A strong Lewis acid imparts high ionic conductivity and interfacial stability to polymer composite electrolytes towards all-solid-state Li-metal batteries - CityU Scholars

<!doctype html><html lang="en"><head> <meta charset="utf-8" /> <meta name="viewport" content="width=device-width, initial-scale=1" /> <title>A strong Lewis acid imparts high ionic conductivity and interfacial stability to polymer composite electrolytes towards all-solid-state Li-metal batteries - CityU Scholars | A Research Hub of Excellence</title> <meta property="og:image" content="/resources/style/gfx/logo_top.png" /> <meta property="og:url" content="https://scholars.cityu.edu.hk/en/publications/a-strong-lewis-acid-imparts-high-ionic-conductivity-and-interfacial-stability-to-polymer-composite-electrolytes-towards-allsolidstate-limetal-batteries(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).html" /> <link rel="image_src" type="image/png" href="/resources/style/gfx/logo_top.png" /> <link rel="icon" href="/resources/style/gfx/favicon.ico" type="image/x-icon" /> <link href="https://fonts.googleapis.com/css?family=Open+Sans:400,300,700,600" rel="stylesheet" type="text/css" /><link 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content="Yunlei Zhong" /><meta name="citation_author_institution" content="University of Macau" /><meta name="citation_author" content="Zhaorui Wen" /><meta name="citation_author_institution" content="University of Macau" /><meta name="citation_author" content="Chaowei Li" /><meta name="citation_author_institution" content="University of Macau" /><meta name="citation_author" content="Jingxin Zhao" /><meta name="citation_author_institution" content="University of Macau" /><meta name="citation_author" content="Mingzheng Ge" /><meta name="citation_author_institution" content="University of Macau" /><meta name="citation_author_institution" content="Nantong University" /><meta name="citation_author" content="Pengfei Zhou" /><meta name="citation_author_institution" content="University of Macau" /><meta name="citation_author" content="Yanyan Zhang" /><meta name="citation_author_institution" content="Fuzhou University" /><meta name="citation_author" content="Yuxin Tang" /><meta name="citation_author_institution" content="Fuzhou University" /><meta name="citation_author" content="Guo Hong" /><meta name="citation_author_institution" content="University of Macau" /><meta name="citation_author_email" content="guohong@cityu.edu.hk" /><meta name="citation_author_orcid" content="0000-0002-5658-2244" /><meta name="citation_publication_date" content="2022/08" /><meta name="citation_online_date" content="2023/04/25" /><meta name="citation_doi" content="10.1007/s40843-021-1908-x" /><meta name="citation_language" content="English" /><meta name="citation_keywords" content="all-solid-state battery; composite electrolyte; interfaces; Li-ion conductivity; polyethylene oxide" /><meta name="citation_journal_title" content="Science China Materials" /><meta name="citation_issn" content="2095-8226" /><meta name="citation_publisher" content="Science in China Press" /><meta name="citation_volume" content="65" /><meta name="citation_issue" content="8" /><meta 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class="type_classification">RGC 21 - Publication in refereed journal</span><span class="type_classification"><span class="type_parent_sep"> › </span>peer-review</span></p></div> <div class="tabs-container"> <ul class="clear"> <li class="selected"><a class="portal_link" href="https://scholars.cityu.edu.hk/en/publications/a-strong-lewis-acid-imparts-high-ionic-conductivity-and-interfacial-stability-to-polymer-composite-electrolytes-towards-allsolidstate-limetal-batteries(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).html"><span>Overview</span></a> </li> </ul> </div> <div class="pub-full"> <div class="pub-top"> <div class="view-box scopus"> <span class="number">32</span> <span>Scopus Citations</span> </div> <div class="view-box viewall-scopus"> <a target="_blank" class="view_all_scopus_button" href="https://www.scopus.com/record/pubmetrics.uri?eid=2-s2.0-85122975931&origin=recordpage"> Scopus Metrics </a> </div> <div class="view-box almetric"> <script type="text/javascript" src="//d1bxh8uas1mnw7.cloudfront.net/assets/embed.js"></script> <div class="altmetric-embed pure_altmetric_component" data-badge-type="2" data-badge-popover="left" data-hide-no-mentions="true" data-link-target="true" data-doi="10.1007/s40843-021-1908-x"></div> </div> <div class="graph_viewer"> <div class="graph"><a class="portal_graphviewer_button" href="javascript:void(0);" id="j_id-222676425_40f6ca2e"><span>View graph of relations</span></a> <script type="text/javascript"></script> <i class="icon-network"></i> </div> </div> <div class="addthis"> <div class="addthis_sharing_toolbox"></div> </div> </div> <div class="view-box"> <h2 class="subheader">Author(s)</h2><div class="rendering rendering_researchoutput rendering_researchoutput_associatesauthorsclassifiedsummarizedlistportal rendering_contributiontojournal rendering_associatesauthorsclassifiedsummarizedlistportal rendering_contributiontojournal_associatesauthorsclassifiedsummarizedlistportal"><ul class="relations persons"><li><a rel="Person" href="https://scholars.cityu.edu.hk/en/persons/guo-hong(0698ee0d-3e35-4cdb-b1e5-dba301b40b57).html" class="link person"><span>Guo Hong</span></a></li><li><a onclick="$(this).up('ul').next('ul').toggleClassName('common_hidden');return false;" href="#" class="all link"><span>And 9 others</span></a></li></ul><ul class="relations persons common_hidden associates_authors_full_list"><li class="external">Litong Wang</li><li class="external">Yunlei Zhong</li><li class="external">Zhaorui Wen</li><li class="external">Chaowei Li</li><li class="external">Jingxin Zhao</li><li class="external">Mingzheng Ge</li><li class="external">Pengfei Zhou</li><li class="external">Yanyan Zhang</li><li class="external">Yuxin Tang</li></ul></div> </div> <div class="view-box"> <h2 class="subheader">Detail(s)</h2><div class="rendering rendering_researchoutput rendering_researchoutput_detailsportal rendering_contributiontojournal rendering_detailsportal rendering_contributiontojournal_detailsportal"><div class="article"><table class="properties"><tbody><tr class="language"><th scope="row">Original language</th><td>English</td></tr><tr><th scope="row">Pages (from-to)</th><td>2179-2188</td></tr><tr><th scope="row">Journal / Publication</th><td><a rel="Journal" href="https://scholars.cityu.edu.hk/en/journals/science-china-materials(7033621d-a67d-4be8-bb45-afc9c2722a9b)/publications.html" class="link"><span>Science China Materials</span></a></td></tr><tr><th scope="row">Volume</th><td>65</td></tr><tr><th scope="row">Issue number</th><td>8</td></tr><tr><th scope="row">Online published</th><td><span class="date">10 Jan 2022</span></td></tr><tr class="status"><th scope="row">Publication status</th><td><span class="prefix">Published - </span><span class="date">Aug 2022</span></td></tr><tr><th scope="row">Externally published</th><td>Yes</td></tr></tbody></table></div></div> </div> <div class="view-box"> <h2 class="subheader">Link(s)</h2> <table class="properties pub-links"> <tr> <th>DOI</th> <td><div class="rendering rendering_researchoutput rendering_researchoutput_versioneddoiextensionportal rendering_contributiontojournal rendering_versioneddoiextensionportal rendering_contributiontojournal_versioneddoiextensionportal"><h2 class="subheader">DOI</h3><ul class="relations links digital_object_identifiers"><li class="embargo_date_ended available open "><a onclick="window.open(this.href, '_blank','noopener,noreferrer'); return false;" href="https://doi.org/10.1007/s40843-021-1908-x" class="link"><span>https://doi.org/10.1007/s40843-021-1908-x</span></a> <span class="common_icon_16" style="background-image: url('/resources/style/icons/type/openaccess16.png');"></span><p class="dimmed">Final Published version</p></li></ul></div> </td> </tr> <tr> <th></th> <td> <span class="sfx-button" title="Check@CityULib"> <a href="https://julac.hosted.exlibrisgroup.com/primo-explore/openurl?ctx_ver=Z39.88-2004&ctx_tim=2024-11-23T20%3A09%3A57HKT&ctx_enc=info%3Aofi%2FencUTF-8&url_ver=Z39.88-2004&url_ctx_fmt=info%3Aofi%2Ffmt%3Akev%3Amtx%3Actx&rft.genre=article&rft_val_fmt=info%3Aofi%2Fkev%3Afmt%3Ajournal&rfr_id=info%3Asid%2F%3Apure&rft.atitle=A%20strong%20Lewis%20acid%20imparts%20high%20ionic%20conductivity%20and%20interfacial%20stability%20to%20polymer%20composite%20electrolytes%20towards%20all-solid-state%20Li-metal%20batteries&rft_id=info%3Adoi%2F10.1007%2Fs40843-021-1908-x&rft.aulast=Wang&rft.aufirst=Litong&rft.auinit=L&rft.date=2022-08&rft.volume=65&rft.issue=8&rft.issn=2095-8226&rft.jtitle=Science%20China%20Materials&rft.pages=2179-2188&institution=CUH_ALMA&vid=CUH" target="_blank"> Check@CityULib </a> </span> </td> </tr> <tr> <th>Link to Scopus</th> <td><a target="_blank" class="scopus-link-pub" href="https://www.scopus.com/record/display.uri?eid=2-s2.0-85122975931&origin=recordpage"> https://www.scopus.com/record/display.uri?eid=2-s2.0-85122975931&origin=recordpage </a></td> </tr> <tr class="permanent_link"> <th>Permanent Link</th> <td> <a href="https://scholars.cityu.edu.hk/en/publications/publication(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).html">https://scholars.cityu.edu.hk/en/publications/publication(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).html</a></td> </tr> </table> </div> <div class="view-box"> <h2 class="subheader">Abstract</h2><div class="rendering rendering_researchoutput rendering_researchoutput_customabstractportal rendering_contributiontojournal rendering_customabstractportal rendering_contributiontojournal_customabstractportal"><div class="textblock">The development of high-performance solid polymer electrolytes is crucial for producing all-solid-state lithium metal batteries with high safety and high energy density. However, the low ionic conductivity of solid polymer electrolytes and their unstable electrolyte/electrode interfaces have hindered their widespread utilization. To address these critical challenges, a strong Lewis acid (aluminum fluoride (AlF<sub>3</sub>)) with dual functionality is introduced into polyethylene oxide) (PEO)-based polymer electrolyte. The AlF<sub>3</sub> facilitates the dissociation of lithium salt, increasing the ion-transfer efficiency due to the Lewis acid-base interaction; further the <i>in-situ </i>formation of lithium fluoride-rich interfacial layer is promoted, which suppresses the uneven lithium deposition and continuous undesired reactions between the Li metal and PEO matrix. Benefiting from our rational design, the symmetric Li/Li battery with the modified electrolyte exhibits much longer cycling stability (over 3600 h) than that of the pure PEO/lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) electrolyte (550 h). Furthermore, the all-solid-state LiFePO<sub>4</sub> full cell with the composite electrolyte displays a much higher Coulombic efficiency (98.4% after 150 cycles) than that of the electrolyte without the AlF<sub>3</sub> additive (63.3% after 150 cycles) at a large voltage window of 2.4–4.2 V, demonstrating the improved interface and cycling stability of solid polymer lithium metal batteries. © Science China Press and Springer-Verlag GmbH Germany, part of Springer Nature 2022.</div></div> </div> <div class="view-box"> <h2 class="subheader">Research Area(s)</h2><div class="rendering rendering_keywordable rendering_keywordgroupsexcludecopyright rendering_keywordable_keywordgroupsexcludecopyright"><div class="keywordcontainers"><ul class="relations keywords"><li>all-solid-state battery, composite electrolyte, interfaces, Li-ion conductivity, polyethylene oxide</li></ul></div><div class="sustainabledevelopmentgoals"><ul class="relations keywords"><li><strong><a 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class="procent">100</span> </div> <div class="finger-info"> <span class="title"> <span class="text">Lithium Metal Batte...</span> </span> <span class="concept_badge less_100" data-content-id="198071491" data-thesauri-acronym="MaterialScience"> <span class="rating rank_100"><em></em></span> <span class="domain"> <span class="text">Material Science</span> </span> </span> </div></span></a> </div> </div> <div class="concept_links"><a class="portal_link" href="https://scholars.cityu.edu.hk/en/publications/a-strong-lewis-acid-imparts-high-ionic-conductivity-and-interfacial-stability-to-polymer-composite-electrolytes-towards-allsolidstate-limetal-batteries(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9)/fingerprints.html"><span>Full Fingerprint ›</span></a> </div> </div> </div> </div> <div class="view-box citations"> <h2 class="subheader">Citation Format(s)</h2> <div class="tabs-container citations clear"> <ul class="citations"> <li class="selected"><a href="#">Standard</a></li> <li><a href="#">Harvard</a></li> <li><a href="#">APA</a></li> <li><a href="#">Vancouver</a></li> <li><a href="#">Author</a></li> </ul> <div class="cite-export"> <span class="publication_export">[ <a class="portal_link" href="https://scholars.cityu.edu.hk/en/publications/a-strong-lewis-acid-imparts-high-ionic-conductivity-and-interfacial-stability-to-polymer-composite-electrolytes-towards-allsolidstate-limetal-batteries(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).ris?download=true"><span>RIS</span></a> ]</span> <span class="publication_export">[ <a class="portal_link" href="https://scholars.cityu.edu.hk/en/publications/a-strong-lewis-acid-imparts-high-ionic-conductivity-and-interfacial-stability-to-polymer-composite-electrolytes-towards-allsolidstate-limetal-batteries(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).bibtex?download=true"><span>BibTeX</span></a> ]</span> </div> </div> <div class="citation-container"> <div class="view-box cite"><div class="rendering rendering_researchoutput rendering_researchoutput_standard rendering_contributiontojournal rendering_standard rendering_contributiontojournal_standard"><a rel="ContributionToJournal" href="https://scholars.cityu.edu.hk/en/publications/a-strong-lewis-acid-imparts-high-ionic-conductivity-and-interfacial-stability-to-polymer-composite-electrolytes-towards-allsolidstate-limetal-batteries(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).html" class="link"><span><strong>A strong Lewis acid imparts high ionic conductivity and interfacial stability to polymer composite electrolytes towards all-solid-state Li-metal batteries.</strong></span></a> / Wang, Litong; Zhong, Yunlei; Wen, Zhaorui et al. <br />In: <a rel="Journal" href="https://scholars.cityu.edu.hk/en/journals/science-china-materials(7033621d-a67d-4be8-bb45-afc9c2722a9b)/publications.html" class="link"><span>Science China Materials</span></a>, Vol. 65, No. 8, 08.2022, p. 2179-2188.<p class="type"><span class="type_family">Research output<span class="type_family_sep">: </span></span><span class="type_classification_parent">Journal Publications and Reviews<span class="type_parent_sep"> › </span></span><span class="type_classification">RGC 21 - Publication in refereed journal</span><span class="type_classification"><span class="type_parent_sep"> › </span>peer-review</span></p></div> </div> <div class="view-box cite" style="display: none;"><div class="rendering rendering_researchoutput rendering_researchoutput_harvard rendering_contributiontojournal rendering_harvard rendering_contributiontojournal_harvard">Wang, L, Zhong, Y, Wen, Z, Li, C, Zhao, J, Ge, M, Zhou, P, Zhang, Y, Tang, Y<a rel="Person" href="https://scholars.cityu.edu.hk/en/persons/guo-hong(0698ee0d-3e35-4cdb-b1e5-dba301b40b57).html" class="link"><span> & Hong, G</span></a> 2022, '<a rel="ContributionToJournal" href="https://scholars.cityu.edu.hk/en/publications/a-strong-lewis-acid-imparts-high-ionic-conductivity-and-interfacial-stability-to-polymer-composite-electrolytes-towards-allsolidstate-limetal-batteries(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).html" class="link harvard_title"><span>A strong Lewis acid imparts high ionic conductivity and interfacial stability to polymer composite electrolytes towards all-solid-state Li-metal batteries</span></a>', <a rel="Journal" href="https://scholars.cityu.edu.hk/en/journals/science-china-materials(7033621d-a67d-4be8-bb45-afc9c2722a9b)/publications.html" class="link"><span><em>Science China Materials</em></span></a>, vol. 65, no. 8, pp. 2179-2188. <a onclick="window.open(this.href, '_blank','noopener,noreferrer'); return false;" href="https://doi.org/10.1007/s40843-021-1908-x" class="link"><span>https://doi.org/10.1007/s40843-021-1908-x</span></a></div> </div> <div class="view-box cite" style="display: none;"><div class="rendering rendering_researchoutput rendering_researchoutput_apa rendering_contributiontojournal rendering_apa rendering_contributiontojournal_apa">Wang, L., Zhong, Y., Wen, Z., Li, C., Zhao, J., Ge, M., Zhou, P., Zhang, Y., Tang, Y.<a rel="Person" href="https://scholars.cityu.edu.hk/en/persons/guo-hong(0698ee0d-3e35-4cdb-b1e5-dba301b40b57).html" class="link"><span>, & Hong, G.</span></a> (2022). <a rel="ContributionToJournal" href="https://scholars.cityu.edu.hk/en/publications/a-strong-lewis-acid-imparts-high-ionic-conductivity-and-interfacial-stability-to-polymer-composite-electrolytes-towards-allsolidstate-limetal-batteries(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).html" class="link"><span>A strong Lewis acid imparts high ionic conductivity and interfacial stability to polymer composite electrolytes towards all-solid-state Li-metal batteries</span></a>. <a rel="Journal" href="https://scholars.cityu.edu.hk/en/journals/science-china-materials(7033621d-a67d-4be8-bb45-afc9c2722a9b)/publications.html" class="link"><span><em>Science China Materials</em></span></a>, <em>65</em>(8), 2179-2188. <a onclick="window.open(this.href, '_blank','noopener,noreferrer'); return false;" href="https://doi.org/10.1007/s40843-021-1908-x" class="link"><span>https://doi.org/10.1007/s40843-021-1908-x</span></a></div> </div> <div class="view-box cite" style="display: none;"><div class="rendering rendering_researchoutput rendering_researchoutput_vancouver rendering_contributiontojournal rendering_vancouver rendering_contributiontojournal_vancouver">Wang L, Zhong Y, Wen Z, Li C, Zhao J, Ge M et al. <span class="title"><a rel="ContributionToJournal" href="https://scholars.cityu.edu.hk/en/publications/a-strong-lewis-acid-imparts-high-ionic-conductivity-and-interfacial-stability-to-polymer-composite-electrolytes-towards-allsolidstate-limetal-batteries(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).html" class="link"><span>A strong Lewis acid imparts high ionic conductivity and interfacial stability to polymer composite electrolytes towards all-solid-state Li-metal batteries</span></a></span>. <a rel="Journal" href="https://scholars.cityu.edu.hk/en/journals/science-china-materials(7033621d-a67d-4be8-bb45-afc9c2722a9b)/publications.html" class="link"><span>Science China Materials</span></a>. 2022 Aug;65(8):2179-2188. Epub 2022 Jan 10. doi: 10.1007/s40843-021-1908-x</div> </div> <div class="view-box cite" style="display: none;"><div class="rendering rendering_researchoutput rendering_researchoutput_author rendering_contributiontojournal rendering_author rendering_contributiontojournal_author">Wang, Litong ; Zhong, Yunlei ; Wen, Zhaorui et al. / <a rel="ContributionToJournal" href="https://scholars.cityu.edu.hk/en/publications/a-strong-lewis-acid-imparts-high-ionic-conductivity-and-interfacial-stability-to-polymer-composite-electrolytes-towards-allsolidstate-limetal-batteries(3d2a7273-64e0-424d-b5a0-08f6ed1ef2b9).html" class="link"><span><strong>A strong Lewis acid imparts high ionic conductivity and interfacial stability to polymer composite electrolytes towards all-solid-state Li-metal batteries</strong></span></a>. In: <a rel="Journal" href="https://scholars.cityu.edu.hk/en/journals/science-china-materials(7033621d-a67d-4be8-bb45-afc9c2722a9b)/publications.html" class="link"><span>Science China Materials</span></a>. 2022 ; Vol. 65, No. 8. pp. 2179-2188.</div> </div> </div> </div> </div> </div> </div> <div class="footer"> <div class="wrapper"> <div class="cityu-scholar-footer-outbox"> <div class="cityu-scholar-footer-inbox"> <a href="https://www.cityu.edu.hk/cityu/privacy/index.htm" title="Footer Privacy Policy" target="_blank">Privacy Policy</a> | <a href="https://www.cityu.edu.hk/cityu/copyright/index.htm#copyright" title="Footer Copyright" target="_blank">Copyright</a> | <a href="https://www.cityu.edu.hk/cityu/disclaimer/index.htm#disclaimer" title="Footer Disclaimer" target="_blank">Disclaimer</a> | <a href="https://www.cityu.edu.hk/cityu/accessibility/" title="Footer Accessibility" target="_blank">Accessibility</a> | <a href="https://www.cityu.edu.hk/cityu/contactus/index.htm" title="Footer Contact Us" target="_blank">Contact Us</a><br /> © City University of Hong Kong. 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