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UFZ - Publikationsverzeichnis - Helmholtz-Zentrum für Umweltforschung UFZ
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<a href="index.php?de=43085" class=" " >UFZ-Chronik</a> </li> <li> <a href="index.php?de=34272" class=" " >Standorte/Anfahrt</a> </li> <li> <a href="index.php?de=39475" class=" " >Übersicht Ansprechpersonen</a> </li> </ul> </nav> <main id="contentwrapper" class="col-sm-9"> <ul class="breadcrumb"> <li> <a href="index.php?de=34257">UFZ</a> </li> <li> <a href="index.php?de=34270">Bibliothek</a> </li> <li> <a href="index.php?de=36296">Service</a> </li> <li> <a href="index.php?de=20939">UFZ - Publikationsverzeichnis</a> </li> <li class="pull-right iconoff hidden-print hidden-xs"> <a href="javascript:window.print();"><i class="fa fa-print fa-lg"></i></a> </li> </ul> <article id="content" class="col-md-12 "> <table style="width:98%"> <tr> <td class="marginoff paddingoff left top borderoff width70p"><h2 class="big">Details zur Publikation</h2></td> <td class="right top borderoff width30p"></td> </tr> </table> <table class="width100p pubappstyle"> <tr> <td class="left top bglightblue bordergray">Kategorie</td> <td class="left top bordergray">Textpublikation</td> </tr> <tr> <td class="left top bglightblue bordergray">Referenztyp</td> <td class="left top bordergray">Zeitschriften</td> </tr> <tr> <td class="left top bglightblue bordergray">DOI</td> <td class="left top bordergray"> <a target="_blank" href="https://doi.org/10.1016/j.cej.2019.122689">10.1016/j.cej.2019.122689</a> </td> </tr> <tr> <td class="left top bglightblue bordergray">Titel (prim盲r)</td> <td class="left top bordergray">Understanding the effect of carbon surface chemistry on adsorption of perfluorinated alkyl substances</td> </tr> <tr> <td class="left top bglightblue bordergray">Autor</td> <td class="left top bordergray"><strong>Saeidi, N.</strong>; <strong>Kopinke, F.-D.</strong>; <strong>Georgi, A.</strong></td> </tr> <tr> <td class="left top bglightblue bordergray">Quelle </td> <td class="left top bordergray">Chemical Engineering Journal</td> </tr> <tr> <td class="left top bglightblue bordergray">Erscheinungsjahr</td> <td class="left top bordergray">2020</td> </tr> <tr> <td class="left top bglightblue bordergray">Department</td> <td class="left top bordergray">TUCHEM</td> </tr> <tr> <td class="left top bglightblue bordergray">Band/Volume</td> <td class="left top bordergray">381</td> </tr> <tr> <td class="left top bglightblue bordergray">Seite von</td> <td class="left top bordergray">art. 122689</td> </tr> <tr> <td class="left top bglightblue bordergray">Sprache</td> <td class="left top bordergray">englisch</td> </tr> <tr> <td class="left top bglightblue bordergray">Keywords</td> <td class="left top bordergray">PFOA; PFOS; Activated carbon felts; Anion exchange capacity; Surface chemistry</td> </tr> <tr> <td class="left top bglightblue bordergray">Abstract</td> <td class="left top bordergray">The adsorption of perfluorooctanoic acid (PFOA) and perfluorooctylsulfonic acid (PFOS) on various activated carbon felts (ACFs) was studied and related to their surface characteristics. The adsorption isotherms of the ACFs studied differ widely in terms of adsorption affinities as well as maximum loadings. Cation and anion exchange capacities (CEC and AEC) at pH 7, as well as point of zero net proton charge (PZC), were identified as good indicators for understanding of each adsorbent鈥檚 behavior towards the perfluorinated alkyl substances (PFAS) in their anionic state. Maximum loadings of the two PFAS are in all cases equal to or lower than the AEC of the ACFs. The superposition of hydrophobic interactions and electrostatic attraction between PFAS anions and positively charged sites of ACF leads to exceptionally high adsorption affinity (<em>K</em><sub>d</sub> up to 10<sup>8</sup>鈥疞/kg). In this respect, positive charges created by proton adsorption to 蟺-electron-rich regions on the basal plane of carbon are more important than basic oxygen-containing groups. The effect of inorganic ions on adsorption of PFAS is variable and is also influenced by the surface chemistry of the ACFs. Dissolved natural organic matter did not significantly affect PFAS adsorption most likely due to size exclusion exerted by the micropores of the ACFs.</td> </tr> <tr> <td class="left top bglightblue bordergray width30p">dauerhafte UFZ-Verlinkung</td> <td class="left top bordergray width70p"><font style="font-size:9px">https://www.ufz.de/index.php?en=20939&ufzPublicationIdentifier=22196</font></td> </tr> <tr> <td class="left top bordergray" colspan="2"><b>Saeidi, N.</b>, <b>Kopinke, F.-D.</b>, <b>Georgi, A.</b> (2020):<br /> Understanding the effect of carbon surface chemistry on adsorption of perfluorinated alkyl substances<br /> <i>Chem. Eng. J.</i> <b>381</b> , art. 122689 <a class="iconoff" target="_blank" href="https://doi.org/10.1016/j.cej.2019.122689">10.1016/j.cej.2019.122689</a></td> </tr> </table> </article> <footer class="col-md-12 hidden-xs"> <ul class="page-info"> <li>Zugriffe: 7045116</li> <li>geändert: 11.02.2016</li> <li>Inhalt: Michael Garbe</li> <li><a href="mailto:kai.morlock@ufz.de">webmaster</a></li> </ul> </footer> </main> </div> </div> </section> <footer class="container"> <nav id="sitemap" class="sitemap row hidden-xs hidden-sm"> <div class="col-xs-2"> <h4><a href="index.php?de=34257">UFZ</a></h4> <hr> <ul class="nav nav-stacked"> <li> <a href="index.php?de=34258"> Mission </a> </li> <li> <a href="index.php?de=34262"> Geschäftsführung </a> </li> <li> <a href="index.php?de=49511"> Nachhaltigkeit am UFZ </a> </li> <li> <a href="index.php?de=39549"> Organisationsstruktur </a> </li> <li> <a href="index.php?de=34261"> Stäbe und Administration </a> </li> <li> <a href="index.php?de=34266"> Gremien und 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