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</div> <p class="title is-5 mathjax"> Anharmonic quantum muon effects in the kagome antiferromagnet Zn-Barlowite </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&amp;query=Hotz%2C+F">Fabian Hotz</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Gomil%C5%A1ek%2C+M">Matja啪 Gomil拧ek</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Arh%2C+T">Tina Arh</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Zorko%2C+A">Andrej Zorko</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Luetkens%2C+H">Hubertus Luetkens</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2408.00185v1-abstract-short" style="display: inline;"> Muon spin spectroscopy ($渭$SR) is a powerful local probe technique e.g. used for the investigation of exotic frustrated magnetism. Ab initio simulations using Density Functional Theory with the muon treated as a point-like defect (DFT+$渭$) are commonly employed to determine the interstitial lattice positions where the muon comes to rest after implantation. These muon stopping sites are critical fo&hellip; <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2408.00185v1-abstract-full').style.display = 'inline'; document.getElementById('2408.00185v1-abstract-short').style.display = 'none';">&#9661; More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2408.00185v1-abstract-full" style="display: none;"> Muon spin spectroscopy ($渭$SR) is a powerful local probe technique e.g. used for the investigation of exotic frustrated magnetism. Ab initio simulations using Density Functional Theory with the muon treated as a point-like defect (DFT+$渭$) are commonly employed to determine the interstitial lattice positions where the muon comes to rest after implantation. These muon stopping sites are critical for accurately interpreting $渭$SR data. For example, for the quantum spin liquid candidate Zn-Barlowite, DFT+$渭$ simulations identify two types of muon stopping sites: a higher-energy site where the muon is located between a fluorine and a bromine atom and three similar sites near an OH group. However, our study shows that the $渭$SR spectra of Zn-Barlowite cannot be adequately described using muon sites determined by the conventional DFT+$渭$ approach. Instead, accurate reproduction of the $渭$SR data requires treating the muon as a spatially extended quantum particle with a skewed wavefunction due to the anharmonicity of the surrounding electrostatic potential. The quantum nature of the muon significantly affects its lattice position and, consequently, the observed $渭$SR spectra. Our findings highlight the potential of $渭$SR to study the localization of quantum particles, using the muon as the probe and particle under investigation. The light mass of the muon amplifies quantum effects, enhancing the sensitivity of our measurements and enabling a detailed comparison between experimental data and theoretical calculations. These results can be directly applied to the theoretical calculations of hydrogen localization, where quantum effects, though smaller, may still be relevant in real materials. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2408.00185v1-abstract-full').style.display = 'none'; document.getElementById('2408.00185v1-abstract-short').style.display = 'inline';">&#9651; Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 31 July, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> August 2024. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2407.09179">arXiv:2407.09179</a> <span>&nbsp;[<a href="https://arxiv.org/pdf/2407.09179">pdf</a>]&nbsp;</span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> </div> <p class="title is-5 mathjax"> Magnetic properties and field-induced phenomena in the Jeff = 1/2 distorted kagome antiferromagnet </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&amp;query=Yadav%2C+A">A. Yadav</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Elghandour%2C+A">A. Elghandour</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Arh%2C+T">T. Arh</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Adroja%2C+D+T">D. T. Adroja</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Le%2C+M+D">M. D. Le</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Stenning%2C+G+B+G">G. B. G. Stenning</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Aouane%2C+M">M. Aouane</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Luther%2C+S">S. Luther</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Hotz%2C+F">F. Hotz</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Hicken%2C+T+J">T. J. Hicken</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Luetkens%2C+H">H. Luetkens</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Zorko%2C+A">A. Zorko</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Klingeler%2C+R">R. Klingeler</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Khuntia%2C+P">P. Khuntia</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2407.09179v2-abstract-short" style="display: inline;"> The intertwining between competing degrees of freedom, anisotropy, and frustration-induced quantum fluctuations offers an ideal ground to realize exotic quantum phenomena in the rare-earth-based kagome lattice. The magnetic susceptibility reveals the presence of two energy scales in agreement with the INS results. The higher energy state is dominated by CEF excitations, where the lowest Kramers gr&hellip; <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2407.09179v2-abstract-full').style.display = 'inline'; document.getElementById('2407.09179v2-abstract-short').style.display = 'none';">&#9661; More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2407.09179v2-abstract-full" style="display: none;"> The intertwining between competing degrees of freedom, anisotropy, and frustration-induced quantum fluctuations offers an ideal ground to realize exotic quantum phenomena in the rare-earth-based kagome lattice. The magnetic susceptibility reveals the presence of two energy scales in agreement with the INS results. The higher energy state is dominated by CEF excitations, where the lowest Kramers ground-state doublet is well separated from the excited state suggesting that the compound realizes a low-energy state at low temperatures. The second energy scale is witnessed via thermodynamic results that reveal an anomaly at 0.3 K typical of a phase transition, which is attributed to the presence of complex magnetic ordering phenomena. The broad maximum in the specific heat well above 0.3 K indicates the presence of short-range spin correlations that is corroborated by muon spin relaxation rate results. The isothermal magnetization reveals a field-induced 1/3 magnetization plateau at low temperatures. muSR relaxation rate experiments, on the other hand, neither show the signature of a phase transition nor spin-freezing down to 34 mK. The ZF muSR relaxation is governed by the Orbach process and reveals the presence of a fluctuating state owing to the depopulation of crystal field levels reflected as a constant value of relaxation rate in the temperature range 0.4-10 K. NMR results indicate the presence of fluctuating Nd3+ moments down to 1.8 K consistent with muSR experiments. Our comprehensive results reveal that a field-induced quantum critical phenomenon is at play in this frustrated kagome magnet and enable us to construct a phase diagram exemplifying the proximity effect of competing magnetic states. This sets the stage to investigate the broad RE3BWO9 family of rare-earth kagome magnets promising to host exotic quantum states driven by spin-orbit coupling and geometrical frustration. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2407.09179v2-abstract-full').style.display = 'none'; document.getElementById('2407.09179v2-abstract-short').style.display = 'inline';">&#9651; Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 18 December, 2024; <span class="has-text-black-bis has-text-weight-semibold">v1</span> submitted 12 July, 2024; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> July 2024. </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2302.07015">arXiv:2302.07015</a> <span>&nbsp;[<a href="https://arxiv.org/pdf/2302.07015">pdf</a>, <a href="https://arxiv.org/format/2302.07015">other</a>]&nbsp;</span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Superconductivity">cond-mat.supr-con</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1073/pnas.2303423120">10.1073/pnas.2303423120 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Designing the stripe-ordered cuprate phase diagram through uniaxial-stress </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&amp;query=Guguchia%2C+Z">Z. Guguchia</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Das%2C+D">D. Das</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Simutis%2C+G">G. Simutis</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Adachi%2C+T">T. Adachi</a>, <a href="/search/cond-mat?searchtype=author&amp;query=K%C3%BCspert%2C+J">J. K眉spert</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Kitajima%2C+N">N. Kitajima</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Elender%2C+M">M. Elender</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Grinenko%2C+V">V. Grinenko</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Ivashko%2C+O">O. Ivashko</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Zimmermann%2C+M+v">M. v. Zimmermann</a>, <a href="/search/cond-mat?searchtype=author&amp;query=M%C3%BCller%2C+M">M. M眉ller</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Mielke%2C+C">C. Mielke III</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Hotz%2C+F">F. Hotz</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Mudry%2C+C">C. Mudry</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Baines%2C+C">C. Baines</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Bartkowiak%2C+M">M. Bartkowiak</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Shiroka%2C+T">T. Shiroka</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Koike%2C+Y">Y. Koike</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Amato%2C+A">A. Amato</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Hicks%2C+C+W">C. W. Hicks</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Gu%2C+G+D">G. D. Gu</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Tranquada%2C+J+M">J. M. Tranquada</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Klauss%2C+H+-">H. -H. Klauss</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Chang%2C+J+J">J. J. Chang</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Janoschek%2C+M">M. Janoschek</a> , et al. (1 additional authors not shown) </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2302.07015v1-abstract-short" style="display: inline;"> The ability to efficiently control charge and spin in the cuprate high-temperature superconductors is crucial for fundamental research and underpins technological development. Here, we explore the tunability of magnetism, superconductivity and crystal structure in the stripe phase of the cuprate La_2-xBa_xCuO_4, with x = 0.115 and 0.135, by employing temperature-dependent (down to 400 mK) muon-spi&hellip; <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2302.07015v1-abstract-full').style.display = 'inline'; document.getElementById('2302.07015v1-abstract-short').style.display = 'none';">&#9661; More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2302.07015v1-abstract-full" style="display: none;"> The ability to efficiently control charge and spin in the cuprate high-temperature superconductors is crucial for fundamental research and underpins technological development. Here, we explore the tunability of magnetism, superconductivity and crystal structure in the stripe phase of the cuprate La_2-xBa_xCuO_4, with x = 0.115 and 0.135, by employing temperature-dependent (down to 400 mK) muon-spin rotation and AC susceptibility, as well as X-ray scattering experiments under compressive uniaxial stress in the CuO_2 plane. A sixfold increase of the 3-dimensional (3D) superconducting critical temperature T_c and a full recovery of the 3D phase coherence is observed in both samples with the application of extremely low uniaxial stress of 0.1 GPa. This finding demonstrates the removal of the well-known 1/8-anomaly of cuprates by uniaxial stress. On the other hand, the spin-stripe order temperature as well as the magnetic fraction at 400 mK show only a modest decrease under stress. Moreover, the onset temperatures of 3D superconductivity and spin-stripe order are very similar in the large stress regime. However, a substantial decrease of the magnetic volume fraction and a full suppression of the low-temperature tetragonal structure is found at elevated temperatures, which is a necessary condition for the development of the 3D superconducting phase with optimal T_c. Our results evidence a remarkable cooperation between the long-range static spin-stripe order and the underlying crystalline order with the three-dimensional fully coherent superconductivity. Overall, these results suggest that the stripe- and the SC order may have a common physical mechanism. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2302.07015v1-abstract-full').style.display = 'none'; document.getElementById('2302.07015v1-abstract-short').style.display = 'inline';">&#9651; Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 14 February, 2023; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> February 2023. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">11 pages, 5 figures. This work builds on our earlier findings on LBCO, arXiv:2008.01159, and substantially expands it</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Proc. Natl. Acd. Sci. U.S.A 121(1), e2303423120 (2024) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2203.05055">arXiv:2203.05055</a> <span>&nbsp;[<a href="https://arxiv.org/pdf/2203.05055">pdf</a>, <a href="https://arxiv.org/format/2203.05055">other</a>]&nbsp;</span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Superconductivity">cond-mat.supr-con</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Materials Science">cond-mat.mtrl-sci</span> </div> </div> <p class="title is-5 mathjax"> Two types of charge order in the superconducting kagome material CsV$_3$Sb$_5$ </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&amp;query=Gupta%2C+R">Ritu Gupta</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Das%2C+D">Debarchan Das</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Mielke%2C+C">Charles Mielke III</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Ritz%2C+E">Ethan Ritz</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Hotz%2C+F">Fabian Hotz</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Yin%2C+Q">Qiangwei Yin</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Tu%2C+Z">Zhijun Tu</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Gong%2C+C">Chunsheng Gong</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Lei%2C+H">Hechang Lei</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Birol%2C+T">Turan Birol</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Fernandes%2C+R+M">Rafael M. Fernandes</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Guguchia%2C+Z">Zurab Guguchia</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Luetkens%2C+H">Hubertus Luetkens</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Khasanov%2C+R">Rustem Khasanov</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2203.05055v1-abstract-short" style="display: inline;"> The kagome metals of the family $A$V$_3$Sb$_5$, featuring a unique structural motif, harbor an array of intriguing phenomena such as chiral charge order and superconductivity. CsV$_3$Sb$_5$ is of particular interest because it displays a double superconducting dome in the region of the temperature-pressure phase diagram where charge order is still present. However, the microscopic origin of such a&hellip; <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2203.05055v1-abstract-full').style.display = 'inline'; document.getElementById('2203.05055v1-abstract-short').style.display = 'none';">&#9661; More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2203.05055v1-abstract-full" style="display: none;"> The kagome metals of the family $A$V$_3$Sb$_5$, featuring a unique structural motif, harbor an array of intriguing phenomena such as chiral charge order and superconductivity. CsV$_3$Sb$_5$ is of particular interest because it displays a double superconducting dome in the region of the temperature-pressure phase diagram where charge order is still present. However, the microscopic origin of such an unusual behavior remains an unsolved issue. Here, to address it, we combine high-pressure, low-temperature muon spin relaxation with first-principles calculations. We observe a pressure-induced threefold enhancement of the superfluid density, which also displays a double peak feature, similar to the superconducting critical temperature. This leads to three distinct regions in the phase diagram, each of which features distinct slopes of the linear relation between superfluid density and the critical temperature. These results are attributed to a possible evolution of the charge order pattern from the superimposed tri-hexagonal Star-of-David phase at low pressures (within the first dome) to the staggered tri-hexagonal phase at intermediate pressures (between the first and second domes). Our findings suggest a change in the nature of the charge ordered state across the phase diagram of CsV$_3$Sb$_5$, with varying degrees of competition with superconductivity. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2203.05055v1-abstract-full').style.display = 'none'; document.getElementById('2203.05055v1-abstract-short').style.display = 'inline';">&#9651; Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 9 March, 2022; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> March 2022. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">9 pages, 4 figures</span> </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/2111.13668">arXiv:2111.13668</a> <span>&nbsp;[<a href="https://arxiv.org/pdf/2111.13668">pdf</a>, <a href="https://arxiv.org/format/2111.13668">other</a>]&nbsp;</span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Superconductivity">cond-mat.supr-con</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevResearch.4.023093">10.1103/PhysRevResearch.4.023093 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> Magnetic correlations in infinite-layer nickelates: an experimental and theoretical multi-method study </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&amp;query=Ortiz%2C+R+A">R. A. Ortiz</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Puphal%2C+P">P. Puphal</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Klett%2C+M">M. Klett</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Hotz%2C+F">F. Hotz</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Kremer%2C+R+K">R. K. Kremer</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Trepka%2C+H">H. Trepka</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Hemmida%2C+M">M. Hemmida</a>, <a href="/search/cond-mat?searchtype=author&amp;query=von+Nidda%2C+H+-+K">H. -A. Krug von Nidda</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Isobe%2C+M">M. Isobe</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Khasanov%2C+R">R. Khasanov</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Luetkens%2C+H">H. Luetkens</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Hansmann%2C+P">P. Hansmann</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Keimer%2C+B">B. Keimer</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Sch%C3%A4fer%2C+T">T. Sch盲fer</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Hepting%2C+M">M. Hepting</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="2111.13668v1-abstract-short" style="display: inline;"> We report a comprehensive study of magnetic correlations in LaNiO$_{2}$, a parent compound of the recently discovered family of infinite-layer (IL) nickelate superconductors, using multiple experimental and theoretical methods. Our specific heat, muon-spin rotation ($渭$SR), and magnetic susceptibility measurements on polycrystalline LaNiO$_{2}$ show that long-range magnetic order remains absent do&hellip; <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2111.13668v1-abstract-full').style.display = 'inline'; document.getElementById('2111.13668v1-abstract-short').style.display = 'none';">&#9661; More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="2111.13668v1-abstract-full" style="display: none;"> We report a comprehensive study of magnetic correlations in LaNiO$_{2}$, a parent compound of the recently discovered family of infinite-layer (IL) nickelate superconductors, using multiple experimental and theoretical methods. Our specific heat, muon-spin rotation ($渭$SR), and magnetic susceptibility measurements on polycrystalline LaNiO$_{2}$ show that long-range magnetic order remains absent down to 2 K. Nevertheless, we detect residual entropy in the low-temperature specific heat, which is compatible with a model fit that includes paramagnon excitations. The $渭$SR and low-field static and dynamic magnetic susceptibility measurements indicate the presence of short-range magnetic correlations and glassy spin dynamics, which we attribute to local oxygen non-stoichiometry in the average infinite-layer crystal structure. This glassy behavior can be suppressed in strong external fields, allowing us to extract the intrinsic paramagnetic susceptibility. Remarkably, we find that the intrinsic susceptibility shows non-Curie-Weiss behavior at high temperatures, in analogy to doped cuprates that possess robust non-local spin fluctuations. The distinct temperature dependence of the intrinsic susceptibility of LaNiO$_{2}$ can be theoretically understood by a multi-method study of the single-band Hubbard model in which we apply complementary cutting-edge quantum many-body techniques (dynamical mean-field theory, cellular dynamical mean-field theory and the dynamical vertex approximation) to investigate the influence of both short- and long-ranged correlations. Our results suggest a profound analogy between the magnetic correlations in parent (undoped) IL nickelates and doped cuprates. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('2111.13668v1-abstract-full').style.display = 'none'; document.getElementById('2111.13668v1-abstract-short').style.display = 'inline';">&#9651; Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 26 November, 2021; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> November 2021. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Comments:</span> <span class="has-text-grey-dark mathjax">18 pages, 14 figures</span> </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Research 4, 023093 (2022) </p> </li> <li class="arxiv-result"> <div class="is-marginless"> <p class="list-title is-inline-block"><a href="https://arxiv.org/abs/1907.07695">arXiv:1907.07695</a> <span>&nbsp;[<a href="https://arxiv.org/pdf/1907.07695">pdf</a>, <a href="https://arxiv.org/format/1907.07695">other</a>]&nbsp;</span> </p> <div class="tags is-inline-block"> <span class="tag is-small is-link tooltip is-tooltip-top" data-tooltip="Strongly Correlated Electrons">cond-mat.str-el</span> <span class="tag is-small is-grey tooltip is-tooltip-top" data-tooltip="Mesoscale and Nanoscale Physics">cond-mat.mes-hall</span> </div> <div class="is-inline-block" style="margin-left: 0.5rem"> <div class="tags has-addons"> <span class="tag is-dark is-size-7">doi</span> <span class="tag is-light is-size-7"><a class="" href="https://doi.org/10.1103/PhysRevResearch.1.033029">10.1103/PhysRevResearch.1.033029 <i class="fa fa-external-link" aria-hidden="true"></i></a></span> </div> </div> </div> <p class="title is-5 mathjax"> An exactly soluble model for a fractionalized Weyl semimetal </p> <p class="authors"> <span class="search-hit">Authors:</span> <a href="/search/cond-mat?searchtype=author&amp;query=Hotz%2C+F">Fabian Hotz</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Tiwari%2C+A">Apoorv Tiwari</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Turker%2C+O">Oguz Turker</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Meng%2C+T">Tobias Meng</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Stern%2C+A">Ady Stern</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Koch-Janusz%2C+M">Maciej Koch-Janusz</a>, <a href="/search/cond-mat?searchtype=author&amp;query=Neupert%2C+T">Titus Neupert</a> </p> <p class="abstract mathjax"> <span class="has-text-black-bis has-text-weight-semibold">Abstract</span>: <span class="abstract-short has-text-grey-dark mathjax" id="1907.07695v1-abstract-short" style="display: inline;"> We construct an exactly solvable lattice model of a fractional Weyl semimetal (FWS). The low energy theory of this strongly interacting state is that of a Weyl semimetal built out of fractionally charged fermions. We show the existence of a universally quantized and fractional circular photogalvanic effect (CPGE) and a violation of the Wiedemann-Franz law in the system. Together with a spectral ga&hellip; <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1907.07695v1-abstract-full').style.display = 'inline'; document.getElementById('1907.07695v1-abstract-short').style.display = 'none';">&#9661; More</a> </span> <span class="abstract-full has-text-grey-dark mathjax" id="1907.07695v1-abstract-full" style="display: none;"> We construct an exactly solvable lattice model of a fractional Weyl semimetal (FWS). The low energy theory of this strongly interacting state is that of a Weyl semimetal built out of fractionally charged fermions. We show the existence of a universally quantized and fractional circular photogalvanic effect (CPGE) and a violation of the Wiedemann-Franz law in the system. Together with a spectral gap in the single-particle electronic Green&#39;s function they provide strong experimental signatures for this exotic gapless state of matter. <a class="is-size-7" style="white-space: nowrap;" onclick="document.getElementById('1907.07695v1-abstract-full').style.display = 'none'; document.getElementById('1907.07695v1-abstract-short').style.display = 'inline';">&#9651; Less</a> </span> </p> <p class="is-size-7"><span class="has-text-black-bis has-text-weight-semibold">Submitted</span> 17 July, 2019; <span class="has-text-black-bis has-text-weight-semibold">originally announced</span> July 2019. </p> <p class="comments is-size-7"> <span class="has-text-black-bis has-text-weight-semibold">Journal ref:</span> Phys. Rev. Research 1, 033029 (2019) </p> </li> </ol> <div class="is-hidden-tablet"> <!-- feedback for mobile only --> <span class="help" style="display: inline-block;"><a href="https://github.com/arXiv/arxiv-search/releases">Search v0.5.6 released 2020-02-24</a>&nbsp;&nbsp;</span> </div> </div> </main> <footer> <div class="columns is-desktop" role="navigation" aria-label="Secondary"> <!-- MetaColumn 1 --> <div class="column"> <div class="columns"> <div class="column"> <ul class="nav-spaced"> <li><a href="https://info.arxiv.org/about">About</a></li> <li><a href="https://info.arxiv.org/help">Help</a></li> </ul> </div> <div class="column"> <ul class="nav-spaced"> <li> <svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 512 512" class="icon filter-black" role="presentation"><title>contact arXiv</title><desc>Click here to contact arXiv</desc><path d="M502.3 190.8c3.9-3.1 9.7-.2 9.7 4.7V400c0 26.5-21.5 48-48 48H48c-26.5 0-48-21.5-48-48V195.6c0-5 5.7-7.8 9.7-4.7 22.4 17.4 52.1 39.5 154.1 113.6 21.1 15.4 56.7 47.8 92.2 47.6 35.7.3 72-32.8 92.3-47.6 102-74.1 131.6-96.3 154-113.7zM256 320c23.2.4 56.6-29.2 73.4-41.4 132.7-96.3 142.8-104.7 173.4-128.7 5.8-4.5 9.2-11.5 9.2-18.9v-19c0-26.5-21.5-48-48-48H48C21.5 64 0 85.5 0 112v19c0 7.4 3.4 14.3 9.2 18.9 30.6 23.9 40.7 32.4 173.4 128.7 16.8 12.2 50.2 41.8 73.4 41.4z"/></svg> <a href="https://info.arxiv.org/help/contact.html"> Contact</a> </li> <li> <svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 512 512" class="icon filter-black" role="presentation"><title>subscribe to arXiv mailings</title><desc>Click here to subscribe</desc><path d="M476 3.2L12.5 270.6c-18.1 10.4-15.8 35.6 2.2 43.2L121 358.4l287.3-253.2c5.5-4.9 13.3 2.6 8.6 8.3L176 407v80.5c0 23.6 28.5 32.9 42.5 15.8L282 426l124.6 52.2c14.2 6 30.4-2.9 33-18.2l72-432C515 7.8 493.3-6.8 476 3.2z"/></svg> <a href="https://info.arxiv.org/help/subscribe"> Subscribe</a> </li> </ul> </div> </div> </div> <!-- end MetaColumn 1 --> <!-- MetaColumn 2 --> <div class="column"> <div class="columns"> <div class="column"> <ul class="nav-spaced"> <li><a href="https://info.arxiv.org/help/license/index.html">Copyright</a></li> <li><a href="https://info.arxiv.org/help/policies/privacy_policy.html">Privacy Policy</a></li> </ul> </div> <div class="column sorry-app-links"> <ul class="nav-spaced"> <li><a href="https://info.arxiv.org/help/web_accessibility.html">Web Accessibility Assistance</a></li> <li> <p class="help"> <a class="a11y-main-link" href="https://status.arxiv.org" target="_blank">arXiv Operational Status <svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 256 512" class="icon filter-dark_grey" role="presentation"><path d="M224.3 273l-136 136c-9.4 9.4-24.6 9.4-33.9 0l-22.6-22.6c-9.4-9.4-9.4-24.6 0-33.9l96.4-96.4-96.4-96.4c-9.4-9.4-9.4-24.6 0-33.9L54.3 103c9.4-9.4 24.6-9.4 33.9 0l136 136c9.5 9.4 9.5 24.6.1 34z"/></svg></a><br> Get status notifications via <a class="is-link" href="https://subscribe.sorryapp.com/24846f03/email/new" target="_blank"><svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 512 512" class="icon filter-black" role="presentation"><path d="M502.3 190.8c3.9-3.1 9.7-.2 9.7 4.7V400c0 26.5-21.5 48-48 48H48c-26.5 0-48-21.5-48-48V195.6c0-5 5.7-7.8 9.7-4.7 22.4 17.4 52.1 39.5 154.1 113.6 21.1 15.4 56.7 47.8 92.2 47.6 35.7.3 72-32.8 92.3-47.6 102-74.1 131.6-96.3 154-113.7zM256 320c23.2.4 56.6-29.2 73.4-41.4 132.7-96.3 142.8-104.7 173.4-128.7 5.8-4.5 9.2-11.5 9.2-18.9v-19c0-26.5-21.5-48-48-48H48C21.5 64 0 85.5 0 112v19c0 7.4 3.4 14.3 9.2 18.9 30.6 23.9 40.7 32.4 173.4 128.7 16.8 12.2 50.2 41.8 73.4 41.4z"/></svg>email</a> or <a class="is-link" href="https://subscribe.sorryapp.com/24846f03/slack/new" target="_blank"><svg xmlns="http://www.w3.org/2000/svg" viewBox="0 0 448 512" class="icon filter-black" role="presentation"><path d="M94.12 315.1c0 25.9-21.16 47.06-47.06 47.06S0 341 0 315.1c0-25.9 21.16-47.06 47.06-47.06h47.06v47.06zm23.72 0c0-25.9 21.16-47.06 47.06-47.06s47.06 21.16 47.06 47.06v117.84c0 25.9-21.16 47.06-47.06 47.06s-47.06-21.16-47.06-47.06V315.1zm47.06-188.98c-25.9 0-47.06-21.16-47.06-47.06S139 32 164.9 32s47.06 21.16 47.06 47.06v47.06H164.9zm0 23.72c25.9 0 47.06 21.16 47.06 47.06s-21.16 47.06-47.06 47.06H47.06C21.16 243.96 0 222.8 0 196.9s21.16-47.06 47.06-47.06H164.9zm188.98 47.06c0-25.9 21.16-47.06 47.06-47.06 25.9 0 47.06 21.16 47.06 47.06s-21.16 47.06-47.06 47.06h-47.06V196.9zm-23.72 0c0 25.9-21.16 47.06-47.06 47.06-25.9 0-47.06-21.16-47.06-47.06V79.06c0-25.9 21.16-47.06 47.06-47.06 25.9 0 47.06 21.16 47.06 47.06V196.9zM283.1 385.88c25.9 0 47.06 21.16 47.06 47.06 0 25.9-21.16 47.06-47.06 47.06-25.9 0-47.06-21.16-47.06-47.06v-47.06h47.06zm0-23.72c-25.9 0-47.06-21.16-47.06-47.06 0-25.9 21.16-47.06 47.06-47.06h117.84c25.9 0 47.06 21.16 47.06 47.06 0 25.9-21.16 47.06-47.06 47.06H283.1z"/></svg>slack</a> </p> </li> </ul> </div> </div> </div> <!-- end MetaColumn 2 --> </div> </footer> <script src="https://static.arxiv.org/static/base/1.0.0a5/js/member_acknowledgement.js"></script> </body> </html>

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