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In this work, we successfully developed a novel strategy to modify a gold" /> <title>(PDF) Site-specific surface functionalization of gold nanorods using DNA origami clamps | Travis Meyer - Academia.edu</title> <link rel="canonical" href="https://www.academia.edu/23614269/Site_specific_surface_functionalization_of_gold_nanorods_using_DNA_origami_clamps" /> <script async src="https://www.googletagmanager.com/gtag/js?id=G-5VKX33P2DS"></script> <script> window.dataLayer = window.dataLayer || []; function gtag(){dataLayer.push(arguments);} gtag('js', new Date()); gtag('config', 'G-5VKX33P2DS', { cookie_domain: 'academia.edu', send_page_view: false, }); gtag('event', 'page_view', { 'controller': "single_work", 'action': "show", 'controller_action': 'single_work#show', 'logged_in': 'false', 'edge': 'unknown', // Send nil if there is no A/B test bucket, in case some records get logged // with missing data - that way we can distinguish between the two cases. // ab_test_bucket should be of the form <ab_test_name>:<bucket> 'ab_test_bucket': null, }) </script> <script> var $controller_name = 'single_work'; var $action_name = "show"; var $rails_env = 'production'; var $app_rev = '9387f500ddcbb8d05c67bef28a2fe0334f1aafb8'; var $domain = 'academia.edu'; var $app_host = "academia.edu"; var $asset_host = "academia-assets.com"; var $start_time = new Date().getTime(); var $recaptcha_key = "6LdxlRMTAAAAADnu_zyLhLg0YF9uACwz78shpjJB"; var $recaptcha_invisible_key = "6Lf3KHUUAAAAACggoMpmGJdQDtiyrjVlvGJ6BbAj"; var $disableClientRecordHit = false; </script> <script> window.require = { config: function() { return function() {} } } </script> <script> window.Aedu = window.Aedu || {}; window.Aedu.hit_data = null; window.Aedu.serverRenderTime = new Date(1733056794000); window.Aedu.timeDifference = new Date().getTime() - 1733056794000; </script> <script type="application/ld+json">{"@context":"https://schema.org","@type":"ScholarlyArticle","abstract":"Precise control over surface functionalities of nanomaterials offers great opportunities for fabricating complex functional nanoarchitectures but still remains challenging. In this work, we successfully developed a novel strategy to modify a gold nanorod (AuNR) with specific surface recognition sites using a DNA origami clamp. AuNRs were encapsulated by the DNA origami through hybridization of single-stranded DNA on the AuNRs and complementary capture strands inside the clamp. Another set of capture strands on the outside of the clamp create the specific recognition sites on the AuNR surface. By means of this strategy, AuNRs were sitespecifically modified with gold nanoparticles at the top, middle, and bottom of the surface, respectively, to construct a series of well-defined heterostructures with controlled “chemical valence”. Our study greatly expands the utility of DNA origami as a tool for building complex nanoarchitectures and represents a new approach for precise tailoring of nanomaterial surfaces.","author":[{"@context":"https://schema.org","@type":"Person","name":"Travis Meyer"}],"contributor":[],"dateCreated":"2016-03-23","dateModified":null,"datePublished":null,"headline":"Site-specific surface functionalization of gold nanorods using DNA origami clamps","inLanguage":"en","keywords":["Dna Nanotechnology","Gold Nanoparticles"],"locationCreated":null,"publication":null,"publisher":{"@context":"https://schema.org","@type":"Organization","name":null},"image":null,"thumbnailUrl":null,"url":"https://www.academia.edu/23614269/Site_specific_surface_functionalization_of_gold_nanorods_using_DNA_origami_clamps","sourceOrganization":[{"@context":"https://schema.org","@type":"EducationalOrganization","name":"gatech"}]}</script><link rel="stylesheet" media="all" 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"https://www.academia.edu/login?post_login_redirect_url=https%3A%2F%2Fwww.academia.edu%2F23614269%2FSite_specific_surface_functionalization_of_gold_nanorods_using_DNA_origami_clamps%3Fauto%3Ddownload"; window.loswp.translateUrl = "https://www.academia.edu/login?post_login_redirect_url=https%3A%2F%2Fwww.academia.edu%2F23614269%2FSite_specific_surface_functionalization_of_gold_nanorods_using_DNA_origami_clamps%3Fshow_translation%3Dtrue"; window.loswp.previewableAttachments = [{"id":44030285,"identifier":"Attachment_44030285","shouldShowBulkDownload":false}]; window.loswp.shouldDetectTimezone = true; window.loswp.shouldShowBulkDownload = true; window.loswp.showSignupCaptcha = false window.loswp.willEdgeCache = false; window.loswp.work = {"work":{"id":23614269,"created_at":"2016-03-23T07:18:38.397-07:00","from_world_paper_id":null,"updated_at":"2024-11-28T22:16:44.951-08:00","_data":{"abstract":"Precise control over surface functionalities\nof nanomaterials offers great opportunities for fabricating\ncomplex functional nanoarchitectures but still remains\nchallenging. In this work, we successfully developed a\nnovel strategy to modify a gold nanorod (AuNR) with\nspecific surface recognition sites using a DNA origami\nclamp. AuNRs were encapsulated by the DNA origami\nthrough hybridization of single-stranded DNA on the\nAuNRs and complementary capture strands inside the\nclamp. Another set of capture strands on the outside of the\nclamp create the specific recognition sites on the AuNR\nsurface. By means of this strategy, AuNRs were sitespecifically\nmodified with gold nanoparticles at the top,\nmiddle, and bottom of the surface, respectively, to\nconstruct a series of well-defined heterostructures with\ncontrolled “chemical valence”. Our study greatly expands\nthe utility of DNA origami as a tool for building complex\nnanoarchitectures and represents a new approach for\nprecise tailoring of nanomaterial surfaces.","ai_title_tag":"DNA Origami Clamps for Site-Specific Functionalization of Gold Nanorods"},"document_type":"paper","pre_hit_view_count_baseline":null,"quality":"high","language":"en","title":"Site-specific surface functionalization of gold nanorods using DNA origami clamps","broadcastable":true,"draft":false,"has_indexable_attachment":true,"indexable":true}}["work"]; window.loswp.workCoauthors = [33570395]; window.loswp.locale = "en"; window.loswp.countryCode = "SG"; window.loswp.cwvAbTestBucket = ""; window.loswp.designVariant = "ds_vanilla"; window.loswp.fullPageMobileSutdModalVariant = "full_page_mobile_sutd_modal"; window.loswp.useOptimizedScribd4genScript = false; window.loswp.appleClientId = 'edu.academia.applesignon';</script><script defer="" src="https://accounts.google.com/gsi/client"></script><div class="ds-loswp-container"><div class="ds-work-card--grid-container"><div class="ds-work-card--container js-loswp-work-card"><div class="ds-work-card--cover"><div class="ds-work-cover--wrapper"><div class="ds-work-cover--container"><button class="ds-work-cover--clickable js-swp-download-button" data-signup-modal="{"location":"swp-splash-paper-cover","attachmentId":44030285,"attachmentType":"pdf"}"><img alt="First page of “Site-specific surface functionalization of gold nanorods using DNA origami clamps”" class="ds-work-cover--cover-thumbnail" src="https://0.academia-photos.com/attachment_thumbnails/44030285/mini_magick20220701-20920-lf51ay.png?1656680769" /><img alt="PDF Icon" class="ds-work-cover--file-icon" src="//a.academia-assets.com/assets/single_work_splash/adobe.icon-574afd46eb6b03a77a153a647fb47e30546f9215c0ee6a25df597a779717f9ef.svg" /><div class="ds-work-cover--hover-container"><span class="material-symbols-outlined" style="font-size: 20px" translate="no">download</span><p>Download Free PDF</p></div><div class="ds-work-cover--ribbon-container">Download Free PDF</div><div class="ds-work-cover--ribbon-triangle"></div></button></div></div></div><div class="ds-work-card--work-information"><h1 class="ds-work-card--work-title">Site-specific surface functionalization of gold nanorods using DNA origami clamps</h1><div class="ds-work-card--work-authors ds-work-card--detail"><a class="ds-work-card--author js-wsj-grid-card-author ds2-5-body-md ds2-5-body-link" data-author-id="33570395" href="https://gatech.academia.edu/TMeyer"><img alt="Profile image of Travis Meyer" class="ds-work-card--author-avatar" src="//a.academia-assets.com/images/s65_no_pic.png" />Travis Meyer</a></div><div class="ds-work-card--detail"><div class="ds-work-card--work-metadata"><div class="ds-work-card--work-metadata__stat"><span class="material-symbols-outlined" style="font-size: 20px" translate="no">visibility</span><p class="ds2-5-body-sm" id="work-metadata-view-count">…</p></div><div class="ds-work-card--work-metadata__stat"><span class="material-symbols-outlined" style="font-size: 20px" translate="no">description</span><p class="ds2-5-body-sm">4 pages</p></div><div class="ds-work-card--work-metadata__stat"><span class="material-symbols-outlined" style="font-size: 20px" translate="no">link</span><p class="ds2-5-body-sm">1 file</p></div></div><script>(async () => { const workId = 23614269; const worksViewsPath = "/v0/works/views?subdomain_param=api&work_ids%5B%5D=23614269"; const getWorkViews = async (workId) => { const response = await fetch(worksViewsPath); if (!response.ok) { throw new Error('Failed to load work views'); } const data = await response.json(); return data.views[workId]; }; // Get the view count for the work - we send this immediately rather than waiting for // the DOM to load, so it can be available as soon as possible (but without holding up // the backend or other resource requests, because it's a bit expensive and not critical). const viewCount = await getWorkViews(workId); const updateViewCount = (viewCount) => { const viewCountNumber = Number(viewCount); if (!viewCountNumber) { throw new Error('Failed to parse view count'); } const commaizedViewCount = viewCountNumber.toLocaleString(); const viewCountBody = document.getElementById('work-metadata-view-count'); if (viewCountBody) { viewCountBody.textContent = `${commaizedViewCount} views`; } else { throw new Error('Failed to find work views element'); } }; // If the DOM is still loading, wait for it to be ready before updating the view count. if (document.readyState === "loading") { document.addEventListener('DOMContentLoaded', () => { updateViewCount(viewCount); }); // Otherwise, just update it immediately. } else { updateViewCount(viewCount); } })();</script></div><p class="ds-work-card--work-abstract ds-work-card--detail ds2-5-body-md">Precise control over surface functionalities of nanomaterials offers great opportunities for fabricating complex functional nanoarchitectures but still remains challenging. In this work, we successfully developed a novel strategy to modify a gold nanorod (AuNR) with specific surface recognition sites using a DNA origami clamp. AuNRs were encapsulated by the DNA origami through hybridization of single-stranded DNA on the AuNRs and complementary capture strands inside the clamp. Another set of capture strands on the outside of the clamp create the specific recognition sites on the AuNR surface. By means of this strategy, AuNRs were sitespecifically modified with gold nanoparticles at the top, middle, and bottom of the surface, respectively, to construct a series of well-defined heterostructures with controlled “chemical valence”. Our study greatly expands the utility of DNA origami as a tool for building complex nanoarchitectures and represents a new approach for precise tailoring of nanomaterial surfaces.</p><div class="ds-work-card--button-container"><button class="ds2-5-button js-swp-download-button" data-signup-modal="{"location":"continue-reading-button--work-card","attachmentId":44030285,"attachmentType":"pdf","workUrl":"https://www.academia.edu/23614269/Site_specific_surface_functionalization_of_gold_nanorods_using_DNA_origami_clamps"}">See full PDF</button><button class="ds2-5-button ds2-5-button--secondary js-swp-download-button" data-signup-modal="{"location":"download-pdf-button--work-card","attachmentId":44030285,"attachmentType":"pdf","workUrl":"https://www.academia.edu/23614269/Site_specific_surface_functionalization_of_gold_nanorods_using_DNA_origami_clamps"}"><span class="material-symbols-outlined" style="font-size: 20px" translate="no">download</span>Download 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Stefani</a></div><p class="ds-related-work--metadata ds2-5-body-xs">Nano Letters, 2014</p><div class="ds-related-work--ctas"><button class="ds2-5-text-link ds2-5-text-link--inline js-swp-download-button" data-signup-modal="{"location":"wsj-grid-card-download-pdf-modal","work_title":"Controlled Reduction of Photobleaching in DNA Origami–Gold Nanoparticle Hybrids","attachmentId":99030693,"attachmentType":"pdf","work_url":"https://www.academia.edu/97397107/Controlled_Reduction_of_Photobleaching_in_DNA_Origami_Gold_Nanoparticle_Hybrids","alternativeTracking":true}"><span class="material-symbols-outlined" style="font-size: 18px" translate="no">download</span><span class="ds2-5-text-link__content">Download free PDF</span></button><a class="ds2-5-text-link ds2-5-text-link--inline js-related-work-grid-card-view-pdf" href="https://www.academia.edu/97397107/Controlled_Reduction_of_Photobleaching_in_DNA_Origami_Gold_Nanoparticle_Hybrids"><span class="ds2-5-text-link__content">View PDF</span><span 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Zheng</a></div><p class="ds-related-work--metadata ds2-5-body-xs">SPIE Proceedings, 2004</p><div class="ds-related-work--ctas"><button class="ds2-5-text-link ds2-5-text-link--inline js-swp-download-button" data-signup-modal="{"location":"wsj-grid-card-download-pdf-modal","work_title":"Self-assembled gold nanowires from nanoparticles: an electronic route towards DNA nanosensors","attachmentId":104221684,"attachmentType":"pdf","work_url":"https://www.academia.edu/104512339/Self_assembled_gold_nanowires_from_nanoparticles_an_electronic_route_towards_DNA_nanosensors","alternativeTracking":true}"><span class="material-symbols-outlined" style="font-size: 18px" translate="no">download</span><span class="ds2-5-text-link__content">Download free PDF</span></button><a class="ds2-5-text-link ds2-5-text-link--inline js-related-work-grid-card-view-pdf" href="https://www.academia.edu/104512339/Self_assembled_gold_nanowires_from_nanoparticles_an_electronic_route_towards_DNA_nanosensors"><span 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