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<button class="button is-small is-link">Go</button> </div> </div> </form> </div> </div> <ol class="breathe-horizontal" start="1"> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2411.01700">arXiv:2411.01700</a> <span> [<a href="https://arxiv.org/pdf/2411.01700">pdf</a>, <a href="https://arxiv.org/format/2411.01700">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Chemical Physics">physics.chem-ph</span> </div> </div> <p class="title is-5 mathjax"> Attosecond Coherent Electron Motion in a Photoionized Aromatic Molecule </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a>, <a href="/search/physics?searchtype=author&query=Guo%2C+Z">Zhaoheng Guo</a>, <a href="/search/physics?searchtype=author&query=Isele%2C+E">Erik Isele</a>, <a href="/search/physics?searchtype=author&query=Grell%2C+G">Gilbert Grell</a>, <a href="/search/physics?searchtype=author&query=Ruberti%2C+M">Marco Ruberti</a>, <a href="/search/physics?searchtype=author&query=ONeal%2C+J+T">Jordan T. ONeal</a>, <a href="/search/physics?searchtype=author&query=Alexander%2C+O">Oliver Alexander</a>, <a href="/search/physics?searchtype=author&query=Beauvarlet%2C+S">Sandra Beauvarlet</a>, <a href="/search/physics?searchtype=author&query=Cesar%2C+D">David Cesar</a>, <a href="/search/physics?searchtype=author&query=Duris%2C+J">Joseph Duris</a>, <a href="/search/physics?searchtype=author&query=Garratt%2C+D">Douglas Garratt</a>, <a href="/search/physics?searchtype=author&query=Larsen%2C+K+A">Kirk A. Larsen</a>, <a href="/search/physics?searchtype=author&query=Li%2C+S">Siqi Li</a>, <a href="/search/physics?searchtype=author&query=Koloren%C4%8D%2C+P">P艡emysl Koloren膷</a>, <a href="/search/physics?searchtype=author&query=McCracken%2C+G+A">Gregory A. McCracken</a>, <a href="/search/physics?searchtype=author&query=Tuthill%2C+D">Daniel Tuthill</a>, <a href="/search/physics?searchtype=author&query=Wang%2C+Z">Zifan Wang</a>, <a href="/search/physics?searchtype=author&query=Berrah%2C+N">Nora Berrah</a>, <a href="/search/physics?searchtype=author&query=Bostedt%2C+C">Christoph Bostedt</a>, <a href="/search/physics?searchtype=author&query=Borne%2C+K">Kurtis Borne</a>, <a href="/search/physics?searchtype=author&query=Cheng%2C+X">Xinxin Cheng</a>, <a href="/search/physics?searchtype=author&query=DiMauro%2C+L+F">Louis F. DiMauro</a>, <a href="/search/physics?searchtype=author&query=Doumy%2C+G">Gilles Doumy</a>, <a href="/search/physics?searchtype=author&query=Franz%2C+P+L">Paris L. Franz</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a> , et al. (28 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2411.01700v1-abstract-short" style="display: inline;"> In molecular systems, the ultrafast motion of electrons initiates the process of chemical change. Tracking this electronic motion across molecules requires coupling attosecond time resolution to atomic-scale spatial sensitivity. In this work, we employ a pair of attosecond x-ray pulses from an x-ray free-electron laser to follow electron motion resulting from the sudden removal of an electron from… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2411.01700v1-abstract-full').style.display = 'inline'; document.getElementById('2411.01700v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2411.01700v1-abstract-full" style="display: none;"> In molecular systems, the ultrafast motion of electrons initiates the process of chemical change. Tracking this electronic motion across molecules requires coupling attosecond time resolution to atomic-scale spatial sensitivity. In this work, we employ a pair of attosecond x-ray pulses from an x-ray free-electron laser to follow electron motion resulting from the sudden removal of an electron from a prototypical aromatic system, para-aminophenol. X-ray absorption enables tracking this motion with atomic-site specificity. Our measurements are compared with state-of-the-art computational modeling, reproducing the observed response across multiple timescales. Sub-femtosecond dynamics are assigned to states undergoing non-radiative decay, while few-femtosecond oscillatory motion is associated with electronic wavepacket motion in stable cation states, that will eventually couple to nuclear motion. Our work provides insight on the ultrafast charge motion preceding and initiating chemical transformations in moderately complex systems, and provides a powerful benchmark for computational models of ultrafast charge motion in matter. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2411.01700v1-abstract-full').style.display = 'none'; document.getElementById('2411.01700v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 3 November, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> November 2024. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2406.13083">arXiv:2406.13083</a> <span> [<a href="https://arxiv.org/pdf/2406.13083">pdf</a>, <a href="https://arxiv.org/format/2406.13083">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Instrumentation and Detectors">physics.ins-det</span> </div> </div> <p class="title is-5 mathjax"> Design and Performance of a Magnetic Bottle Electron Spectrometer for High-Energy Photoelectron Spectroscopy </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Borne%2C+K">Kurtis Borne</a>, <a href="/search/physics?searchtype=author&query=ONeal%2C+J+T">Jordan T ONeal</a>, <a href="/search/physics?searchtype=author&query=Wang%2C+J">Jun Wang</a>, <a href="/search/physics?searchtype=author&query=Isele%2C+E">Erk Isele</a>, <a href="/search/physics?searchtype=author&query=Obaid%2C+R">Razib Obaid</a>, <a href="/search/physics?searchtype=author&query=Berrah%2C+N">Nora Berrah</a>, <a href="/search/physics?searchtype=author&query=Cheng%2C+X">Xinxin Cheng</a>, <a href="/search/physics?searchtype=author&query=Bucksbaum%2C+P+H">Philip H Bucksbaum</a>, <a href="/search/physics?searchtype=author&query=James%2C+J">Justin James</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andri Kamalov</a>, <a href="/search/physics?searchtype=author&query=Larsen%2C+K+A">Kirk A Larsen</a>, <a href="/search/physics?searchtype=author&query=Li%2C+X">Xiang Li</a>, <a href="/search/physics?searchtype=author&query=Lin%2C+M">Ming-Fu Lin</a>, <a href="/search/physics?searchtype=author&query=Liu%2C+Y">Yusong Liu</a>, <a href="/search/physics?searchtype=author&query=Marinelli%2C+A">Agostino Marinelli</a>, <a href="/search/physics?searchtype=author&query=Summers%2C+A">Adam Summers</a>, <a href="/search/physics?searchtype=author&query=Thierstein%2C+E">Emily Thierstein</a>, <a href="/search/physics?searchtype=author&query=Wolf%2C+T">Thomas Wolf</a>, <a href="/search/physics?searchtype=author&query=Rolles%2C+D">Daniel Rolles</a>, <a href="/search/physics?searchtype=author&query=Walter%2C+P">Peter Walter</a>, <a href="/search/physics?searchtype=author&query=Cryan%2C+J+P">James P Cryan</a>, <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2406.13083v2-abstract-short" style="display: inline;"> We describe the design and performance of a magnetic bottle electron spectrometer~(MBES) for high-energy electron spectroscopy. Our design features a ${\sim2}$~m long electron drift tube and electrostatic retardation lens, achieving sub-electronvolt (eV) electron kinetic energy resolution for high energy (several hundred eV) electrons with close to 4$蟺$ collection efficiency. A segmented anode… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2406.13083v2-abstract-full').style.display = 'inline'; document.getElementById('2406.13083v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2406.13083v2-abstract-full" style="display: none;"> We describe the design and performance of a magnetic bottle electron spectrometer~(MBES) for high-energy electron spectroscopy. Our design features a ${\sim2}$~m long electron drift tube and electrostatic retardation lens, achieving sub-electronvolt (eV) electron kinetic energy resolution for high energy (several hundred eV) electrons with close to 4$蟺$ collection efficiency. A segmented anode electron detector enables the simultaneous collection of photoelectron spectra in high resolution and high collection efficiency modes. This versatile instrument is installed at the TMO endstation at the LCLS x-ray free-electron laser (XFEL). In this paper, we demonstrate its high resolution, collection efficiency and spatial selectivity in measurements where it is coupled to an XFEL source. These combined characteristics are designed to enable high-resolution time-resolved measurements using x-ray photoelectron, absorption, and Auger-Meitner spectroscopy. We also describe the pervasive artifact in MBES time-of-flight spectra that arises from a periodic modulation in electron detection efficiency, and present a robust analysis procedure for its removal. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2406.13083v2-abstract-full').style.display = 'none'; document.getElementById('2406.13083v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 4 July, 2024; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 18 June, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> June 2024. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2402.17685">arXiv:2402.17685</a> <span> [<a href="https://arxiv.org/pdf/2402.17685">pdf</a>, <a href="https://arxiv.org/format/2402.17685">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Chemical Physics">physics.chem-ph</span> </div> </div> <p class="title is-5 mathjax"> Attosecond X-ray Chronoscopy of Core-level Photoemission </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Ji%2C+J">Jia-Bao Ji</a>, <a href="/search/physics?searchtype=author&query=Guo%2C+Z">Zhaoheng Guo</a>, <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a>, <a href="/search/physics?searchtype=author&query=Trevisan%2C+C+S">Cynthia S. Trevisan</a>, <a href="/search/physics?searchtype=author&query=Cesar%2C+D">David Cesar</a>, <a href="/search/physics?searchtype=author&query=Cheng%2C+X">Xinxin Cheng</a>, <a href="/search/physics?searchtype=author&query=Duris%2C+J">Joseph Duris</a>, <a href="/search/physics?searchtype=author&query=Franz%2C+P+L">Paris L. Franz</a>, <a href="/search/physics?searchtype=author&query=Glownia%2C+J">James Glownia</a>, <a href="/search/physics?searchtype=author&query=Gong%2C+X">Xiaochun Gong</a>, <a href="/search/physics?searchtype=author&query=Hammerland%2C+D">Daniel Hammerland</a>, <a href="/search/physics?searchtype=author&query=Han%2C+M">Meng Han</a>, <a href="/search/physics?searchtype=author&query=Heck%2C+S">Saijoscha Heck</a>, <a href="/search/physics?searchtype=author&query=Hoffmann%2C+M">Matthias Hoffmann</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Larsen%2C+K+A">Kirk A. Larsen</a>, <a href="/search/physics?searchtype=author&query=Li%2C+X">Xiang Li</a>, <a href="/search/physics?searchtype=author&query=Lin%2C+M">Ming-Fu Lin</a>, <a href="/search/physics?searchtype=author&query=Liu%2C+Y">Yuchen Liu</a>, <a href="/search/physics?searchtype=author&query=McCurdy%2C+C+W">C. William McCurdy</a>, <a href="/search/physics?searchtype=author&query=Obaid%2C+R">Razib Obaid</a>, <a href="/search/physics?searchtype=author&query=ONeal%2C+J+T">Jordan T. ONeal</a>, <a href="/search/physics?searchtype=author&query=Rescigno%2C+T+N">Thomas N. Rescigno</a>, <a href="/search/physics?searchtype=author&query=Robles%2C+R+R">River R. Robles</a>, <a href="/search/physics?searchtype=author&query=Sudar%2C+N">Nicholas Sudar</a> , et al. (10 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2402.17685v3-abstract-short" style="display: inline;"> Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits to the complexity of systems that can be studied and the information that can be retrieved, respectively. Using attosecond X-ray pulses from LCLS, we demonstrat… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2402.17685v3-abstract-full').style.display = 'inline'; document.getElementById('2402.17685v3-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2402.17685v3-abstract-full" style="display: none;"> Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits to the complexity of systems that can be studied and the information that can be retrieved, respectively. Using attosecond X-ray pulses from LCLS, we demonstrate the key advantages of measuring core-level delays: the photoelectron spectra remain atom-like, the measurements become element specific and the observed scattering dynamics originate from a point-like source. We exploit these unique features to reveal the effects of electronegativity and symmetry on attosecond scattering dynamics by measuring the photoionization delays between N-1s and C-1s core shells of a series of aromatic azabenzene molecules. Remarkably, the delays systematically increase with the number of nitrogen atoms in the molecule and reveal multiple resonances. We identify two previously unknown mechanisms regulating the associated attosecond dynamics, namely the enhanced confinement of the trapped wavefunction with increasing electronegativity of the atoms and the decrease of the coupling strength among the photoemitted partial waves with increasing symmetry. This study demonstrates the unique opportunities opened by measurements of core-level photoionization delays for unravelling attosecond electron dynamics in complex matter. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2402.17685v3-abstract-full').style.display = 'none'; document.getElementById('2402.17685v3-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 8 April, 2024; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 27 February, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> February 2024. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2402.12764">arXiv:2402.12764</a> <span> [<a href="https://arxiv.org/pdf/2402.12764">pdf</a>, <a href="https://arxiv.org/format/2402.12764">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> </div> <p class="title is-5 mathjax"> Attosecond Delays in X-ray Molecular Ionization </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a>, <a href="/search/physics?searchtype=author&query=Mountney%2C+M">Miles Mountney</a>, <a href="/search/physics?searchtype=author&query=Wang%2C+J">Jun Wang</a>, <a href="/search/physics?searchtype=author&query=Ortmann%2C+L">Lisa Ortmann</a>, <a href="/search/physics?searchtype=author&query=Al-Haddad%2C+A">Andre Al-Haddad</a>, <a href="/search/physics?searchtype=author&query=Berrah%2C+N">Nora Berrah</a>, <a href="/search/physics?searchtype=author&query=Bostedt%2C+C">Christoph Bostedt</a>, <a href="/search/physics?searchtype=author&query=Champenois%2C+E+G">Elio G. Champenois</a>, <a href="/search/physics?searchtype=author&query=DiMauro%2C+L+F">Louis F. DiMauro</a>, <a href="/search/physics?searchtype=author&query=Duris%2C+J">Joseph Duris</a>, <a href="/search/physics?searchtype=author&query=Garratt%2C+D">Douglas Garratt</a>, <a href="/search/physics?searchtype=author&query=Glownia%2C+J+M">James M. Glownia</a>, <a href="/search/physics?searchtype=author&query=Guo%2C+Z">Zhaoheng Guo</a>, <a href="/search/physics?searchtype=author&query=Haxton%2C+D">Daniel Haxton</a>, <a href="/search/physics?searchtype=author&query=Isele%2C+E">Erik Isele</a>, <a href="/search/physics?searchtype=author&query=Ivanov%2C+I">Igor Ivanov</a>, <a href="/search/physics?searchtype=author&query=Ji%2C+J">Jiabao Ji</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Li%2C+S">Siqi Li</a>, <a href="/search/physics?searchtype=author&query=Lin%2C+M">Ming-Fu Lin</a>, <a href="/search/physics?searchtype=author&query=Marangos%2C+J+P">Jon P. Marangos</a>, <a href="/search/physics?searchtype=author&query=Obaid%2C+R">Razib Obaid</a>, <a href="/search/physics?searchtype=author&query=O%27Neal%2C+J+T">Jordan T. O'Neal</a>, <a href="/search/physics?searchtype=author&query=Rosenberger%2C+P">Philipp Rosenberger</a>, <a href="/search/physics?searchtype=author&query=Shivaram%2C+N+H">Niranjan H. Shivaram</a> , et al. (12 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2402.12764v1-abstract-short" style="display: inline;"> The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the requisite tools to resolve the dynamics of photoionization. Accordingly, the past decade has produced a large volume of work on photoionization delays following single photon absorption of an extreme ultraviolet (XUV) phot… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2402.12764v1-abstract-full').style.display = 'inline'; document.getElementById('2402.12764v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2402.12764v1-abstract-full" style="display: none;"> The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the requisite tools to resolve the dynamics of photoionization. Accordingly, the past decade has produced a large volume of work on photoionization delays following single photon absorption of an extreme ultraviolet (XUV) photon. However, the measurement of time-resolved core-level photoionization remained out of reach. The required x-ray photon energies needed for core-level photoionization were not available with attosecond tabletop sources. We have now measured the x-ray photoemission delay of core-level electrons, and here report unexpectedly large delays, ranging up to 700 attoseconds in NO near the oxygen K-shell threshold. These measurements exploit attosecond soft x-ray pulses from a free-electron laser (XFEL) to scan across the entire region near the K-shell threshold. Furthermore, we find the delay spectrum is richly modulated, suggesting several contributions including transient trapping of the photoelectron due to shape resonances, collisions with the Auger-Meitner electron that is emitted in the rapid non-radiative relaxation of the molecule, and multi-electron scattering effects. The results demonstrate how x-ray attosecond experiments, supported by comprehensive theoretical modelling, can unravel the complex correlated dynamics of core-level photoionization. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2402.12764v1-abstract-full').style.display = 'none'; document.getElementById('2402.12764v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 20 February, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> February 2024. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2401.15250">arXiv:2401.15250</a> <span> [<a href="https://arxiv.org/pdf/2401.15250">pdf</a>, <a href="https://arxiv.org/format/2401.15250">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Accelerator Physics">physics.acc-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> </div> </div> <p class="title is-5 mathjax"> Experimental Demonstration of Attosecond Pump-Probe Spectroscopy with an X-ray Free-Electron Laser </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Guo%2C+Z">Zhaoheng Guo</a>, <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a>, <a href="/search/physics?searchtype=author&query=Beauvarlet%2C+S">Sandra Beauvarlet</a>, <a href="/search/physics?searchtype=author&query=Cesar%2C+D">David Cesar</a>, <a href="/search/physics?searchtype=author&query=Duris%2C+J">Joseph Duris</a>, <a href="/search/physics?searchtype=author&query=Franz%2C+P+L">Paris L. Franz</a>, <a href="/search/physics?searchtype=author&query=Alexander%2C+O">Oliver Alexander</a>, <a href="/search/physics?searchtype=author&query=Bohler%2C+D">Dorian Bohler</a>, <a href="/search/physics?searchtype=author&query=Bostedt%2C+C">Christoph Bostedt</a>, <a href="/search/physics?searchtype=author&query=Averbukh%2C+V">Vitali Averbukh</a>, <a href="/search/physics?searchtype=author&query=Cheng%2C+X">Xinxin Cheng</a>, <a href="/search/physics?searchtype=author&query=DiMauro%2C+L+F">Louis F. DiMauro</a>, <a href="/search/physics?searchtype=author&query=Doumy%2C+G">Gilles Doumy</a>, <a href="/search/physics?searchtype=author&query=Forbes%2C+R">Ruaridh Forbes</a>, <a href="/search/physics?searchtype=author&query=Gessner%2C+O">Oliver Gessner</a>, <a href="/search/physics?searchtype=author&query=Glownia%2C+J+M">James M. Glownia</a>, <a href="/search/physics?searchtype=author&query=Isele%2C+E">Erik Isele</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Larsen%2C+K+A">Kirk A. Larsen</a>, <a href="/search/physics?searchtype=author&query=Li%2C+S">Siqi Li</a>, <a href="/search/physics?searchtype=author&query=Li%2C+X">Xiang Li</a>, <a href="/search/physics?searchtype=author&query=Lin%2C+M">Ming-Fu Lin</a>, <a href="/search/physics?searchtype=author&query=McCracken%2C+G+A">Gregory A. McCracken</a>, <a href="/search/physics?searchtype=author&query=Obaid%2C+R">Razib Obaid</a>, <a href="/search/physics?searchtype=author&query=ONeal%2C+J+T">Jordan T. ONeal</a> , et al. (25 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2401.15250v1-abstract-short" style="display: inline;"> Pump-probe experiments with sub-femtosecond resolution are the key to understanding electronic dynamics in quantum systems. Here we demonstrate the generation and control of sub-femtosecond pulse pairs from a two-colour X-ray free-electron laser (XFEL). By measuring the delay between the two pulses with an angular streaking diagnostic, we characterise the group velocity of the XFEL and demonstrate… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2401.15250v1-abstract-full').style.display = 'inline'; document.getElementById('2401.15250v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2401.15250v1-abstract-full" style="display: none;"> Pump-probe experiments with sub-femtosecond resolution are the key to understanding electronic dynamics in quantum systems. Here we demonstrate the generation and control of sub-femtosecond pulse pairs from a two-colour X-ray free-electron laser (XFEL). By measuring the delay between the two pulses with an angular streaking diagnostic, we characterise the group velocity of the XFEL and demonstrate control of the pulse delay down to 270 as. We demonstrate the application of this technique to a pump-probe measurement in core-excited para-aminophenol. These results demonstrate the ability to perform pump-probe experiments with sub-femtosecond resolution and atomic site specificity. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2401.15250v1-abstract-full').style.display = 'none'; document.getElementById('2401.15250v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 26 January, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2024. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">55 pages, main manuscript (5 figures) + supplementary materials (25 figures), 30 figures total. Submitted to Nature Photonics</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2305.05169">arXiv:2305.05169</a> <span> [<a href="https://arxiv.org/pdf/2305.05169">pdf</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Instrumentation and Detectors">physics.ins-det</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Optics">physics.optics</span> </div> </div> <p class="title is-5 mathjax"> A compact single-shot soft X-ray photon spectrometer for free electron laser diagnostics </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Larsen%2C+K+A">Kirk A. Larsen</a>, <a href="/search/physics?searchtype=author&query=Borne%2C+K">Kurtis Borne</a>, <a href="/search/physics?searchtype=author&query=Obaid%2C+R">Razib Obaid</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Liu%2C+Y">Yusong Liu</a>, <a href="/search/physics?searchtype=author&query=Cheng%2C+X">Xinxin Cheng</a>, <a href="/search/physics?searchtype=author&query=James%2C+J">Justin James</a>, <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a>, <a href="/search/physics?searchtype=author&query=Li%2C+K">Kenan Li</a>, <a href="/search/physics?searchtype=author&query=Liu%2C+Y">Yanwei Liu</a>, <a href="/search/physics?searchtype=author&query=Sakdinawat%2C+A">Anne Sakdinawat</a>, <a href="/search/physics?searchtype=author&query=David%2C+C">Christian David</a>, <a href="/search/physics?searchtype=author&query=Wolf%2C+T+J+A">Thomas J. A. Wolf</a>, <a href="/search/physics?searchtype=author&query=Cryan%2C+J">James Cryan</a>, <a href="/search/physics?searchtype=author&query=Walter%2C+P">Peter Walter</a>, <a href="/search/physics?searchtype=author&query=Lin%2C+M">Ming-Fu Lin</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2305.05169v1-abstract-short" style="display: inline;"> The photon spectrum from free-electron laser (FEL) light sources offers valuable information in time-resolved experiments and machine optimization in the spectral and temporal domains. We have developed a compact single-shot photon spectrometer to diagnose soft X-ray spectra. The spectrometer consists of an array of off-axis Fresnel zone plates (FZP) that act as transmission-imaging gratings, a Ce… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2305.05169v1-abstract-full').style.display = 'inline'; document.getElementById('2305.05169v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2305.05169v1-abstract-full" style="display: none;"> The photon spectrum from free-electron laser (FEL) light sources offers valuable information in time-resolved experiments and machine optimization in the spectral and temporal domains. We have developed a compact single-shot photon spectrometer to diagnose soft X-ray spectra. The spectrometer consists of an array of off-axis Fresnel zone plates (FZP) that act as transmission-imaging gratings, a Ce-YAG scintillator, and a microscope objective to image the scintillation target onto a two-dimensional imaging detector. This spectrometer operates in an energy range which covers absorption edges associated with several atomic constituents carbon, nitrogen, oxygen, and neon. The spectrometer's performance is demonstrated at a repetition rate of 120 Hz, but our detection scheme can be easily extended to 200 kHz spectral collection by employing a fast complementary metal oxide semiconductor (CMOS) line-scan camera to detect the light from the scintillator. This compact photon spectrometer provides an opportunity for monitoring the spectrum downstream of an endstation in a limited space environment with subelectronvolt energy resolution. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2305.05169v1-abstract-full').style.display = 'none'; document.getElementById('2305.05169v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 9 May, 2023; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> May 2023. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">14 pages, 5 figures, 1 table</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2209.05233">arXiv:2209.05233</a> <span> [<a href="https://arxiv.org/pdf/2209.05233">pdf</a>, <a href="https://arxiv.org/format/2209.05233">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Instrumentation and Detectors">physics.ins-det</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Data Analysis, Statistics and Probability">physics.data-an</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1007/978-3-031-23606-8_7">10.1007/978-3-031-23606-8_7 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> At-the-edge Data Processing for Low Latency High Throughput Machine Learning Algorithms </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Hirschman%2C+J">Jack Hirschman</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Obaid%2C+R">Razib Obaid</a>, <a href="/search/physics?searchtype=author&query=O%27Shea%2C+F+H">Finn H. O'Shea</a>, <a href="/search/physics?searchtype=author&query=Coffee%2C+R+N">Ryan N Coffee</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2209.05233v1-abstract-short" style="display: inline;"> High throughput and low latency data processing is essential for systems requiring live decision making, control, and machine learning-optimized data reduction. We focus on two distinct use cases for in-flight streaming data processing for a) X-ray pulse reconstruction at SLAC's LCLS-II Free-Electron Laser and b) control diagnostics at the DIII-D tokamak fusion reactor. Both cases exemplify high t… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2209.05233v1-abstract-full').style.display = 'inline'; document.getElementById('2209.05233v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2209.05233v1-abstract-full" style="display: none;"> High throughput and low latency data processing is essential for systems requiring live decision making, control, and machine learning-optimized data reduction. We focus on two distinct use cases for in-flight streaming data processing for a) X-ray pulse reconstruction at SLAC's LCLS-II Free-Electron Laser and b) control diagnostics at the DIII-D tokamak fusion reactor. Both cases exemplify high throughput and low latency control feedback and motivate our focus on machine learning at the edge where data processing and machine learning algorithms can be implemented in field programmable gate array based hardware immediately after the diagnostic sensors. We present our recent work on a data preprocessing chain which requires fast featurization for information encoding. We discuss several options for such algorithms with the primary focus on our discrete cosine and sine transform-based approach adapted for streaming data. These algorithms are primarily aimed at implementation in field programmable gate arrays, favoring linear algebra operations that are also aligned with the recent advances in inference accelerators for the computational edge. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2209.05233v1-abstract-full').style.display = 'none'; document.getElementById('2209.05233v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 6 September, 2022; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> September 2022. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">18 pages, 7 figures; To be published in Smoky Mountains Computational Sciences and Engineering Conference 2022 (SMC 2022) proceedings</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2112.00863">arXiv:2112.00863</a> <span> [<a href="https://arxiv.org/pdf/2112.00863">pdf</a>, <a href="https://arxiv.org/format/2112.00863">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Instrumentation and Detectors">physics.ins-det</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Accelerator Physics">physics.acc-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1107/S1600577522004283">10.1107/S1600577522004283 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> The Time-resolved Atomic, Molecular and Optical Science Instrument at the Linac Coherent Light Source </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Walter%2C+P">Peter Walter</a>, <a href="/search/physics?searchtype=author&query=Osipov%2C+T">Timur Osipov</a>, <a href="/search/physics?searchtype=author&query=Lin%2C+M">Ming-Fu Lin</a>, <a href="/search/physics?searchtype=author&query=Cryan%2C+J">James Cryan</a>, <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Marinelli%2C+A">Agostino Marinelli</a>, <a href="/search/physics?searchtype=author&query=Robinson%2C+J">Joe Robinson</a>, <a href="/search/physics?searchtype=author&query=Seaberg%2C+M">Matt Seaberg</a>, <a href="/search/physics?searchtype=author&query=Wolf%2C+T+J+A">Thomas J. A. Wolf</a>, <a href="/search/physics?searchtype=author&query=Aldrich%2C+J">Jeff Aldrich</a>, <a href="/search/physics?searchtype=author&query=Brown%2C+N">Nolan Brown</a>, <a href="/search/physics?searchtype=author&query=Champenois%2C+E+G">Elio G. Champenois</a>, <a href="/search/physics?searchtype=author&query=Cheng%2C+X">Xinxin Cheng</a>, <a href="/search/physics?searchtype=author&query=Cocco%2C+D">Daniele Cocco</a>, <a href="/search/physics?searchtype=author&query=Conder%2C+A">Alan Conder</a>, <a href="/search/physics?searchtype=author&query=Curiel%2C+I">Ivan Curiel</a>, <a href="/search/physics?searchtype=author&query=Egger%2C+A">Adam Egger</a>, <a href="/search/physics?searchtype=author&query=Glownia%2C+J+M">James M. Glownia</a>, <a href="/search/physics?searchtype=author&query=Heimann%2C+P">Philip Heimann</a>, <a href="/search/physics?searchtype=author&query=Holmes%2C+M">Michael Holmes</a>, <a href="/search/physics?searchtype=author&query=Johnson%2C+T">Tyler Johnson</a>, <a href="/search/physics?searchtype=author&query=Li%2C+X">Xiang Li</a>, <a href="/search/physics?searchtype=author&query=Moeller%2C+S">Stefan Moeller</a>, <a href="/search/physics?searchtype=author&query=Morton%2C+D">DanielS Morton</a> , et al. (17 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2112.00863v1-abstract-short" style="display: inline;"> The newly constructed Time-resolved atomic, Molecular and Optical science instrument (TMO), is configured to take full advantage of both linear accelerators at SLAC National Accelerator Laboratory, the copper accelerator operating at a repetition rate of 120 Hz providing high per pulse energy, as well as the superconducting accelerator operating at a repetition rate of about 1 MHz providing high a… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2112.00863v1-abstract-full').style.display = 'inline'; document.getElementById('2112.00863v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2112.00863v1-abstract-full" style="display: none;"> The newly constructed Time-resolved atomic, Molecular and Optical science instrument (TMO), is configured to take full advantage of both linear accelerators at SLAC National Accelerator Laboratory, the copper accelerator operating at a repetition rate of 120 Hz providing high per pulse energy, as well as the superconducting accelerator operating at a repetition rate of about 1 MHz providing high average intensity. Both accelerators build a soft X-ray free electron laser with the new variable gab undulator section. With this flexible light sources, TMO supports many experimental techniques not previously available at LCLS and will have two X-ray beam focus spots in line. Thereby, TMO supports Atomic, Molecular and Optical (AMO), strong-field and nonlinear science and will host a designated new dynamic reaction microscope with a sub-micron X-ray focus spot. The flexible instrument design is optimized for studying ultrafast electronic and molecular phenomena and can take full advantage of the sub-femtosecond soft X-ray pulse generation program. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2112.00863v1-abstract-full').style.display = 'none'; document.getElementById('2112.00863v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 1 December, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> December 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Report number:</span> gb5129 </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Journal of Synchrotron Radiation 2022 </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2105.08854">arXiv:2105.08854</a> <span> [<a href="https://arxiv.org/pdf/2105.08854">pdf</a>, <a href="https://arxiv.org/format/2105.08854">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Chemical Physics">physics.chem-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1126/science.abj2096">10.1126/science.abj2096 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Attosecond Coherent Electron Motion in Auger-Meitner Decay </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Li%2C+S">Siqi Li</a>, <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a>, <a href="/search/physics?searchtype=author&query=Rosenberger%2C+P">Philipp Rosenberger</a>, <a href="/search/physics?searchtype=author&query=Champenois%2C+E+G">Elio G. Champenois</a>, <a href="/search/physics?searchtype=author&query=Duris%2C+J">Joseph Duris</a>, <a href="/search/physics?searchtype=author&query=Al-Haddad%2C+A">Andre Al-Haddad</a>, <a href="/search/physics?searchtype=author&query=Averbukh%2C+V">Vitali Averbukh</a>, <a href="/search/physics?searchtype=author&query=Barnard%2C+J+C+T">Jonathan C. T. Barnard</a>, <a href="/search/physics?searchtype=author&query=Berrah%2C+N">Nora Berrah</a>, <a href="/search/physics?searchtype=author&query=Bostedt%2C+C">Christoph Bostedt</a>, <a href="/search/physics?searchtype=author&query=Bucksbaum%2C+P+H">Philip H. Bucksbaum</a>, <a href="/search/physics?searchtype=author&query=Coffee%2C+R">Ryan Coffee</a>, <a href="/search/physics?searchtype=author&query=DiMauro%2C+L+F">Louis F. DiMauro</a>, <a href="/search/physics?searchtype=author&query=Fang%2C+L">Li Fang</a>, <a href="/search/physics?searchtype=author&query=Garratt%2C+D">Douglas Garratt</a>, <a href="/search/physics?searchtype=author&query=Gatton%2C+A">Averell Gatton</a>, <a href="/search/physics?searchtype=author&query=Guo%2C+Z">Zhaoheng Guo</a>, <a href="/search/physics?searchtype=author&query=Hartmann%2C+G">Gregor Hartmann</a>, <a href="/search/physics?searchtype=author&query=Haxton%2C+D">Daniel Haxton</a>, <a href="/search/physics?searchtype=author&query=Helml%2C+W">Wolfram Helml</a>, <a href="/search/physics?searchtype=author&query=Huang%2C+Z">Zhirong Huang</a>, <a href="/search/physics?searchtype=author&query=LaForge%2C+A+C">Aaron C. LaForge</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Knurr%2C+J">Jonas Knurr</a>, <a href="/search/physics?searchtype=author&query=Lin%2C+M">Ming-Fu Lin</a> , et al. (16 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2105.08854v1-abstract-short" style="display: inline;"> In quantum systems, coherent superpositions of electronic states evolve on ultrafast timescales (few femtosecond to attosecond, 1 as = 0.001 fs = 10^{-18} s), leading to a time dependent charge density. Here we exploit the first attosecond soft x-ray pulses produced by an x-ray free-electron laser to induce a coherent core-hole excitation in nitric oxide. Using an additional circularly polarized i… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2105.08854v1-abstract-full').style.display = 'inline'; document.getElementById('2105.08854v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2105.08854v1-abstract-full" style="display: none;"> In quantum systems, coherent superpositions of electronic states evolve on ultrafast timescales (few femtosecond to attosecond, 1 as = 0.001 fs = 10^{-18} s), leading to a time dependent charge density. Here we exploit the first attosecond soft x-ray pulses produced by an x-ray free-electron laser to induce a coherent core-hole excitation in nitric oxide. Using an additional circularly polarized infrared laser pulse we create a clock to time-resolve the electron dynamics, and demonstrate control of the coherent electron motion by tuning the photon energy of the x-ray pulse. Core-excited states offer a fundamental test bed for studying coherent electron dynamics in highly excited and strongly correlated matter. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2105.08854v1-abstract-full').style.display = 'none'; document.getElementById('2105.08854v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 18 May, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> May 2021. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2103.07603">arXiv:2103.07603</a> <span> [<a href="https://arxiv.org/pdf/2103.07603">pdf</a>, <a href="https://arxiv.org/format/2103.07603">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Instrumentation and Detectors">physics.ins-det</span> </div> </div> <p class="title is-5 mathjax"> Multi-Resolution Electron Spectrometer Array for Future Free-Electron Laser Experiments </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Walter%2C+P">Peter Walter</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Gatton%2C+A">Averell Gatton</a>, <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a>, <a href="/search/physics?searchtype=author&query=Bhogadi%2C+D">Dileep Bhogadi</a>, <a href="/search/physics?searchtype=author&query=Castagna%2C+J">Jean-Charles Castagna</a>, <a href="/search/physics?searchtype=author&query=Cheng%2C+X">Xianchao Cheng</a>, <a href="/search/physics?searchtype=author&query=Shi%2C+H">Hongliang Shi</a>, <a href="/search/physics?searchtype=author&query=Cryan%2C+J">James Cryan</a>, <a href="/search/physics?searchtype=author&query=Helml%2C+W">Wolfram Helml</a>, <a href="/search/physics?searchtype=author&query=Ilchen%2C+M">Markus Ilchen</a>, <a href="/search/physics?searchtype=author&query=Coffee%2C+R+N">Ryan N. Coffee</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2103.07603v1-abstract-short" style="display: inline;"> We report the design of an angular array of electron Time-of-Flight (eToF) spectrometers intended for non-invasive spectral, temporal, and polarization characterization of single shots of high-repetition rate, quasi-continuous, short-wavelength Free-Electron Lasers (FELs) such as the LCLS-II at SLAC. This array also enables angle-resolved, high-resolution eToF spectroscopy to address a variety of… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2103.07603v1-abstract-full').style.display = 'inline'; document.getElementById('2103.07603v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2103.07603v1-abstract-full" style="display: none;"> We report the design of an angular array of electron Time-of-Flight (eToF) spectrometers intended for non-invasive spectral, temporal, and polarization characterization of single shots of high-repetition rate, quasi-continuous, short-wavelength Free-Electron Lasers (FELs) such as the LCLS-II at SLAC. This array also enables angle-resolved, high-resolution eToF spectroscopy to address a variety of scientific questions of ultrafast and nonlinear light--matter interaction at FELs. The presented device is specifically designed for the Time-resolved atomic, Molecular and Optical science end station (TMO) at LCLS-II. In its final version, it can comprise of up to 20 eToF spectrometers aligned to collect electrons from the interaction point defined by the intersection of the incoming FEL radiation and a gaseous target. There are 16 such spectrometers forming a circular equiangular array in the plane normal to x-ray propagation and 4 spectrometers at 54.7$^\circ$ angle relative to the principle linear x-ray polarization axis. The spectrometers are capable of independent and minimally chromatic electrostatic lensing and retardation in order to enable simultaneous angle-resolved photo-electron and Auger electron spectroscopy with high energy resolution. They are designed to ensure energy resolution of 0.25 eV across an energy window of up to 75 eV which can be individually centered via the adjustable retardation to cover ranges of electron kinetic energies relevant to soft x-ray methods, 0--2 keV. The full spectrometer array will enable non-invasive and online spectral-polarimetry measurements, polarization-sensitive attoclock spectroscopy for characterizing the full time--energy structure of even SASE or seeded LCLS-II pulses, and also supports emerging trends in molecular frame spectroscopy measurements. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2103.07603v1-abstract-full').style.display = 'none'; document.getElementById('2103.07603v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 12 March, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> March 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">under review</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1909.07441">arXiv:1909.07441</a> <span> [<a href="https://arxiv.org/pdf/1909.07441">pdf</a>, <a href="https://arxiv.org/format/1909.07441">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Chemical Physics">physics.chem-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Optics">physics.optics</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Quantum Physics">quant-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1039/C9CP03951A">10.1039/C9CP03951A <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Attosecond Transient Absorption Spooktroscopy: a ghost imaging approach to ultrafast absorption spectroscopy </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a>, <a href="/search/physics?searchtype=author&query=Li%2C+S">Siqi Li</a>, <a href="/search/physics?searchtype=author&query=Champenois%2C+E+G">Elio G. Champenois</a>, <a href="/search/physics?searchtype=author&query=Duris%2C+J">Joseph Duris</a>, <a href="/search/physics?searchtype=author&query=Ratner%2C+D">Daniel Ratner</a>, <a href="/search/physics?searchtype=author&query=Lane%2C+T">TJ Lane</a>, <a href="/search/physics?searchtype=author&query=Rosenberger%2C+P">Philipp Rosenberger</a>, <a href="/search/physics?searchtype=author&query=Al-Haddad%2C+A">Andre Al-Haddad</a>, <a href="/search/physics?searchtype=author&query=Averbukh%2C+V">Vitali Averbukh</a>, <a href="/search/physics?searchtype=author&query=Barnard%2C+T">Toby Barnard</a>, <a href="/search/physics?searchtype=author&query=Berrah%2C+N">Nora Berrah</a>, <a href="/search/physics?searchtype=author&query=Bostedt%2C+C">Christoph Bostedt</a>, <a href="/search/physics?searchtype=author&query=Bucksbaum%2C+P+H">Philip H. Bucksbaum</a>, <a href="/search/physics?searchtype=author&query=Coffee%2C+R">Ryan Coffee</a>, <a href="/search/physics?searchtype=author&query=DiMauro%2C+L+F">Louis F. DiMauro</a>, <a href="/search/physics?searchtype=author&query=Fang%2C+L">Li Fang</a>, <a href="/search/physics?searchtype=author&query=Garratt%2C+D">Douglas Garratt</a>, <a href="/search/physics?searchtype=author&query=Gatton%2C+A">Averell Gatton</a>, <a href="/search/physics?searchtype=author&query=Guo%2C+Z">Zhaoheng Guo</a>, <a href="/search/physics?searchtype=author&query=Hartmann%2C+G">Gregor Hartmann</a>, <a href="/search/physics?searchtype=author&query=Haxton%2C+D">Daniel Haxton</a>, <a href="/search/physics?searchtype=author&query=Helml%2C+W">Wolfram Helml</a>, <a href="/search/physics?searchtype=author&query=Huang%2C+Z">Zhirong Huang</a>, <a href="/search/physics?searchtype=author&query=LaForge%2C+A">Aaron LaForge</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a> , et al. (16 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1909.07441v1-abstract-short" style="display: inline;"> The recent demonstration of isolated attosecond pulses from an X-ray free-electron laser (XFEL) opens the possibility for probing ultrafast electron dynamics at X-ray wavelengths. An established experimental method for probing ultrafast dynamics is X-ray transient absorption spectroscopy, where the X-ray absorption spectrum is measured by scanning the central photon energy and recording the result… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1909.07441v1-abstract-full').style.display = 'inline'; document.getElementById('1909.07441v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1909.07441v1-abstract-full" style="display: none;"> The recent demonstration of isolated attosecond pulses from an X-ray free-electron laser (XFEL) opens the possibility for probing ultrafast electron dynamics at X-ray wavelengths. An established experimental method for probing ultrafast dynamics is X-ray transient absorption spectroscopy, where the X-ray absorption spectrum is measured by scanning the central photon energy and recording the resultant photoproducts. The spectral bandwidth inherent to attosecond pulses is wide compared to the resonant features typically probed, which generally precludes the application of this technique in the attosecond regime. In this paper we propose and demonstrate a new technique to conduct transient absorption spectroscopy with broad bandwidth attosecond pulses with the aid of ghost imaging, recovering sub-bandwidth resolution in photoproduct-based absorption measurements. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1909.07441v1-abstract-full').style.display = 'none'; document.getElementById('1909.07441v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 16 September, 2019; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> September 2019. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">13 pages, 3 figures</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1906.10728">arXiv:1906.10728</a> <span> [<a href="https://arxiv.org/pdf/1906.10728">pdf</a>, <a href="https://arxiv.org/format/1906.10728">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Optics">physics.optics</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Quantum Physics">quant-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevA.102.023118">10.1103/PhysRevA.102.023118 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Electron Correlation Effects in Attosecond Photoionization of CO$_{2}$ </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Wang%2C+A+L">Anna L. Wang</a>, <a href="/search/physics?searchtype=author&query=Bucksbaum%2C+P+H">Philip H. Bucksbaum</a>, <a href="/search/physics?searchtype=author&query=Haxton%2C+D+J">Daniel J. Haxton</a>, <a href="/search/physics?searchtype=author&query=Cryan%2C+J+P">James P. Cryan</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1906.10728v1-abstract-short" style="display: inline;"> A technique for measuring photoionization time delays with attosecond precision is combined with calculations of photoionization matrix elements to demonstrate how multi-electron dynamics affect photoionization time delays in carbon dioxide. Electron correlation is observed to affect the time delays through two mechanisms: autoionization of molecular Rydberg states and accelerated escape from a co… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1906.10728v1-abstract-full').style.display = 'inline'; document.getElementById('1906.10728v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1906.10728v1-abstract-full" style="display: none;"> A technique for measuring photoionization time delays with attosecond precision is combined with calculations of photoionization matrix elements to demonstrate how multi-electron dynamics affect photoionization time delays in carbon dioxide. Electron correlation is observed to affect the time delays through two mechanisms: autoionization of molecular Rydberg states and accelerated escape from a continuum shape resonance. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1906.10728v1-abstract-full').style.display = 'none'; document.getElementById('1906.10728v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 25 June, 2019; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> June 2019. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. A 102, 023118 (2020) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1906.10649">arXiv:1906.10649</a> <span> [<a href="https://arxiv.org/pdf/1906.10649">pdf</a>, <a href="https://arxiv.org/format/1906.10649">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Optics">physics.optics</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Accelerator Physics">physics.acc-ph</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1038/s41566-019-0549-5">10.1038/s41566-019-0549-5 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Tunable Isolated Attosecond X-ray Pulses with Gigawatt Peak Power from a Free-Electron Laser </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Duris%2C+J">Joseph Duris</a>, <a href="/search/physics?searchtype=author&query=Li%2C+S">Siqi Li</a>, <a href="/search/physics?searchtype=author&query=Driver%2C+T">Taran Driver</a>, <a href="/search/physics?searchtype=author&query=Champenois%2C+E+G">Elio G. Champenois</a>, <a href="/search/physics?searchtype=author&query=MacArthur%2C+J+P">James P. MacArthur</a>, <a href="/search/physics?searchtype=author&query=Lutman%2C+A+A">Alberto A. Lutman</a>, <a href="/search/physics?searchtype=author&query=Zhang%2C+Z">Zhen Zhang</a>, <a href="/search/physics?searchtype=author&query=Rosenberger%2C+P">Philipp Rosenberger</a>, <a href="/search/physics?searchtype=author&query=Aldrich%2C+J+W">Jeff W. Aldrich</a>, <a href="/search/physics?searchtype=author&query=Coffee%2C+R">Ryan Coffee</a>, <a href="/search/physics?searchtype=author&query=Coslovich%2C+G">Giacomo Coslovich</a>, <a href="/search/physics?searchtype=author&query=Decker%2C+F">Franz-Josef Decker</a>, <a href="/search/physics?searchtype=author&query=Glownia%2C+J+M">James M. Glownia</a>, <a href="/search/physics?searchtype=author&query=Hartmann%2C+G">Gregor Hartmann</a>, <a href="/search/physics?searchtype=author&query=Helml%2C+W">Wolfram Helml</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Knurr%2C+J">Jonas Knurr</a>, <a href="/search/physics?searchtype=author&query=Krzywinski%2C+J">Jacek Krzywinski</a>, <a href="/search/physics?searchtype=author&query=Lin%2C+M">Ming-Fu Lin</a>, <a href="/search/physics?searchtype=author&query=Nantel%2C+M">Megan Nantel</a>, <a href="/search/physics?searchtype=author&query=Natan%2C+A">Adi Natan</a>, <a href="/search/physics?searchtype=author&query=O%27Neal%2C+J">Jordan O'Neal</a>, <a href="/search/physics?searchtype=author&query=Shivaram%2C+N">Niranjan Shivaram</a>, <a href="/search/physics?searchtype=author&query=Walter%2C+P">Peter Walter</a>, <a href="/search/physics?searchtype=author&query=Wang%2C+A">Anna Wang</a> , et al. (9 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1906.10649v1-abstract-short" style="display: inline;"> The quantum mechanical motion of electrons in molecules and solids occurs on the sub-femtosecond timescale. Consequently, the study of ultrafast electronic phenomena requires the generation of laser pulses shorter than 1 fs and of sufficient intensity to interact with their target with high probability. Probing these dynamics with atomic-site specificity requires the extension of sub-femtosecond p… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1906.10649v1-abstract-full').style.display = 'inline'; document.getElementById('1906.10649v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1906.10649v1-abstract-full" style="display: none;"> The quantum mechanical motion of electrons in molecules and solids occurs on the sub-femtosecond timescale. Consequently, the study of ultrafast electronic phenomena requires the generation of laser pulses shorter than 1 fs and of sufficient intensity to interact with their target with high probability. Probing these dynamics with atomic-site specificity requires the extension of sub-femtosecond pulses to the soft X-ray spectral region. Here we report the generation of isolated GW-scale soft X-ray attosecond pulses with an X-ray free-electron laser. Our source has a pulse energy that is six orders of magnitude larger than any other source of isolated attosecond pulses in the soft X-ray spectral region, with a peak power in the tens of gigawatts. This unique combination of high intensity, high photon energy and short pulse duration enables the investigation of electron dynamics with X-ray non-linear spectroscopy and single-particle imaging. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1906.10649v1-abstract-full').style.display = 'none'; document.getElementById('1906.10649v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 25 June, 2019; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> June 2019. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Duris, J., Li, S., Driver, T. et al. Nat. Photonics 14, 30-36 (2020) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1504.06811">arXiv:1504.06811</a> <span> [<a href="https://arxiv.org/pdf/1504.06811">pdf</a>, <a href="https://arxiv.org/ps/1504.06811">ps</a>, <a href="https://arxiv.org/format/1504.06811">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Quantum Physics">quant-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Atomic Physics">physics.atom-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Chemical Physics">physics.chem-ph</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Optics">physics.optics</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevLett.115.203002">10.1103/PhysRevLett.115.203002 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Observation of Bloch oscillations in molecular rotation </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Flo%C3%9F%2C+J">Johannes Flo脽</a>, <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Averbukh%2C+I+S">Ilya Sh. Averbukh</a>, <a href="/search/physics?searchtype=author&query=Bucksbaum%2C+P+H">Philip H. Bucksbaum</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1504.06811v1-abstract-short" style="display: inline;"> The periodically kicked quantum rotor is known for non-classical effects such as quantum localisation in angular momentum space or quantum resonances in rotational excitation. These phenomena have been studied in diverse systems mimicking the kicked rotor, such as cold atoms in optical lattices, or coupled photonic structures. Recently, it was predicted that several solid state quantum localisatio… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1504.06811v1-abstract-full').style.display = 'inline'; document.getElementById('1504.06811v1-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1504.06811v1-abstract-full" style="display: none;"> The periodically kicked quantum rotor is known for non-classical effects such as quantum localisation in angular momentum space or quantum resonances in rotational excitation. These phenomena have been studied in diverse systems mimicking the kicked rotor, such as cold atoms in optical lattices, or coupled photonic structures. Recently, it was predicted that several solid state quantum localisation phenomena - Anderson localisation, Bloch oscillations, and Tamm-Shockley surface states - may manifest themselves in the rotational dynamics of laser-kicked molecules. Here, we report the first observation of rotational Bloch oscillations in a gas of nitrogen molecules kicked by a periodic train of femtosecond laser pulses. A controllable detuning from the quantum resonance creates an effective accelerating potential in angular momentum space, inducing Bloch-like oscillations of the rotational excitation. These oscillations are measured via the temporal modulation of the refractive index of the gas. Our results introduce room-temperature laser-kicked molecules as a new laboratory for studies of localisation phenomena in quantum transport. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1504.06811v1-abstract-full').style.display = 'none'; document.getElementById('1504.06811v1-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 26 April, 2015; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> April 2015. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">5 pages, 5 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Lett. 115, 203002 (2015) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1501.04136">arXiv:1501.04136</a> <span> [<a href="https://arxiv.org/pdf/1501.04136">pdf</a>, <a href="https://arxiv.org/ps/1501.04136">ps</a>, <a href="https://arxiv.org/format/1501.04136">other</a>] </span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Optics">physics.optics</span> </div> </div> <p class="title is-5 mathjax"> Dynamical Localization in Molecular Alignment of Kicked Quantum Rotors </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/physics?searchtype=author&query=Kamalov%2C+A">Andrei Kamalov</a>, <a href="/search/physics?searchtype=author&query=Broege%2C+D+W">Douglas W. Broege</a>, <a href="/search/physics?searchtype=author&query=Bucksbaum%2C+P+H">Philip H. Bucksbaum</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1501.04136v2-abstract-short" style="display: inline;"> The periodically $未$-kicked quantum linear rotor is known to experience non-classical bounded energy growth due to quantum dynamical localization in angular momentum space. We study the effect of random deviations of the kick period in simulations and experiments. This breaks the energy and angular momentum localization and increases the rotational alignment, which is the analog of the onset of An… <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1501.04136v2-abstract-full').style.display = 'inline'; document.getElementById('1501.04136v2-abstract-short').style.display = 'none';">▽ More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1501.04136v2-abstract-full" style="display: none;"> The periodically $未$-kicked quantum linear rotor is known to experience non-classical bounded energy growth due to quantum dynamical localization in angular momentum space. We study the effect of random deviations of the kick period in simulations and experiments. This breaks the energy and angular momentum localization and increases the rotational alignment, which is the analog of the onset of Anderson localization in 1-D chains. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1501.04136v2-abstract-full').style.display = 'none'; document.getElementById('1501.04136v2-abstract-short').style.display = 'inline';">△ Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 31 March, 2015; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 16 January, 2015; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> January 2015. </p> </li> </ol> <div class="is-hidden-tablet">  <span class="help" style="display: inline-block;"><a href="https://github.com/arXiv/arxiv-search/releases">Search v0.5.6 released 2020-02-24</a>  </span> </div> </div> </main> <footer> <div class="columns is-desktop" 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