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class="user-content-wrapper"><div class="uploads-container" id="social-redesign-work-container"><div class="upload-header"><h2 class="ds2-5-heading-sans-serif-xs">Uploads</h2></div><div class="documents-container backbone-social-profile-documents" style="width: 100%;"><div class="u-taCenter"></div><div class="profile--tab_content_container js-tab-pane tab-pane active" id="all"><div class="profile--tab_heading_container js-section-heading" data-section="Papers" id="Papers"><h3 class="profile--tab_heading_container">Papers by Richard Tuckett</h3></div><div class="js-work-strip profile--work_container" data-work-id="125490149"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490149/The_near_infra_red_emission_band_of_DO_sub_2_sub_determination_of_the_molecular_geometry"><img alt="Research paper thumbnail of The near infra-red emission band of DO<sub>2</sub>: determination of the molecular geometry" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490149/The_near_infra_red_emission_band_of_DO_sub_2_sub_determination_of_the_molecular_geometry">The near infra-red emission band of DO<sub>2</sub>: determination of the molecular geometry</a></div><div class="wp-workCard_item"><span>Molecular Physics</span><span>, Feb 1, 1979</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The 2A&amp;amp;#x27; --&amp;amp;amp;gt;2A&amp;amp;#x27;&amp;amp;#x27; spectrum of DO2 has been re...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The 2A&amp;amp;#x27; --&amp;amp;amp;gt;2A&amp;amp;#x27;&amp;amp;#x27; spectrum of DO2 has been recorded at high resolution in order to determine the geometry of HO2 in these two electronic states. The results obtained are: The HOO bond angle shows little change between the two states.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490149"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490149"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490149; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490149]").text(description); $(".js-view-count[data-work-id=125490149]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490149; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490149']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490149, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490149]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490149,"title":"The near infra-red emission band of DO\u003csub\u003e2\u003c/sub\u003e: determination of the molecular geometry","translated_title":"","metadata":{"abstract":"The 2A\u0026amp;amp;#x27; --\u0026amp;amp;amp;gt;2A\u0026amp;amp;#x27;\u0026amp;amp;#x27; spectrum of DO2 has been recorded at high resolution in order to determine the geometry of HO2 in these two electronic states. The results obtained are: The HOO bond angle shows little change between the two states.","publisher":"Taylor \u0026 Francis","publication_date":{"day":1,"month":2,"year":1979,"errors":{}},"publication_name":"Molecular Physics"},"translated_abstract":"The 2A\u0026amp;amp;#x27; --\u0026amp;amp;amp;gt;2A\u0026amp;amp;#x27;\u0026amp;amp;#x27; spectrum of DO2 has been recorded at high resolution in order to determine the geometry of HO2 in these two electronic states. The results obtained are: The HOO bond angle shows little change between the two states.","internal_url":"https://www.academia.edu/125490149/The_near_infra_red_emission_band_of_DO_sub_2_sub_determination_of_the_molecular_geometry","translated_internal_url":"","created_at":"2024-11-12T08:56:48.561-08:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"The_near_infra_red_emission_band_of_DO_sub_2_sub_determination_of_the_molecular_geometry","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"The 2A\u0026amp;amp;#x27; --\u0026amp;amp;amp;gt;2A\u0026amp;amp;#x27;\u0026amp;amp;#x27; spectrum of DO2 has been recorded at high resolution in order to determine the geometry of HO2 in these two electronic states. The results obtained are: The HOO bond angle shows little change between the two states.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":513,"name":"Molecular Physics","url":"https://www.academia.edu/Documents/in/Molecular_Physics"},{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":54418,"name":"Geometry","url":"https://www.academia.edu/Documents/in/Geometry"},{"id":116193,"name":"Solid State electronic devices","url":"https://www.academia.edu/Documents/in/Solid_State_electronic_devices"},{"id":309086,"name":"High 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href="https://www.academia.edu/125490147/Use_of_threshold_electron_and_fluorescence_coincidence_techniques_to_probe_the_decay_dynamics_of_the_valence_states_of_CF_sup_sup_sub_4_sub_SiF_sup_sup_sub_4_sub_SiCl_sup_sup_sub_4_sub_and_GeCl_sup_sup_sub_4_sub_"><img alt="Research paper thumbnail of Use of threshold electron and fluorescence coincidence techniques to probe the decay dynamics of the valence states of CF<sup>+</sup><sub>4</sub>, SiF<sup>+</sup><sub>4</sub>, SiCl<sup>+</sup><sub>4</sub>, and GeCl<sup>+</sup><sub>4</sub>" class="work-thumbnail" src="https://attachments.academia-assets.com/119523598/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490147/Use_of_threshold_electron_and_fluorescence_coincidence_techniques_to_probe_the_decay_dynamics_of_the_valence_states_of_CF_sup_sup_sub_4_sub_SiF_sup_sup_sub_4_sub_SiCl_sup_sup_sub_4_sub_and_GeCl_sup_sup_sub_4_sub_">Use of threshold electron and fluorescence coincidence techniques to probe the decay dynamics of the valence states of CF<sup>+</sup><sub>4</sub>, SiF<sup>+</sup><sub>4</sub>, SiCl<sup>+</sup><sub>4</sub>, and GeCl<sup>+</sup><sub>4</sub></a></div><div class="wp-workCard_item"><span>Journal of Chemical Physics</span><span>, Dec 15, 1994</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="ce92eec9ee2586ccd9c3069a593105bb" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":119523598,"asset_id":125490147,"asset_type":"Work","button_location":"profile"}" 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src="https://attachments.academia-assets.com/119523597/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490145/PHOTOELECTRON_PHOTOION_COINCIDENCE_STUDY_OF_THE_FRAGMENTATION_OF_VALENCE_STATES_OF_CHF2_CH3_IN_THE_RANGE_12_25_eV">PHOTOELECTRON PHOTOION COINCIDENCE STUDY OF THE FRAGMENTATION OF VALENCE STATES OF CHF2–CH3+ IN THE RANGE 12–25 eV</a></div><div class="wp-workCard_item"><span>International Journal of Modern Physics B</span><span>, Jun 10, 2009</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="ca4bffcdc91fdc08a5c3c6acc67cbf23" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" 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href="https://www.academia.edu/125490144/Electronic_Fluorescence_Spectra_of_Gas_Phase_Positive_Ions"><img alt="Research paper thumbnail of Electronic Fluorescence Spectra of Gas-Phase Positive Ions" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490144/Electronic_Fluorescence_Spectra_of_Gas_Phase_Positive_Ions">Electronic Fluorescence Spectra of Gas-Phase Positive Ions</a></div><div class="wp-workCard_item"><span>Springer eBooks</span><span>, 1983</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">We describe here a novel technique to observe electronic spectra of gas-phase positive ions. The ...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">We describe here a novel technique to observe electronic spectra of gas-phase positive ions. The ions are formed by electron impact on a supersonic beam of neutral molecules, and the fluorescent radiation from the ions is dispersed. The two particular properties of supersonic beams that we exploit are: (a.) The density of molecules in a beam can be high, yet they all travel in the same direction in a collision-free environment. Collisional deactivation of the ion by fast ion-molecule reactions is therefore absent. (b.) In the expansion, random motion of the molecules is converted into forward directed flow, producing a beam of internally cold molecules; the rotational temperature can be less than 1°K.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490144"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490144"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490144; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490144]").text(description); $(".js-view-count[data-work-id=125490144]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490144; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490144']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490144, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490144]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490144,"title":"Electronic Fluorescence Spectra of Gas-Phase Positive Ions","translated_title":"","metadata":{"abstract":"We describe here a novel technique to observe electronic spectra of gas-phase positive ions. 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In the expansion, random motion of the molecules is converted into forward directed flow, producing a beam of internally cold molecules; the rotational temperature can be less than 1°K.","internal_url":"https://www.academia.edu/125490144/Electronic_Fluorescence_Spectra_of_Gas_Phase_Positive_Ions","translated_internal_url":"","created_at":"2024-11-12T08:56:47.453-08:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"Electronic_Fluorescence_Spectra_of_Gas_Phase_Positive_Ions","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"We describe here a novel technique to observe electronic spectra of gas-phase positive ions. The ions are formed by electron impact on a supersonic beam of neutral molecules, and the fluorescent radiation from the ions is dispersed. 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In the expansion, random motion of the molecules is converted into forward directed flow, producing a beam of internally cold molecules; the rotational temperature can be less than 1°K.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":511,"name":"Materials Science","url":"https://www.academia.edu/Documents/in/Materials_Science"},{"id":7698,"name":"Fluorescence","url":"https://www.academia.edu/Documents/in/Fluorescence"},{"id":11740,"name":"Atomic Physics","url":"https://www.academia.edu/Documents/in/Atomic_Physics"},{"id":348756,"name":"Ion","url":"https://www.academia.edu/Documents/in/Ion"},{"id":883316,"name":"Gas Phase","url":"https://www.academia.edu/Documents/in/Gas_Phase"},{"id":1029023,"name":"Molecule","url":"https://www.academia.edu/Documents/in/Molecule"},{"id":2778229,"name":"Supersonic speed","url":"https://www.academia.edu/Documents/in/Supersonic_speed"},{"id":3647879,"name":"Springer Ebooks","url":"https://www.academia.edu/Documents/in/Springer_Ebooks"}],"urls":[{"id":45586979,"url":"https://doi.org/10.1007/978-1-4613-3664-8_13"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="125490143"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490143/Vacuum_UV_fluorescence_excitation_spectroscopy_of_BCl3in_the_range_35_140_nm"><img alt="Research paper thumbnail of Vacuum UV fluorescence excitation spectroscopy of BCl3in the range 35–140 nm" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490143/Vacuum_UV_fluorescence_excitation_spectroscopy_of_BCl3in_the_range_35_140_nm">Vacuum UV fluorescence excitation spectroscopy of BCl3in the range 35–140 nm</a></div><div class="wp-workCard_item"><span>Molecular Physics</span><span>, Jun 10, 1993</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metas...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies &gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. The two strongest resonant peaks at 13·1 a...</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490143"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490143"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490143; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490143]").text(description); $(".js-view-count[data-work-id=125490143]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490143; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490143']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490143, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490143]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490143,"title":"Vacuum UV fluorescence excitation spectroscopy of BCl3in the range 35–140 nm","translated_title":"","metadata":{"abstract":"The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. 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The two strongest resonant peaks at 13·1 a...","publisher":"Taylor \u0026 Francis","publication_date":{"day":10,"month":6,"year":1993,"errors":{}},"publication_name":"Molecular Physics"},"translated_abstract":"The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies \u0026gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. 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"profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="125490142"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490142/The_vacuum_ultraviolet_photoelectron_spectra_of_CH2F2_and_CH2Cl2_revisited"><img alt="Research paper thumbnail of The vacuum-ultraviolet photoelectron spectra of CH2F2 and CH2Cl2 revisited" class="work-thumbnail" src="https://attachments.academia-assets.com/119526016/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490142/The_vacuum_ultraviolet_photoelectron_spectra_of_CH2F2_and_CH2Cl2_revisited">The vacuum-ultraviolet photoelectron spectra of CH2F2 and CH2Cl2 revisited</a></div><div class="wp-workCard_item"><span>Journal of Molecular Spectroscopy</span><span>, Sep 1, 2015</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="1701d856fdf544bd1686b24d6893f789" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":119526016,"asset_id":125490142,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/119526016/download_file?st=MTczMzkwNzA3Miw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490142"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span 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12–25 eV" class="work-thumbnail" src="https://attachments.academia-assets.com/119523593/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490141/Fragmentation_of_valence_electronic_states_of_CF_sub_3_sub_CH_sub_2_sub_F_sup_sup_and_CHF_sub_2_sub_CHF_sub_2_sub_sup_sup_in_the_range_12_25_eV">Fragmentation of valence electronic states of CF<sub>3</sub>–CH<sub>2</sub>F<sup>+</sup>and CHF<sub>2</sub>–CHF<sub>2</sub><sup>+</sup>in the range 12–25 eV</a></div><div class="wp-workCard_item"><span>Physical Chemistry Chemical Physics</span><span>, 2002</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="78172433ba7fd98872e2bb9e3c426702" class="wp-workCard--action" rel="nofollow" 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Physics","url":"https://www.academia.edu/Documents/in/Atomic_Physics"},{"id":22300,"name":"Chemical Physics","url":"https://www.academia.edu/Documents/in/Chemical_Physics"},{"id":118582,"name":"Physical sciences","url":"https://www.academia.edu/Documents/in/Physical_sciences"},{"id":260118,"name":"CHEMICAL SCIENCES","url":"https://www.academia.edu/Documents/in/CHEMICAL_SCIENCES"},{"id":348756,"name":"Ion","url":"https://www.academia.edu/Documents/in/Ion"},{"id":2620537,"name":"Physical chemistry and chemical physics","url":"https://www.academia.edu/Documents/in/Physical_chemistry_and_chemical_physics"}],"urls":[{"id":45586976,"url":"http://pure-oai.bham.ac.uk/ws/files/2922101/Tuckett15PhysChemChemPhys2002.pdf"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="125490140"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490140/Vacuum_UV_fluorescence_excitation_spectroscopy_of_BF3in_the_range_45_125_nm"><img alt="Research paper thumbnail of Vacuum UV fluorescence excitation spectroscopy of BF3in the range 45–125 nm" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490140/Vacuum_UV_fluorescence_excitation_spectroscopy_of_BF3in_the_range_45_125_nm">Vacuum UV fluorescence excitation spectroscopy of BF3in the range 45–125 nm</a></div><div class="wp-workCard_item"><span>Molecular Physics</span><span>, Mar 1, 1993</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metas...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies &gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. The two strongest resonant peaks at 13·1 a...</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490140"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490140"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490140; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490140]").text(description); $(".js-view-count[data-work-id=125490140]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490140; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490140']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490140, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490140]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490140,"title":"Vacuum UV fluorescence excitation spectroscopy of BF3in the range 45–125 nm","translated_title":"","metadata":{"abstract":"The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies \u0026gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. The two strongest resonant peaks at 13·1 a...","publisher":"Taylor \u0026 Francis","publication_date":{"day":1,"month":3,"year":1993,"errors":{}},"publication_name":"Molecular Physics"},"translated_abstract":"The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies \u0026gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. The two strongest resonant peaks at 13·1 a...","internal_url":"https://www.academia.edu/125490140/Vacuum_UV_fluorescence_excitation_spectroscopy_of_BF3in_the_range_45_125_nm","translated_internal_url":"","created_at":"2024-11-12T08:56:44.799-08:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"Vacuum_UV_fluorescence_excitation_spectroscopy_of_BF3in_the_range_45_125_nm","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies \u0026gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. The two strongest resonant peaks at 13·1 a...","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":513,"name":"Molecular Physics","url":"https://www.academia.edu/Documents/in/Molecular_Physics"},{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":923,"name":"Technology","url":"https://www.academia.edu/Documents/in/Technology"},{"id":1525,"name":"Fluorescence Spectroscopy","url":"https://www.academia.edu/Documents/in/Fluorescence_Spectroscopy"},{"id":5427,"name":"Spectroscopy","url":"https://www.academia.edu/Documents/in/Spectroscopy"},{"id":7698,"name":"Fluorescence","url":"https://www.academia.edu/Documents/in/Fluorescence"},{"id":11740,"name":"Atomic 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cross section for the H+D<sub>2</sub>→HD(<i>v</i>′=4, <i>J</i>′=3)+D reaction at a collision energy of 2.2 eV</a></div><div class="wp-workCard_item"><span>Journal of Chemical Physics</span><span>, Sep 22, 1995</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="3d975b7bc6107d22294c562da9318fc1" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":119523623,"asset_id":125490138,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/119523623/download_file?st=MTczMzkwNzA3Miw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490138"><a 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Abstracting Service, delivering concise information at a glance t...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">ABSTRACT ChemInform is a weekly Abstracting Service, delivering concise information at a glance that was extracted from about 100 leading journals. 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$(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="125490133"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490133/The_A_2%CE%A0u_X_2%CE%A0g_emission_spectrum_of_I2_"><img alt="Research paper thumbnail of The A 2Πu-X 2Πg emission spectrum of I2+" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490133/The_A_2%CE%A0u_X_2%CE%A0g_emission_spectrum_of_I2_">The A 2Πu-X 2Πg emission spectrum of I2+</a></div><div class="wp-workCard_item"><span>Chemical Physics Letters</span><span>, Aug 1, 1989</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">Abstract The A 2Πu-X 2Πg electronic emission spectrum of I2+ has been recorded at a low rotationa...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">Abstract The A 2Πu-X 2Πg electronic emission spectrum of I2+ has been recorded at a low rotational temperature in a crossed molecular beam/electron beam apparatus. Six vibrational sequences with five or more members have been assigned to progressions in ν′, giving ω′e = 122±8 cm−1, but a full vibrational analysis has not been possible. It is not known whether this is due to the relatively poor resolution (≈5 cm−1) at which the spectrum has been recorded or because the A 2Πu state is perturbed in one or both spin-orbit components. Existing data on the A state of I2+ are reviewed.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490133"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490133"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490133; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490133]").text(description); $(".js-view-count[data-work-id=125490133]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490133; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490133']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490133, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490133]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490133,"title":"The A 2Πu-X 2Πg emission spectrum of I2+","translated_title":"","metadata":{"abstract":"Abstract The A 2Πu-X 2Πg electronic emission spectrum of I2+ has been recorded at a low rotational temperature in a crossed molecular beam/electron beam apparatus. Six vibrational sequences with five or more members have been assigned to progressions in ν′, giving ω′e = 122±8 cm−1, but a full vibrational analysis has not been possible. It is not known whether this is due to the relatively poor resolution (≈5 cm−1) at which the spectrum has been recorded or because the A 2Πu state is perturbed in one or both spin-orbit components. Existing data on the A state of I2+ are reviewed.","publisher":"Elsevier BV","publication_date":{"day":1,"month":8,"year":1989,"errors":{}},"publication_name":"Chemical Physics Letters"},"translated_abstract":"Abstract The A 2Πu-X 2Πg electronic emission spectrum of I2+ has been recorded at a low rotational temperature in a crossed molecular beam/electron beam apparatus. Six vibrational sequences with five or more members have been assigned to progressions in ν′, giving ω′e = 122±8 cm−1, but a full vibrational analysis has not been possible. It is not known whether this is due to the relatively poor resolution (≈5 cm−1) at which the spectrum has been recorded or because the A 2Πu state is perturbed in one or both spin-orbit components. Existing data on the A state of I2+ are reviewed.","internal_url":"https://www.academia.edu/125490133/The_A_2%CE%A0u_X_2%CE%A0g_emission_spectrum_of_I2_","translated_internal_url":"","created_at":"2024-11-12T08:56:42.670-08:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"The_A_2Πu_X_2Πg_emission_spectrum_of_I2_","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"Abstract The A 2Πu-X 2Πg electronic emission spectrum of I2+ has been recorded at a low rotational temperature in a crossed molecular beam/electron beam apparatus. Six vibrational sequences with five or more members have been assigned to progressions in ν′, giving ω′e = 122±8 cm−1, but a full vibrational analysis has not been possible. It is not known whether this is due to the relatively poor resolution (≈5 cm−1) at which the spectrum has been recorded or because the A 2Πu state is perturbed in one or both spin-orbit components. Existing data on the A state of I2+ are reviewed.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":923,"name":"Technology","url":"https://www.academia.edu/Documents/in/Technology"},{"id":11740,"name":"Atomic Physics","url":"https://www.academia.edu/Documents/in/Atomic_Physics"},{"id":39585,"name":"Molecular beam epitaxy","url":"https://www.academia.edu/Documents/in/Molecular_beam_epitaxy"},{"id":118582,"name":"Physical sciences","url":"https://www.academia.edu/Documents/in/Physical_sciences"},{"id":260118,"name":"CHEMICAL 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data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490132/Vacuum_UV_negative_photoion_spectroscopy_of_CH3F_CH3Cl_and_CH3Br">Vacuum-UV negative photoion spectroscopy of CH3F, CH3Cl and CH3Br</a></div><div class="wp-workCard_item"><span>Physical Chemistry Chemical Physics</span><span>, 2010</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="535769d99166c98505f915a9d0206df7" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":119523588,"asset_id":125490132,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/119523588/download_file?st=MTczMzkwNzA3Myw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span 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class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490076/Vacuum_UV_fluorescence_spectroscopy_of_CCl3F_CCl3H_and_CCl3Br_in_the_range_8_30_eV"><img alt="Research paper thumbnail of Vacuum-UV fluorescence spectroscopy of CCl3F, CCl3H and CCl3Br in the range 8–30 eV" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490076/Vacuum_UV_fluorescence_spectroscopy_of_CCl3F_CCl3H_and_CCl3Br_in_the_range_8_30_eV">Vacuum-UV fluorescence spectroscopy of CCl3F, CCl3H and CCl3Br in the range 8–30 eV</a></div><div class="wp-workCard_item"><span>Physical Chemistry Chemical Physics</span><span>, 1999</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The fluorescence spectroscopy of CCl3X (X=F, H, Br) in the range 200–700 nm is reported, using va...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The fluorescence spectroscopy of CCl3X (X=F, H, Br) in the range 200–700 nm is reported, using vacuum-UV radiation in the range 8–30 eV from a synchrotron as a tunable photoexcitation source. Excitation spectra, with undispersed detection of the fluorescence, have been recorded at the Daresbury UK source with a resolution of 0.1 nm, corresponding to an average energy resolution of ca. 0.015 eV. Dispersed emission spectra in the range 200–700 nm have been recorded at the BESSY 1 Germany source with an optical resolution of 8 nm, following photoexcitation at the energies of the peaks in the excitation spectra. Action spectra, in which the vacuum-UV energy is scanned with detection of the fluorescence at a specific wavelength, have also been recorded at BESSY 1 with a resolution of 0.3 nm; thresholds for production of a particular excited state of a fragment are then obtained. Using single-bunch mode, lifetimes of all the emitting states that fall in the range ca. 3–100 ns have been measured. For photon energies in the range 8–12 eV, emission is due to both CCl2 A1B1–1A1 and CXCl A1A″–1A′. These products form by photodissociation of low-lying Rydberg states of CCl3X, and the thresholds for their production therefore relate to energies of the Rydberg states of the parent molecule. It is not possible to say whether the other products form as two halogen atoms or a diatomic molecule. For energies in the range 13–17 eV, emission is due to diatomic fragments; CCl A2Δ, CF B2Δ, CH B2Σ- and A2Δ, CBr A2Δ, and Cl2 D′ 23Πg. From their threshold energies, there is now accumulated evidence that the excited state of CCl or CX forms in association with three isolated atoms. Our results yield no information on whether the three bonds in CCl3X* break simultaneously or sequentially. In the range 13–17 eV, Cl2* almost certainly forms in conjunction with ground-state CX+Cl. This ion-pair state of Cl2 also forms at higher excitation energies around 20 eV, probably with atomic products C+X+Cl. In no cases is emission observed from excited states of either the CCl3 radical or the parent molecular ion, CCl3X+.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490076"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490076"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490076; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490076]").text(description); $(".js-view-count[data-work-id=125490076]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490076; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490076']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490076, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490076]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490076,"title":"Vacuum-UV fluorescence spectroscopy of CCl3F, CCl3H and CCl3Br in the range 8–30 eV","translated_title":"","metadata":{"abstract":"The fluorescence spectroscopy of CCl3X (X=F, H, Br) in the range 200–700 nm is reported, using vacuum-UV radiation in the range 8–30 eV from a synchrotron as a tunable photoexcitation source. Excitation spectra, with undispersed detection of the fluorescence, have been recorded at the Daresbury UK source with a resolution of 0.1 nm, corresponding to an average energy resolution of ca. 0.015 eV. Dispersed emission spectra in the range 200–700 nm have been recorded at the BESSY 1 Germany source with an optical resolution of 8 nm, following photoexcitation at the energies of the peaks in the excitation spectra. Action spectra, in which the vacuum-UV energy is scanned with detection of the fluorescence at a specific wavelength, have also been recorded at BESSY 1 with a resolution of 0.3 nm; thresholds for production of a particular excited state of a fragment are then obtained. Using single-bunch mode, lifetimes of all the emitting states that fall in the range ca. 3–100 ns have been measured. For photon energies in the range 8–12 eV, emission is due to both CCl2 A1B1–1A1 and CXCl A1A″–1A′. These products form by photodissociation of low-lying Rydberg states of CCl3X, and the thresholds for their production therefore relate to energies of the Rydberg states of the parent molecule. It is not possible to say whether the other products form as two halogen atoms or a diatomic molecule. For energies in the range 13–17 eV, emission is due to diatomic fragments; CCl A2Δ, CF B2Δ, CH B2Σ- and A2Δ, CBr A2Δ, and Cl2 D′ 23Πg. From their threshold energies, there is now accumulated evidence that the excited state of CCl or CX forms in association with three isolated atoms. Our results yield no information on whether the three bonds in CCl3X* break simultaneously or sequentially. In the range 13–17 eV, Cl2* almost certainly forms in conjunction with ground-state CX+Cl. This ion-pair state of Cl2 also forms at higher excitation energies around 20 eV, probably with atomic products C+X+Cl. In no cases is emission observed from excited states of either the CCl3 radical or the parent molecular ion, CCl3X+.","publisher":"Royal Society of Chemistry","publication_date":{"day":null,"month":null,"year":1999,"errors":{}},"publication_name":"Physical Chemistry Chemical Physics"},"translated_abstract":"The fluorescence spectroscopy of CCl3X (X=F, H, Br) in the range 200–700 nm is reported, using vacuum-UV radiation in the range 8–30 eV from a synchrotron as a tunable photoexcitation source. Excitation spectra, with undispersed detection of the fluorescence, have been recorded at the Daresbury UK source with a resolution of 0.1 nm, corresponding to an average energy resolution of ca. 0.015 eV. Dispersed emission spectra in the range 200–700 nm have been recorded at the BESSY 1 Germany source with an optical resolution of 8 nm, following photoexcitation at the energies of the peaks in the excitation spectra. Action spectra, in which the vacuum-UV energy is scanned with detection of the fluorescence at a specific wavelength, have also been recorded at BESSY 1 with a resolution of 0.3 nm; thresholds for production of a particular excited state of a fragment are then obtained. Using single-bunch mode, lifetimes of all the emitting states that fall in the range ca. 3–100 ns have been measured. For photon energies in the range 8–12 eV, emission is due to both CCl2 A1B1–1A1 and CXCl A1A″–1A′. These products form by photodissociation of low-lying Rydberg states of CCl3X, and the thresholds for their production therefore relate to energies of the Rydberg states of the parent molecule. It is not possible to say whether the other products form as two halogen atoms or a diatomic molecule. For energies in the range 13–17 eV, emission is due to diatomic fragments; CCl A2Δ, CF B2Δ, CH B2Σ- and A2Δ, CBr A2Δ, and Cl2 D′ 23Πg. From their threshold energies, there is now accumulated evidence that the excited state of CCl or CX forms in association with three isolated atoms. Our results yield no information on whether the three bonds in CCl3X* break simultaneously or sequentially. In the range 13–17 eV, Cl2* almost certainly forms in conjunction with ground-state CX+Cl. This ion-pair state of Cl2 also forms at higher excitation energies around 20 eV, probably with atomic products C+X+Cl. In no cases is emission observed from excited states of either the CCl3 radical or the parent molecular ion, CCl3X+.","internal_url":"https://www.academia.edu/125490076/Vacuum_UV_fluorescence_spectroscopy_of_CCl3F_CCl3H_and_CCl3Br_in_the_range_8_30_eV","translated_internal_url":"","created_at":"2024-11-12T08:55:42.919-08:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"Vacuum_UV_fluorescence_spectroscopy_of_CCl3F_CCl3H_and_CCl3Br_in_the_range_8_30_eV","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"The fluorescence spectroscopy of CCl3X (X=F, H, Br) in the range 200–700 nm is reported, using vacuum-UV radiation in the range 8–30 eV from a synchrotron as a tunable photoexcitation source. Excitation spectra, with undispersed detection of the fluorescence, have been recorded at the Daresbury UK source with a resolution of 0.1 nm, corresponding to an average energy resolution of ca. 0.015 eV. Dispersed emission spectra in the range 200–700 nm have been recorded at the BESSY 1 Germany source with an optical resolution of 8 nm, following photoexcitation at the energies of the peaks in the excitation spectra. Action spectra, in which the vacuum-UV energy is scanned with detection of the fluorescence at a specific wavelength, have also been recorded at BESSY 1 with a resolution of 0.3 nm; thresholds for production of a particular excited state of a fragment are then obtained. Using single-bunch mode, lifetimes of all the emitting states that fall in the range ca. 3–100 ns have been measured. For photon energies in the range 8–12 eV, emission is due to both CCl2 A1B1–1A1 and CXCl A1A″–1A′. These products form by photodissociation of low-lying Rydberg states of CCl3X, and the thresholds for their production therefore relate to energies of the Rydberg states of the parent molecule. It is not possible to say whether the other products form as two halogen atoms or a diatomic molecule. For energies in the range 13–17 eV, emission is due to diatomic fragments; CCl A2Δ, CF B2Δ, CH B2Σ- and A2Δ, CBr A2Δ, and Cl2 D′ 23Πg. From their threshold energies, there is now accumulated evidence that the excited state of CCl or CX forms in association with three isolated atoms. Our results yield no information on whether the three bonds in CCl3X* break simultaneously or sequentially. In the range 13–17 eV, Cl2* almost certainly forms in conjunction with ground-state CX+Cl. This ion-pair state of Cl2 also forms at higher excitation energies around 20 eV, probably with atomic products C+X+Cl. In no cases is emission observed from excited states of either the CCl3 radical or the parent molecular ion, CCl3X+.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":5427,"name":"Spectroscopy","url":"https://www.academia.edu/Documents/in/Spectroscopy"},{"id":11740,"name":"Atomic Physics","url":"https://www.academia.edu/Documents/in/Atomic_Physics"},{"id":118582,"name":"Physical sciences","url":"https://www.academia.edu/Documents/in/Physical_sciences"},{"id":260118,"name":"CHEMICAL SCIENCES","url":"https://www.academia.edu/Documents/in/CHEMICAL_SCIENCES"},{"id":2376080,"name":"Photoexcitation","url":"https://www.academia.edu/Documents/in/Photoexcitation"},{"id":2620537,"name":"Physical chemistry and chemical physics","url":"https://www.academia.edu/Documents/in/Physical_chemistry_and_chemical_physics"}],"urls":[{"id":45586923,"url":"https://doi.org/10.1039/a809422e"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="121518323"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/121518323/The_i_Dtilde_i_sup_2_sup_i_A_i_sub_1_sub_i_Ctilde_i_sup_2_sup_i_T_i_sub_2_sub_emission_band_system_of_SiF_sup_sup_sub_4_sub_"><img alt="Research paper thumbnail of The<i>[Dtilde]</i><sup>2</sup><i>A</i><sub>1</sub>-<i>[Ctilde]</i><sup>2</sup><i>T</i><sub>2</sub>emission band system of SiF<sup>+</sup><sub>4</sub>" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/121518323/The_i_Dtilde_i_sup_2_sup_i_A_i_sub_1_sub_i_Ctilde_i_sup_2_sup_i_T_i_sub_2_sub_emission_band_system_of_SiF_sup_sup_sub_4_sub_">The<i>[Dtilde]</i><sup>2</sup><i>A</i><sub>1</sub>-<i>[Ctilde]</i><sup>2</sup><i>T</i><sub>2</sub>emission band system of SiF<sup>+</sup><sub>4</sub></a></div><div class="wp-workCard_item"><span>Molecular Physics</span><span>, Mar 1, 1987</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The [Dtilde] 2 A 1-[Ctilde] 2 T 2 emission spectrum of SiF+ 4 is observed at a low rotational tem...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The [Dtilde] 2 A 1-[Ctilde] 2 T 2 emission spectrum of SiF+ 4 is observed at a low rotational temperature in a crossed molecular beam/electron beam apparatus. The narrow rotational envelope of the bands confirms the assignment of the emitter as the parent molecular ion of SiF4. The spectrum is analysed, and the results compare excellently with photoelectron data for SiF4. Spin-orbit splitting and Jahn-Teller distortion are observed in the [Ctilde] 2 T 2 state, with both v 2(e) and v 4(t 2) being Jahn-Teller active vibrations.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="121518323"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="121518323"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 121518323; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=121518323]").text(description); $(".js-view-count[data-work-id=121518323]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 121518323; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='121518323']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 121518323, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=121518323]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":121518323,"title":"The\u003ci\u003e[Dtilde]\u003c/i\u003e\u003csup\u003e2\u003c/sup\u003e\u003ci\u003eA\u003c/i\u003e\u003csub\u003e1\u003c/sub\u003e-\u003ci\u003e[Ctilde]\u003c/i\u003e\u003csup\u003e2\u003c/sup\u003e\u003ci\u003eT\u003c/i\u003e\u003csub\u003e2\u003c/sub\u003eemission band system of SiF\u003csup\u003e+\u003c/sup\u003e\u003csub\u003e4\u003c/sub\u003e","translated_title":"","metadata":{"abstract":"The [Dtilde] 2 A 1-[Ctilde] 2 T 2 emission spectrum of SiF+ 4 is observed at a low rotational temperature in a crossed molecular beam/electron beam apparatus. The narrow rotational envelope of the bands confirms the assignment of the emitter as the parent molecular ion of SiF4. The spectrum is analysed, and the results compare excellently with photoelectron data for SiF4. Spin-orbit splitting and Jahn-Teller distortion are observed in the [Ctilde] 2 T 2 state, with both v 2(e) and v 4(t 2) being Jahn-Teller active vibrations.","publisher":"Taylor \u0026 Francis","publication_date":{"day":1,"month":3,"year":1987,"errors":{}},"publication_name":"Molecular Physics"},"translated_abstract":"The [Dtilde] 2 A 1-[Ctilde] 2 T 2 emission spectrum of SiF+ 4 is observed at a low rotational temperature in a crossed molecular beam/electron beam apparatus. The narrow rotational envelope of the bands confirms the assignment of the emitter as the parent molecular ion of SiF4. The spectrum is analysed, and the results compare excellently with photoelectron data for SiF4. Spin-orbit splitting and Jahn-Teller distortion are observed in the [Ctilde] 2 T 2 state, with both v 2(e) and v 4(t 2) being Jahn-Teller active vibrations.","internal_url":"https://www.academia.edu/121518323/The_i_Dtilde_i_sup_2_sup_i_A_i_sub_1_sub_i_Ctilde_i_sup_2_sup_i_T_i_sub_2_sub_emission_band_system_of_SiF_sup_sup_sub_4_sub_","translated_internal_url":"","created_at":"2024-06-25T23:56:56.667-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"The_i_Dtilde_i_sup_2_sup_i_A_i_sub_1_sub_i_Ctilde_i_sup_2_sup_i_T_i_sub_2_sub_emission_band_system_of_SiF_sup_sup_sub_4_sub_","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"The [Dtilde] 2 A 1-[Ctilde] 2 T 2 emission spectrum of SiF+ 4 is observed at a low rotational temperature in a crossed molecular beam/electron beam apparatus. The narrow rotational envelope of the bands confirms the assignment of the emitter as the parent molecular ion of SiF4. The spectrum is analysed, and the results compare excellently with photoelectron data for SiF4. Spin-orbit splitting and Jahn-Teller distortion are observed in the [Ctilde] 2 T 2 state, with both v 2(e) and v 4(t 2) being Jahn-Teller active vibrations.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":513,"name":"Molecular Physics","url":"https://www.academia.edu/Documents/in/Molecular_Physics"},{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":11740,"name":"Atomic Physics","url":"https://www.academia.edu/Documents/in/Atomic_Physics"},{"id":348756,"name":"Ion","url":"https://www.academia.edu/Documents/in/Ion"},{"id":645605,"name":"THEORETICAL AND COMPUTATIONAL CHEMISTRY","url":"https://www.academia.edu/Documents/in/THEORETICAL_AND_COMPUTATIONAL_CHEMISTRY"},{"id":1213686,"name":"Jahn Teller Effect","url":"https://www.academia.edu/Documents/in/Jahn_Teller_Effect"}],"urls":[{"id":43238747,"url":"https://doi.org/10.1080/00268978700100531"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="121518322"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/121518322/Fragmentation_of_Energy_Selected_SF5CF3_Probed_by_Threshold_Photoelectron_Photoion_Coincidence_Spectroscopy_Bond_Dissociation_Energy_of_SF5_CF3_and_Its_Atmospheric_Implications"><img alt="Research paper thumbnail of Fragmentation of Energy-Selected SF5CF3+ Probed by Threshold Photoelectron Photoion Coincidence Spectroscopy: Bond Dissociation Energy of SF5-CF3 and Its Atmospheric Implications" class="work-thumbnail" src="https://attachments.academia-assets.com/116371908/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/121518322/Fragmentation_of_Energy_Selected_SF5CF3_Probed_by_Threshold_Photoelectron_Photoion_Coincidence_Spectroscopy_Bond_Dissociation_Energy_of_SF5_CF3_and_Its_Atmospheric_Implications">Fragmentation of Energy-Selected SF5CF3+ Probed by Threshold Photoelectron Photoion Coincidence Spectroscopy: Bond Dissociation Energy of SF5-CF3 and Its Atmospheric Implications</a></div><div class="wp-workCard_item"><span>Journal of Physical Chemistry A</span><span>, Aug 24, 2001</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">Where a licence is displayed above, please note the terms and conditions of the licence govern yo...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">Where a licence is displayed above, please note the terms and conditions of the licence govern your use of this document. When citing, please reference the published version. Take down policy While the University of Birmingham exercises care and attention in making items available there are rare occasions when an item has been uploaded in error or has been deemed to be commercially or otherwise sensitive.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="c0b035e053c424a9c1803e0dabd86417" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":116371908,"asset_id":121518322,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/116371908/download_file?st=MTczMzkwNzA3Myw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="121518322"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="121518322"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 121518322; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=121518322]").text(description); $(".js-view-count[data-work-id=121518322]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 121518322; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='121518322']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 121518322, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (true){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "c0b035e053c424a9c1803e0dabd86417" } } $('.js-work-strip[data-work-id=121518322]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":121518322,"title":"Fragmentation of Energy-Selected SF5CF3+ Probed by Threshold Photoelectron Photoion Coincidence Spectroscopy: Bond Dissociation Energy of SF5-CF3 and Its Atmospheric Implications","translated_title":"","metadata":{"publisher":"American Chemical Society","grobid_abstract":"Where a licence is displayed above, please note the terms and conditions of the licence govern your use of this document. When citing, please reference the published version. Take down policy While the University of Birmingham exercises care and attention in making items available there are rare occasions when an item has been uploaded in error or has been deemed to be commercially or otherwise sensitive.","publication_date":{"day":24,"month":8,"year":2001,"errors":{}},"publication_name":"Journal of Physical Chemistry A","grobid_abstract_attachment_id":116371908},"translated_abstract":null,"internal_url":"https://www.academia.edu/121518322/Fragmentation_of_Energy_Selected_SF5CF3_Probed_by_Threshold_Photoelectron_Photoion_Coincidence_Spectroscopy_Bond_Dissociation_Energy_of_SF5_CF3_and_Its_Atmospheric_Implications","translated_internal_url":"","created_at":"2024-06-25T23:56:56.456-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[{"id":116371908,"title":"","file_type":"pdf","scribd_thumbnail_url":"https://attachments.academia-assets.com/116371908/thumbnails/1.jpg","file_name":"Tuckett8JPhysChemA2001.pdf","download_url":"https://www.academia.edu/attachments/116371908/download_file?st=MTczMzkwNzA3Myw4LjIyMi4yMDguMTQ2&","bulk_download_file_name":"Fragmentation_of_Energy_Selected_SF5CF3.pdf","bulk_download_url":"https://d1wqtxts1xzle7.cloudfront.net/116371908/Tuckett8JPhysChemA2001-libre.pdf?1719392273=\u0026response-content-disposition=attachment%3B+filename%3DFragmentation_of_Energy_Selected_SF5CF3.pdf\u0026Expires=1733910673\u0026Signature=Z-ZHF08tt4EPbenORT4dlfeylfcW5b0FToxmzzhcjRqFENNj4KsEizHkn5SH2XYExLII4OCetAfYvXH9tFSIl59LoKq~VGp38FgVSqz5xb7roatxUXedVxE7MiMp2ubmsGKesWo9www~9JFDyBeY9NEobg9fHPFP-cXoUEypWUwcPQcVlxiH28FN-Po~Isw2~vVk350ER2Rswp8HiGFc11LGQA34vwmE2IVflrPC~5dxlmJJX7GT7sZXyEOAC8U4R6siBjfFwPEcYD72ke5enCwPu6xBt907hGchqMIiazoXu3SWpTEBzlq2zdUYs0D-CWn28LurJO3R0XD~3GupDQ__\u0026Key-Pair-Id=APKAJLOHF5GGSLRBV4ZA"}],"slug":"Fragmentation_of_Energy_Selected_SF5CF3_Probed_by_Threshold_Photoelectron_Photoion_Coincidence_Spectroscopy_Bond_Dissociation_Energy_of_SF5_CF3_and_Its_Atmospheric_Implications","translated_slug":"","page_count":32,"language":"en","content_type":"Work","summary":"Where a licence is displayed above, please note the terms and conditions of the licence govern your use of this document. When citing, please reference the published version. 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The ions are produced by electron impact on a supersonic molecular beam, and the resulting fluorescent radiation is dispersed. Some results on N 2 , N 2 O and CO 2 are presented. They suggest that this technique could be most productive for studying large polyatomic cations.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="121518321"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="121518321"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 121518321; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=121518321]").text(description); $(".js-view-count[data-work-id=121518321]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 121518321; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='121518321']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 121518321, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=121518321]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":121518321,"title":"Electronic fluorescence spectra of gas-phase positive molecular ions","translated_title":"","metadata":{"abstract":"Abstract A new technique for observing electronic spectra of gas-phase positive molecular ions is described. 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They suggest that this technique could be most productive for studying large polyatomic cations.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":923,"name":"Technology","url":"https://www.academia.edu/Documents/in/Technology"},{"id":7698,"name":"Fluorescence","url":"https://www.academia.edu/Documents/in/Fluorescence"},{"id":39585,"name":"Molecular beam epitaxy","url":"https://www.academia.edu/Documents/in/Molecular_beam_epitaxy"},{"id":118582,"name":"Physical sciences","url":"https://www.academia.edu/Documents/in/Physical_sciences"},{"id":260118,"name":"CHEMICAL SCIENCES","url":"https://www.academia.edu/Documents/in/CHEMICAL_SCIENCES"},{"id":348756,"name":"Ion","url":"https://www.academia.edu/Documents/in/Ion"},{"id":883316,"name":"Gas Phase","url":"https://www.academia.edu/Documents/in/Gas_Phase"},{"id":2778229,"name":"Supersonic speed","url":"https://www.academia.edu/Documents/in/Supersonic_speed"}],"urls":[{"id":43238745,"url":"https://doi.org/10.1016/0009-2614(80)85005-6"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> </div><div class="profile--tab_content_container js-tab-pane tab-pane" data-section-id="12423179" id="papers"><div class="js-work-strip profile--work_container" data-work-id="125490149"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490149/The_near_infra_red_emission_band_of_DO_sub_2_sub_determination_of_the_molecular_geometry"><img alt="Research paper thumbnail of The near infra-red emission band of DO<sub>2</sub>: determination of the molecular geometry" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490149/The_near_infra_red_emission_band_of_DO_sub_2_sub_determination_of_the_molecular_geometry">The near infra-red emission band of DO<sub>2</sub>: determination of the molecular geometry</a></div><div class="wp-workCard_item"><span>Molecular Physics</span><span>, Feb 1, 1979</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The 2A&amp;amp;#x27; --&amp;amp;amp;gt;2A&amp;amp;#x27;&amp;amp;#x27; spectrum of DO2 has been re...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The 2A&amp;amp;#x27; --&amp;amp;amp;gt;2A&amp;amp;#x27;&amp;amp;#x27; spectrum of DO2 has been recorded at high resolution in order to determine the geometry of HO2 in these two electronic states. The results obtained are: The HOO bond angle shows little change between the two states.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490149"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490149"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490149; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490149]").text(description); $(".js-view-count[data-work-id=125490149]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490149; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490149']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490149, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490149]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490149,"title":"The near infra-red emission band of DO\u003csub\u003e2\u003c/sub\u003e: determination of the molecular geometry","translated_title":"","metadata":{"abstract":"The 2A\u0026amp;amp;#x27; --\u0026amp;amp;amp;gt;2A\u0026amp;amp;#x27;\u0026amp;amp;#x27; spectrum of DO2 has been recorded at high resolution in order to determine the geometry of HO2 in these two electronic states. The results obtained are: The HOO bond angle shows little change between the two states.","publisher":"Taylor \u0026 Francis","publication_date":{"day":1,"month":2,"year":1979,"errors":{}},"publication_name":"Molecular Physics"},"translated_abstract":"The 2A\u0026amp;amp;#x27; --\u0026amp;amp;amp;gt;2A\u0026amp;amp;#x27;\u0026amp;amp;#x27; spectrum of DO2 has been recorded at high resolution in order to determine the geometry of HO2 in these two electronic states. The results obtained are: The HOO bond angle shows little change between the two states.","internal_url":"https://www.academia.edu/125490149/The_near_infra_red_emission_band_of_DO_sub_2_sub_determination_of_the_molecular_geometry","translated_internal_url":"","created_at":"2024-11-12T08:56:48.561-08:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"The_near_infra_red_emission_band_of_DO_sub_2_sub_determination_of_the_molecular_geometry","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"The 2A\u0026amp;amp;#x27; --\u0026amp;amp;amp;gt;2A\u0026amp;amp;#x27;\u0026amp;amp;#x27; spectrum of DO2 has been recorded at high resolution in order to determine the geometry of HO2 in these two electronic states. The results obtained are: The HOO bond angle shows little change between the two states.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":513,"name":"Molecular Physics","url":"https://www.academia.edu/Documents/in/Molecular_Physics"},{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":54418,"name":"Geometry","url":"https://www.academia.edu/Documents/in/Geometry"},{"id":116193,"name":"Solid State electronic devices","url":"https://www.academia.edu/Documents/in/Solid_State_electronic_devices"},{"id":309086,"name":"High 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href="https://www.academia.edu/125490147/Use_of_threshold_electron_and_fluorescence_coincidence_techniques_to_probe_the_decay_dynamics_of_the_valence_states_of_CF_sup_sup_sub_4_sub_SiF_sup_sup_sub_4_sub_SiCl_sup_sup_sub_4_sub_and_GeCl_sup_sup_sub_4_sub_"><img alt="Research paper thumbnail of Use of threshold electron and fluorescence coincidence techniques to probe the decay dynamics of the valence states of CF<sup>+</sup><sub>4</sub>, SiF<sup>+</sup><sub>4</sub>, SiCl<sup>+</sup><sub>4</sub>, and GeCl<sup>+</sup><sub>4</sub>" class="work-thumbnail" src="https://attachments.academia-assets.com/119523598/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490147/Use_of_threshold_electron_and_fluorescence_coincidence_techniques_to_probe_the_decay_dynamics_of_the_valence_states_of_CF_sup_sup_sub_4_sub_SiF_sup_sup_sub_4_sub_SiCl_sup_sup_sub_4_sub_and_GeCl_sup_sup_sub_4_sub_">Use of threshold electron and fluorescence coincidence techniques to probe the decay dynamics of the valence states of CF<sup>+</sup><sub>4</sub>, SiF<sup>+</sup><sub>4</sub>, SiCl<sup>+</sup><sub>4</sub>, and GeCl<sup>+</sup><sub>4</sub></a></div><div class="wp-workCard_item"><span>Journal of Chemical Physics</span><span>, Dec 15, 1994</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="ce92eec9ee2586ccd9c3069a593105bb" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":119523598,"asset_id":125490147,"asset_type":"Work","button_location":"profile"}" 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href="https://www.academia.edu/125490144/Electronic_Fluorescence_Spectra_of_Gas_Phase_Positive_Ions"><img alt="Research paper thumbnail of Electronic Fluorescence Spectra of Gas-Phase Positive Ions" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490144/Electronic_Fluorescence_Spectra_of_Gas_Phase_Positive_Ions">Electronic Fluorescence Spectra of Gas-Phase Positive Ions</a></div><div class="wp-workCard_item"><span>Springer eBooks</span><span>, 1983</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">We describe here a novel technique to observe electronic spectra of gas-phase positive ions. The ...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">We describe here a novel technique to observe electronic spectra of gas-phase positive ions. The ions are formed by electron impact on a supersonic beam of neutral molecules, and the fluorescent radiation from the ions is dispersed. The two particular properties of supersonic beams that we exploit are: (a.) The density of molecules in a beam can be high, yet they all travel in the same direction in a collision-free environment. Collisional deactivation of the ion by fast ion-molecule reactions is therefore absent. (b.) In the expansion, random motion of the molecules is converted into forward directed flow, producing a beam of internally cold molecules; the rotational temperature can be less than 1°K.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490144"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490144"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490144; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490144]").text(description); $(".js-view-count[data-work-id=125490144]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490144; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490144']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490144, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490144]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490144,"title":"Electronic Fluorescence Spectra of Gas-Phase Positive Ions","translated_title":"","metadata":{"abstract":"We describe here a novel technique to observe electronic spectra of gas-phase positive ions. 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In the expansion, random motion of the molecules is converted into forward directed flow, producing a beam of internally cold molecules; the rotational temperature can be less than 1°K.","internal_url":"https://www.academia.edu/125490144/Electronic_Fluorescence_Spectra_of_Gas_Phase_Positive_Ions","translated_internal_url":"","created_at":"2024-11-12T08:56:47.453-08:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"Electronic_Fluorescence_Spectra_of_Gas_Phase_Positive_Ions","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"We describe here a novel technique to observe electronic spectra of gas-phase positive ions. The ions are formed by electron impact on a supersonic beam of neutral molecules, and the fluorescent radiation from the ions is dispersed. 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In the expansion, random motion of the molecules is converted into forward directed flow, producing a beam of internally cold molecules; the rotational temperature can be less than 1°K.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":511,"name":"Materials Science","url":"https://www.academia.edu/Documents/in/Materials_Science"},{"id":7698,"name":"Fluorescence","url":"https://www.academia.edu/Documents/in/Fluorescence"},{"id":11740,"name":"Atomic Physics","url":"https://www.academia.edu/Documents/in/Atomic_Physics"},{"id":348756,"name":"Ion","url":"https://www.academia.edu/Documents/in/Ion"},{"id":883316,"name":"Gas Phase","url":"https://www.academia.edu/Documents/in/Gas_Phase"},{"id":1029023,"name":"Molecule","url":"https://www.academia.edu/Documents/in/Molecule"},{"id":2778229,"name":"Supersonic speed","url":"https://www.academia.edu/Documents/in/Supersonic_speed"},{"id":3647879,"name":"Springer Ebooks","url":"https://www.academia.edu/Documents/in/Springer_Ebooks"}],"urls":[{"id":45586979,"url":"https://doi.org/10.1007/978-1-4613-3664-8_13"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="125490143"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490143/Vacuum_UV_fluorescence_excitation_spectroscopy_of_BCl3in_the_range_35_140_nm"><img alt="Research paper thumbnail of Vacuum UV fluorescence excitation spectroscopy of BCl3in the range 35–140 nm" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490143/Vacuum_UV_fluorescence_excitation_spectroscopy_of_BCl3in_the_range_35_140_nm">Vacuum UV fluorescence excitation spectroscopy of BCl3in the range 35–140 nm</a></div><div class="wp-workCard_item"><span>Molecular Physics</span><span>, Jun 10, 1993</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metas...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies &gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. The two strongest resonant peaks at 13·1 a...</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490143"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490143"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490143; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490143]").text(description); $(".js-view-count[data-work-id=125490143]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490143; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490143']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490143, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490143]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490143,"title":"Vacuum UV fluorescence excitation spectroscopy of BCl3in the range 35–140 nm","translated_title":"","metadata":{"abstract":"The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. 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The two strongest resonant peaks at 13·1 a...","publisher":"Taylor \u0026 Francis","publication_date":{"day":10,"month":6,"year":1993,"errors":{}},"publication_name":"Molecular Physics"},"translated_abstract":"The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies \u0026gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. 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The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies \u0026gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. 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12–25 eV" class="work-thumbnail" src="https://attachments.academia-assets.com/119523593/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490141/Fragmentation_of_valence_electronic_states_of_CF_sub_3_sub_CH_sub_2_sub_F_sup_sup_and_CHF_sub_2_sub_CHF_sub_2_sub_sup_sup_in_the_range_12_25_eV">Fragmentation of valence electronic states of CF<sub>3</sub>–CH<sub>2</sub>F<sup>+</sup>and CHF<sub>2</sub>–CHF<sub>2</sub><sup>+</sup>in the range 12–25 eV</a></div><div class="wp-workCard_item"><span>Physical Chemistry Chemical Physics</span><span>, 2002</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="78172433ba7fd98872e2bb9e3c426702" class="wp-workCard--action" rel="nofollow" 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hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490140/Vacuum_UV_fluorescence_excitation_spectroscopy_of_BF3in_the_range_45_125_nm"><img alt="Research paper thumbnail of Vacuum UV fluorescence excitation spectroscopy of BF3in the range 45–125 nm" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490140/Vacuum_UV_fluorescence_excitation_spectroscopy_of_BF3in_the_range_45_125_nm">Vacuum UV fluorescence excitation spectroscopy of BF3in the range 45–125 nm</a></div><div class="wp-workCard_item"><span>Molecular Physics</span><span>, Mar 1, 1993</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metas...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies &gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. The two strongest resonant peaks at 13·1 a...</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490140"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490140"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490140; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490140]").text(description); $(".js-view-count[data-work-id=125490140]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490140; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490140']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490140, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490140]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490140,"title":"Vacuum UV fluorescence excitation spectroscopy of BF3in the range 45–125 nm","translated_title":"","metadata":{"abstract":"The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. 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The two strongest resonant peaks at 13·1 a...","publisher":"Taylor \u0026 Francis","publication_date":{"day":1,"month":3,"year":1993,"errors":{}},"publication_name":"Molecular Physics"},"translated_abstract":"The fluorescence following excitation of BF3 is studied using two techniques: (a) He* (23S) metastable excitation with dispersed fluorescence detection, (b) photon excitation using tunable vacuum UV radiation from a synchrotron source with undispersed detection. The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies \u0026gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. 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The He* experiment gives an extensive spectrum between 200 and 300 nm with two long progressions, each of separation 525 ± 30 cm-1. They are assigned to transitions to the v 2 bending mode of BF2 [Xtilde] 2A1, probably from the first excited state A 2B1. Using photons in the energy range 10–28 eV two different fluorescence decay channels are observed: (1) BF2 fluorescence for photon energies below 17eV, (2) BF3 + fluorescence for energies \u0026gt; 21·5eV. The shapes of the excitation functions confirm that (1) is a resonant process via Rydberg states of BF3, whereas (2) is a non-resonant photoionization process. The emitting state in BF3 + is the [Etilde]2A′1 state with a vertical ionization potential of 21·5eV. 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class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490138/Measurement_of_the_state_specific_differential_cross_section_for_the_H_D_sub_2_sub_HD_i_v_i_4_i_J_i_3_D_reaction_at_a_collision_energy_of_2_2_eV"><img alt="Research paper thumbnail of Measurement of the state‐specific differential cross section for the H+D<sub>2</sub>→HD(<i>v</i>′=4, <i>J</i>′=3)+D reaction at a collision energy of 2.2 eV" class="work-thumbnail" src="https://attachments.academia-assets.com/119523623/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490138/Measurement_of_the_state_specific_differential_cross_section_for_the_H_D_sub_2_sub_HD_i_v_i_4_i_J_i_3_D_reaction_at_a_collision_energy_of_2_2_eV">Measurement of the state‐specific differential cross section for the H+D<sub>2</sub>→HD(<i>v</i>′=4, <i>J</i>′=3)+D reaction at a collision energy of 2.2 eV</a></div><div class="wp-workCard_item"><span>Journal of Chemical Physics</span><span>, Sep 22, 1995</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="3d975b7bc6107d22294c562da9318fc1" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":119523623,"asset_id":125490138,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/119523623/download_file?st=MTczMzkwNzA3Myw4LjIyMi4yMDguMTQ2&st=MTczMzkwNzA3Miw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" 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href="https://www.academia.edu/125490134/The_use_of_threshold_photoelectron_fluorescence_photon_coincidence_spectroscopy_for_the_measurement_of_the_radiative_lifetimes_of_emitting_states_of_CF3X_X_F_H_Cl_Br_ions"><img alt="Research paper thumbnail of The use of threshold photoelectron - fluorescence photon coincidence spectroscopy for the measurement of the radiative lifetimes of emitting states of CF3X+ (X = F, H, Cl, Br) ions" class="work-thumbnail" src="https://attachments.academia-assets.com/119523622/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490134/The_use_of_threshold_photoelectron_fluorescence_photon_coincidence_spectroscopy_for_the_measurement_of_the_radiative_lifetimes_of_emitting_states_of_CF3X_X_F_H_Cl_Br_ions">The use of threshold photoelectron - fluorescence photon coincidence spectroscopy for the measurement of the radiative lifetimes of emitting states of CF3X+ (X = F, H, Cl, Br) ions</a></div><div class="wp-workCard_item"><span>Chemical Physics</span><span>, 1997</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="9e823f1a0685f016e9dc239722777000" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":119523622,"asset_id":125490134,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/119523622/download_file?st=MTczMzkwNzA3Myw4LjIyMi4yMDguMTQ2&st=MTczMzkwNzA3Myw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" 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class="js-work-strip profile--work_container" data-work-id="125490133"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490133/The_A_2%CE%A0u_X_2%CE%A0g_emission_spectrum_of_I2_"><img alt="Research paper thumbnail of The A 2Πu-X 2Πg emission spectrum of I2+" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490133/The_A_2%CE%A0u_X_2%CE%A0g_emission_spectrum_of_I2_">The A 2Πu-X 2Πg emission spectrum of I2+</a></div><div class="wp-workCard_item"><span>Chemical Physics Letters</span><span>, Aug 1, 1989</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">Abstract The A 2Πu-X 2Πg electronic emission spectrum of I2+ has been recorded at a low rotationa...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">Abstract The A 2Πu-X 2Πg electronic emission spectrum of I2+ has been recorded at a low rotational temperature in a crossed molecular beam/electron beam apparatus. Six vibrational sequences with five or more members have been assigned to progressions in ν′, giving ω′e = 122±8 cm−1, but a full vibrational analysis has not been possible. It is not known whether this is due to the relatively poor resolution (≈5 cm−1) at which the spectrum has been recorded or because the A 2Πu state is perturbed in one or both spin-orbit components. Existing data on the A state of I2+ are reviewed.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490133"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490133"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490133; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490133]").text(description); $(".js-view-count[data-work-id=125490133]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490133; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490133']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490133, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490133]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490133,"title":"The A 2Πu-X 2Πg emission spectrum of I2+","translated_title":"","metadata":{"abstract":"Abstract The A 2Πu-X 2Πg electronic emission spectrum of I2+ has been recorded at a low rotational temperature in a crossed molecular beam/electron beam apparatus. Six vibrational sequences with five or more members have been assigned to progressions in ν′, giving ω′e = 122±8 cm−1, but a full vibrational analysis has not been possible. It is not known whether this is due to the relatively poor resolution (≈5 cm−1) at which the spectrum has been recorded or because the A 2Πu state is perturbed in one or both spin-orbit components. Existing data on the A state of I2+ are reviewed.","publisher":"Elsevier BV","publication_date":{"day":1,"month":8,"year":1989,"errors":{}},"publication_name":"Chemical Physics Letters"},"translated_abstract":"Abstract The A 2Πu-X 2Πg electronic emission spectrum of I2+ has been recorded at a low rotational temperature in a crossed molecular beam/electron beam apparatus. Six vibrational sequences with five or more members have been assigned to progressions in ν′, giving ω′e = 122±8 cm−1, but a full vibrational analysis has not been possible. It is not known whether this is due to the relatively poor resolution (≈5 cm−1) at which the spectrum has been recorded or because the A 2Πu state is perturbed in one or both spin-orbit components. Existing data on the A state of I2+ are reviewed.","internal_url":"https://www.academia.edu/125490133/The_A_2%CE%A0u_X_2%CE%A0g_emission_spectrum_of_I2_","translated_internal_url":"","created_at":"2024-11-12T08:56:42.670-08:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"The_A_2Πu_X_2Πg_emission_spectrum_of_I2_","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"Abstract The A 2Πu-X 2Πg electronic emission spectrum of I2+ has been recorded at a low rotational temperature in a crossed molecular beam/electron beam apparatus. Six vibrational sequences with five or more members have been assigned to progressions in ν′, giving ω′e = 122±8 cm−1, but a full vibrational analysis has not been possible. It is not known whether this is due to the relatively poor resolution (≈5 cm−1) at which the spectrum has been recorded or because the A 2Πu state is perturbed in one or both spin-orbit components. Existing data on the A state of I2+ are reviewed.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":923,"name":"Technology","url":"https://www.academia.edu/Documents/in/Technology"},{"id":11740,"name":"Atomic Physics","url":"https://www.academia.edu/Documents/in/Atomic_Physics"},{"id":39585,"name":"Molecular beam epitaxy","url":"https://www.academia.edu/Documents/in/Molecular_beam_epitaxy"},{"id":118582,"name":"Physical sciences","url":"https://www.academia.edu/Documents/in/Physical_sciences"},{"id":260118,"name":"CHEMICAL 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data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490132/Vacuum_UV_negative_photoion_spectroscopy_of_CH3F_CH3Cl_and_CH3Br">Vacuum-UV negative photoion spectroscopy of CH3F, CH3Cl and CH3Br</a></div><div class="wp-workCard_item"><span>Physical Chemistry Chemical Physics</span><span>, 2010</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><a id="535769d99166c98505f915a9d0206df7" class="wp-workCard--action" rel="nofollow" data-click-track="profile-work-strip-download" data-download="{"attachment_id":119523588,"asset_id":125490132,"asset_type":"Work","button_location":"profile"}" href="https://www.academia.edu/attachments/119523588/download_file?st=MTczMzkwNzA3Myw4LjIyMi4yMDguMTQ2&st=MTczMzkwNzA3Myw4LjIyMi4yMDguMTQ2&s=profile"><span><i class="fa fa-arrow-down"></i></span><span>Download</span></a><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: 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class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/125490076/Vacuum_UV_fluorescence_spectroscopy_of_CCl3F_CCl3H_and_CCl3Br_in_the_range_8_30_eV"><img alt="Research paper thumbnail of Vacuum-UV fluorescence spectroscopy of CCl3F, CCl3H and CCl3Br in the range 8–30 eV" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/125490076/Vacuum_UV_fluorescence_spectroscopy_of_CCl3F_CCl3H_and_CCl3Br_in_the_range_8_30_eV">Vacuum-UV fluorescence spectroscopy of CCl3F, CCl3H and CCl3Br in the range 8–30 eV</a></div><div class="wp-workCard_item"><span>Physical Chemistry Chemical Physics</span><span>, 1999</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The fluorescence spectroscopy of CCl3X (X=F, H, Br) in the range 200–700 nm is reported, using va...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The fluorescence spectroscopy of CCl3X (X=F, H, Br) in the range 200–700 nm is reported, using vacuum-UV radiation in the range 8–30 eV from a synchrotron as a tunable photoexcitation source. Excitation spectra, with undispersed detection of the fluorescence, have been recorded at the Daresbury UK source with a resolution of 0.1 nm, corresponding to an average energy resolution of ca. 0.015 eV. Dispersed emission spectra in the range 200–700 nm have been recorded at the BESSY 1 Germany source with an optical resolution of 8 nm, following photoexcitation at the energies of the peaks in the excitation spectra. Action spectra, in which the vacuum-UV energy is scanned with detection of the fluorescence at a specific wavelength, have also been recorded at BESSY 1 with a resolution of 0.3 nm; thresholds for production of a particular excited state of a fragment are then obtained. Using single-bunch mode, lifetimes of all the emitting states that fall in the range ca. 3–100 ns have been measured. For photon energies in the range 8–12 eV, emission is due to both CCl2 A1B1–1A1 and CXCl A1A″–1A′. These products form by photodissociation of low-lying Rydberg states of CCl3X, and the thresholds for their production therefore relate to energies of the Rydberg states of the parent molecule. It is not possible to say whether the other products form as two halogen atoms or a diatomic molecule. For energies in the range 13–17 eV, emission is due to diatomic fragments; CCl A2Δ, CF B2Δ, CH B2Σ- and A2Δ, CBr A2Δ, and Cl2 D′ 23Πg. From their threshold energies, there is now accumulated evidence that the excited state of CCl or CX forms in association with three isolated atoms. Our results yield no information on whether the three bonds in CCl3X* break simultaneously or sequentially. In the range 13–17 eV, Cl2* almost certainly forms in conjunction with ground-state CX+Cl. This ion-pair state of Cl2 also forms at higher excitation energies around 20 eV, probably with atomic products C+X+Cl. In no cases is emission observed from excited states of either the CCl3 radical or the parent molecular ion, CCl3X+.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="125490076"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="125490076"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 125490076; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=125490076]").text(description); $(".js-view-count[data-work-id=125490076]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 125490076; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='125490076']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 125490076, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=125490076]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":125490076,"title":"Vacuum-UV fluorescence spectroscopy of CCl3F, CCl3H and CCl3Br in the range 8–30 eV","translated_title":"","metadata":{"abstract":"The fluorescence spectroscopy of CCl3X (X=F, H, Br) in the range 200–700 nm is reported, using vacuum-UV radiation in the range 8–30 eV from a synchrotron as a tunable photoexcitation source. Excitation spectra, with undispersed detection of the fluorescence, have been recorded at the Daresbury UK source with a resolution of 0.1 nm, corresponding to an average energy resolution of ca. 0.015 eV. Dispersed emission spectra in the range 200–700 nm have been recorded at the BESSY 1 Germany source with an optical resolution of 8 nm, following photoexcitation at the energies of the peaks in the excitation spectra. Action spectra, in which the vacuum-UV energy is scanned with detection of the fluorescence at a specific wavelength, have also been recorded at BESSY 1 with a resolution of 0.3 nm; thresholds for production of a particular excited state of a fragment are then obtained. Using single-bunch mode, lifetimes of all the emitting states that fall in the range ca. 3–100 ns have been measured. For photon energies in the range 8–12 eV, emission is due to both CCl2 A1B1–1A1 and CXCl A1A″–1A′. These products form by photodissociation of low-lying Rydberg states of CCl3X, and the thresholds for their production therefore relate to energies of the Rydberg states of the parent molecule. It is not possible to say whether the other products form as two halogen atoms or a diatomic molecule. For energies in the range 13–17 eV, emission is due to diatomic fragments; CCl A2Δ, CF B2Δ, CH B2Σ- and A2Δ, CBr A2Δ, and Cl2 D′ 23Πg. From their threshold energies, there is now accumulated evidence that the excited state of CCl or CX forms in association with three isolated atoms. Our results yield no information on whether the three bonds in CCl3X* break simultaneously or sequentially. In the range 13–17 eV, Cl2* almost certainly forms in conjunction with ground-state CX+Cl. This ion-pair state of Cl2 also forms at higher excitation energies around 20 eV, probably with atomic products C+X+Cl. In no cases is emission observed from excited states of either the CCl3 radical or the parent molecular ion, CCl3X+.","publisher":"Royal Society of Chemistry","publication_date":{"day":null,"month":null,"year":1999,"errors":{}},"publication_name":"Physical Chemistry Chemical Physics"},"translated_abstract":"The fluorescence spectroscopy of CCl3X (X=F, H, Br) in the range 200–700 nm is reported, using vacuum-UV radiation in the range 8–30 eV from a synchrotron as a tunable photoexcitation source. Excitation spectra, with undispersed detection of the fluorescence, have been recorded at the Daresbury UK source with a resolution of 0.1 nm, corresponding to an average energy resolution of ca. 0.015 eV. Dispersed emission spectra in the range 200–700 nm have been recorded at the BESSY 1 Germany source with an optical resolution of 8 nm, following photoexcitation at the energies of the peaks in the excitation spectra. Action spectra, in which the vacuum-UV energy is scanned with detection of the fluorescence at a specific wavelength, have also been recorded at BESSY 1 with a resolution of 0.3 nm; thresholds for production of a particular excited state of a fragment are then obtained. Using single-bunch mode, lifetimes of all the emitting states that fall in the range ca. 3–100 ns have been measured. For photon energies in the range 8–12 eV, emission is due to both CCl2 A1B1–1A1 and CXCl A1A″–1A′. These products form by photodissociation of low-lying Rydberg states of CCl3X, and the thresholds for their production therefore relate to energies of the Rydberg states of the parent molecule. It is not possible to say whether the other products form as two halogen atoms or a diatomic molecule. For energies in the range 13–17 eV, emission is due to diatomic fragments; CCl A2Δ, CF B2Δ, CH B2Σ- and A2Δ, CBr A2Δ, and Cl2 D′ 23Πg. From their threshold energies, there is now accumulated evidence that the excited state of CCl or CX forms in association with three isolated atoms. Our results yield no information on whether the three bonds in CCl3X* break simultaneously or sequentially. In the range 13–17 eV, Cl2* almost certainly forms in conjunction with ground-state CX+Cl. This ion-pair state of Cl2 also forms at higher excitation energies around 20 eV, probably with atomic products C+X+Cl. In no cases is emission observed from excited states of either the CCl3 radical or the parent molecular ion, CCl3X+.","internal_url":"https://www.academia.edu/125490076/Vacuum_UV_fluorescence_spectroscopy_of_CCl3F_CCl3H_and_CCl3Br_in_the_range_8_30_eV","translated_internal_url":"","created_at":"2024-11-12T08:55:42.919-08:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"Vacuum_UV_fluorescence_spectroscopy_of_CCl3F_CCl3H_and_CCl3Br_in_the_range_8_30_eV","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"The fluorescence spectroscopy of CCl3X (X=F, H, Br) in the range 200–700 nm is reported, using vacuum-UV radiation in the range 8–30 eV from a synchrotron as a tunable photoexcitation source. Excitation spectra, with undispersed detection of the fluorescence, have been recorded at the Daresbury UK source with a resolution of 0.1 nm, corresponding to an average energy resolution of ca. 0.015 eV. Dispersed emission spectra in the range 200–700 nm have been recorded at the BESSY 1 Germany source with an optical resolution of 8 nm, following photoexcitation at the energies of the peaks in the excitation spectra. Action spectra, in which the vacuum-UV energy is scanned with detection of the fluorescence at a specific wavelength, have also been recorded at BESSY 1 with a resolution of 0.3 nm; thresholds for production of a particular excited state of a fragment are then obtained. Using single-bunch mode, lifetimes of all the emitting states that fall in the range ca. 3–100 ns have been measured. For photon energies in the range 8–12 eV, emission is due to both CCl2 A1B1–1A1 and CXCl A1A″–1A′. These products form by photodissociation of low-lying Rydberg states of CCl3X, and the thresholds for their production therefore relate to energies of the Rydberg states of the parent molecule. It is not possible to say whether the other products form as two halogen atoms or a diatomic molecule. For energies in the range 13–17 eV, emission is due to diatomic fragments; CCl A2Δ, CF B2Δ, CH B2Σ- and A2Δ, CBr A2Δ, and Cl2 D′ 23Πg. From their threshold energies, there is now accumulated evidence that the excited state of CCl or CX forms in association with three isolated atoms. Our results yield no information on whether the three bonds in CCl3X* break simultaneously or sequentially. In the range 13–17 eV, Cl2* almost certainly forms in conjunction with ground-state CX+Cl. This ion-pair state of Cl2 also forms at higher excitation energies around 20 eV, probably with atomic products C+X+Cl. In no cases is emission observed from excited states of either the CCl3 radical or the parent molecular ion, CCl3X+.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":5427,"name":"Spectroscopy","url":"https://www.academia.edu/Documents/in/Spectroscopy"},{"id":11740,"name":"Atomic Physics","url":"https://www.academia.edu/Documents/in/Atomic_Physics"},{"id":118582,"name":"Physical sciences","url":"https://www.academia.edu/Documents/in/Physical_sciences"},{"id":260118,"name":"CHEMICAL SCIENCES","url":"https://www.academia.edu/Documents/in/CHEMICAL_SCIENCES"},{"id":2376080,"name":"Photoexcitation","url":"https://www.academia.edu/Documents/in/Photoexcitation"},{"id":2620537,"name":"Physical chemistry and chemical physics","url":"https://www.academia.edu/Documents/in/Physical_chemistry_and_chemical_physics"}],"urls":[{"id":45586923,"url":"https://doi.org/10.1039/a809422e"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="121518323"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/121518323/The_i_Dtilde_i_sup_2_sup_i_A_i_sub_1_sub_i_Ctilde_i_sup_2_sup_i_T_i_sub_2_sub_emission_band_system_of_SiF_sup_sup_sub_4_sub_"><img alt="Research paper thumbnail of The<i>[Dtilde]</i><sup>2</sup><i>A</i><sub>1</sub>-<i>[Ctilde]</i><sup>2</sup><i>T</i><sub>2</sub>emission band system of SiF<sup>+</sup><sub>4</sub>" class="work-thumbnail" src="https://a.academia-assets.com/images/blank-paper.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/121518323/The_i_Dtilde_i_sup_2_sup_i_A_i_sub_1_sub_i_Ctilde_i_sup_2_sup_i_T_i_sub_2_sub_emission_band_system_of_SiF_sup_sup_sub_4_sub_">The<i>[Dtilde]</i><sup>2</sup><i>A</i><sub>1</sub>-<i>[Ctilde]</i><sup>2</sup><i>T</i><sub>2</sub>emission band system of SiF<sup>+</sup><sub>4</sub></a></div><div class="wp-workCard_item"><span>Molecular Physics</span><span>, Mar 1, 1987</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">The [Dtilde] 2 A 1-[Ctilde] 2 T 2 emission spectrum of SiF+ 4 is observed at a low rotational tem...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">The [Dtilde] 2 A 1-[Ctilde] 2 T 2 emission spectrum of SiF+ 4 is observed at a low rotational temperature in a crossed molecular beam/electron beam apparatus. The narrow rotational envelope of the bands confirms the assignment of the emitter as the parent molecular ion of SiF4. The spectrum is analysed, and the results compare excellently with photoelectron data for SiF4. Spin-orbit splitting and Jahn-Teller distortion are observed in the [Ctilde] 2 T 2 state, with both v 2(e) and v 4(t 2) being Jahn-Teller active vibrations.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="121518323"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="121518323"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 121518323; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=121518323]").text(description); $(".js-view-count[data-work-id=121518323]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 121518323; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='121518323']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 121518323, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=121518323]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":121518323,"title":"The\u003ci\u003e[Dtilde]\u003c/i\u003e\u003csup\u003e2\u003c/sup\u003e\u003ci\u003eA\u003c/i\u003e\u003csub\u003e1\u003c/sub\u003e-\u003ci\u003e[Ctilde]\u003c/i\u003e\u003csup\u003e2\u003c/sup\u003e\u003ci\u003eT\u003c/i\u003e\u003csub\u003e2\u003c/sub\u003eemission band system of SiF\u003csup\u003e+\u003c/sup\u003e\u003csub\u003e4\u003c/sub\u003e","translated_title":"","metadata":{"abstract":"The [Dtilde] 2 A 1-[Ctilde] 2 T 2 emission spectrum of SiF+ 4 is observed at a low rotational temperature in a crossed molecular beam/electron beam apparatus. The narrow rotational envelope of the bands confirms the assignment of the emitter as the parent molecular ion of SiF4. The spectrum is analysed, and the results compare excellently with photoelectron data for SiF4. Spin-orbit splitting and Jahn-Teller distortion are observed in the [Ctilde] 2 T 2 state, with both v 2(e) and v 4(t 2) being Jahn-Teller active vibrations.","publisher":"Taylor \u0026 Francis","publication_date":{"day":1,"month":3,"year":1987,"errors":{}},"publication_name":"Molecular Physics"},"translated_abstract":"The [Dtilde] 2 A 1-[Ctilde] 2 T 2 emission spectrum of SiF+ 4 is observed at a low rotational temperature in a crossed molecular beam/electron beam apparatus. The narrow rotational envelope of the bands confirms the assignment of the emitter as the parent molecular ion of SiF4. The spectrum is analysed, and the results compare excellently with photoelectron data for SiF4. Spin-orbit splitting and Jahn-Teller distortion are observed in the [Ctilde] 2 T 2 state, with both v 2(e) and v 4(t 2) being Jahn-Teller active vibrations.","internal_url":"https://www.academia.edu/121518323/The_i_Dtilde_i_sup_2_sup_i_A_i_sub_1_sub_i_Ctilde_i_sup_2_sup_i_T_i_sub_2_sub_emission_band_system_of_SiF_sup_sup_sub_4_sub_","translated_internal_url":"","created_at":"2024-06-25T23:56:56.667-07:00","preview_url":null,"current_user_can_edit":null,"current_user_is_owner":null,"owner_id":32346837,"coauthors_can_edit":true,"document_type":"paper","co_author_tags":[],"downloadable_attachments":[],"slug":"The_i_Dtilde_i_sup_2_sup_i_A_i_sub_1_sub_i_Ctilde_i_sup_2_sup_i_T_i_sub_2_sub_emission_band_system_of_SiF_sup_sup_sub_4_sub_","translated_slug":"","page_count":null,"language":"en","content_type":"Work","summary":"The [Dtilde] 2 A 1-[Ctilde] 2 T 2 emission spectrum of SiF+ 4 is observed at a low rotational temperature in a crossed molecular beam/electron beam apparatus. The narrow rotational envelope of the bands confirms the assignment of the emitter as the parent molecular ion of SiF4. The spectrum is analysed, and the results compare excellently with photoelectron data for SiF4. Spin-orbit splitting and Jahn-Teller distortion are observed in the [Ctilde] 2 T 2 state, with both v 2(e) and v 4(t 2) being Jahn-Teller active vibrations.","owner":{"id":32346837,"first_name":"Richard","middle_initials":null,"last_name":"Tuckett","page_name":"RichardTuckett","domain_name":"bham","created_at":"2015-06-19T03:00:24.265-07:00","display_name":"Richard Tuckett","url":"https://bham.academia.edu/RichardTuckett"},"attachments":[],"research_interests":[{"id":513,"name":"Molecular Physics","url":"https://www.academia.edu/Documents/in/Molecular_Physics"},{"id":523,"name":"Chemistry","url":"https://www.academia.edu/Documents/in/Chemistry"},{"id":11740,"name":"Atomic Physics","url":"https://www.academia.edu/Documents/in/Atomic_Physics"},{"id":348756,"name":"Ion","url":"https://www.academia.edu/Documents/in/Ion"},{"id":645605,"name":"THEORETICAL AND COMPUTATIONAL CHEMISTRY","url":"https://www.academia.edu/Documents/in/THEORETICAL_AND_COMPUTATIONAL_CHEMISTRY"},{"id":1213686,"name":"Jahn Teller Effect","url":"https://www.academia.edu/Documents/in/Jahn_Teller_Effect"}],"urls":[{"id":43238747,"url":"https://doi.org/10.1080/00268978700100531"}]}, dispatcherData: dispatcherData }); $(this).data('initialized', true); } }); $a.trackClickSource(".js-work-strip-work-link", "profile_work_strip") }); </script> <div class="js-work-strip profile--work_container" data-work-id="121518322"><div class="profile--work_thumbnail hidden-xs"><a class="js-work-strip-work-link" data-click-track="profile-work-strip-thumbnail" href="https://www.academia.edu/121518322/Fragmentation_of_Energy_Selected_SF5CF3_Probed_by_Threshold_Photoelectron_Photoion_Coincidence_Spectroscopy_Bond_Dissociation_Energy_of_SF5_CF3_and_Its_Atmospheric_Implications"><img alt="Research paper thumbnail of Fragmentation of Energy-Selected SF5CF3+ Probed by Threshold Photoelectron Photoion Coincidence Spectroscopy: Bond Dissociation Energy of SF5-CF3 and Its Atmospheric Implications" class="work-thumbnail" src="https://attachments.academia-assets.com/116371908/thumbnails/1.jpg" /></a></div><div class="wp-workCard wp-workCard_itemContainer"><div class="wp-workCard_item wp-workCard--title"><a class="js-work-strip-work-link text-gray-darker" data-click-track="profile-work-strip-title" href="https://www.academia.edu/121518322/Fragmentation_of_Energy_Selected_SF5CF3_Probed_by_Threshold_Photoelectron_Photoion_Coincidence_Spectroscopy_Bond_Dissociation_Energy_of_SF5_CF3_and_Its_Atmospheric_Implications">Fragmentation of Energy-Selected SF5CF3+ Probed by Threshold Photoelectron Photoion Coincidence Spectroscopy: Bond Dissociation Energy of SF5-CF3 and Its Atmospheric Implications</a></div><div class="wp-workCard_item"><span>Journal of Physical Chemistry A</span><span>, Aug 24, 2001</span></div><div class="wp-workCard_item"><span class="js-work-more-abstract-truncated">Where a licence is displayed above, please note the terms and conditions of the licence govern yo...</span><a class="js-work-more-abstract" data-broccoli-component="work_strip.more_abstract" data-click-track="profile-work-strip-more-abstract" href="javascript:;"><span> more </span><span><i class="fa fa-caret-down"></i></span></a><span class="js-work-more-abstract-untruncated hidden">Where a licence is displayed above, please note the terms and conditions of the licence govern your use of this document. 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The ions are produced by electron impact on a supersonic molecular beam, and the resulting fluorescent radiation is dispersed. Some results on N 2 , N 2 O and CO 2 are presented. They suggest that this technique could be most productive for studying large polyatomic cations.</span></div><div class="wp-workCard_item wp-workCard--actions"><span class="work-strip-bookmark-button-container"></span><span class="wp-workCard--action visible-if-viewed-by-owner inline-block" style="display: none;"><span class="js-profile-work-strip-edit-button-wrapper profile-work-strip-edit-button-wrapper" data-work-id="121518321"><a class="js-profile-work-strip-edit-button" tabindex="0"><span><i class="fa fa-pencil"></i></span><span>Edit</span></a></span></span><span id="work-strip-rankings-button-container"></span></div><div class="wp-workCard_item wp-workCard--stats"><span><span><span class="js-view-count view-count u-mr2x" data-work-id="121518321"><i class="fa fa-spinner fa-spin"></i></span><script>$(function () { var workId = 121518321; window.Academia.workViewCountsFetcher.queue(workId, function (count) { var description = window.$h.commaizeInt(count) + " " + window.$h.pluralize(count, 'View'); $(".js-view-count[data-work-id=121518321]").text(description); $(".js-view-count[data-work-id=121518321]").attr('title', description).tooltip(); }); });</script></span></span><span><span class="percentile-widget hidden"><span class="u-mr2x work-percentile"></span></span><script>$(function () { var workId = 121518321; window.Academia.workPercentilesFetcher.queue(workId, function (percentileText) { var container = $(".js-work-strip[data-work-id='121518321']"); container.find('.work-percentile').text(percentileText.charAt(0).toUpperCase() + percentileText.slice(1)); container.find('.percentile-widget').show(); container.find('.percentile-widget').removeClass('hidden'); }); });</script></span><span><script>$(function() { new Works.PaperRankView({ workId: 121518321, container: "", }); });</script></span></div><div id="work-strip-premium-row-container"></div></div></div><script> require.config({ waitSeconds: 90 })(["https://a.academia-assets.com/assets/wow_profile-f77ea15d77ce96025a6048a514272ad8becbad23c641fc2b3bd6e24ca6ff1932.js","https://a.academia-assets.com/assets/work_edit-ad038b8c047c1a8d4fa01b402d530ff93c45fee2137a149a4a5398bc8ad67560.js"], function() { // from javascript_helper.rb var dispatcherData = {} if (false){ window.WowProfile.dispatcher = window.WowProfile.dispatcher || _.clone(Backbone.Events); dispatcherData = { dispatcher: window.WowProfile.dispatcher, downloadLinkId: "-1" } } $('.js-work-strip[data-work-id=121518321]').each(function() { if (!$(this).data('initialized')) { new WowProfile.WorkStripView({ el: this, workJSON: {"id":121518321,"title":"Electronic fluorescence spectra of gas-phase positive molecular ions","translated_title":"","metadata":{"abstract":"Abstract A new technique for observing electronic spectra of gas-phase positive molecular ions is described. 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