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class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Weller%2C+M">M. Weller</a>, <a href="/search/physics?searchtype=author&query=Kastirke%2C+G">G. Kastirke</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Goy%2C+C">C. Goy</a>, <a href="/search/physics?searchtype=author&query=Khan%2C+A">A. Khan</a>, <a href="/search/physics?searchtype=author&query=Kircher%2C+M">M. Kircher</a>, <a href="/search/physics?searchtype=author&query=Rauch%2C+C">C. Rauch</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Sisourat%2C+N">N. Sisourat</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2411.14620v1-abstract-short" style="display: inline;"> Electronically excited atoms or molecules may deexcite by emission of a secondary electron through an Auger-Meitner decay. This deexcitation process is typically considered to be exponential in time. This is strictly speaking, however, only true for the case of an atom. Here, we present a study experimentally demonstrating the non-exponential time dependence of the decay of an inner-shell hole in… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2411.14620v1-abstract-full').style.display = 'inline'; document.getElementById('2411.14620v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2411.14620v1-abstract-full" style="display: none;"> Electronically excited atoms or molecules may deexcite by emission of a secondary electron through an Auger-Meitner decay. This deexcitation process is typically considered to be exponential in time. This is strictly speaking, however, only true for the case of an atom. Here, we present a study experimentally demonstrating the non-exponential time dependence of the decay of an inner-shell hole in a diatomic molecule. In addition, we provide an intuitive explanation for the origin of the observed variation of the molecular lifetimes and their dependence on the kinetic energy of the ionic fragments measured in coincidence with the photoelectrons. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2411.14620v1-abstract-full').style.display = 'none'; document.getElementById('2411.14620v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 21 November, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> November 2024. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">5 pages, 4 figures</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2402.03215">arXiv:2402.03215</a> <span> [<a href="https://arxiv.org/pdf/2402.03215">pdf</a>, <a href="https://arxiv.org/format/2402.03215">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Quantum Physics">quant-ph</span> </div> </div> <p class="title is-5 mathjax"> Sub-cycle resolved strong field ionization of chiral molecules and the origin of chiral photoelectron asymmetries </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Hofmann%2C+M">M. Hofmann</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Geyer%2C+A">A. Geyer</a>, <a href="/search/physics?searchtype=author&query=Anders%2C+N">N. Anders</a>, <a href="/search/physics?searchtype=author&query=Kruse%2C+J">J. Kruse</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2402.03215v1-abstract-short" style="display: inline;"> We report on strong field ionization of S- and R-propylene oxide in circularly polarized two-color laser fields. We find that the relative helicity of the two single color laser fields affects the photoelectron circular dichroism (PECD). Further, we observe that PECD is modulated as a function of the sub-cycle release time of the electron. Our experimental observations are successfully described b… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2402.03215v1-abstract-full').style.display = 'inline'; document.getElementById('2402.03215v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2402.03215v1-abstract-full" style="display: none;"> We report on strong field ionization of S- and R-propylene oxide in circularly polarized two-color laser fields. We find that the relative helicity of the two single color laser fields affects the photoelectron circular dichroism (PECD). Further, we observe that PECD is modulated as a function of the sub-cycle release time of the electron. Our experimental observations are successfully described by a heuristic model based on electrons in chiral initial states, which are selectively liberated by the laser field and, after tunneling, interact with an achiral Coulomb potential. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2402.03215v1-abstract-full').style.display = 'none'; document.getElementById('2402.03215v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 5 February, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> February 2024. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2110.08601">arXiv:2110.08601</a> <span> [<a href="https://arxiv.org/pdf/2110.08601">pdf</a>, <a href="https://arxiv.org/format/2110.08601">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.128.023201">10.1103/PhysRevLett.128.023201 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Magnetic-field effect in high-order above-threshold ionization </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Lin%2C+K">Kang Lin</a>, <a href="/search/physics?searchtype=author&query=Brennecke%2C+S">Simon Brennecke</a>, <a href="/search/physics?searchtype=author&query=Ni%2C+H">Hongcheng Ni</a>, <a href="/search/physics?searchtype=author&query=Chen%2C+X">Xiang Chen</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">Alexander Hartung</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">Daniel Trabert</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">Kilian Fehre</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">Jonas Rist</a>, <a href="/search/physics?searchtype=author&query=Tong%2C+X">Xiao-Min Tong</a>, <a href="/search/physics?searchtype=author&query=Burgd%C3%B6rfer%2C+J">Joachim Burgd枚rfer</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">Lothar. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">Markus S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">Till Jahnke</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">Maksim Kunitski</a>, <a href="/search/physics?searchtype=author&query=He%2C+F">Feng He</a>, <a href="/search/physics?searchtype=author&query=Lein%2C+M">Manfred Lein</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">Sebastian Eckart</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">Reinhard D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2110.08601v1-abstract-short" style="display: inline;"> We experimentally and theoretically investigate the influence of the magnetic component of an electromagnetic field on high-order above-threshold ionization of xenon atoms driven by ultrashort femtosecond laser pulses. The nondipole shift of the electron momentum distribution along the light-propagation direction for high energy electrons beyond the classical cutoff is found to be vastly different… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2110.08601v1-abstract-full').style.display = 'inline'; document.getElementById('2110.08601v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2110.08601v1-abstract-full" style="display: none;"> We experimentally and theoretically investigate the influence of the magnetic component of an electromagnetic field on high-order above-threshold ionization of xenon atoms driven by ultrashort femtosecond laser pulses. The nondipole shift of the electron momentum distribution along the light-propagation direction for high energy electrons beyond the classical cutoff is found to be vastly different from that below the cutoff. A V-shape structure in the momentum dependence of the nondipole shift above the cutoff is identified for the first time. With the help of classical and quantum-orbit analysis, we show that large-angle rescattering of the electrons strongly alters the partitioning of the photon momentum between electron and ion. The sensitivity of the observed nondipole shift to the electronic structure of the target atom is confirmed by three-dimensional time-dependent Schr枚dinger equation simulations for different model potentials. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2110.08601v1-abstract-full').style.display = 'none'; document.getElementById('2110.08601v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 16 October, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> October 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">6 pages, 3 figures</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2110.04027">arXiv:2110.04027</a> <span> [<a href="https://arxiv.org/pdf/2110.04027">pdf</a>, <a href="https://arxiv.org/format/2110.04027">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> </div> <p class="title is-5 mathjax"> Photoelectron energy peaks shift against the radiation pressure in strong field ionization </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Lin%2C+K">Kang Lin</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">Sebastian Eckart</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">Alexander Hartung</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">Daniel Trabert</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">Kilian Fehre</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">Jonas Rist</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">Markus S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">Till Jahnke</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">Maksim Kunitski</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">Reinhard D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2110.04027v1-abstract-short" style="display: inline;"> The photoelectric effect describes the ejection of an electron upon absorption of one or several photons. The kinetic energy of this electron is determined by the photon energy reduced by the binding energy of the electron and, if strong laser fields are involved, by the ponderomotive potential in addition. It has therefore been widely taken for granted that for atoms and molecules the photoelectr… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2110.04027v1-abstract-full').style.display = 'inline'; document.getElementById('2110.04027v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2110.04027v1-abstract-full" style="display: none;"> The photoelectric effect describes the ejection of an electron upon absorption of one or several photons. The kinetic energy of this electron is determined by the photon energy reduced by the binding energy of the electron and, if strong laser fields are involved, by the ponderomotive potential in addition. It has therefore been widely taken for granted that for atoms and molecules the photoelectron energy does not depend on the electron's emission direction but theoretical studies have questioned this since 1990. Here we provide experimental evidence, that the energies of photoelectrons emitted against the light-propagation direction are shifted towards higher values while those electrons that are emitted along the light-propagation direction are shifted to lower values. We attribute the energy shift to a nondipole contribution from the interaction of the moving electrons with the incident photons. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2110.04027v1-abstract-full').style.display = 'none'; document.getElementById('2110.04027v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 8 October, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> October 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">6 pages, 4 figures</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2108.10426">arXiv:2108.10426</a> <span> [<a href="https://arxiv.org/pdf/2108.10426">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Quantum Physics">quant-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1126/sciadv.abq8227">10.1126/sciadv.abq8227 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Ultrafast preparation and strong-field ionization of an atomic Bell-like state </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Geyer%2C+A">A. Geyer</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2108.10426v1-abstract-short" style="display: inline;"> Molecules are many body systems with a substantial amount of entanglement between their electrons. Is there a way to break the molecular bond of a diatomic molecule and obtain two atoms in their ground state which are still entangled and form a Bell-like state? We present a scheme that allows for the preparation of such entangled atomic states from single oxygen molecules on femtosecond time scale… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2108.10426v1-abstract-full').style.display = 'inline'; document.getElementById('2108.10426v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2108.10426v1-abstract-full" style="display: none;"> Molecules are many body systems with a substantial amount of entanglement between their electrons. Is there a way to break the molecular bond of a diatomic molecule and obtain two atoms in their ground state which are still entangled and form a Bell-like state? We present a scheme that allows for the preparation of such entangled atomic states from single oxygen molecules on femtosecond time scales. The two neutral oxygen atoms are entangled in the magnetic quantum number of their valence electrons. In a time-delayed probe step, we employ non-adiabatic tunnel ionization, which is a magnetic quantum number-sensitive mechanism. We then investigate correlations by comparing single and double ionization probabilities of the Bell-like state. The experimental results agree with the predictions for an entangled state. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2108.10426v1-abstract-full').style.display = 'none'; document.getElementById('2108.10426v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 23 August, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> August 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">20 pages, 7 figures, 1 table</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Sci. Adv. 9 (2023) eabq8227 </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2107.05994">arXiv:2107.05994</a> <span> [<a href="https://arxiv.org/pdf/2107.05994">pdf</a>, <a href="https://arxiv.org/format/2107.05994">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1038/s41467-021-26994-2">10.1038/s41467-021-26994-2 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Measuring the photoelectron emission delay in the molecular frame </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Rist%2C+J">Jonas Rist</a>, <a href="/search/physics?searchtype=author&query=Klyssek%2C+K">Kim Klyssek</a>, <a href="/search/physics?searchtype=author&query=Novikovskiy%2C+N+M">Nikolay M. Novikovskiy</a>, <a href="/search/physics?searchtype=author&query=Kircher%2C+M">Max Kircher</a>, <a href="/search/physics?searchtype=author&query=Vela-P%C3%A9rez%2C+I">Isabel Vela-P茅rez</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">Daniel Trabert</a>, <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">Sven Grundmann</a>, <a href="/search/physics?searchtype=author&query=Tsitsonis%2C+D">Dimitrios Tsitsonis</a>, <a href="/search/physics?searchtype=author&query=Siebert%2C+J">Juliane Siebert</a>, <a href="/search/physics?searchtype=author&query=Geyer%2C+A">Angelina Geyer</a>, <a href="/search/physics?searchtype=author&query=Melzer%2C+N">Niklas Melzer</a>, <a href="/search/physics?searchtype=author&query=Schwarz%2C+C">Christian Schwarz</a>, <a href="/search/physics?searchtype=author&query=Anders%2C+N">Nils Anders</a>, <a href="/search/physics?searchtype=author&query=Kaiser%2C+L">Leon Kaiser</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">Kilian Fehre</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">Alexander Hartung</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">Sebastian Eckart</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">Lothar Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">Markus S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Davis%2C+V+T">Vernon T. Davis</a>, <a href="/search/physics?searchtype=author&query=Williams%2C+J+B">Joshua B. Williams</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">Florian Trinter</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">Reinhard D枚rner</a>, <a href="/search/physics?searchtype=author&query=Demekhin%2C+P+V">Philipp V. Demekhin</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">Till Jahnke</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2107.05994v1-abstract-short" style="display: inline;"> If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort intervals became possible. While these types of studies require attosecond experimental precision, we present here a novel measurement approach that avoids tho… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2107.05994v1-abstract-full').style.display = 'inline'; document.getElementById('2107.05994v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2107.05994v1-abstract-full" style="display: none;"> If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort intervals became possible. While these types of studies require attosecond experimental precision, we present here a novel measurement approach that avoids those experimental difficulties. We instead extract the emission delay from the interference pattern generated as the emitted photoelectron is diffracted by the parent ion's potential. Targeting core electrons in CO, we measured a 2d map of photoelectron emission delays in the molecular frame over a wide range of electron energies. The measured emission times depend drastically on the emission direction and exhibit characteristic changes along the shape resonance of the molecule. Our approach can be routinely extended to other electron orbitals and more complex molecules. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2107.05994v1-abstract-full').style.display = 'none'; document.getElementById('2107.05994v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 13 July, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> July 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Nat Commun 12, 6657 (2021) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2106.14170">arXiv:2106.14170</a> <span> [<a href="https://arxiv.org/pdf/2106.14170">pdf</a>, <a href="https://arxiv.org/format/2106.14170">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic and Molecular Clusters">physics.atm-clus</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.127.103201">10.1103/PhysRevLett.127.103201 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Fourfold Differential Photoelectron Circular Dichroism </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Novikovskiy%2C+N+M">N. M. Novikovskiy</a>, <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">S. Grundmann</a>, <a href="/search/physics?searchtype=author&query=Kastirke%2C+G">G. Kastirke</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">A. Hartung</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Janke%2C+C">C. Janke</a>, <a href="/search/physics?searchtype=author&query=Nalin%2C+G">G. Nalin</a>, <a href="/search/physics?searchtype=author&query=Pitzer%2C+M">M. Pitzer</a>, <a href="/search/physics?searchtype=author&query=Zeller%2C+S">S. Zeller</a>, <a href="/search/physics?searchtype=author&query=Wiegandt%2C+F">F. Wiegandt</a>, <a href="/search/physics?searchtype=author&query=Weller%2C+M">M. Weller</a>, <a href="/search/physics?searchtype=author&query=Kircher%2C+M">M. Kircher</a>, <a href="/search/physics?searchtype=author&query=Hofmann%2C+M">M. Hofmann</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Knie%2C+A">A. Knie</a>, <a href="/search/physics?searchtype=author&query=Hans%2C+A">A. Hans</a>, <a href="/search/physics?searchtype=author&query=Ltaief%2C+L+B">L. Ben Ltaief</a>, <a href="/search/physics?searchtype=author&query=Ehresmann%2C+A">A. Ehresmann</a>, <a href="/search/physics?searchtype=author&query=Berger%2C+R">R. Berger</a>, <a href="/search/physics?searchtype=author&query=Fukuzawa%2C+H">H. Fukuzawa</a>, <a href="/search/physics?searchtype=author&query=Ueda%2C+K">K. Ueda</a> , et al. (6 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2106.14170v1-abstract-short" style="display: inline;"> We report on a joint experimental and theoretical study of photoelectron circular dichroism (PECD) in methyloxirane. By detecting O 1s-photoelectrons in coincidence with fragment ions, we deduce the molecule's orientation and photoelectron emission direction in the laboratory frame. Thereby, we retrieve a fourfold differential PECD clearly beyond 50%. This strong chiral asymmetry is reproduced by… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2106.14170v1-abstract-full').style.display = 'inline'; document.getElementById('2106.14170v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2106.14170v1-abstract-full" style="display: none;"> We report on a joint experimental and theoretical study of photoelectron circular dichroism (PECD) in methyloxirane. By detecting O 1s-photoelectrons in coincidence with fragment ions, we deduce the molecule's orientation and photoelectron emission direction in the laboratory frame. Thereby, we retrieve a fourfold differential PECD clearly beyond 50%. This strong chiral asymmetry is reproduced by ab initio electronic structure calculations. Providing such a pronounced contrast makes PECD of fixed-in-space chiral molecules an even more sensitive tool for chiral recognition in the gas phase. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2106.14170v1-abstract-full').style.display = 'none'; document.getElementById('2106.14170v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 27 June, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> June 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">5 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 127, 103201 (2021) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2105.11897">arXiv:2105.11897</a> <span> [<a href="https://arxiv.org/pdf/2105.11897">pdf</a>, <a href="https://arxiv.org/format/2105.11897">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1039/D2CP05942H">10.1039/D2CP05942H <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> High-Energy Molecular-Frame Photoelectron Angular Distributions: A Molecular Bond-Length Ruler </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Vela-Per%C3%A9z%2C+I">Isabel Vela-Per茅z</a>, <a href="/search/physics?searchtype=author&query=Ota%2C+F">Fukiko Ota</a>, <a href="/search/physics?searchtype=author&query=Mhamdi%2C+A">Abir Mhamdi</a>, <a href="/search/physics?searchtype=author&query=Tamura%2C+Y">Yoshiaki Tamura</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">Jonas Rist</a>, <a href="/search/physics?searchtype=author&query=Melzer%2C+N">Niklas Melzer</a>, <a href="/search/physics?searchtype=author&query=Uerken%2C+S">Safak Uerken</a>, <a href="/search/physics?searchtype=author&query=Nalin%2C+G">Giammarco Nalin</a>, <a href="/search/physics?searchtype=author&query=Anders%2C+N">Nils Anders</a>, <a href="/search/physics?searchtype=author&query=You%2C+D">Daehyun You</a>, <a href="/search/physics?searchtype=author&query=Kircher%2C+M">Max Kircher</a>, <a href="/search/physics?searchtype=author&query=Janke%2C+C">Christian Janke</a>, <a href="/search/physics?searchtype=author&query=Waitz%2C+M">Markus Waitz</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">Florian Trinter</a>, <a href="/search/physics?searchtype=author&query=Guillemin%2C+R">Renaud Guillemin</a>, <a href="/search/physics?searchtype=author&query=Piancastelli%2C+M+N">Maria Novella Piancastelli</a>, <a href="/search/physics?searchtype=author&query=Simon%2C+M">Marc Simon</a>, <a href="/search/physics?searchtype=author&query=Davis%2C+V+T">Vernon T. Davis</a>, <a href="/search/physics?searchtype=author&query=Williams%2C+J+B">Joshua B. Williams</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">Reinhard D枚rner</a>, <a href="/search/physics?searchtype=author&query=Hatada%2C+K">Keisuke Hatada</a>, <a href="/search/physics?searchtype=author&query=Yamazaki%2C+K">Kaoru Yamazaki</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">Kilian Fehre</a>, <a href="/search/physics?searchtype=author&query=Demekhin%2C+P+V">Philipp V. Demekhin</a>, <a href="/search/physics?searchtype=author&query=Ueda%2C+K">Kiyoshi Ueda</a> , et al. (2 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2105.11897v1-abstract-short" style="display: inline;"> We present an experimental and theoretical study of core-level ionization of small hetero- and homo-nuclear molecules employing circularly polarized light and address molecular-frame photoelectron angular distributions in the light's polarization plane (CP-MFPADs). We find that the main forward-scattering peaks of CP-MFPADs are slightly tilted with respect to the molecular axis. We show that this… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2105.11897v1-abstract-full').style.display = 'inline'; document.getElementById('2105.11897v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2105.11897v1-abstract-full" style="display: none;"> We present an experimental and theoretical study of core-level ionization of small hetero- and homo-nuclear molecules employing circularly polarized light and address molecular-frame photoelectron angular distributions in the light's polarization plane (CP-MFPADs). We find that the main forward-scattering peaks of CP-MFPADs are slightly tilted with respect to the molecular axis. We show that this tilt angle can be directly connected to the molecular bond length by a simple, universal formula. The extraction of the bond length becomes more accurate as the photoelectron energy is increased. We apply the derived formula to several examples of CP-MFPADs of C 1s and O 1s photoelectrons of CO, which have been measured experimentally or obtained by means of ab initio modeling. The photoelectron kinetic energies range from 70 to 1000~eV and the extracted bond lengths agree well with the known bond length of the CO molecule in its ground state. In addition, we discuss the influence of the back-scattering contribution that is superimposed over the analyzed forward-scattering peak in case of homo-nuclear diatomic molecules as N$_2$. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2105.11897v1-abstract-full').style.display = 'none'; document.getElementById('2105.11897v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 25 May, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> May 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Chem. Chem. Phys., 2023, 25, 13784-13791 </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2105.02028">arXiv:2105.02028</a> <span> [<a href="https://arxiv.org/pdf/2105.02028">pdf</a>, <a href="https://arxiv.org/format/2105.02028">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.123.193001">10.1103/PhysRevLett.123.193001 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Photon-momentum-induced molecular dynamics in photoionization of N$_2$ at $h谓=40$ keV </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Kircher%2C+M">M. Kircher</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">S. Grundmann</a>, <a href="/search/physics?searchtype=author&query=Waitz%2C+M">M. Waitz</a>, <a href="/search/physics?searchtype=author&query=Melzer%2C+N">N. Melzer</a>, <a href="/search/physics?searchtype=author&query=Vela-Perez%2C+I">I. Vela-Perez</a>, <a href="/search/physics?searchtype=author&query=Mletzko%2C+T">T. Mletzko</a>, <a href="/search/physics?searchtype=author&query=Pier%2C+A">A. Pier</a>, <a href="/search/physics?searchtype=author&query=Strenger%2C+N">N. Strenger</a>, <a href="/search/physics?searchtype=author&query=Siebert%2C+J">J. Siebert</a>, <a href="/search/physics?searchtype=author&query=Janssen%2C+R">R. Janssen</a>, <a href="/search/physics?searchtype=author&query=Honkim%C3%A4ki%2C+V">V. Honkim盲ki</a>, <a href="/search/physics?searchtype=author&query=Drnec%2C+J">J. Drnec</a>, <a href="/search/physics?searchtype=author&query=Demekhin%2C+P+V">Ph. V. Demekhin</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2105.02028v1-abstract-short" style="display: inline;"> We investigate K-shell ionization of N$_2$ at 40 keV photon energy. Using a COLTRIMS reaction microscope we determine the vector momenta of the photoelectron, the Auger electron and both N$^+$ fragments. These fully differential data show that the dissociation process of the N$_2^{2+}$ ion is significantly modified not only by the recoil momentum of the photoelectron, but also by the photon moment… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2105.02028v1-abstract-full').style.display = 'inline'; document.getElementById('2105.02028v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2105.02028v1-abstract-full" style="display: none;"> We investigate K-shell ionization of N$_2$ at 40 keV photon energy. Using a COLTRIMS reaction microscope we determine the vector momenta of the photoelectron, the Auger electron and both N$^+$ fragments. These fully differential data show that the dissociation process of the N$_2^{2+}$ ion is significantly modified not only by the recoil momentum of the photoelectron, but also by the photon momentum and the momentum of the emitted Auger electron. We find that the recoil energy introduced by the photon and the photoelectron momentum is partitioned with a ratio of approximately 30/70 between the Auger electron and fragment ion kinetic energies, respectively. We also observe that the photon momentum induces an additional rotation of the molecular ion. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2105.02028v1-abstract-full').style.display = 'none'; document.getElementById('2105.02028v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 5 May, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> May 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">5 pages, 2 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 123, 193001 (2019) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2105.01955">arXiv:2105.01955</a> <span> [<a href="https://arxiv.org/pdf/2105.01955">pdf</a>, <a href="https://arxiv.org/format/2105.01955">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.123.243201">10.1103/PhysRevLett.123.243201 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Recoil-Induced Asymmetry of Nondipole Molecular Frame Photoelectron Angular Distributions in the Hard X-ray Regime </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Kircher%2C+M">M. Kircher</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">S. Grundmann</a>, <a href="/search/physics?searchtype=author&query=Waitz%2C+M">M. Waitz</a>, <a href="/search/physics?searchtype=author&query=Melzer%2C+N">N. Melzer</a>, <a href="/search/physics?searchtype=author&query=Vela-Perez%2C+I">I. Vela-Perez</a>, <a href="/search/physics?searchtype=author&query=Mletzko%2C+T">T. Mletzko</a>, <a href="/search/physics?searchtype=author&query=Pier%2C+A">A. Pier</a>, <a href="/search/physics?searchtype=author&query=Strenger%2C+N">N. Strenger</a>, <a href="/search/physics?searchtype=author&query=Siebert%2C+J">J. Siebert</a>, <a href="/search/physics?searchtype=author&query=Janssen%2C+R">R. Janssen</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Artemyev%2C+A+N">A. N. Artemyev</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a>, <a href="/search/physics?searchtype=author&query=Demekhin%2C+P+V">Ph. V. Demekhin</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2105.01955v1-abstract-short" style="display: inline;"> We investigate angular emission distributions of the 1s-photoelectrons of N$_2$ ionized by linearly polarized synchrotron radiation at $h 谓=40$ keV. As expected, nondipole contributions cause a very strong forward-backward asymmetry in the measured emission distributions. In addition, we observe an unexpected asymmetry with respect to the polarization direction, which depends on the direction of t… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2105.01955v1-abstract-full').style.display = 'inline'; document.getElementById('2105.01955v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2105.01955v1-abstract-full" style="display: none;"> We investigate angular emission distributions of the 1s-photoelectrons of N$_2$ ionized by linearly polarized synchrotron radiation at $h 谓=40$ keV. As expected, nondipole contributions cause a very strong forward-backward asymmetry in the measured emission distributions. In addition, we observe an unexpected asymmetry with respect to the polarization direction, which depends on the direction of the molecular fragmentation. In particular, photoelectrons are predominantly emitted in the direction of the forward nitrogen atom. This observation cannot be explained via asymmetries introduced by the initial bound and final continuum electronic states of the oriented molecule. The present simulations assign this asymmetry to a novel nontrivial effect of the recoil imposed to the nuclei by the fast photoelectrons and high-energy photons, which results in a propensity for the ions to break up along the axis of the recoil momentum. The results are of particular importance for the interpretation of future experiments at XFELs operating in the few tens of keV regime, where such nondipole and recoil effects will be essential. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2105.01955v1-abstract-full').style.display = 'none'; document.getElementById('2105.01955v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 5 May, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> May 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">6 pages, 2 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 123, 243201 (2019) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2101.03375">arXiv:2101.03375</a> <span> [<a href="https://arxiv.org/pdf/2101.03375">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Chemical Physics">physics.chem-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Applied Physics">physics.app-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1039/D2CP03090J">10.1039/D2CP03090J <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> A new route for enantio-sensitive structure determination by photoelectron scattering on molecules in the gas phase </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Novikovskiy%2C+N+M">N. M. Novikovskiy</a>, <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">S. Grundmann</a>, <a href="/search/physics?searchtype=author&query=Kastirke%2C+G">G. Kastirke</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">A. Hartung</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Janke%2C+C">Ch. Janke</a>, <a href="/search/physics?searchtype=author&query=Pitzer%2C+M">M. Pitzer</a>, <a href="/search/physics?searchtype=author&query=Zeller%2C+S">S. Zeller</a>, <a href="/search/physics?searchtype=author&query=Wiegandt%2C+F">F. Wiegandt</a>, <a href="/search/physics?searchtype=author&query=Weller%2C+M">M. Weller</a>, <a href="/search/physics?searchtype=author&query=Kircher%2C+M">M. Kircher</a>, <a href="/search/physics?searchtype=author&query=Nalin%2C+G">G. Nalin</a>, <a href="/search/physics?searchtype=author&query=Hofmann%2C+M">M. Hofmann</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Knie%2C+A">A. Knie</a>, <a href="/search/physics?searchtype=author&query=Hans%2C+A">A. Hans</a>, <a href="/search/physics?searchtype=author&query=Ltaief%2C+L+B">L. Ben Ltaief</a>, <a href="/search/physics?searchtype=author&query=Ehresmann%2C+A">A. Ehresmann</a>, <a href="/search/physics?searchtype=author&query=Berger%2C+R">R. Berger</a>, <a href="/search/physics?searchtype=author&query=Fukuzawa%2C+H">H. Fukuzawa</a>, <a href="/search/physics?searchtype=author&query=Ueda%2C+K">K. Ueda</a> , et al. (6 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2101.03375v2-abstract-short" style="display: inline;"> X-ray as well as electron diffraction are powerful tools for structure determination of molecules. Studies on randomly oriented molecules in the gas-phase address cases in which molecular crystals cannot be generated or the interaction-free molecular structure is to be addressed. Such studies usually yield partial geometrical information, such as interatomic distances. Here, we present a complemen… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2101.03375v2-abstract-full').style.display = 'inline'; document.getElementById('2101.03375v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2101.03375v2-abstract-full" style="display: none;"> X-ray as well as electron diffraction are powerful tools for structure determination of molecules. Studies on randomly oriented molecules in the gas-phase address cases in which molecular crystals cannot be generated or the interaction-free molecular structure is to be addressed. Such studies usually yield partial geometrical information, such as interatomic distances. Here, we present a complementary approach, which allows obtaining insight to the structure, handedness and even detailed geometrical features of molecules in the gas phase. Our approach combines Coulomb explosion imaging, the information that is encoded in the molecular frame diffraction pattern of core-shell photoelectrons and ab initio computations. Using a loop-like analysis scheme we are able to deduce specific molecular coordinates with sensitivity even to the handedness of chiral molecules and the positions of individual atoms, as, e.g., protons. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2101.03375v2-abstract-full').style.display = 'none'; document.getElementById('2101.03375v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 23 January, 2023; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 9 January, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">13 pages, 3 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Chem. Chem. Phys. 24, 26458-26465 (2022) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2011.08554">arXiv:2011.08554</a> <span> [<a href="https://arxiv.org/pdf/2011.08554">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.126.083201">10.1103/PhysRevLett.126.083201 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Strong Differential Photoion Circular Dichroism in Strong-Field Ionization of Chiral Molecules </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a>, <a href="/search/physics?searchtype=author&query=Janke%2C+C">C. Janke</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Hofmann%2C+M">M. Hofmann</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Weller%2C+M">M. Weller</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">A. Hartung</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Braun%2C+H">H. Braun</a>, <a href="/search/physics?searchtype=author&query=Baumert%2C+T">T. Baumert</a>, <a href="/search/physics?searchtype=author&query=Stohner%2C+J">J. Stohner</a>, <a href="/search/physics?searchtype=author&query=Demekhin%2C+P+V">Ph. V. Demekhin</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2011.08554v1-abstract-short" style="display: inline;"> We investigate the differential ionization probability of chiral molecules in the strong field regime as a function of the helicity of the incident light. To this end, we analyze the fourfold ionization of bromochlorofluoromethane (CHBrClF) with subsequent fragmentation into four charged fragments and different dissociation channels of the singly ionized methyloxirane. We observe a variation of th… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2011.08554v1-abstract-full').style.display = 'inline'; document.getElementById('2011.08554v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2011.08554v1-abstract-full" style="display: none;"> We investigate the differential ionization probability of chiral molecules in the strong field regime as a function of the helicity of the incident light. To this end, we analyze the fourfold ionization of bromochlorofluoromethane (CHBrClF) with subsequent fragmentation into four charged fragments and different dissociation channels of the singly ionized methyloxirane. We observe a variation of the differential ionization probability in a range of several percent. Accordingly, we conclude that the helicity of light is a quantity that should be considered for the theoretical description of the strong field ionization rate of chiral molecules. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2011.08554v1-abstract-full').style.display = 'none'; document.getElementById('2011.08554v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 17 November, 2020; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> November 2020. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">12 pages, 6 figures, submitted</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">MSC Class:</span> v1 </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 126, 083201 (2021) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2008.07638">arXiv:2008.07638</a> <span> [<a href="https://arxiv.org/pdf/2008.07638">pdf</a>, <a href="https://arxiv.org/format/2008.07638">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.126.053202">10.1103/PhysRevLett.126.053202 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Electric Nondipole Effect in Strong-Field Ionization </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Hartung%2C+A">A. Hartung</a>, <a href="/search/physics?searchtype=author&query=Brennecke%2C+S">S. Brennecke</a>, <a href="/search/physics?searchtype=author&query=Lin%2C+K">K. Lin</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a>, <a href="/search/physics?searchtype=author&query=Lein%2C+M">M. Lein</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2008.07638v3-abstract-short" style="display: inline;"> Strong-field ionization of atoms by circularly polarized femtosecond laser pulses produces a donut-shaped electron momentum distribution. Within the dipole approximation this distribution is symmetric with respect to the polarization plane. The magnetic component of the light field is known to shift this distribution forward. Here, we show that this magnetic non-dipole effect is not the only non-d… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2008.07638v3-abstract-full').style.display = 'inline'; document.getElementById('2008.07638v3-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2008.07638v3-abstract-full" style="display: none;"> Strong-field ionization of atoms by circularly polarized femtosecond laser pulses produces a donut-shaped electron momentum distribution. Within the dipole approximation this distribution is symmetric with respect to the polarization plane. The magnetic component of the light field is known to shift this distribution forward. Here, we show that this magnetic non-dipole effect is not the only non-dipole effect in strong-field ionization. We find that an electric non-dipole effect arises that is due to the position dependence of the electric field and which can be understood in analogy to the Doppler effect. This electric non-dipole effect manifests as an increase of the radius of the donut-shaped photoelectron momentum distribution for forward-directed momenta and as a decrease of this radius for backwards-directed electrons. We present experimental data showing this fingerprint of the electric non-dipole effect and compare our findings with a classical model and quantum calculations. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2008.07638v3-abstract-full').style.display = 'none'; document.getElementById('2008.07638v3-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 4 February, 2021; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 17 August, 2020; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> August 2020. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">6 pages, 3 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 126, 053202 (2021) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2005.04148">arXiv:2005.04148</a> <span> [<a href="https://arxiv.org/pdf/2005.04148">pdf</a>, <a href="https://arxiv.org/format/2005.04148">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevA.102.043115">10.1103/PhysRevA.102.043115 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Sideband Modulation by Sub-Cycle Interference </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Geyer%2C+A">A. Geyer</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Lin%2C+K">K. Lin</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2005.04148v4-abstract-short" style="display: inline;"> We experimentally and theoretically show that the electron energy spectra strongly depend on the relative helicity in highly intense, circularly polarized two-color laser fields which is an unexpected finding. The employed counter-rotating two-color (CRTC) fields and the co-rotating two-color (CoRTC) fields are both a superposition of circularly polarized laser pulses at a central wavelength of 39… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2005.04148v4-abstract-full').style.display = 'inline'; document.getElementById('2005.04148v4-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2005.04148v4-abstract-full" style="display: none;"> We experimentally and theoretically show that the electron energy spectra strongly depend on the relative helicity in highly intense, circularly polarized two-color laser fields which is an unexpected finding. The employed counter-rotating two-color (CRTC) fields and the co-rotating two-color (CoRTC) fields are both a superposition of circularly polarized laser pulses at a central wavelength of 390 nm and 780 nm (intensitiy ratio $I_{390}/I_{780}\approx 250$). For the CRTC field, the measured electron energy spectrum is dominated by peaks that are spaced by 3.18 eV (corresponds to the photon energy of light at a wavelength of 390 nm). For the CoRTC field, we observe additional energy peaks (sidebands). Using our semi-classical, trajectory-based models, we conclude that the sideband intensity is modulated by a sub-cycle interference, which sensitively depends on the relative helicity in circularly polarized two-color fields. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2005.04148v4-abstract-full').style.display = 'none'; document.getElementById('2005.04148v4-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 26 October, 2020; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 8 May, 2020; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> May 2020. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">7 pages, 4 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. A 102, 043115 (2020) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2003.10706">arXiv:2003.10706</a> <span> [<a href="https://arxiv.org/pdf/2003.10706">pdf</a>, <a href="https://arxiv.org/format/2003.10706">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.124.233201">10.1103/PhysRevLett.124.233201 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Observation of Photoion Backward Emission in Photoionization of He and N2 </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">Sven Grundmann</a>, <a href="/search/physics?searchtype=author&query=Kircher%2C+M">Max Kircher</a>, <a href="/search/physics?searchtype=author&query=Vela-Perez%2C+I">Isabel Vela-Perez</a>, <a href="/search/physics?searchtype=author&query=Nalin%2C+G">Giammarco Nalin</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">Daniel Trabert</a>, <a href="/search/physics?searchtype=author&query=Anders%2C+N">Nils Anders</a>, <a href="/search/physics?searchtype=author&query=Melzer%2C+N">Niklas Melzer</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">Jonas Rist</a>, <a href="/search/physics?searchtype=author&query=Pier%2C+A">Andreas Pier</a>, <a href="/search/physics?searchtype=author&query=Strenger%2C+N">Nico Strenger</a>, <a href="/search/physics?searchtype=author&query=Siebert%2C+J">Juliane Siebert</a>, <a href="/search/physics?searchtype=author&query=Demekhin%2C+P+V">Philipp V. Demekhin</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">Lothar Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">Florian Trinter</a>, <a href="/search/physics?searchtype=author&query=Schoeffler%2C+M+S">Markus S. Schoeffler</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">Till Jahnke</a>, <a href="/search/physics?searchtype=author&query=Doerner%2C+R">Reinhard Doerner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2003.10706v1-abstract-short" style="display: inline;"> We experimentally investigate the effects of the linear photon momentum on the momentum distributions of photoions and photoelectrons generated in one-photon ionization in an energy range of 300 eV $\leq~E_纬~\leq$ 40 keV. Our results show that for each ionization event the photon momentum is imparted onto the photoion, which is essentially the system's center of mass. Nevertheless, the mean value… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2003.10706v1-abstract-full').style.display = 'inline'; document.getElementById('2003.10706v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2003.10706v1-abstract-full" style="display: none;"> We experimentally investigate the effects of the linear photon momentum on the momentum distributions of photoions and photoelectrons generated in one-photon ionization in an energy range of 300 eV $\leq~E_纬~\leq$ 40 keV. Our results show that for each ionization event the photon momentum is imparted onto the photoion, which is essentially the system's center of mass. Nevertheless, the mean value of the ion momentum distribution along the light propagation direction is backward-directed by $-3/5$ times the photon momentum. These results experimentally confirm a 90 year old prediction. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2003.10706v1-abstract-full').style.display = 'none'; document.getElementById('2003.10706v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 24 March, 2020; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> March 2020. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">5 pages, 3 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 124, 233201 (2020) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2001.07713">arXiv:2001.07713</a> <span> [<a href="https://arxiv.org/pdf/2001.07713">pdf</a>, <a href="https://arxiv.org/format/2001.07713">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevResearch.2.033080">10.1103/PhysRevResearch.2.033080 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Revealing the Two-Electron Cusp in the Ground States of He and H2 via Quasifree Double Photoionization </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">S. Grundmann</a>, <a href="/search/physics?searchtype=author&query=Serov%2C+V">V. Serov</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Strenger%2C+N">N. Strenger</a>, <a href="/search/physics?searchtype=author&query=Pier%2C+A">A. Pier</a>, <a href="/search/physics?searchtype=author&query=Kircher%2C+M">M. Kircher</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Weller%2C+M">M. Weller</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Kaiser%2C+L">L. Kaiser</a>, <a href="/search/physics?searchtype=author&query=Bray%2C+A+W">A. W. Bray</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Williams%2C+J+B">J. B. Williams</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Kheifets%2C+A+S">A. S. Kheifets</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2001.07713v2-abstract-short" style="display: inline;"> We report on kinematically complete measurements and ab initio non-perturbative calculations of double ionization of He and H2 by a single 800 eV circularly polarized photon. We confirm the quasifree mechanism of photoionization for H2 and show how it originates from the two-electron cusp in the ground state of a two-electron target. Our approach establishes a new method for mapping electrons rela… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2001.07713v2-abstract-full').style.display = 'inline'; document.getElementById('2001.07713v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2001.07713v2-abstract-full" style="display: none;"> We report on kinematically complete measurements and ab initio non-perturbative calculations of double ionization of He and H2 by a single 800 eV circularly polarized photon. We confirm the quasifree mechanism of photoionization for H2 and show how it originates from the two-electron cusp in the ground state of a two-electron target. Our approach establishes a new method for mapping electrons relative to each other and provides valuable insight into photoionization beyond the electric-dipole approximation. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2001.07713v2-abstract-full').style.display = 'none'; document.getElementById('2001.07713v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 1 July, 2020; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 21 January, 2020; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2020. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">7 pages, 4 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Research 2, 033080 (2020) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1911.04780">arXiv:1911.04780</a> <span> [<a href="https://arxiv.org/pdf/1911.04780">pdf</a>, <a href="https://arxiv.org/format/1911.04780">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1038/s41567-020-0880-2">10.1038/s41567-020-0880-2 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Kinematically complete experimental study of Compton scattering at helium atoms near the ionization threshold </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Kircher%2C+M">Max Kircher</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">Florian Trinter</a>, <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">Sven Grundmann</a>, <a href="/search/physics?searchtype=author&query=Vela-Perez%2C+I">Isabel Vela-Perez</a>, <a href="/search/physics?searchtype=author&query=Brennecke%2C+S">Simon Brennecke</a>, <a href="/search/physics?searchtype=author&query=Eicke%2C+N">Nicolas Eicke</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">Jonas Rist</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">Sebastian Eckart</a>, <a href="/search/physics?searchtype=author&query=Houamer%2C+S">Salim Houamer</a>, <a href="/search/physics?searchtype=author&query=Chuluunbaatar%2C+O">Ochbadrakh Chuluunbaatar</a>, <a href="/search/physics?searchtype=author&query=Popov%2C+Y+V">Yuri V. Popov</a>, <a href="/search/physics?searchtype=author&query=Volobuev%2C+I+P">Igor P. Volobuev</a>, <a href="/search/physics?searchtype=author&query=Bagschik%2C+K">Kai Bagschik</a>, <a href="/search/physics?searchtype=author&query=Piancastelli%2C+M+N">Maria Novella Piancastelli</a>, <a href="/search/physics?searchtype=author&query=Lein%2C+M">Manfred Lein</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">Till Jahnke</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">Markus S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">Reinhard D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1911.04780v2-abstract-short" style="display: inline;"> Compton scattering is one of the fundamental interaction processes of light with matter. Already upon its discovery [1] it was described as a billiard-type collision of a photon kicking a quasi-free electron. With decreasing photon energy, the maximum possible momentum transfer becomes so small that the corresponding energy falls below the binding energy of the electron. Then ionization by Compton… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1911.04780v2-abstract-full').style.display = 'inline'; document.getElementById('1911.04780v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1911.04780v2-abstract-full" style="display: none;"> Compton scattering is one of the fundamental interaction processes of light with matter. Already upon its discovery [1] it was described as a billiard-type collision of a photon kicking a quasi-free electron. With decreasing photon energy, the maximum possible momentum transfer becomes so small that the corresponding energy falls below the binding energy of the electron. Then ionization by Compton scattering becomes an intriguing quantum phenomenon. Here we report a kinematically complete experiment on Compton scattering at helium atoms below that threshold. We determine the momentum correlations of the electron, the recoiling ion, and the scattered photon in a coincidence experiment finding that electrons are not only emitted in the direction of the momentum transfer, but that there is a second peak of ejection to the backward direction. This finding links Compton scattering to processes as ionization by ultrashort optical pulses [2], electron impact ionization [3,4], ion impact ionization [5,6], and neutron scattering [7] where similar momentum patterns occur. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1911.04780v2-abstract-full').style.display = 'none'; document.getElementById('1911.04780v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 5 November, 2020; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 12 November, 2019; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> November 2019. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">7 pages, 4 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Nature Physics 16, 756-760 (2020) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1902.07278">arXiv:1902.07278</a> <span> [<a href="https://arxiv.org/pdf/1902.07278">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1038/s41567-019-0653-y">10.1038/s41567-019-0653-y <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Magnetic fields alter tunneling in strong-field ionization </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Hartung%2C+A">A. Hartung</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Brennecke%2C+S">S. Brennecke</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Richter%2C+M">M. Richter</a>, <a href="/search/physics?searchtype=author&query=Sann%2C+H">H. Sann</a>, <a href="/search/physics?searchtype=author&query=Zeller%2C+S">S. Zeller</a>, <a href="/search/physics?searchtype=author&query=Henrichs%2C+K">K. Henrichs</a>, <a href="/search/physics?searchtype=author&query=Kastirke%2C+G">G. Kastirke</a>, <a href="/search/physics?searchtype=author&query=Hoehl%2C+J">J. Hoehl</a>, <a href="/search/physics?searchtype=author&query=Kalinin%2C+A">A. Kalinin</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Lein%2C+M">M. Lein</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1902.07278v1-abstract-short" style="display: inline;"> When a strong laser pulse induces the ionization of an atom, momentum conservation dictates that the absorbed photons transfer their momentum $p_纬=E_纬/c$ to the electron and its parent ion. Even after 30 years of studying strong-field ionization, the sharing of the photon momentum between the two particles and its underlying mechanism are still under debate in theory. Corresponding experiments are… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1902.07278v1-abstract-full').style.display = 'inline'; document.getElementById('1902.07278v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1902.07278v1-abstract-full" style="display: none;"> When a strong laser pulse induces the ionization of an atom, momentum conservation dictates that the absorbed photons transfer their momentum $p_纬=E_纬/c$ to the electron and its parent ion. Even after 30 years of studying strong-field ionization, the sharing of the photon momentum between the two particles and its underlying mechanism are still under debate in theory. Corresponding experiments are very challenging due to the extremely small photon momentum ($~10^{-4}$ a.u.) and their precision has been too limited, so far, to ultimately resolve the debate. Here, by utilizing a novel experimental approach of two counter-propagating laser pulses, we present a detailed study on the effects of the photon momentum in strong-field ionization. The high precision and self-referencing of the method allows to unambiguously demonstrate the action of the light's magnetic field on the electron while it is under the tunnel barrier, confirming theoretical predictions, disproving others. Our results deepen the understanding of, for example, molecular imaging and time-resolved photoelectron holography. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1902.07278v1-abstract-full').style.display = 'none'; document.getElementById('1902.07278v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 19 February, 2019; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> February 2019. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1810.07415">arXiv:1810.07415</a> <span> [<a href="https://arxiv.org/pdf/1810.07415">pdf</a>, <a href="https://arxiv.org/format/1810.07415">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic and Molecular Clusters">physics.atm-clus</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.121.243002">10.1103/PhysRevLett.121.243002 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Breakdown of the spectator concept in low-electron-energy resonant decay processes </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Mhamdi%2C+A">A. Mhamdi</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Aslit%C3%BCrk%2C+D">D. Aslit眉rk</a>, <a href="/search/physics?searchtype=author&query=Weller%2C+M">M. Weller</a>, <a href="/search/physics?searchtype=author&query=Melzer%2C+N">N. Melzer</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Kircher%2C+M">M. Kircher</a>, <a href="/search/physics?searchtype=author&query=Vela-Perez%2C+I">I. Vela-Perez</a>, <a href="/search/physics?searchtype=author&query=Siebert%2C+J">J. Siebert</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">S. Grundmann</a>, <a href="/search/physics?searchtype=author&query=Kastirke%2C+G">G. Kastirke</a>, <a href="/search/physics?searchtype=author&query=Waitz%2C+M">M. Waitz</a>, <a href="/search/physics?searchtype=author&query=Khan%2C+A">A. Khan</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Demekhin%2C+P+V">Ph. V. Demekhin</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1810.07415v1-abstract-short" style="display: inline;"> We suggest that low energy electrons, released by resonant decay processes, experience substantial scattering on the electron density of excited electrons, which remain a spectator during the decay. As a result, the angular emission distribution is altered significantly. This effect is expected to be a common feature of low energy secondary electron emission. In this letter, we exemplify our idea… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1810.07415v1-abstract-full').style.display = 'inline'; document.getElementById('1810.07415v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1810.07415v1-abstract-full" style="display: none;"> We suggest that low energy electrons, released by resonant decay processes, experience substantial scattering on the electron density of excited electrons, which remain a spectator during the decay. As a result, the angular emission distribution is altered significantly. This effect is expected to be a common feature of low energy secondary electron emission. In this letter, we exemplify our idea by examining the spectator resonant interatomic Coulombic decay (sRICD) of Ne dimers. Our theoretical predictions are confirmed by a corresponding coincidence experiment. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1810.07415v1-abstract-full').style.display = 'none'; document.getElementById('1810.07415v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 17 October, 2018; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> October 2018. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">5 pages two figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 121, 243002 (2018) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1808.03516">arXiv:1808.03516</a> <span> [<a href="https://arxiv.org/pdf/1808.03516">pdf</a>, <a href="https://arxiv.org/format/1808.03516">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevA.98.043405">10.1103/PhysRevA.98.043405 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Multiphoton Double Ionization of Helium at 394nm - a Fully Differential Experiment </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Henrichs%2C+K">K. Henrichs</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">A. Hartung</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Sann%2C+H">H. Sann</a>, <a href="/search/physics?searchtype=author&query=Pitzer%2C+M">M. Pitzer</a>, <a href="/search/physics?searchtype=author&query=Richter%2C+M">M. Richter</a>, <a href="/search/physics?searchtype=author&query=Kang%2C+H">H. Kang</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1808.03516v1-abstract-short" style="display: inline;"> We report on a kinematically complete experiment on strong field double ionization of helium using laser pulses with a wavelength of 394\,nm and intensities of $3.5-5.7\times10^{14}\,W/cm^2$. Our experiment reaches the most complete level of detail which previously has only been reached for single photon double ionization. We give an overview over the observables on many levels of integration, sta… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1808.03516v1-abstract-full').style.display = 'inline'; document.getElementById('1808.03516v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1808.03516v1-abstract-full" style="display: none;"> We report on a kinematically complete experiment on strong field double ionization of helium using laser pulses with a wavelength of 394\,nm and intensities of $3.5-5.7\times10^{14}\,W/cm^2$. Our experiment reaches the most complete level of detail which previously has only been reached for single photon double ionization. We give an overview over the observables on many levels of integration, starting from the ratio of double to single ionization, the individual electron and ion momentum distributions over joint momentum and energy distributions to fully differential cross sections showing the correlated angular momentum distributions. Within the studied intensity range the ratio of double to single ionization changes from $2\times 10^{-4}$ to $1.5\times 10^{-3}$. We find the momentum distributions of the $\rm{He}^{2+}$ ions and the correlated two electron momentum distributions to vary substantially. Only at the highest intensity both electrons are emitted to the same direction while at the lowest intensity back-to-back emission dominates. The joint energy distribution of the electrons shows discrete structures from the energy quantization of the photon field which allows us to count the number of absorbed photons and thus access the parity of the final state. We find the energy of the individual electron to show a peak structure indicating a quantized sharing of the overall energy absorbed from the field. The joint angular momentum distributions of the two electrons show a highly directed emission of both electrons along the polarization axis as well as clear imprints of electron repulsion. They strongly change with the energy sharing between the electrons. The aspect of selection rules in double ionization which are also visible in the presented dataset has been subject to a preceding publication [1]. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1808.03516v1-abstract-full').style.display = 'none'; document.getElementById('1808.03516v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 10 August, 2018; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> August 2018. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">10 pages, 13 figures, submitted to PRA</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. A 98, 043405 (2018) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1806.06276">arXiv:1806.06276</a> <span> [<a href="https://arxiv.org/pdf/1806.06276">pdf</a>, <a href="https://arxiv.org/format/1806.06276">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic and Molecular Clusters">physics.atm-clus</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevA.98.050701">10.1103/PhysRevA.98.050701 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Frustrated Coulomb explosion of small helium clusters </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Kazandjian%2C+S">S. Kazandjian</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Weller%2C+M">M. Weller</a>, <a href="/search/physics?searchtype=author&query=Wiegandt%2C+F">F. Wiegandt</a>, <a href="/search/physics?searchtype=author&query=Aslit%C3%BCrk%2C+D">D. Aslit眉rk</a>, <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">S. Grundmann</a>, <a href="/search/physics?searchtype=author&query=Kircher%2C+M">M. Kircher</a>, <a href="/search/physics?searchtype=author&query=Nalin%2C+G">G. Nalin</a>, <a href="/search/physics?searchtype=author&query=Pitters%2C+D">D. Pitters</a>, <a href="/search/physics?searchtype=author&query=P%C3%A9rez%2C+I+V">I. Vela P茅rez</a>, <a href="/search/physics?searchtype=author&query=Waitz%2C+M">M. Waitz</a>, <a href="/search/physics?searchtype=author&query=Schiwietz%2C+G">G. Schiwietz</a>, <a href="/search/physics?searchtype=author&query=Griffin%2C+B">B. Griffin</a>, <a href="/search/physics?searchtype=author&query=Williams%2C+J+B">J. B. Williams</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M">M. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Miteva%2C+T">T. Miteva</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Sisourat%2C+N">N. Sisourat</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1806.06276v2-abstract-short" style="display: inline;"> Almost ten years ago, energetic neutral hydrogen atoms were detected after a strong-field double ionization of H$_2$. This process, called 'frustrated tunneling ionization', occurs when an ionized electron is recaptured after being driven back to its parent ion by the electric field of a femtosecond laser. In the present study we demonstrate that a related process naturally occurs in clusters with… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1806.06276v2-abstract-full').style.display = 'inline'; document.getElementById('1806.06276v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1806.06276v2-abstract-full" style="display: none;"> Almost ten years ago, energetic neutral hydrogen atoms were detected after a strong-field double ionization of H$_2$. This process, called 'frustrated tunneling ionization', occurs when an ionized electron is recaptured after being driven back to its parent ion by the electric field of a femtosecond laser. In the present study we demonstrate that a related process naturally occurs in clusters without the need of an external field: we observe a charge hopping that occurs during a Coulomb explosion of a small helium cluster, which leads to an energetic neutral helium atom. This claim is supported by theoretical evidence. As an analog to 'frustrated tunneling ionization', we term this process 'frustrated Coulomb explosion'. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1806.06276v2-abstract-full').style.display = 'none'; document.getElementById('1806.06276v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 19 June, 2018; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 16 June, 2018; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> June 2018. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. A 98, 050701 (2018) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1806.05214">arXiv:1806.05214</a> <span> [<a href="https://arxiv.org/pdf/1806.05214">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic and Molecular Clusters">physics.atm-clus</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevA.100.022707">10.1103/PhysRevA.100.022707 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Direct observation of interatomic Coulombic decay and subsequent ion-atom scattering in helium nanodroplets </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Wiegandt%2C+F">F. Wiegandt</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Henrichs%2C+K">K. Henrichs</a>, <a href="/search/physics?searchtype=author&query=Metz%2C+D">D. Metz</a>, <a href="/search/physics?searchtype=author&query=Pitzer%2C+M">M. Pitzer</a>, <a href="/search/physics?searchtype=author&query=Waitz%2C+M">M. Waitz</a>, <a href="/search/physics?searchtype=author&query=Maalouf%2C+E+J+a">E. Jabbour al Maalouf</a>, <a href="/search/physics?searchtype=author&query=Janke%2C+C">C. Janke</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Wechselberger%2C+N">N. Wechselberger</a>, <a href="/search/physics?searchtype=author&query=Miteva%2C+T">T. Miteva</a>, <a href="/search/physics?searchtype=author&query=Kazandjian%2C+S">S. Kazandjian</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M">M. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Sisourat%2C+N">N. Sisourat</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1806.05214v4-abstract-short" style="display: inline;"> We report on the experimental observation of interatomic Coulombic decay (ICD) in pure $^4$He nanoclusters of mean sizes between $N \approx$ 5000 and 30000 and the subsequent scattering of energetic He$^+$ fragments inside the neutral cluster by using cold target recoil ion momentum spectroscopy. ICD is induced in He clusters by using vacuum ultraviolet light of $h谓=$ 67 eV from the BESSY II synch… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1806.05214v4-abstract-full').style.display = 'inline'; document.getElementById('1806.05214v4-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1806.05214v4-abstract-full" style="display: none;"> We report on the experimental observation of interatomic Coulombic decay (ICD) in pure $^4$He nanoclusters of mean sizes between $N \approx$ 5000 and 30000 and the subsequent scattering of energetic He$^+$ fragments inside the neutral cluster by using cold target recoil ion momentum spectroscopy. ICD is induced in He clusters by using vacuum ultraviolet light of $h谓=$ 67 eV from the BESSY II synchrotron. The electronic decay creates two neighboring ions in the cluster at a well-defined distance. The measured fragment energies and angular correlations show that a main energy loss mechanism of these ions inside the cluster is a single hard binary collision with one atom of the cluster. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1806.05214v4-abstract-full').style.display = 'none'; document.getElementById('1806.05214v4-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 4 September, 2019; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 13 June, 2018; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> June 2018. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">6 pages, 4 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. A 100, 022707 (2019) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1805.05898">arXiv:1805.05898</a> <span> [<a href="https://arxiv.org/pdf/1805.05898">pdf</a>, <a href="https://arxiv.org/ps/1805.05898">ps</a>, <a href="https://arxiv.org/format/1805.05898">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.121.163202">10.1103/PhysRevLett.121.163202 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Direct Experimental Access to the Nonadiabatic Initial Momentum Offset upon Tunnel Ionization </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Eicke%2C+N">N. Eicke</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">A. Hartung</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Strenger%2C+N">N. Strenger</a>, <a href="/search/physics?searchtype=author&query=Pier%2C+A">A. Pier</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Lein%2C+M">M. Lein</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1805.05898v2-abstract-short" style="display: inline;"> We report on the non-adiabatic offset of the initial electron momentum distribution in the plane of polarization upon single ionization of argon by strong field tunneling and show how to experimentally control the degree of non-adiabaticity. Two-color counter- and co-rotating fields (390 and 780 nm) are compared to show that the non-adiabatic offset strongly depends on the temporal evolution of th… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1805.05898v2-abstract-full').style.display = 'inline'; document.getElementById('1805.05898v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1805.05898v2-abstract-full" style="display: none;"> We report on the non-adiabatic offset of the initial electron momentum distribution in the plane of polarization upon single ionization of argon by strong field tunneling and show how to experimentally control the degree of non-adiabaticity. Two-color counter- and co-rotating fields (390 and 780 nm) are compared to show that the non-adiabatic offset strongly depends on the temporal evolution of the laser electric field. We introduce a simple method for the direct access to the non-adiabatic offset using two-color counter- and co-rotating fields. Further, for a single-color circularly polarized field at 780 nm we show that the radius of the experimentally observed donut-like distribution increases for increasing momentum in the light propagation direction. Our observed initial momentum offsets are well reproduced by the strong-field approximation (SFA). A mechanistic picture is introduced that links the measured non-adiabatic offset to the magnetic quantum number of virtually populated intermediate states. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1805.05898v2-abstract-full').style.display = 'none'; document.getElementById('1805.05898v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 16 October, 2018; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 15 May, 2018; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> May 2018. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">6 pages, 4 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 121, 163202 (2018) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1803.10841">arXiv:1803.10841</a> <span> [<a href="https://arxiv.org/pdf/1803.10841">pdf</a>, <a href="https://arxiv.org/ps/1803.10841">ps</a>, <a href="https://arxiv.org/format/1803.10841">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.121.173003">10.1103/PhysRevLett.121.173003 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Separating Dipole and Quadrupole Contributions to Single-Photon Double Ionization </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Grundmann%2C+S">S. Grundmann</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Bray%2C+A+W">A. W. Bray</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Kastirke%2C+G">G. Kastirke</a>, <a href="/search/physics?searchtype=author&query=Metz%2C+D">D. Metz</a>, <a href="/search/physics?searchtype=author&query=Klumpp%2C+S">S. Klumpp</a>, <a href="/search/physics?searchtype=author&query=Viefhaus%2C+J">J. Viefhaus</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Williams%2C+J+B">J. B. Williams</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Kheifets%2C+A+S">A. S. Kheifets</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1803.10841v2-abstract-short" style="display: inline;"> We report on a kinematically complete measurement of double ionization of helium by a single 1100 eV circularly polarized photon. By exploiting dipole selection rules in the two-electron continuum state, we observed the angular emission pattern of electrons originating from a pure quadrupole transition. Our fully differential experimental data and companion ab initio nonperturbative theory show th… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1803.10841v2-abstract-full').style.display = 'inline'; document.getElementById('1803.10841v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1803.10841v2-abstract-full" style="display: none;"> We report on a kinematically complete measurement of double ionization of helium by a single 1100 eV circularly polarized photon. By exploiting dipole selection rules in the two-electron continuum state, we observed the angular emission pattern of electrons originating from a pure quadrupole transition. Our fully differential experimental data and companion ab initio nonperturbative theory show the separation of dipole and quadrupole contributions to photo-double-ionization and provide new insight into the nature of the quasifree mechanism. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1803.10841v2-abstract-full').style.display = 'none'; document.getElementById('1803.10841v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 8 October, 2018; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 28 March, 2018; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> March 2018. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">5 Pages, 3 Figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 121, 173003 (2018) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1802.06630">arXiv:1802.06630</a> <span> [<a href="https://arxiv.org/pdf/1802.06630">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1038/s41567-018-0080-5">10.1038/s41567-018-0080-5 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Ultrafast Preparation and Detection of Ring Currents in Single Atoms </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Eckart%2C+S">Sebastian Eckart</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">Maksim Kunitski</a>, <a href="/search/physics?searchtype=author&query=Richter%2C+M">Martin Richter</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">Alexander Hartung</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">Jonas Rist</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">Florian Trinter</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">Kilian Fehre</a>, <a href="/search/physics?searchtype=author&query=Schlott%2C+N">Nikolai Schlott</a>, <a href="/search/physics?searchtype=author&query=Henrichs%2C+K">Kevin Henrichs</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">Lothar Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">Till Jahnke</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M">Markus Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Liu%2C+K">Kunlong Liu</a>, <a href="/search/physics?searchtype=author&query=Barth%2C+I">Ingo Barth</a>, <a href="/search/physics?searchtype=author&query=Kaushal%2C+J">Jivesh Kaushal</a>, <a href="/search/physics?searchtype=author&query=Morales%2C+F">Felipe Morales</a>, <a href="/search/physics?searchtype=author&query=Ivanov%2C+M">Misha Ivanov</a>, <a href="/search/physics?searchtype=author&query=Smirnova%2C+O">Olga Smirnova</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">Reinhard D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1802.06630v1-abstract-short" style="display: inline;"> Quantum particles can penetrate potential barriers by tunneling (1). If that barrier is rotating, the tunneling process is modified (2,3). This is typical for electrons in atoms, molecules or solids exposed to strong circularly polarized laser pulses (4,5). Here we measure how the transmission probability through a rotating tunnel depends on the sign of the magnetic quantum number m of the electro… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1802.06630v1-abstract-full').style.display = 'inline'; document.getElementById('1802.06630v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1802.06630v1-abstract-full" style="display: none;"> Quantum particles can penetrate potential barriers by tunneling (1). If that barrier is rotating, the tunneling process is modified (2,3). This is typical for electrons in atoms, molecules or solids exposed to strong circularly polarized laser pulses (4,5). Here we measure how the transmission probability through a rotating tunnel depends on the sign of the magnetic quantum number m of the electron and thus on the initial sense of rotation of its quantum phase. We further show that the electron keeps part of that rotary motion on its way through the tunnel by measuring m-dependent modification of the electron emission pattern. These findings are relevant for attosecond metrology as well as for interpretation of strong field electron emission from atoms and molecules (6-13) and directly demonstrates the creation of ring currents in bound states of ions with attosecond precision. In solids, this could open a way to inducing and controlling ring-current related topological phenomena (14). <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1802.06630v1-abstract-full').style.display = 'none'; document.getElementById('1802.06630v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 19 February, 2018; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> February 2018. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">19 pages, 6 figures, Nature Physics accepted</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Nat Phys 14, 701-704 (2018) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1711.08361">arXiv:1711.08361</a> <span> [<a href="https://arxiv.org/pdf/1711.08361">pdf</a>, <a href="https://arxiv.org/ps/1711.08361">ps</a>, <a href="https://arxiv.org/format/1711.08361">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevA.97.031405">10.1103/PhysRevA.97.031405 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Experimental Evidence for Selection Rules in Multiphoton Double Ionization of Helium </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Henrichs%2C+K">K. Henrichs</a>, <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">A. Hartung</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Sann%2C+H">H. Sann</a>, <a href="/search/physics?searchtype=author&query=Pitzer%2C+M">M. Pitzer</a>, <a href="/search/physics?searchtype=author&query=Richter%2C+M">M. Richter</a>, <a href="/search/physics?searchtype=author&query=Kang%2C+H">H. Kang</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1711.08361v2-abstract-short" style="display: inline;"> We report on the observation of phase space modulations in the correlated electron emission after strong field double ionization of helium using laser pulses with a wavelength of 394~nm and an intensity of $3\cdot10^{14}$W/cm$^2$. Those modulations are identified as direct results of quantum mechanical selection rules predicted by many theoretical calculations. They only occur for an odd number of… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1711.08361v2-abstract-full').style.display = 'inline'; document.getElementById('1711.08361v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1711.08361v2-abstract-full" style="display: none;"> We report on the observation of phase space modulations in the correlated electron emission after strong field double ionization of helium using laser pulses with a wavelength of 394~nm and an intensity of $3\cdot10^{14}$W/cm$^2$. Those modulations are identified as direct results of quantum mechanical selection rules predicted by many theoretical calculations. They only occur for an odd number of absorbed photons. By that we attribute this effect to the parity of the continuum wave function. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1711.08361v2-abstract-full').style.display = 'none'; document.getElementById('1711.08361v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 6 February, 2018; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 22 November, 2017; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> November 2017. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">5 pages, 3 figures, submitted to Phys. Rev. Lett</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. A 97, 031405 (2018) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1711.03880">arXiv:1711.03880</a> <span> [<a href="https://arxiv.org/pdf/1711.03880">pdf</a>, <a href="https://arxiv.org/ps/1711.03880">ps</a>, <a href="https://arxiv.org/format/1711.03880">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevA.97.041402">10.1103/PhysRevA.97.041402 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Sub-Cycle Interference upon Tunnel-Ionization by Counterrotating Two-Color Fields </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a>, <a href="/search/physics?searchtype=author&query=Ivanov%2C+I">I. Ivanov</a>, <a href="/search/physics?searchtype=author&query=Richter%2C+M">M. Richter</a>, <a href="/search/physics?searchtype=author&query=Fehre%2C+K">K. Fehre</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">A. Hartung</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Henrichs%2C+K">K. Henrichs</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">D. Trabert</a>, <a href="/search/physics?searchtype=author&query=Schlott%2C+N">N. Schlott</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Kheifets%2C+A">A. Kheifets</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1711.03880v2-abstract-short" style="display: inline;"> We report on three-dimensional (3D) electron momentum distributions from single ionization of helium by a laser pulse consisting of two counterrotating circularly polarized fields (390 nm and 780 nm). A pronounced 3D low energy structure and sub-cycle interferences are observed experimentally and reproduced numerically using a trajectory based semi-classical simulation. The orientation of the low… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1711.03880v2-abstract-full').style.display = 'inline'; document.getElementById('1711.03880v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1711.03880v2-abstract-full" style="display: none;"> We report on three-dimensional (3D) electron momentum distributions from single ionization of helium by a laser pulse consisting of two counterrotating circularly polarized fields (390 nm and 780 nm). A pronounced 3D low energy structure and sub-cycle interferences are observed experimentally and reproduced numerically using a trajectory based semi-classical simulation. The orientation of the low energy structure in the polarization plane is verified by numerical simulations solving the time dependent Schr枚dinger equation. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1711.03880v2-abstract-full').style.display = 'none'; document.getElementById('1711.03880v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 23 March, 2018; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 10 November, 2017; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> November 2017. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">5 pages, 4 figures, PRA Rapid Communications accepted</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. A 97, 041402 (2018) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1609.03828">arXiv:1609.03828</a> <span> [<a href="https://arxiv.org/pdf/1609.03828">pdf</a>, <a href="https://arxiv.org/format/1609.03828">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Chemical Physics">physics.chem-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1021/acs.jpclett.7b01000">10.1021/acs.jpclett.7b01000 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Observation of enhanced chiral asymmetries in the inner-shell photoionization of uniaxially oriented methyloxirane enantiomers </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Tia%2C+M">Maurice Tia</a>, <a href="/search/physics?searchtype=author&query=Pitzer%2C+M">Martin Pitzer</a>, <a href="/search/physics?searchtype=author&query=Kastirke%2C+G">Gregor Kastirke</a>, <a href="/search/physics?searchtype=author&query=Gatzke%2C+J">Janine Gatzke</a>, <a href="/search/physics?searchtype=author&query=Kim%2C+H">Hong-Keun Kim</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">Florian Trinter</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">Jonas Rist</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">Alexander Hartung</a>, <a href="/search/physics?searchtype=author&query=Trabert%2C+D">Daniel Trabert</a>, <a href="/search/physics?searchtype=author&query=Siebert%2C+J">Juliane Siebert</a>, <a href="/search/physics?searchtype=author&query=Henrichs%2C+K">Kevin Henrichs</a>, <a href="/search/physics?searchtype=author&query=Becht%2C+J">Jasper Becht</a>, <a href="/search/physics?searchtype=author&query=Zeller%2C+S">Stefan Zeller</a>, <a href="/search/physics?searchtype=author&query=Gassert%2C+H">Helena Gassert</a>, <a href="/search/physics?searchtype=author&query=Wiegandt%2C+F">Florian Wiegandt</a>, <a href="/search/physics?searchtype=author&query=Wallauer%2C+R">Robert Wallauer</a>, <a href="/search/physics?searchtype=author&query=Kuhlins%2C+A">Andreas Kuhlins</a>, <a href="/search/physics?searchtype=author&query=Schober%2C+C">Carl Schober</a>, <a href="/search/physics?searchtype=author&query=Bauer%2C+T">Tobias Bauer</a>, <a href="/search/physics?searchtype=author&query=Wechselberger%2C+N">Natascha Wechselberger</a>, <a href="/search/physics?searchtype=author&query=Burzynski%2C+P">Phillip Burzynski</a>, <a href="/search/physics?searchtype=author&query=Neff%2C+J">Jonathan Neff</a>, <a href="/search/physics?searchtype=author&query=Weller%2C+M">Miriam Weller</a>, <a href="/search/physics?searchtype=author&query=Metz%2C+D">Daniel Metz</a>, <a href="/search/physics?searchtype=author&query=Kircher%2C+M">Max Kircher</a> , et al. (16 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1609.03828v2-abstract-short" style="display: inline;"> Most large molecules are chiral in their structure: they exist as two enantiomers, which are mirror images of each other. Whereas the rovibronic sublevels of two enantiomers are almost identical, it turns out that the photoelectric effect is sensitive to the absolute configuration of the ionized enantiomer - an effect termed Photoelectron Circular Dichroism (PECD). Our comprehensive study demonstr… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1609.03828v2-abstract-full').style.display = 'inline'; document.getElementById('1609.03828v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1609.03828v2-abstract-full" style="display: none;"> Most large molecules are chiral in their structure: they exist as two enantiomers, which are mirror images of each other. Whereas the rovibronic sublevels of two enantiomers are almost identical, it turns out that the photoelectric effect is sensitive to the absolute configuration of the ionized enantiomer - an effect termed Photoelectron Circular Dichroism (PECD). Our comprehensive study demonstrates that the origin of PECD can be found in the molecular frame electron emission pattern connecting PECD to other fundamental photophysical effects as the circular dichroism in angular distributions (CDAD). Accordingly, orienting a chiral molecule in space enhances the PECD by a factor of about 10. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1609.03828v2-abstract-full').style.display = 'none'; document.getElementById('1609.03828v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 16 February, 2017; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 13 September, 2016; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> September 2016. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> J. Phys. Chem. Lett. (2017) 8 pp 2780-2786 </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1606.07303">arXiv:1606.07303</a> <span> [<a href="https://arxiv.org/pdf/1606.07303">pdf</a>, <a href="https://arxiv.org/format/1606.07303">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.117.133202">10.1103/PhysRevLett.117.133202 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Non-Sequential Double Ionization by Counter Rotating Circularly Polarized Two-Color Laser Fields </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Eckart%2C+S">S. Eckart</a>, <a href="/search/physics?searchtype=author&query=Richter%2C+M">M. Richter</a>, <a href="/search/physics?searchtype=author&query=Kunitski%2C+M">M. Kunitski</a>, <a href="/search/physics?searchtype=author&query=Hartung%2C+A">A. Hartung</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Henrichs%2C+K">K. Henrichs</a>, <a href="/search/physics?searchtype=author&query=Schlott%2C+N">N. Schlott</a>, <a href="/search/physics?searchtype=author&query=Kang%2C+H">H. Kang</a>, <a href="/search/physics?searchtype=author&query=Bauer%2C+T">T. Bauer</a>, <a href="/search/physics?searchtype=author&query=Sann%2C+H">H. Sann</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M">M. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1606.07303v2-abstract-short" style="display: inline;"> We report on non-sequential double ionization of Ar by a laser pulse consisting of two counter rotating circularly polarized fields (390 nm and 780 nm). The double ionization probability depends strongly on the relative intensity of the two fields and shows a "knee"-like structure as function of intensity. We conclude that double ionization is driven by a beam of nearly monoenergetic recolliding e… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1606.07303v2-abstract-full').style.display = 'inline'; document.getElementById('1606.07303v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1606.07303v2-abstract-full" style="display: none;"> We report on non-sequential double ionization of Ar by a laser pulse consisting of two counter rotating circularly polarized fields (390 nm and 780 nm). The double ionization probability depends strongly on the relative intensity of the two fields and shows a "knee"-like structure as function of intensity. We conclude that double ionization is driven by a beam of nearly monoenergetic recolliding electrons, which can be controlled in intensity and energy by the field parameters. The electron momentum distributions show the recolliding electron as well as a second electron which escapes from an intermediate excited state of Ar$^+$. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1606.07303v2-abstract-full').style.display = 'none'; document.getElementById('1606.07303v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 16 August, 2016; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 23 June, 2016; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> June 2016. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">6 pages, 3 figures, Phys.Rev.Lett. accepted</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 117, 133202 (2016) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1601.06012">arXiv:1601.06012</a> <span> [<a href="https://arxiv.org/pdf/1601.06012">pdf</a>, <a href="https://arxiv.org/format/1601.06012">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Atomic and Molecular Clusters">physics.atm-clus</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.116.043001">10.1103/PhysRevLett.116.043001 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Electron localization in dissociating $H_2^+$ by retroaction of a photoelectron onto its source </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Waitz%2C+M">M. Waitz</a>, <a href="/search/physics?searchtype=author&query=Aslit%C3%BCrk%2C+D">D. Aslit眉rk</a>, <a href="/search/physics?searchtype=author&query=Wechselberger%2C+N">N. Wechselberger</a>, <a href="/search/physics?searchtype=author&query=Gill%2C+H+K">H. K. Gill</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Wiegandt%2C+F">F. Wiegandt</a>, <a href="/search/physics?searchtype=author&query=Goihl%2C+C">C. Goihl</a>, <a href="/search/physics?searchtype=author&query=Kastirke%2C+G">G. Kastirke</a>, <a href="/search/physics?searchtype=author&query=Weller%2C+M">M. Weller</a>, <a href="/search/physics?searchtype=author&query=Bauer%2C+T">T. Bauer</a>, <a href="/search/physics?searchtype=author&query=Metz%2C+D">D. Metz</a>, <a href="/search/physics?searchtype=author&query=Sturm%2C+F+P">F. P. Sturm</a>, <a href="/search/physics?searchtype=author&query=Voigtsberger%2C+J">J. Voigtsberger</a>, <a href="/search/physics?searchtype=author&query=Zeller%2C+S">S. Zeller</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Schiwietz%2C+G">G. Schiwietz</a>, <a href="/search/physics?searchtype=author&query=Weber%2C+T">T. Weber</a>, <a href="/search/physics?searchtype=author&query=Williams%2C+J+B">J. B. Williams</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1601.06012v1-abstract-short" style="display: inline;"> We investigate the dissociation of $H_2^+$ into a proton and a $H^0$ after single ionization with photons of an energy close to the threshold. We find that the $p^+$ and the $H^0$ do not emerge symmetrically in case of the $H_2^+$ dissociating along the $1s蟽_g$ ground state. Instead, a preference for the ejection of the $p^+$ in the direction of the escaping photoelectron can be observed. This sym… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1601.06012v1-abstract-full').style.display = 'inline'; document.getElementById('1601.06012v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1601.06012v1-abstract-full" style="display: none;"> We investigate the dissociation of $H_2^+$ into a proton and a $H^0$ after single ionization with photons of an energy close to the threshold. We find that the $p^+$ and the $H^0$ do not emerge symmetrically in case of the $H_2^+$ dissociating along the $1s蟽_g$ ground state. Instead, a preference for the ejection of the $p^+$ in the direction of the escaping photoelectron can be observed. This symmetry breaking is strongest for very small electron energies. Our experiment is consistent with a recent prediction by Serov and Kheifets [Phys. Rev. A 89, 031402 (2014)]. In their model, which treats the photoelectron classically, the symmetry breaking is induced by the retroaction of the long range Coulomb potential onto the dissociating $H_2^+$. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1601.06012v1-abstract-full').style.display = 'none'; document.getElementById('1601.06012v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 22 January, 2016; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2016. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">Accepted for publication in Phys.Rev.Lett. 1/11/2016</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 116, 043001 (2016) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1509.02349">arXiv:1509.02349</a> <span> [<a href="https://arxiv.org/pdf/1509.02349">pdf</a>, <a href="https://arxiv.org/format/1509.02349">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.116.073201">10.1103/PhysRevLett.116.073201 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Agreement at last: an experimental and theoretical study on the single ionization of helium by fast proton impact </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Gassert%2C+H">H. Gassert</a>, <a href="/search/physics?searchtype=author&query=Chuluunbaatar%2C+O">O. Chuluunbaatar</a>, <a href="/search/physics?searchtype=author&query=Waitz%2C+M">M. Waitz</a>, <a href="/search/physics?searchtype=author&query=Trinter%2C+F">F. Trinter</a>, <a href="/search/physics?searchtype=author&query=Kim%2C+H+-">H. -K. Kim</a>, <a href="/search/physics?searchtype=author&query=Bauer%2C+T">T. Bauer</a>, <a href="/search/physics?searchtype=author&query=Laucke%2C+A">A. Laucke</a>, <a href="/search/physics?searchtype=author&query=M%C3%BCller%2C+C">Ch. M眉ller</a>, <a href="/search/physics?searchtype=author&query=Voigtsberger%2C+J">J. Voigtsberger</a>, <a href="/search/physics?searchtype=author&query=Weller%2C+M">M. Weller</a>, <a href="/search/physics?searchtype=author&query=Rist%2C+J">J. Rist</a>, <a href="/search/physics?searchtype=author&query=Pitzer%2C+M">M. Pitzer</a>, <a href="/search/physics?searchtype=author&query=Zeller%2C+S">S. Zeller</a>, <a href="/search/physics?searchtype=author&query=Jahnke%2C+T">T. Jahnke</a>, <a href="/search/physics?searchtype=author&query=Schmidt%2C+L+P+H">L. Ph. H. Schmidt</a>, <a href="/search/physics?searchtype=author&query=Williams%2C+J+B">J. B. Williams</a>, <a href="/search/physics?searchtype=author&query=Zaytsev%2C+S+A">S. A. Zaytsev</a>, <a href="/search/physics?searchtype=author&query=Bulychev%2C+A+A">A. A. Bulychev</a>, <a href="/search/physics?searchtype=author&query=Kouzakov%2C+K+A">K. A. Kouzakov</a>, <a href="/search/physics?searchtype=author&query=Schmidt-B%C3%B6cking%2C+H">H. Schmidt-B枚cking</a>, <a href="/search/physics?searchtype=author&query=D%C3%B6rner%2C+R">R. D枚rner</a>, <a href="/search/physics?searchtype=author&query=Popov%2C+Y+V">Yu. V. Popov</a>, <a href="/search/physics?searchtype=author&query=Sch%C3%B6ffler%2C+M+S">M. S. Sch枚ffler</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1509.02349v1-abstract-short" style="display: inline;"> Even though ion/atom-collision is a mature field of atomic physics great discrepancies between experiment and theoretical calculations are still common. Here we present experimental results with highest momentum resolution on single ionization of helium induced by 1\,MeV protons and compare these to different theoretical calculations. The overall agreement is strikingly good and already the first… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1509.02349v1-abstract-full').style.display = 'inline'; document.getElementById('1509.02349v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1509.02349v1-abstract-full" style="display: none;"> Even though ion/atom-collision is a mature field of atomic physics great discrepancies between experiment and theoretical calculations are still common. Here we present experimental results with highest momentum resolution on single ionization of helium induced by 1\,MeV protons and compare these to different theoretical calculations. The overall agreement is strikingly good and already the first Born approximation yields good agreement between theory and experiment. This has been expected since several decades, but so far has not been accomplished. The influence of projectile coherence effects on the measured data is shortly discussed in line with an ongoing dispute on the existence of nodal structures in the electron angular emission distributions. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1509.02349v1-abstract-full').style.display = 'none'; document.getElementById('1509.02349v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 8 September, 2015; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> September 2015. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">15 pages, 4 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 116, 073201 (2016) </p> </li> </ol> <div class="is-hidden-tablet"> <!-- feedback for mobile only --> <span class="help" style="display: inline-block;"><a href="https://github.com/arXiv/arxiv-search/releases">Search v0.5.6 released 2020-02-24</a> </span> </div> </div> </main> <footer> <div class="columns is-desktop" role="navigation" aria-label="Secondary"> <!-- MetaColumn 1 --> <div class="column"> <div class="columns"> <div class="column"> <ul class="nav-spaced"> <li><a href="https://info.arxiv.org/about">About</a></li> <li><a href="https://info.arxiv.org/help">Help</a></li> </ul> </div> <div class="column"> <ul class="nav-spaced"> <li> <svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 512 512" class="icon filter-black" role="presentation"><title>contact arXiv</title><desc>Click here to contact arXiv</desc><path d="M502.3 190.8c3.9-3.1 9.7-.2 9.7 4.7V400c0 26.5-21.5 48-48 48H48c-26.5 0-48-21.5-48-48V195.6c0-5 5.7-7.8 9.7-4.7 22.4 17.4 52.1 39.5 154.1 113.6 21.1 15.4 56.7 47.8 92.2 47.6 35.7.3 72-32.8 92.3-47.6 102-74.1 131.6-96.3 154-113.7zM256 320c23.2.4 56.6-29.2 73.4-41.4 132.7-96.3 142.8-104.7 173.4-128.7 5.8-4.5 9.2-11.5 9.2-18.9v-19c0-26.5-21.5-48-48-48H48C21.5 64 0 85.5 0 112v19c0 7.4 3.4 14.3 9.2 18.9 30.6 23.9 40.7 32.4 173.4 128.7 16.8 12.2 50.2 41.8 73.4 41.4z"/></svg> <a href="https://info.arxiv.org/help/contact.html"> Contact</a> </li> <li> <svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 512 512" class="icon filter-black" role="presentation"><title>subscribe to arXiv mailings</title><desc>Click here to subscribe</desc><path d="M476 3.2L12.5 270.6c-18.1 10.4-15.8 35.6 2.2 43.2L121 358.4l287.3-253.2c5.5-4.9 13.3 2.6 8.6 8.3L176 407v80.5c0 23.6 28.5 32.9 42.5 15.8L282 426l124.6 52.2c14.2 6 30.4-2.9 33-18.2l72-432C515 7.8 493.3-6.8 476 3.2z"/></svg> <a href="https://info.arxiv.org/help/subscribe"> Subscribe</a> </li> </ul> </div> </div> </div> <!-- end MetaColumn 1 --> <!-- MetaColumn 2 --> <div class="column"> <div class="columns"> <div class="column"> <ul class="nav-spaced"> <li><a href="https://info.arxiv.org/help/license/index.html">Copyright</a></li> <li><a href="https://info.arxiv.org/help/policies/privacy_policy.html">Privacy Policy</a></li> </ul> </div> <div class="column sorry-app-links"> <ul class="nav-spaced"> <li><a href="https://info.arxiv.org/help/web_accessibility.html">Web Accessibility Assistance</a></li> <li> <p class="help"> <a class="a11y-main-link" href="https://status.arxiv.org" target="_blank">arXiv Operational Status <svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 256 512" class="icon filter-dark_grey" role="presentation"><path d="M224.3 273l-136 136c-9.4 9.4-24.6 9.4-33.9 0l-22.6-22.6c-9.4-9.4-9.4-24.6 0-33.9l96.4-96.4-96.4-96.4c-9.4-9.4-9.4-24.6 0-33.9L54.3 103c9.4-9.4 24.6-9.4 33.9 0l136 136c9.5 9.4 9.5 24.6.1 34z"/></svg></a><br> Get status notifications via <a class="is-link" href="https://subscribe.sorryapp.com/24846f03/email/new" target="_blank"><svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 512 512" class="icon filter-black" role="presentation"><path d="M502.3 190.8c3.9-3.1 9.7-.2 9.7 4.7V400c0 26.5-21.5 48-48 48H48c-26.5 0-48-21.5-48-48V195.6c0-5 5.7-7.8 9.7-4.7 22.4 17.4 52.1 39.5 154.1 113.6 21.1 15.4 56.7 47.8 92.2 47.6 35.7.3 72-32.8 92.3-47.6 102-74.1 131.6-96.3 154-113.7zM256 320c23.2.4 56.6-29.2 73.4-41.4 132.7-96.3 142.8-104.7 173.4-128.7 5.8-4.5 9.2-11.5 9.2-18.9v-19c0-26.5-21.5-48-48-48H48C21.5 64 0 85.5 0 112v19c0 7.4 3.4 14.3 9.2 18.9 30.6 23.9 40.7 32.4 173.4 128.7 16.8 12.2 50.2 41.8 73.4 41.4z"/></svg>email</a> or <a class="is-link" href="https://subscribe.sorryapp.com/24846f03/slack/new" target="_blank"><svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 448 512" class="icon filter-black" role="presentation"><path d="M94.12 315.1c0 25.9-21.16 47.06-47.06 47.06S0 341 0 315.1c0-25.9 21.16-47.06 47.06-47.06h47.06v47.06zm23.72 0c0-25.9 21.16-47.06 47.06-47.06s47.06 21.16 47.06 47.06v117.84c0 25.9-21.16 47.06-47.06 47.06s-47.06-21.16-47.06-47.06V315.1zm47.06-188.98c-25.9 0-47.06-21.16-47.06-47.06S139 32 164.9 32s47.06 21.16 47.06 47.06v47.06H164.9zm0 23.72c25.9 0 47.06 21.16 47.06 47.06s-21.16 47.06-47.06 47.06H47.06C21.16 243.96 0 222.8 0 196.9s21.16-47.06 47.06-47.06H164.9zm188.98 47.06c0-25.9 21.16-47.06 47.06-47.06 25.9 0 47.06 21.16 47.06 47.06s-21.16 47.06-47.06 47.06h-47.06V196.9zm-23.72 0c0 25.9-21.16 47.06-47.06 47.06-25.9 0-47.06-21.16-47.06-47.06V79.06c0-25.9 21.16-47.06 47.06-47.06 25.9 0 47.06 21.16 47.06 47.06V196.9zM283.1 385.88c25.9 0 47.06 21.16 47.06 47.06 0 25.9-21.16 47.06-47.06 47.06-25.9 0-47.06-21.16-47.06-47.06v-47.06h47.06zm0-23.72c-25.9 0-47.06-21.16-47.06-47.06 0-25.9 21.16-47.06 47.06-47.06h117.84c25.9 0 47.06 21.16 47.06 47.06 0 25.9-21.16 47.06-47.06 47.06H283.1z"/></svg>slack</a> </p> </li> </ul> </div> </div> </div> <!-- end MetaColumn 2 --> </div> </footer> <script src="https://static.arxiv.org/static/base/1.0.0a5/js/member_acknowledgement.js"></script> </body> </html>