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贾建华/童明良Angew. Chem. Int. Ed.：阴离子客体调控光致变色Ag(I)-MOFs的拓扑结构、动态发光以及光热转换性能 | 中山大学化学学院
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Chem. Int. Ed.：阴离子客体调控光致变色Ag(I)-MOFs的拓扑结构、动态发光以及光热转换性能 </li> </ul> </nav> </div> </div> </div> <div class="row"> <div class="col-sm-12 col-md-3 hidden-xs region-left"> <div class="block-region-left"> <div data-block-plugin-id="block_content:e18c4d49-b07a-417a-ae63-950c210a1a8c" class="block"> </div> <div data-block-plugin-id="page_qr_code" class="block"> <div class="page-url-qr-code t-c"> <img src="https://ce.sysu.edu.cn/sites/default/files/qrcode/B4MKd9rPD6qo8V1-LzrknqWUiVQ91J8MbJcmHrxMY5g.png"> <div class="qr-title t-c outside-min-tb">扫描此二维码分享</div> </div> </div> </div> </div> <div class="col-sm-12 col-md-9 region-right"> <div class="block-region-right"> <div data-block-plugin-id="article_tilte_block" class="block"> <div class="article-header outside-min-tb"> <div class="article-title"> <h1 class="inside-min-tb">贾建华/童明良Angew. Chem. Int. Ed.：阴离子客体调控光致变色Ag(I)-MOFs的拓扑结构、动态发光以及光热转换性能</h1> </div> <div class="article-submit inside-min-tb"> <span class="article-owner">发布人：陈昱昀</span> <span class="article-approver">责任审核人：冯双</span> <span class="article-date">发布日期：2024-10-24</span> </div> </div> </div> <div data-block-plugin-id="entity_field:node:body" class="block"> <div class="field field-body field-type-text-with-summary field-label-hidden field-item"><p style="line-height:150%;"><span style="font-family:"Times New Roman",serif;font-size:14.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p style="line-height:150%;text-indent:24.0pt;"><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">随着人工智能的快速崛起，智能分子材料迎来广阔的应用场景。光致变色分子是一类光敏智能材料，具有两种可切换的稳定或亚稳定状态以及对比鲜明的颜色和物理化学性质变化，在智能窗户、变色装饰、光存储器和防伪器件等领域具有重要的商业价值。定量调节和快速响应对于光敏智能材料至关重要，自由基诱导光致变色分子能提供有效方案。通过监测光致变色金属</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">-</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">有机框架材料</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> (MOFs) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">中光生自由基的浓度可探究光致发光的动态过程。但是，在自由基富集过程中</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOFs</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">大多表现出单调的发光猝灭行为，只有少数能够激发荧光，而与发光猝灭紧密相关的非辐射跃迁过程又能诱发光热转换行为。因此，如何在晶态</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOFs</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">中实现荧光发射和光热转换的协同调控极具挑战性。</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p style="line-height:150%;text-indent:24.0pt;"><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">近期，贾建华副教授和童明良教授团队基于前期光致变色配合物的工作，通过引入自由基介导光致变色基团构建多功能光致变色</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Ag(I)-MOFs</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">，采用静电补偿策略实现阴离子客体对框架拓扑结构、动态发光以及光热转换性能的调控。选用光活性配体</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">TEPE (1,1,2,2-</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">四</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">(</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">吡啶</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">-4-</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">基</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">乙烯</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">作为连接子与</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Ag(I)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">以及稠环羧基</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">AC<sup>─</sup> (9-</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">蒽甲酸</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">或</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">NC<sup>─</sup> (1-</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">萘甲酸</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">作为阴离子客体构筑两例框架材料，</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>1</strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">和</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2</strong> (</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">图</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">1) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">。由于阳离子主体与阴离子客体之间丰富的静电相互作用，不同尺寸的稠环羧基客体诱导形成两种截然不同的拓扑结构。值得一提的是，本工作首次报道的</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>1</strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">是一种全新的拓扑网络</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;"> </span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">(4,4,4,4-c net)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">，并被命名为</span><em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">sfm</span></em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> (</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">即</span><em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">silver framework material</span></em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">。</span></p><p style="line-height:150%;text-indent:24.0pt;"><span style="font-family:宋体;font-size:12.0pt;line-height:150%;"><img src="/sites/default/files/inline-images/image_125.png" data-entity-uuid="39cd0196-e83b-4ae0-9fda-486d35b25375" data-entity-type="file" width="839" height="444" loading="lazy"></span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p class="text-align-center" style="line-height:150%;"><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p style="line-height:150%;"><span style="font-family:宋体;font-size:12.0pt;line-height:150%;"><strong>图</strong></span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><strong>1.</strong> MOF-<strong>1</strong> (a) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">和</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2</strong> (b) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">中</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Ag(I)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">的配位结构示意图；</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>1</strong> (c) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">和</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2</strong> (d) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">沿</span><em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">c</span></em><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">轴方向三维堆积结构示意图；</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>1</strong> (e) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">和</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2</strong> (f) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">中阳离子主体框架与阴离子客体之间的相互作用示意图。</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p> </p><p style="line-height:150%;text-indent:24.0pt;"><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">时间依赖荧光发射光谱证实了光生自由基调控</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Ag-MOFs</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">发光行为的可行性。在</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">CIE</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">色坐标中，</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>1</strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">显示为从黄色到红色的线性变化轨迹，</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2</strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">则表现出由蓝色到橙色的曲线变化轨迹。可视化的色坐标位移表明</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Ag-MOFs</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">具有灵活的光致发光性质可调性，其原因来自于光照产生的自由基</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> (</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">图</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">2)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">。此外，经过远程紫外光的照射，辐照产物</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>1<sup>*</sup></strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">和</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2<sup>*</sup></strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">表现出良好的光热转换效果，在功率为</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">1 W cm<sup>-2</sup></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">的</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">808 nm</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">激光照射下，</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Ag-MOFs</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">产物表面温度分别达</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">~160°C (MOF-<strong>1<sup>*</sup></strong>) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">和</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">~120°C (MOF-<strong>2<sup>*</sup></strong>)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">。而且，</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Ag-MOFs</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">光照后不仅展现出高效的近红外光热转换效率</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> (MOF-<strong>1<sup>*</sup></strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">，</span><em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">η </span></em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">= 51.8%</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">；</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2<sup>*</sup></strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">，</span><em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">η</span></em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> = 36.2%)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">，还具有良好的可循环性</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> (</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">图</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">3)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">。以上结果表明，在</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Ag-MOFs</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">中引入</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">π</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">共轭客体阴离子有利于增强自由基的稳定性，从而实现优异的光热转换性能。</span></p><p style="line-height:150%;text-indent:24.0pt;"><img src="/sites/default/files/inline-images/image_126.png" data-entity-uuid="43e54770-20bc-4c04-8e31-b7d3189c72f4" data-entity-type="file" width="839" height="430" loading="lazy"></p><p style="line-height:150%;text-indent:24.0pt;"><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p class="text-align-center" style="line-height:150%;"><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p style="line-height:150%;"><span style="font-family:宋体;font-size:12.0pt;line-height:150%;"><strong>图</strong></span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><strong>2</strong>. (a) MOF-<strong>1</strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">和</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2</strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">以及自由</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">TEPE</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">配体的固态</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">EPR</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">谱图；</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF<strong>-1</strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">的时间依赖荧光发射光谱</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;"> </span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">(b) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">及其</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">CIE</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">坐标变化轨迹示意图</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> (c)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">；</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2</strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">的时间依赖荧光发射光谱</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;"> </span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">(d) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">及其</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">CIE</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">坐标变化轨迹示意图</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> (e)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">。</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p class="text-align-center" style="line-height:150%;"><span lang="EN-US"><img src="/sites/default/files/inline-images/image_124.png" data-entity-uuid="a7187146-41ce-48b8-b89d-ee5cec3eec3e" data-entity-type="file" width="1285" height="832" uploadprocessed="true" loading="lazy"></span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p style="line-height:150%;"><span style="font-family:宋体;font-size:12.0pt;line-height:150%;"><strong>图</strong></span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><strong>3</strong>. </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">辐照产物</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>1<sup>*</sup></strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">和</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2<sup>*</sup></strong></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">的光热转换曲线</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;"> </span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">(a) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">以及五次加热</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">-</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">冷却循环测试曲线</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> (b)</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">；</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>1<sup>*</sup></strong> (c) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">和</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">MOF-<strong>2<sup>*</sup></strong> (d) </span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">在功率为</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">1 W cm<sup>-2</sup></span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">的</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">808 nm</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">激光辐照下的红外热成像图。</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p style="line-height:150%;"> </p><p style="line-height:150%;text-indent:24.0pt;"><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">本工作利用静电补偿策略将π共轭阴离子客体引入到阳离子主体框架中，克服了在中性框架内难以精确引入定量客体的挑战，并实现辐照产物高效的近红外光热转换性能。本研究以</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">“Radical-Induced Photochromic Silver(I) Metal-Organic Frameworks: Alternative Topology, Dynamic Photoluminescence and Efficient Photothermal Conversion Modulated by Anionic Guests”</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">为题，发表于综合性学术期刊</span><em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Angew. Chem. Int. Ed.</span></em><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">，并被选为</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Very Important Paper</span><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">。中山大学化学学院、绿色化学与分子工程研究院为该成果的第一完成单位，论文通讯作者为中山大学化学学院贾建华副教授和童明良教授。该研究得到国家重点研发计划、国家自然科学基金和广东省珠江人才计划项目的资助。</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p style="line-height:150%;text-indent:24.0pt;"> </p><p style="line-height:150%;"><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">论文信息：</span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p style="line-height:150%;"><span style="color:black;"><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Pei-Yu Liao, Jia-Xin Li, Jia-Chuan Liu, Qi Xiong, Ze-Yu Ruan, Tao Li, Wei Deng, Shang-Da Jiang, Jian-Hua Jia</span></span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><strong><sup>*</sup></strong></span><span style="color:black;"><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> and Ming-Liang Tong</span></span><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><strong><sup>*</sup></strong></span><span style="color:black;"><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">. Radical-Induced Photochromic Silver(I) Metal-Organic Frameworks: Alternative Topology, Dynamic Photoluminescence and Efficient Photothermal Conversion Modulated by Anionic Guests, </span><em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">Angew. Chem. Int. Ed. </span></em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><strong>2024</strong>,</span><em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"> 63, </span></em><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">e202401448.<o:p></o:p></span></span></p><p style="line-height:150%;"><span style="font-family:宋体;font-size:12.0pt;line-height:150%;">全文链接：</span><a href="https://onlinelibrary.wiley.com/doi/epdf/10.1002/anie.202401448"><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US">https://onlinelibrary.wiley.com/doi/epdf/10.1002/anie.202401448</span></a><span style="font-family:"Times New Roman",serif;font-size:12.0pt;line-height:150%;" lang="EN-US"><o:p></o:p></span></p><p style="line-height:150%;"> </p></div> </div> </div> </div> </div> </div> </div> </article> </div> </div> <div id="footer"> 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