) has revolutionized fundamental science, from atomic to condensed matter physics, from chemistry to biology, giving researchers access to X-rays with unprecedented brightness, coherence, and pulse duration. All XFEL facilities built until recently provided X-ray pulses at a relatively low repetition rate, with limited data statistics. Here, we presen… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2201.06350v2-abstract-full').style.display = 'inline'; document.getElementById('2201.06350v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2201.06350v2-abstract-full" style="display: none;"> The advent of X-ray free-electron lasers (XFELs) has revolutionized fundamental science, from atomic to condensed matter physics, from chemistry to biology, giving researchers access to X-rays with unprecedented brightness, coherence, and pulse duration. All XFEL facilities built until recently provided X-ray pulses at a relatively low repetition rate, with limited data statistics. Here, we present the results from the first megahertz repetition rate X-ray scattering experiments at the Spectroscopy and Coherent Scattering (SCS) instrument of the European XFEL. We illustrate the experimental capabilities that the SCS instrument offers, resulting from the operation at MHz repetition rates and the availability of the novel DSSC 2D imaging detector. Time-resolved magnetic X-ray scattering and holographic imaging experiments in solid state samples were chosen as representative, providing an ideal test-bed for operation at megahertz rates. Our results are relevant and applicable to any other non-destructive XFEL experiments in the soft X-ray range. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2201.06350v2-abstract-full').style.display = 'none'; document.getElementById('2201.06350v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 20 January, 2022; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 17 January, 2022; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2022. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">13 pages, 5 figures. Supplementary Information as ancillary file</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> J. Synchrotron Rad. (2022), 29 </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2102.13502">arXiv:2102.13502</a> <span> [<a href="https://arxiv.org/pdf/2102.13502">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> </div> <p class="title is-5 mathjax"> Direct imaging of chiral domain walls and N茅el-type skyrmionium in ferrimagnetic alloys </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Seng%2C+B">Boris Seng</a>, <a href="/search/cond-mat?searchtype=author&query=Sch%C3%B6nke%2C+D">Daniel Sch枚nke</a>, <a href="/search/cond-mat?searchtype=author&query=Yeste%2C+J">Javier Yeste</a>, <a href="/search/cond-mat?searchtype=author&query=Reeve%2C+R+M">Robert M. Reeve</a>, <a href="/search/cond-mat?searchtype=author&query=Kerber%2C+N">Nico Kerber</a>, <a href="/search/cond-mat?searchtype=author&query=Lacour%2C+D">Daniel Lacour</a>, <a href="/search/cond-mat?searchtype=author&query=Bello%2C+J">Jean-Lo茂s Bello</a>, <a href="/search/cond-mat?searchtype=author&query=Bergeard%2C+N">Nicolas Bergeard</a>, <a href="/search/cond-mat?searchtype=author&query=Kammerbauer%2C+F">Fabian Kammerbauer</a>, <a href="/search/cond-mat?searchtype=author&query=Bhukta%2C+M">Mona Bhukta</a>, <a href="/search/cond-mat?searchtype=author&query=Fert%C3%A9%2C+T">Tom Fert茅</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">Christine Boeglin</a>, <a href="/search/cond-mat?searchtype=author&query=Radu%2C+F">Florin Radu</a>, <a href="/search/cond-mat?searchtype=author&query=Abrudan%2C+R">Radu Abrudan</a>, <a href="/search/cond-mat?searchtype=author&query=Kachel%2C+T">Torsten Kachel</a>, <a href="/search/cond-mat?searchtype=author&query=Mangin%2C+S">St茅phane Mangin</a>, <a href="/search/cond-mat?searchtype=author&query=Hehn%2C+M">Michel Hehn</a>, <a href="/search/cond-mat?searchtype=author&query=Kl%C3%A4ui%2C+M">Mathias Kl盲ui</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2102.13502v2-abstract-short" style="display: inline;"> The evolution of chiral spin structures is studied in ferrimagnet Ta/Ir/Fe/GdFeCo/Pt multilayers as a function of temperature using scanning electron microscopy with polarization analysis (SEMPA). The GdFeCo ferrimagnet exhibits pure right-hand N茅el-type domain wall (DW) spin textures over a large temperature range. This indicates the presence of a negative Dzyaloshinskii-Moriya interaction (DMI)… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2102.13502v2-abstract-full').style.display = 'inline'; document.getElementById('2102.13502v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2102.13502v2-abstract-full" style="display: none;"> The evolution of chiral spin structures is studied in ferrimagnet Ta/Ir/Fe/GdFeCo/Pt multilayers as a function of temperature using scanning electron microscopy with polarization analysis (SEMPA). The GdFeCo ferrimagnet exhibits pure right-hand N茅el-type domain wall (DW) spin textures over a large temperature range. This indicates the presence of a negative Dzyaloshinskii-Moriya interaction (DMI) that can originate from both the top Fe/Pt and the Co/Pt interfaces. From measurements of the DW width, as well as complementary magnetic characterization, the exchange stiffness as a function of temperature is ascertained. The exchange stiffness is surprisingly mostly constant, which is explained by theoretical predictions. Beyond single skyrmions, we find by direct imaging a pure N茅el-type skyrmionium, which due to the absence of a skyrmion Hall angle is a promising topological spin structure to enable high impact potential applications in the next generation of spintronic devices. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2102.13502v2-abstract-full').style.display = 'none'; document.getElementById('2102.13502v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 21 July, 2021; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 26 February, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> February 2021. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1910.13143">arXiv:1910.13143</a> <span> [<a href="https://arxiv.org/pdf/1910.13143">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> </div> <p class="title is-5 mathjax"> Laser induced ultrafast 3d and 4f spin dynamics in CoDy ferrimagnetic alloys as a function of temperature </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Fert%C3%A9%2C+T">Tom Fert茅</a>, <a href="/search/cond-mat?searchtype=author&query=Malinowski%2C+G">Gr茅gory Malinowski</a>, <a href="/search/cond-mat?searchtype=author&query=Terrier%2C+E">Erwan Terrier</a>, <a href="/search/cond-mat?searchtype=author&query=Halt%C3%A9%2C+V">Val茅rie Halt茅</a>, <a href="/search/cond-mat?searchtype=author&query=Guyader%2C+L+L">Lo茂c Le Guyader</a>, <a href="/search/cond-mat?searchtype=author&query=Holldack%2C+K">Karsten Holldack</a>, <a href="/search/cond-mat?searchtype=author&query=Hehn%2C+M">Michel Hehn</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">Christine Boeglin</a>, <a href="/search/cond-mat?searchtype=author&query=Bergeard%2C+N">Nicolas Bergeard</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1910.13143v2-abstract-short" style="display: inline;"> We report on an element- and time-resolved investigation of femtosecond laser induced ultrafast dynamics of 3d and 4f spins in a ferrimagnetic Co80Dy20 alloy as a function of temperature. We observe an increase of the Co3d characteristic demagnetization time and a decrease of the Dy4f demagnetization time when the temperature is approaching the Curie temperature. It suggests that the critical slow… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1910.13143v2-abstract-full').style.display = 'inline'; document.getElementById('1910.13143v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1910.13143v2-abstract-full" style="display: none;"> We report on an element- and time-resolved investigation of femtosecond laser induced ultrafast dynamics of 3d and 4f spins in a ferrimagnetic Co80Dy20 alloy as a function of temperature. We observe an increase of the Co3d characteristic demagnetization time and a decrease of the Dy4f demagnetization time when the temperature is approaching the Curie temperature. It suggests that the critical slowing down regime, which affects the laser induced ultrafast dynamics in pure 3d transition metals and 4f rare-earth ferromagnetic layers, vanishes for the Dy sublattice in the CoDy alloy, in line with the theoretical predictions of the Landau-Lifshitz-Bloch model. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1910.13143v2-abstract-full').style.display = 'none'; document.getElementById('1910.13143v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 15 June, 2020; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 29 October, 2019; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> October 2019. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1708.08919">arXiv:1708.08919</a> <span> [<a href="https://arxiv.org/pdf/1708.08919">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevB.96.144427">10.1103/PhysRevB.96.144427 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Ultrafast hot-electron induced quenching of Tb4f magnetic order </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Ferte%2C+T">T. Ferte</a>, <a href="/search/cond-mat?searchtype=author&query=Bergeard%2C+N">N. Bergeard</a>, <a href="/search/cond-mat?searchtype=author&query=Malinowski%2C+G">G. Malinowski</a>, <a href="/search/cond-mat?searchtype=author&query=Abrudan%2C+R">R. Abrudan</a>, <a href="/search/cond-mat?searchtype=author&query=Kachel%2C+T">T. Kachel</a>, <a href="/search/cond-mat?searchtype=author&query=Holldack%2C+K">K. Holldack</a>, <a href="/search/cond-mat?searchtype=author&query=Hehn%2C+M">M. Hehn</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">C. Boeglin</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1708.08919v2-abstract-short" style="display: inline;"> We have investigated ultrafast quenching of the Tb4f magnetic order in Co74Tb26 alloys, induced by femtosecond hot-electrons pulses. The hot-electron pulses were produced in specific non-magnetic capping layers by infrared fs laser pulses. Our experimental results show that sub-picosecond dynamics of Tb4f magnetic moments can be induced by non-thermal and thermal hot-electrons. We further demonstr… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1708.08919v2-abstract-full').style.display = 'inline'; document.getElementById('1708.08919v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1708.08919v2-abstract-full" style="display: none;"> We have investigated ultrafast quenching of the Tb4f magnetic order in Co74Tb26 alloys, induced by femtosecond hot-electrons pulses. The hot-electron pulses were produced in specific non-magnetic capping layers by infrared fs laser pulses. Our experimental results show that sub-picosecond dynamics of Tb4f magnetic moments can be induced by non-thermal and thermal hot-electrons. We further demonstrate that the demagnetization efficiencies of non-thermal and thermal hot electrons are similar. However, the characteristic demagnetization times show values of 0.35 ps for non-thermal hot-electrons excitations and 1.2 ps for thermal hot-electrons excitations. We explain this temporal elongation by the propagation time of thermal hot-electrons through the 15 nm thick CoTb film. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1708.08919v2-abstract-full').style.display = 'none'; document.getElementById('1708.08919v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 31 August, 2017; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 29 August, 2017; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> August 2017. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">14 pages, 3 Figures and 1 Table</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. B 96, 144427 (2017) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1708.08918">arXiv:1708.08918</a> <span> [<a href="https://arxiv.org/pdf/1708.08918">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevB.96.134303">10.1103/PhysRevB.96.134303 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Element-resolved ultrafast demagnetization rates in ferrimagnetic CoDy </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Ferte%2C+T">T. Ferte</a>, <a href="/search/cond-mat?searchtype=author&query=Bergeard%2C+N">N. Bergeard</a>, <a href="/search/cond-mat?searchtype=author&query=Guyader%2C+L+L">L. Le Guyader</a>, <a href="/search/cond-mat?searchtype=author&query=Hehn%2C+M">M. Hehn</a>, <a href="/search/cond-mat?searchtype=author&query=Malinowski%2C+G">G. Malinowski</a>, <a href="/search/cond-mat?searchtype=author&query=Terrier%2C+E">E. Terrier</a>, <a href="/search/cond-mat?searchtype=author&query=Otero%2C+E">E. Otero</a>, <a href="/search/cond-mat?searchtype=author&query=Holldack%2C+K">K. Holldack</a>, <a href="/search/cond-mat?searchtype=author&query=Pontius%2C+N">N. Pontius</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">C. Boeglin</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1708.08918v2-abstract-short" style="display: inline;"> Femtosecond laser induced ultrafast magnetization dynamics have been studied in multisublattice CoxDy1-x alloys. By performing element and time-resolved X-ray spectroscopy, we distinguish the ultrafast quenching of Co3d and Dy4f magnetic order when the initial temperatures are below (T=150K) or above (T=270K) the temperature of magnetic compensation (Tcomp). In accordance with former element-resol… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1708.08918v2-abstract-full').style.display = 'inline'; document.getElementById('1708.08918v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1708.08918v2-abstract-full" style="display: none;"> Femtosecond laser induced ultrafast magnetization dynamics have been studied in multisublattice CoxDy1-x alloys. By performing element and time-resolved X-ray spectroscopy, we distinguish the ultrafast quenching of Co3d and Dy4f magnetic order when the initial temperatures are below (T=150K) or above (T=270K) the temperature of magnetic compensation (Tcomp). In accordance with former element-resolved investigations and theoretical calculations, we observe different dynamics for Co3d and Dy4f spins. In addition we observe that, for a given laser fluence, the demagnetization amplitudes and demagnetization times are not affected by the existence of a temperature of magnetic compensation. However, our experiment reveals a twofold increase of the ultrafast demagnetization rates for the Dy sublattice at low temperature. In parallel, we measure a constant demagnetization rate of the Co3d sublattice above and below Tcomp. This intriguing difference between the Dy4f and Co3d sublattices calls for further theoretical and experimental investigations. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1708.08918v2-abstract-full').style.display = 'none'; document.getElementById('1708.08918v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 31 August, 2017; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 29 August, 2017; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> August 2017. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">6 Figure, 2 Tables</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. B 96, 134303 (2017) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1701.01375">arXiv:1701.01375</a> <span> [<a href="https://arxiv.org/pdf/1701.01375">pdf</a>, <a href="https://arxiv.org/format/1701.01375">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevB.95.184422">10.1103/PhysRevB.95.184422 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Structural dynamics during laser induced ultrafast demagnetization </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Jal%2C+E">Emmanuelle Jal</a>, <a href="/search/cond-mat?searchtype=author&query=L%C3%B3pez-Flores%2C+V">Victor L贸pez-Flores</a>, <a href="/search/cond-mat?searchtype=author&query=Pontius%2C+N">Niko Pontius</a>, <a href="/search/cond-mat?searchtype=author&query=Fert%C3%A9%2C+T">Tom Fert茅</a>, <a href="/search/cond-mat?searchtype=author&query=Bergeard%2C+N">Nicolas Bergeard</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">Christine Boeglin</a>, <a href="/search/cond-mat?searchtype=author&query=Vodungbo%2C+B">Boris Vodungbo</a>, <a href="/search/cond-mat?searchtype=author&query=L%C3%BCning%2C+J">Jan L眉ning</a>, <a href="/search/cond-mat?searchtype=author&query=Jaouen%2C+N">Nicolas Jaouen</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1701.01375v3-abstract-short" style="display: inline;"> The mechanism underlying femtosecond laser pulse induced ultrafast magnetization dynamics remains elusive despite two decades of intense research on this phenomenon. Most experiments focused so far on characterizing magnetization and charge carrier dynamics, while first direct measurements of structural dynamics during ultrafast demagnetization were reported only very recently. We here present our… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1701.01375v3-abstract-full').style.display = 'inline'; document.getElementById('1701.01375v3-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1701.01375v3-abstract-full" style="display: none;"> The mechanism underlying femtosecond laser pulse induced ultrafast magnetization dynamics remains elusive despite two decades of intense research on this phenomenon. Most experiments focused so far on characterizing magnetization and charge carrier dynamics, while first direct measurements of structural dynamics during ultrafast demagnetization were reported only very recently. We here present our investigation of the infrared laser pulse induced ultrafast demagnetization process in a thin Ni film, which characterizes simultaneously magnetization and structural dynamics. This is achieved by employing femtosecond time resolved X-ray resonant magnetic reflectivity (tr-XRMR) as probe technique. The experimental results reveal unambiguously that the sub-picosecond magnetization quenching is accompanied by strong changes in non-magnetic X-ray reflectivity. These changes vary with reflection angle and changes up to 30$\%$ have been observed. Modeling the X-ray reflectivity of the investigated thin film, we can reproduce these changes by a variation of the apparent Ni layer thickness of up to 1$\%$. Extending these simulations to larger incidence angles we show that tr-XRMR can be employed to discriminate experimentally between currently discussed models describing the ultrafast demagnetization phenomenon. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1701.01375v3-abstract-full').style.display = 'none'; document.getElementById('1701.01375v3-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 7 December, 2017; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 5 January, 2017; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2017. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. B 95, 184422 (2017) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1502.00786">arXiv:1502.00786</a> <span> [<a href="https://arxiv.org/pdf/1502.00786">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevB.91.054416">10.1103/PhysRevB.91.054416 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Irreversible transformation of ferromagnetic ordered stripe domains in single-shot IR pump - resonant X-ray scattering probe experiments </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Bergeard%2C+N">Nicolas Bergeard</a>, <a href="/search/cond-mat?searchtype=author&query=Schaffert%2C+S">Stefan Schaffert</a>, <a href="/search/cond-mat?searchtype=author&query=L%C3%B3pez-Flores%2C+V">V铆ctor L贸pez-Flores</a>, <a href="/search/cond-mat?searchtype=author&query=Jaouen%2C+N">Nicolas Jaouen</a>, <a href="/search/cond-mat?searchtype=author&query=Geilhufe%2C+J">Jan Geilhufe</a>, <a href="/search/cond-mat?searchtype=author&query=G%C3%BCnther%2C+C+M">Christian M. G眉nther</a>, <a href="/search/cond-mat?searchtype=author&query=Schneider%2C+M">Michael Schneider</a>, <a href="/search/cond-mat?searchtype=author&query=Graves%2C+C">Catherine Graves</a>, <a href="/search/cond-mat?searchtype=author&query=Wang%2C+T">Tianhan Wang</a>, <a href="/search/cond-mat?searchtype=author&query=Wu%2C+B">Benny Wu</a>, <a href="/search/cond-mat?searchtype=author&query=Scherz%2C+A">Andreas Scherz</a>, <a href="/search/cond-mat?searchtype=author&query=Baumier%2C+C">C茅dric Baumier</a>, <a href="/search/cond-mat?searchtype=author&query=Delaunay%2C+R">Renaud Delaunay</a>, <a href="/search/cond-mat?searchtype=author&query=Fortuna%2C+F">Franck Fortuna</a>, <a href="/search/cond-mat?searchtype=author&query=Tortarolo%2C+M">Marina Tortarolo</a>, <a href="/search/cond-mat?searchtype=author&query=Tudu%2C+B">Bharati Tudu</a>, <a href="/search/cond-mat?searchtype=author&query=Krupin%2C+O">Oleg Krupin</a>, <a href="/search/cond-mat?searchtype=author&query=Minitti%2C+M+P">Michael P. Minitti</a>, <a href="/search/cond-mat?searchtype=author&query=Robinson%2C+J">Joe Robinson</a>, <a href="/search/cond-mat?searchtype=author&query=Schlotter%2C+W+F">William F. Schlotter</a>, <a href="/search/cond-mat?searchtype=author&query=Turner%2C+J+J">Joshua J. Turner</a>, <a href="/search/cond-mat?searchtype=author&query=L%C3%BCning%2C+J">Jan L眉ning</a>, <a href="/search/cond-mat?searchtype=author&query=Eisebitt%2C+S">Stefan Eisebitt</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">Christine Boeglin</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1502.00786v1-abstract-short" style="display: inline;"> The evolution of a magnetic domain structure upon excitation by an intense, femtosecond Infra-Red (IR) laser pulse has been investigated using single-shot based time-resolved resonant X-ray scattering at the X-ray Free Electron laser LCLS. A well-ordered stripe domain pattern as present in a thin CoPd alloy film has been used as prototype magnetic domain structure for this study. The fluence of th… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1502.00786v1-abstract-full').style.display = 'inline'; document.getElementById('1502.00786v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1502.00786v1-abstract-full" style="display: none;"> The evolution of a magnetic domain structure upon excitation by an intense, femtosecond Infra-Red (IR) laser pulse has been investigated using single-shot based time-resolved resonant X-ray scattering at the X-ray Free Electron laser LCLS. A well-ordered stripe domain pattern as present in a thin CoPd alloy film has been used as prototype magnetic domain structure for this study. The fluence of the IR laser pump pulse was sufficient to lead to an almost complete quenching of the magnetization within the ultrafast demagnetization process taking place within the first few hundreds of femtoseconds following the IR laser pump pulse excitation. On longer time scales this excitation gave rise to subsequent irreversible transformations of the magnetic domain structure. Under our specific experimental conditions, it took about 2 nanoseconds before the magnetization started to recover. After about 5 nanoseconds the previously ordered stripe domain structure had evolved into a disordered labyrinth domain structure. Surprisingly, we observe after about 7 nanoseconds the occurrence of a partially ordered stripe domain structure reoriented into a novel direction. It is this domain structure in which the sample's magnetization stabilizes as revealed by scattering patterns recorded long after the initial pump-probe cycle. Using micro-magnetic simulations we can explain this observation based on changes of the magnetic anisotropy going along with heat dissipation in the film. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1502.00786v1-abstract-full').style.display = 'none'; document.getElementById('1502.00786v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 3 February, 2015; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> February 2015. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">16 pages, 6 figures</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1301.4885">arXiv:1301.4885</a> <span> [<a href="https://arxiv.org/pdf/1301.4885">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevB.87.214412">10.1103/PhysRevB.87.214412 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Role of critical spin fluctuations in ultrafast demagnetization of transition-metal rare-earth alloys </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&query=Lopez-Flores%2C+V">V. Lopez-Flores</a>, <a href="/search/cond-mat?searchtype=author&query=Bergeard%2C+N">N. Bergeard</a>, <a href="/search/cond-mat?searchtype=author&query=Halte%2C+V">V. Halte</a>, <a href="/search/cond-mat?searchtype=author&query=Stamm%2C+C">C Stamm</a>, <a href="/search/cond-mat?searchtype=author&query=Pontius%2C+N">N. Pontius</a>, <a href="/search/cond-mat?searchtype=author&query=Hehn%2C+M">M. Hehn</a>, <a href="/search/cond-mat?searchtype=author&query=Otero%2C+E">E. Otero</a>, <a href="/search/cond-mat?searchtype=author&query=Beaurepaire%2C+E">E. Beaurepaire</a>, <a href="/search/cond-mat?searchtype=author&query=Boeglin%2C+C">C. Boeglin</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1301.4885v3-abstract-short" style="display: inline;"> Ultrafast magnetization dynamics induced by femtosecond laser pulses have been measured in ferrimagnetic Co0.8Gd0.2, Co.74Tb.26 and Co.86Tb.14 alloys. Using element sensitivity of X-ray magnetic circular dichroism at the Co L3, Tb M5 and Gd M5 edges we evidence that the demagnetization dynamics is element dependent. We show that a thermalization time as fast as 280 fs is observed for the rare-eart… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1301.4885v3-abstract-full').style.display = 'inline'; document.getElementById('1301.4885v3-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1301.4885v3-abstract-full" style="display: none;"> Ultrafast magnetization dynamics induced by femtosecond laser pulses have been measured in ferrimagnetic Co0.8Gd0.2, Co.74Tb.26 and Co.86Tb.14 alloys. Using element sensitivity of X-ray magnetic circular dichroism at the Co L3, Tb M5 and Gd M5 edges we evidence that the demagnetization dynamics is element dependent. We show that a thermalization time as fast as 280 fs is observed for the rare-earth in the alloy, when the laser excited state temperature is below the compensation temperature. It is limited to 500 fs when the laser excited state temperature is below the Curie temperature (Tc). We propose critical spin fluctuations in the vicinity of TC as the mechanism which reduces the demagnetization rates of the 4f electrons in transition-metal rare-earth alloys whereas at any different temperature the limited demagnetization rates could be avoided. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1301.4885v3-abstract-full').style.display = 'none'; document.getElementById('1301.4885v3-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 7 May, 2013; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 21 January, 2013; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2013. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">11 pages, 4 figures</span> </p> </li> 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