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Green Catalysis, Ionic Liquids and Metal-Organic Frameworks in Environmental Catalysis – Catalysis
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<main class="site-main" id="main"> <article id="post-100" class="post-100 post type-post status-publish format-standard has-post-thumbnail hentry category-green-catalysis tag-biodiesel-production tag-catalytic-performance tag-environmental-catalysis tag-green-catalysis tag-hybrid-catalysts tag-ionic-liquids tag-metal-organic-frameworks tag-oxidative-desulfurization tag-recyclability tag-sustainable-development" itemtype="https://schema.org/CreativeWork" itemscope> <div class="inside-article"> <div class="featured-image page-header-image-single "> <img width="1200" height="628" src="https://catalysis.blog/archive/wp-content/uploads/2024/09/image-_22_-min-1-1-scaled-e1726233982203.jpg" class="attachment-full size-full" alt="" itemprop="image" decoding="async" fetchpriority="high" /> </div> <header class="entry-header"> <h1 class="entry-title" itemprop="headline">Green Catalysis, Ionic Liquids and Metal-Organic Frameworks in Environmental Catalysis</h1> <div class="entry-meta"> <span class="posted-on"><time class="updated" datetime="2024-09-13T18:56:29+05:30" itemprop="dateModified">September 13, 2024</time><time class="entry-date published" datetime="2024-09-13T17:31:48+05:30" itemprop="datePublished">September 13, 2024</time></span> <span class="byline">by <span class="author vcard" itemprop="author" itemtype="https://schema.org/Person" itemscope><a class="url fn n" href="https://catalysis.blog/archive/author/catalysis/" title="View all posts by catalysis" rel="author" itemprop="url"><span class="author-name" itemprop="name">catalysis</span></a></span></span> </div> </header> <div class="entry-content" itemprop="text"> <p><span style="font-weight: 400;">Sustainable development has been eagerly sought after in recent times. Green catalysis has evolved as a prospective area that seeks to reduce the impact on the environment while maximizing efficiency in chemical processes. Two prominent players in this domain are ionic liquids and metal-organic frameworks. These advanced materials manifest special properties, which make them very efficient in many catalytic applications, especially in the field of environmental catalysis. Combinatorial chemistry of ILs and MOFs has gone a long way in achieving tremendous improvements in processes such as oxidative desulfurization, biodiesel production, and deep desulfurization of fuels. Elucidation of the symmetricality-related efficiency of reactions constitutes the main focus of the continuation of this article section.</span></p> <h3><b>Applications of Combinatorial Chemistry in ILs and MOFs</b></h3> <p><span style="font-weight: 400;">Ionic liquids are considered liquids at relatively low temperatures, usually less than 100 °C. They are composed of an organic cation and an inorganic or organic anion. These IL properties bestow it with low volatility, high thermal stability, and tunable solubility, making them very appropriate media for various catalytic applications. One of the most important advantages is that ILs can play the role of both a solvent and a catalyst, thus giving opportunities to further simplify the reaction process and increase its effectiveness.</span></p> <p><span style="font-weight: 400;">In the context of green catalysis, ILs have been used in large quantities in processes of oxidative desulfurization. ODS is an important technique for desulfurizing fuels since its application is urgently required by strict environmental regulations. ILs make this process quick by enhancing the solubility of sulfur compounds and stabilizing catalytic intermediates. For example, IL-modified heteropolyacids displayed excellent catalytic activity in the process of ODS, realizing high efficiency in sulfur removal under very mild conditions. ILs have been incorporated into catalytic systems, and not only the activity has shown improvement but also the recyclability and stability of the catalyst.</span></p> <p></div></div> <div style="background: #f7f7f7;border: 1px solid rgba(0, 0, 0, 0.07);"> <div style="padding: 30px;"><div class="Adblock-main"> <div class="Adblock-head"> <h2>Yearwise Publication Trend on <b>“<a href="https://catalysis.blog/publication-trends/index/green catalysis" target="_blank" title="green catalysis - yearwise publication trends">green catalysis</a>”</b></h2> </div> </div><div class="results-container"><div class="chart-block" style="padding:15px;"> <div class="left"> <div id="results" class="results"></div> </div> <div class="right"> <div class="chart-container"><canvas id="publicationChart"></canvas></div> </div> <div class="keywordsdiv"> <div style="text-align:center;"><b>Find publication trends on relevant topics</b> </div> <span class="gp-icon icon-tags"><svg viewBox="0 0 512 512" aria-hidden="true" xmlns="http://www.w3.org/2000/svg" width="1em" height="1em"><path d="M20 39.5c-8.836 0-16 7.163-16 16v176c0 4.243 1.686 8.313 4.687 11.314l224 224c6.248 6.248 16.378 6.248 22.626 0l176-176c6.244-6.244 6.25-16.364.013-22.615l-223.5-224A15.999 15.999 0 00196.5 39.5H20zm56 96c0-13.255 10.745-24 24-24s24 10.745 24 24-10.745 24-24 24-24-10.745-24-24z"></path><path d="M259.515 43.015c4.686-4.687 12.284-4.687 16.97 0l228 228c4.686 4.686 4.686 12.284 0 16.97l-180 180c-4.686 4.687-12.284 4.687-16.97 0-4.686-4.686-4.686-12.284 0-16.97L479.029 279.5 259.515 59.985c-4.686-4.686-4.686-12.284 0-16.97z"></path></svg></span> <span id="keyword-stats"></span> </div> </div></div></div><div class="inside-article"><style> table { margin: 0 0 1.5em; 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In their intrinsic form, MOFs possess an exceptionally high surface area, tunable pore size, and diverse chemical functionalities, which make them very versatile in catalysis. The diversity in the nature of metals and organic linkers makes them amenable to designing catalysts with targeted activity for target applications.</span></p> <p><span style="font-weight: 400;">MOFs have been used traditionally in environmental catalysis for oxidative desulfurization, the production of biodiesel, and the destruction of refractory sulfur compounds. MOFs encapsulated with polyoxometalates have exhibited remarkably high catalytic activity and stability in ODS processes. On their part, the high surface area and porous characteristics of MOFs help to enhance the catalytic performance by favoring the diffusion of reactants and products. Moreover, several active species can be bonded to them for proper functionalization, and MOFs can be easily tuned for the preparation of highly effective and recyclable catalysts.</span></p> <h3><b>Synergy between Ionic Liquids and Metal-Organic Frameworks</b></h3> <p><span style="font-weight: 400;">The synergy introduced a new catalytic system that was much more efficient as well as stable. On the surfaces of MOF-based materials or inside their cavities, ILs could be immobilized in an exemplary way to show synergy in performance, increasing the activity and selectivity of the catalyst. For example, IL-modified MOFs exhibited better activity than individual components in the oxidative desulfurization process. For the activation of sulfur compounds, the ILs can provide an appropriate setting, while the MOFs may provide both a high surface area and a stable framework for catalytic reactions.</span></p> <p><span style="font-weight: 400;">One such example is the use of IL-modified MOFs in the case of the oxidative desulfurization of diesel fuel. Such hybrid catalysts show high efficiency in the removal of sulfur compounds from diesel fuel, like dibenzothiophene, even under very mild conditions. The ILs enhance the solubility of sulfur compounds and promote their oxidation, while the MOFs provide a very strong platform for the catalytic reaction. Therein, the synergy has led to high catalytic activity, excellent selectivity, and improved recyclability, which is ideal for industrial applications.</span></p> <h3><b>Recent Developments and Applications</b></h3> <p><span style="font-weight: 400;">New studies in this area have focused on designing and synthesizing IL-MOF hybrids in relation to environmental catalysis and the improvement of performance. The further advancement in the synthesizing technique has made possible accurate control over the composition and structure of the IL-MOF hybrids, which is responsible for the enhanced catalytic activity and stability.</span></p> <p><span style="font-weight: 400;">MOFs encapsulated with Zr-doped polyoxometalates for biodiesel production are a perfect example of such advancement. It is evident that the esterification of oleic acid with methanol to afford high-yielding biodiesel was highly active on these catalysts. The Zr-doped polyoxometalates provide strong acid sites for the catalytic reaction, and the MOFs offer a high surface area and a porous structure for the diffusion of reactants and products. Such an introduction of ILs within MOFs also leads to increased catalytic activity and stability, making the hybrid catalysts highly efficient and recyclable.</span></p> <p><span style="font-weight: 400;">One more interesting development concerns the application of IL-modified MOFs to remove refractory sulfur compounds from fuels. These catalytic systems have manifested high performance in the oxidative desulfurization of diesel fuel under mild conditions with respect to temperature. The ILs improve the solubility of sulfur compounds and promote their oxidation process, while the MOFs provide an ideal framework for catalysis. Such a combination guarantees high catalytic activity, high selectivity, improved recyclability, and consequently makes these IL-MOF hybrid catalysts suitable for industrial applications.</span></p> <p></div></div> <div style="background: #f7f7f7;border: 1px solid rgba(0, 0, 0, 0.07);"> <div style="padding: 30px;"><div class="Adblock-main"> <div class="Adblock-head"> <h2>Recent Publications on <b>“<a href="https://catalysis.blog/recent-publications/index/green catalysis" target="_blank" rel="noopener" title="green catalysis - yearwise publication list">green catalysis</a>”</b></h2> </div> </div> <div class="pb-main"><div class="article-scroll"><div id="results_recent" class="results"></div></div><div class="keywordsdiv" style="margin: 0px 15px;margin-top:20px;"> <div style="text-align:center;"><b>Find publications on relevant topics</b> </div> <span class="gp-icon icon-tags"><svg viewBox="0 0 512 512" aria-hidden="true" xmlns="http://www.w3.org/2000/svg" width="1em" height="1em"><path 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</style> <script> function decodeString(str) { str = str.replace(/\\'/g, "'"); str = str.replace(/\\'/g, "'"); str = str.replace(/\\'/g, "'"); return str; } function displayResults_recent(papers) { var resultsContainer = document.getElementById('results_recent'); if (!papers || papers.length === 0) { resultsContainer.innerHTML = '<p>No recent publications found.</p>'; return; } papers.forEach(paper => { var publicationBlock = document.createElement('div'); publicationBlock.className = 'publication-block'; var title_de = decodeString(paper.title); var publicationHTML = ` <div style="margin-bottom: 10px;line-height: 24px;"><a href="${paper.url}" target="_blank" title="${title_de}">${title_de}</a></div> <p><strong>Issue Release:</strong> ${paper.publishedDate}</p> `; publicationBlock.innerHTML = publicationHTML; resultsContainer.appendChild(publicationBlock); }); } function displayKeywordPapers(keywords) { var resultsContainer = document.getElementById('keyword-papers'); resultsContainer.innerHTML = ''; if (!keywords || keywords.length === 0) { resultsContainer.innerHTML = '<p>No data found.</p>'; return; } var keywordHTML = ''; keywords.forEach((key, index) => { let key_replace = key.replace(/ /g, '-'); key_replace = key_replace.toLowerCase(); keywordHTML += `<a href="https://catalysis.blog/recent-publications/index/${key_replace}" target="_blank" title="${key} - publication list">${key}</a>`; if (index < keywords.length - 1) { keywordHTML += ', '; } }); resultsContainer.innerHTML = keywordHTML; } // Call the function with the PHP data var recent_papers = [ { "title": "Niobic acid as a support for microheterogeneous nanocatalysis of sodium borohydride hydrolysis under mild conditions.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38887643", "publishedDate": "2024" }, { "title": "Enzyme-mediated green synthesis of glycosaminoglycans and catalytic process intensification.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38857660", "publishedDate": "2024" }, { "title": "Nanotechnology for the enhancement of algal cultivation and bioprocessing: Bridging gaps and unlocking potential.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38914236", "publishedDate": "2024" }, { "title": "Green-synthesized CuO and ZnO nanoparticles derived from Calotropis gigantea (Apple of Sodom): enhancing plant growth, efficient dye removal, and potent antibacterial applications.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38958855", "publishedDate": "2024" }, { "title": "Electronic Structure and Functions of Carbon Nitride in Frontier Green Catalysis.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/39107898", "publishedDate": "2024" }, { "title": "Green Synthesis of Carbon Quantum Dots and Carbon Quantum Dot-Gold Nanoparticles for Applications in Bacterial Imaging and Catalytic Reduction of Aromatic Nitro Compounds.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38854549", "publishedDate": "2024" }, { "title": "Green synthesis for diverse bioactive benzo-fused spiroindolines through DBU-catalysed post-Ugi double cyclization.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38689553", "publishedDate": "2024" }, { "title": "Engineering cascade biocatalysis in whole cells for syringic acid bioproduction.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38824548", "publishedDate": "2024" }, { "title": "Photoredox Catalysis by 21-Thiaporphyrins: A green and Efficient Approach for C-N Borylation and C-H Arylation.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38825798", "publishedDate": "2024" }, { "title": "Progress on metabolites of Astragalus medicinal plants and a new factor affecting their formation: Biotransformation of endophytic fungi.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38838334", "publishedDate": "2024" }, { "title": "Cu-chelated polydopamine nanozymes with laccase-like activity for photothermal catalytic degradation of dyes.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38735253", "publishedDate": "2024" }, { "title": "Classification and functional origins of stereocomplementary alcohol dehydrogenases for asymmetric synthesis of chiral secondary alcohols: A review.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38729463", "publishedDate": "2024" }, { "title": "Isomerization Engineering of Oxygen-Enriched Carbon Quantum Dots for Efficient Electrochemical Hydrogen Peroxide Production.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38713154", "publishedDate": "2024" }, { "title": "Progress and Perspective for \\\\\\\"Green\\\\\\\" Strategies of Catalytic Plastics Conversion into Fuels by Regulating Half-Reactions.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38832898", "publishedDate": "2024" }, { "title": "Surface viscosity of liquid interfaces from Green-Kubo relations.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38775241", "publishedDate": "2024" }, { "title": "Spontaneous Formation of Ultrasmall Noble Metal Nanoparticles on Cobalt-Based Layered Double Hydroxide for Electrochemical and Environmental Catalysis.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38189520", "publishedDate": "2024" }, { "title": "The Synergistic Impact of Crystal Seed and Fluoride Ion in the Synthesis of Silicalite-1 Zeolite in Low-Template Systems.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38204118", "publishedDate": "2024" }, { "title": "Biosynthesis of Nicotinamide Mononucleotide: Synthesis Method, Enzyme, and Biocatalytic System.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38330904", "publishedDate": "2024" }, { "title": "Rare Earths-The Answer to Everything.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38338432", "publishedDate": "2024" }, { "title": "Structural characterization of lignin from the green pretreatments for co-producing xylo-oligosaccharides and glucose: Toward full biomass utilization.", "url": "https:\/\/pubmed.ncbi.nlm.nih.gov\/38211916", "publishedDate": "2024" } ]; var keywordsArray = ["Green catalysis","Ionic liquids","Metal-organic frameworks","Environmental catalysis","Oxidative desulfurization","Biodiesel production","Hybrid catalysts","Sustainable development","Catalytic performance","Recyclability"]; displayResults_recent(recent_papers); displayKeywordPapers(keywordsArray); // function stripslashes(str) { // if (typeof str === 'string') { // return str.replace(/\/g, ''); // } // } </script></p> <h3><b>Challenges and Future Directions</b></h3> <p><span style="font-weight: 400;">In spite of the many steps accomplished in the area, different challenges remain. For example, in the said catalysts, scalability comes into play if they are to be applied industrially, since a synthesis route for ILs and MOFs can be very sophisticated and costly. Furthermore, additional studies are required to understand the stability with harsh reaction conditions of the IL-MOF hybrids so that the long-term performance can be assured.</span></p> <p><span style="font-weight: 400;">Further research in this direction must target the development of low-cost methods, which are also scalable, for the synthesis of IL-MOF hybrids. In the coming future, the discovery of a new genre of ILs and MOFs with better properties and functions is also going to be very important to further promote the application of this kind of material in green catalysis. Additionally, the implementation of such IL-MOF hybrids within continuous flow reactors and other modern catalytic systems can really bring great impetus to their practical applications within industrial processes.</span></p> <h3><b>Conclusion</b></h3> <p><span style="font-weight: 400;">The combination of ionic liquids with metal-organic frameworks can furnish a truly worthwhile strategy toward green catalysis related to environmental applications. The properties of anion ordering, high surface area, good to tunable porosity, and enhanced catalytic activity make the ionic liquids and metal-organic frameworks ideal candidates for various catalytic applications. Such a synergism between IL and MOF could lead to the development of highly efficient and recyclable catalysts with superior performance in the fields of oxidative desulfurization, biodiesel production, and other environmental applications. Further research and development related to such hybrids will open the way toward sustainable and proficient exploitation of IL-MOF hybrid catalysts in industries and finally a road to a cleaner and greener future.</span></p> <p></p> <h3><b>References</b></h3> <ol> <li>Wei Z, Wang J, Yu H, Han S, Wei Y. <a href="https://pubmed.ncbi.nlm.nih.gov/36014452/">Recent Advances of Anderson-Type Polyoxometalates as Catalysts Largely for Oxidative Transformations of Organic Molecules.</a> Molecules. 2022 Aug 16;27(16):5212. doi: 10.3390/molecules27165212. PMID: 36014452; PMCID: PMC9412380.</li> <li>Liu, H., Li, Z., Dong, J., Liu, D., Liu, C., Chi, Y. and Hu, C., 2020. <a href="https://pubs.rsc.org/en/content/articlelanding/2020/nr/d0nr03951a/unauth">Polyoxometalates encapsulated into hollow double-shelled nanospheres as amphiphilic nanoreactors for an effective oxidative desulfurization.</a> <i>Nanoscale</i>, <i>12</i>(31), pp.16586-16595.</li> <li>Zhang, Q., Lei, D., Luo, Q., Wang, J., Deng, T., Zhang, Y. and Ma, P., 2020. <a href="https://pubs.rsc.org/en/content/articlehtml/2020/ra/d0ra00141d">Efficient biodiesel production from oleic acid using metal–organic framework encapsulated Zr-doped polyoxometalate nano-hybrids.</a> <i>RSC advances</i>, <i>10</i>(15), pp.8766-8772.</li> <li>Wu, L., Miao, G., Dai, X., Dong, L., Li, Z. and Xiao, J., 2019. <a href="https://pubs.acs.org/doi/abs/10.1021/acs.energyfuels.9b01896">Ultra-deep desulfurization of real diesel using two-layer silica gels under mild conditions. </a><i>Energy & Fuels</i>, <i>33</i>(8), pp.7287-7296.</li> <li>Luo, J., Chao, Y., Tang, Z., Hua, M., Li, X., Wei, Y., Ji, H., Xiong, J., Zhu, W. and Li, H., 2019. <a href="https://pubs.acs.org/doi/abs/10.1021/acs.iecr.9b01745">Design of lewis acid centers in bundlelike boron nitride for boosting adsorptive desulfurization performance.</a> <i>Industrial & Engineering Chemistry Research</i>, <i>58</i>(29), pp.13303-13312.</li> <li>Li, S.W., Gao, R.M. and Zhao, J.S., 2018. <a href="https://pubs.acs.org/doi/abs/10.1021/acssuschemeng.8b04524">Deep oxidative desulfurization of fuel catalyzed by modified heteropolyacid: The comparison performance of three kinds of ionic liquids.</a> <i>ACS Sustainable Chemistry & Engineering</i>, <i>6</i>(11), pp.15858-15866.</li> <li>Wagle, D.V., Zhao, H., Deakyne, C.A. and Baker, G.A., 2018. <a href="https://pubs.acs.org/doi/abs/10.1021/acssuschemeng.8b00224">Quantum chemical evaluation of deep eutectic solvents for the extractive desulfurization of fuel.</a> <i>ACS Sustainable Chemistry & Engineering</i>, <i>6</i>(6), pp.7525-7531.</li> <li>Bhadra, B.N., Song, J.Y., Khan, N.A. and Jhung, S.H., 2017. <a href="https://pubs.acs.org/doi/abs/10.1021/acsami.7b10336">TiO2-containing carbon derived from a metal–organic framework composite: a highly active catalyst for oxidative desulfurization.</a> <i>ACS applied materials & interfaces</i>, <i>9</i>(36), pp.31192-31202.</li> </ol> <div class="citation-actions"></div> <div></div></div> <div style="background: #f7f7f7;border: 1px solid rgba(0, 0, 0, 0.07);"> <div style="padding: 30px;"><div class="Adblock-main"> <div class="Adblock-head"> <h2>Top Experts on “<b style="color:#000;font-size:22px;">green catalysis</b>“</h2> </div> </div><div class="author-main"><div id="results_author"></div><div style="text-align: center;"><a class="register-button" href="https://catalysis.blog/expert-search" target="_blank" rel="noopener">Find experts on any field</a></div></div><div class="inside-article" style="background: none;border: none;box-shadow: none;margin-top: -70px;"> <style> .author-block { padding: 15px; 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China ", "email": "yaoyong1986@ntu.edu.cn", "slug_tail": "xin-yan" }, "gfMxK4wBWBy50K-r97ZT": { "aid": "gfMxK4wBWBy50K-r97ZT", "name": "Changbo Zhao", "citation_count": 24, "hindex": 3, "paper_count": 6, "affiliation": "Institute of Low-Dimensional Materials Genome Initiative, College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen 518060, China. ", "email": "czzhu@szu.edu.cn", "slug_tail": "changbo-zhao" }, "1tRhK4wBWBy50K-rs7aI": { "aid": "1tRhK4wBWBy50K-rs7aI", "name": "Chakrabhavi Dhananjaya Mohan", "citation_count": 43, "hindex": 2, "paper_count": 2, "affiliation": "Department of Studies in Molecular Biology, University of Mysore, Manasagangotri, Mysore 570006, India. ", "email": "cd.mohan@yahoo.com", "slug_tail": "chakrabhavi-dhananjaya-mohan" } }; //console.log(authors_data); displayResults_author(authors_data); var keywordsArray = ["Green catalysis","Ionic liquids","Metal-organic frameworks","Environmental catalysis","Oxidative desulfurization","Biodiesel production","Hybrid catalysts","Sustainable development","Catalytic performance","Recyclability"]; displayKeywordAuthors(keywordsArray); </script></div> </div> <footer class="entry-meta" aria-label="Entry meta"> <span class="cat-links"><span class="gp-icon icon-categories"><svg viewBox="0 0 512 512" aria-hidden="true" xmlns="http://www.w3.org/2000/svg" width="1em" height="1em"><path d="M0 112c0-26.51 21.49-48 48-48h110.014a48 48 0 0143.592 27.907l12.349 26.791A16 16 0 00228.486 128H464c26.51 0 48 21.49 48 48v224c0 26.51-21.49 48-48 48H48c-26.51 0-48-21.49-48-48V112z" /></svg></span><span class="screen-reader-text">Categories </span><a 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