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<!DOCTYPE html> <html lang="en" class="grade-c"> <head> <title>Distinct switching of chiral transport in the kagome metals KV3Sb5 and CsV3Sb5 | npj Quantum Materials</title> <link rel="alternate" type="application/rss+xml" href="https://www.nature.com/npjquantmats.rss"/> <link rel="preconnect" href="https://cmp.nature.com" crossorigin> <meta http-equiv="X-UA-Compatible" content="IE=edge"> <meta name="applicable-device" content="pc,mobile"> <meta name="viewport" content="width=device-width,initial-scale=1.0,maximum-scale=5,user-scalable=yes"> <meta name="360-site-verification" content="5a2dc4ab3fcb9b0393241ffbbb490480" /> <script data-test="dataLayer"> window.dataLayer = [{"content":{"category":{"contentType":"article","legacy":{"webtrendsPrimaryArticleType":"research","webtrendsSubjectTerms":"electronic-properties-and-materials","webtrendsContentCategory":null,"webtrendsContentCollection":"Ordered States in Kagome Metals","webtrendsContentGroup":"npj Quantum Materials","webtrendsContentGroupType":null,"webtrendsContentSubGroup":"Article","status":null}},"article":{"doi":"10.1038/s41535-024-00629-3"},"attributes":{"cms":null,"deliveryPlatform":"oscar","copyright":{"open":true,"legacy":{"webtrendsLicenceType":"http://creativecommons.org/licenses/by/4.0/"}}},"contentInfo":{"authors":["Chunyu Guo","Maarten R. van Delft","Martin Gutierrez-Amigo","Dong Chen","Carsten Putzke","Glenn Wagner","Mark H. 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So far, no consensus on the microscopic nature of these states has been reached as the proposals struggle to explain all their exotic physical properties. Among these, field-switchable electric magneto-chiral anisotropy (eMChA) in CsV3Sb5 provides intriguing evidence for a rewindable electronic chirality, yet the other family members have not been likewise investigated. Here, we present a comparative study of magneto-chiral transport between CsV3Sb5 and KV3Sb5. Despite their similar electronic structure, KV3Sb5 displays negligible eMChA, if any, and with no field switchability. This is in stark contrast to the non-saturating eMChA in CsV3Sb5 even in high fields up to 35 T. In light of their similar band structures, the stark difference in eMChA suggests its origin in the correlated states. 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class="c-article-header"> <header> <ul class="c-article-identifiers" data-test="article-identifier"> <li class="c-article-identifiers__item" data-test="article-category">Article</li> <li class="c-article-identifiers__item"> <a href="https://www.springernature.com/gp/open-research/about/the-fundamentals-of-open-access-and-open-research" data-track="click" data-track-action="open access" data-track-label="link" class="u-color-open-access" data-test="open-access">Open access</a> </li> <li class="c-article-identifiers__item">Published: <time datetime="2024-02-22">22 February 2024</time></li> </ul> <h1 class="c-article-title" data-test="article-title" data-article-title="">Distinct switching of chiral transport in the kagome metals KV<sub>3</sub>Sb<sub>5</sub> and CsV<sub>3</sub>Sb<sub>5</sub></h1> <ul class="c-article-author-list c-article-author-list--short" data-test="authors-list" data-component-authors-activator="authors-list"><li class="c-article-author-list__item"><a data-test="author-name" data-track="click" data-track-action="open author" data-track-label="link" href="#auth-Chunyu-Guo-Aff1" data-author-popup="auth-Chunyu-Guo-Aff1" data-author-search="Guo, Chunyu" data-corresp-id="c1">Chunyu Guo<svg width="16" height="16" focusable="false" role="img" aria-hidden="true" class="u-icon"><use xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="#icon-eds-i-mail-medium"></use></svg></a><span class="u-js-hide"> <a class="js-orcid" href="http://orcid.org/0000-0001-8339-7477"><span class="u-visually-hidden">ORCID: </span>orcid.org/0000-0001-8339-7477</a></span><sup class="u-js-hide"><a href="#Aff1">1</a></sup>, </li><li class="c-article-author-list__item"><a data-test="author-name" data-track="click" data-track-action="open author" data-track-label="link" href="#auth-Maarten_R_-Delft-Aff2-Aff3" data-author-popup="auth-Maarten_R_-Delft-Aff2-Aff3" data-author-search="van Delft, Maarten R.">Maarten R. van Delft</a><sup class="u-js-hide"><a 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Moll<svg width="16" height="16" focusable="false" role="img" aria-hidden="true" class="u-icon"><use xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="#icon-eds-i-mail-medium"></use></svg></a><span class="u-js-hide"> <a class="js-orcid" href="http://orcid.org/0000-0002-7616-5886"><span class="u-visually-hidden">ORCID: </span>orcid.org/0000-0002-7616-5886</a></span><sup class="u-js-hide"><a href="#Aff1">1</a></sup> </li></ul><button aria-expanded="false" class="c-article-author-list__button"><svg width="16" height="16" focusable="false" role="img" aria-hidden="true" class="u-icon"><use xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="#icon-eds-i-chevron-down-medium"></use></svg><span>Show authors</span></button> <p class="c-article-info-details" data-container-section="info"> <a data-test="journal-link" href="/npjquantmats" data-track="click" data-track-action="journal homepage" data-track-category="article body" data-track-label="link"><i data-test="journal-title">npj Quantum Materials</i></a> <b data-test="journal-volume"><span class="u-visually-hidden">volume</span> 9</b>, Article number: <span data-test="article-number">20</span> (<span data-test="article-publication-year">2024</span>) <a href="#citeas" class="c-article-info-details__cite-as u-hide-print" data-track="click" data-track-action="cite this article" data-track-label="link">Cite this article</a> </p> <div class="c-article-metrics-bar__wrapper u-clear-both"> <ul class="c-article-metrics-bar u-list-reset"> <li class=" c-article-metrics-bar__item" data-test="access-count"> <p class="c-article-metrics-bar__count">2375 <span class="c-article-metrics-bar__label">Accesses</span></p> </li> <li class="c-article-metrics-bar__item" data-test="citation-count"> <p class="c-article-metrics-bar__count">3 <span class="c-article-metrics-bar__label">Citations</span></p> </li> <li class="c-article-metrics-bar__item" data-test="altmetric-score"> <p class="c-article-metrics-bar__count">1 <span class="c-article-metrics-bar__label">Altmetric</span></p> </li> <li class="c-article-metrics-bar__item"> <p class="c-article-metrics-bar__details"><a href="/articles/s41535-024-00629-3/metrics" data-track="click" data-track-action="view metrics" data-track-label="link" rel="nofollow">Metrics <span class="u-visually-hidden">details</span></a></p> </li> </ul> </div> </header> <div class="u-js-hide" data-component="article-subject-links"> <h3 class="c-article__sub-heading">Subjects</h3> <ul class="c-article-subject-list"> <li class="c-article-subject-list__subject"><a href="/subjects/electronic-properties-and-materials" data-track="click" data-track-action="view subject" data-track-label="link">Electronic properties and materials</a></li> </ul> </div> </div> <div class="c-article-body"> <section aria-labelledby="Abs1" data-title="Abstract" lang="en"><div class="c-article-section" id="Abs1-section"><h2 class="c-article-section__title js-section-title js-c-reading-companion-sections-item" id="Abs1">Abstract</h2><div class="c-article-section__content" id="Abs1-content"><p>The kagome metals AV<sub>3</sub>Sb<sub>5</sub> (A = K, Rb, Cs) present an ideal sandbox to study the interrelation between multiple coexisting correlated phases such as charge order and superconductivity. So far, no consensus on the microscopic nature of these states has been reached as the proposals struggle to explain all their exotic physical properties. Among these, field-switchable electric magneto-chiral anisotropy (eMChA) in CsV<sub>3</sub>Sb<sub>5</sub> provides intriguing evidence for a rewindable electronic chirality, yet the other family members have not been likewise investigated. Here, we present a comparative study of magneto-chiral transport between CsV<sub>3</sub>Sb<sub>5</sub> and KV<sub>3</sub>Sb<sub>5</sub>. Despite their similar electronic structure, KV<sub>3</sub>Sb<sub>5</sub> displays negligible eMChA, if any, and with no field switchability. This is in stark contrast to the non-saturating eMChA in CsV<sub>3</sub>Sb<sub>5</sub> even in high fields up to 35 T. In light of their similar band structures, the stark difference in eMChA suggests its origin in the correlated states. Clearly, the V kagome nets alone are not sufficient to describe the physics and the interactions with their environment are crucial in determining the nature of their low-temperature state.</p></div></div></section> <section aria-labelledby="inline-recommendations" data-title="Inline Recommendations" class="c-article-recommendations" data-track-component="inline-recommendations"> <h3 class="c-article-recommendations-title" id="inline-recommendations">Similar content being viewed by others</h3> <div class="c-article-recommendations-list"> <div class="c-article-recommendations-list__item"> <article class="c-article-recommendations-card" itemscope itemtype="http://schema.org/ScholarlyArticle"> <div class="c-article-recommendations-card__img"><img src="https://media.springernature.com/w215h120/springer-static/image/art%3A10.1038%2Fs41586-022-05127-9/MediaObjects/41586_2022_5127_Fig1_HTML.png" loading="lazy" alt=""></div> <div class="c-article-recommendations-card__main"> <h3 class="c-article-recommendations-card__heading" itemprop="name headline"> <a class="c-article-recommendations-card__link" itemprop="url" href="https://www.nature.com/articles/s41586-022-05127-9?fromPaywallRec=false" data-track="select_recommendations_1" data-track-context="inline recommendations" data-track-action="click recommendations inline - 1" data-track-label="10.1038/s41586-022-05127-9">Switchable chiral transport in charge-ordered kagome metal CsV<sub>3</sub>Sb<sub>5</sub> </a> </h3> <div class="c-article-meta-recommendations" data-test="recommendation-info"> <span class="c-article-meta-recommendations__item-type">Article</span> <span class="c-article-meta-recommendations__access-type">Open access</span> <span class="c-article-meta-recommendations__date">12 October 2022</span> </div> </div> </article> </div> <div class="c-article-recommendations-list__item"> <article class="c-article-recommendations-card" itemscope itemtype="http://schema.org/ScholarlyArticle"> <div class="c-article-recommendations-card__img"><img src="https://media.springernature.com/w215h120/springer-static/image/art%3A10.1038%2Fs42005-022-01011-0/MediaObjects/42005_2022_1011_Fig1_HTML.png" loading="lazy" alt=""></div> <div class="c-article-recommendations-card__main"> <h3 class="c-article-recommendations-card__heading" itemprop="name headline"> <a class="c-article-recommendations-card__link" itemprop="url" href="https://www.nature.com/articles/s42005-022-01011-0?fromPaywallRec=false" data-track="select_recommendations_2" data-track-context="inline recommendations" data-track-action="click recommendations inline - 2" data-track-label="10.1038/s42005-022-01011-0">Two types of charge order with distinct interplay with superconductivity in the kagome material CsV<sub>3</sub>Sb<sub>5</sub> </a> </h3> <div class="c-article-meta-recommendations" data-test="recommendation-info"> <span class="c-article-meta-recommendations__item-type">Article</span> <span class="c-article-meta-recommendations__access-type">Open access</span> <span class="c-article-meta-recommendations__date">21 September 2022</span> </div> </div> </article> </div> <div class="c-article-recommendations-list__item"> <article class="c-article-recommendations-card" itemscope itemtype="http://schema.org/ScholarlyArticle"> <div class="c-article-recommendations-card__img"><img src="https://media.springernature.com/w215h120/springer-static/image/art%3A10.1038%2Fs41567-023-02374-z/MediaObjects/41567_2023_2374_Fig1_HTML.png" loading="lazy" alt=""></div> <div class="c-article-recommendations-card__main"> <h3 class="c-article-recommendations-card__heading" itemprop="name headline"> <a class="c-article-recommendations-card__link" itemprop="url" href="https://www.nature.com/articles/s41567-023-02374-z?fromPaywallRec=false" data-track="select_recommendations_3" data-track-context="inline recommendations" data-track-action="click recommendations inline - 3" data-track-label="10.1038/s41567-023-02374-z">Correlated order at the tipping point in the kagome metal CsV<sub>3</sub>Sb<sub>5</sub> </a> </h3> <div class="c-article-meta-recommendations" data-test="recommendation-info"> <span class="c-article-meta-recommendations__item-type">Article</span> <span class="c-article-meta-recommendations__access-type">Open access</span> <span class="c-article-meta-recommendations__date">31 January 2024</span> </div> </div> </article> </div> </div> </section> <script> window.dataLayer = window.dataLayer || []; window.dataLayer.push({ recommendations: { recommender: 'semantic', model: 'specter', policy_id: 'NA', timestamp: 1734193094, embedded_user: 'null' } }); </script> <div class="main-content"> <section data-title="Introduction"><div class="c-article-section" id="Sec1-section"><h2 class="c-article-section__title js-section-title js-c-reading-companion-sections-item" id="Sec1">Introduction</h2><div class="c-article-section__content" id="Sec1-content"><p>Metals hosting kagome nets have recently proven to be a fruitful avenue to explore correlated topological materials<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Yin, J.-X., Lian, B. & Hasan, M. Z. Topological kagome magnets and superconductors. Nature 612, 647 (2022)." href="#ref-CR1" id="ref-link-section-d105397969e741">1</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Syôzi, I. Statistics of kagomé lattice. Prog. Theor. Phys. 6, 306 (1951)." href="#ref-CR2" id="ref-link-section-d105397969e741_1">2</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Kang, M. et al. Topological flat bands in frustrated kagome lattice CoSn. Nat. Commun. 11, 4004 (2020)." href="#ref-CR3" id="ref-link-section-d105397969e741_2">3</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Kang, M. et al. Dirac fermions and flat bands in the ideal kagome metal FeSn. Nat. Mat. 19, 163 (2020)." href="#ref-CR4" id="ref-link-section-d105397969e741_3">4</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Yin, J.-X. et al. Quantum-limit Chern topological magnetism in TbMn6Sn6. Nature 583, 533 (2020)." href="#ref-CR5" id="ref-link-section-d105397969e741_4">5</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Yin, J.-X. et al. Giant and anisotropic many-body spin–orbit tunability in a strongly correlated kagome magnet. Nature 562, 91 (2018)." href="#ref-CR6" id="ref-link-section-d105397969e741_5">6</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Ye, L. et al. Massive Dirac fermions in a ferromagnetic kagome metal. Nature 555, 638 (2018)." href="#ref-CR7" id="ref-link-section-d105397969e741_6">7</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Howard, S. et al. Evidence for one-dimensional chiral edge states in a magnetic Weyl semimetal Co3Sn2S2. Nat. Commun. 12, 4269 (2021)." href="#ref-CR8" id="ref-link-section-d105397969e741_7">8</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 9" title="Ortiz, B. R. et al. New kagome prototype materials: discovery of KV3Sb5, Rb3Sb5, and CsV3Sb5. Phys. Rev. Mater. 3, 094407 (2019)." href="/articles/s41535-024-00629-3#ref-CR9" id="ref-link-section-d105397969e744">9</a></sup>. Their orbital and magnetic frustration generically gives rise to Dirac points and potentially flat bands, which are associated with non-trivial behavior such as giant intrinsic anomalous Hall effect<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 5" title="Yin, J.-X. et al. Quantum-limit Chern topological magnetism in TbMn6Sn6. Nature 583, 533 (2020)." href="/articles/s41535-024-00629-3#ref-CR5" id="ref-link-section-d105397969e748">5</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 7" title="Ye, L. et al. Massive Dirac fermions in a ferromagnetic kagome metal. Nature 555, 638 (2018)." href="/articles/s41535-024-00629-3#ref-CR7" id="ref-link-section-d105397969e751">7</a></sup> and topologically protected boundary states<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 5" title="Yin, J.-X. et al. Quantum-limit Chern topological magnetism in TbMn6Sn6. Nature 583, 533 (2020)." href="/articles/s41535-024-00629-3#ref-CR5" id="ref-link-section-d105397969e755">5</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 8" title="Howard, S. et al. Evidence for one-dimensional chiral edge states in a magnetic Weyl semimetal Co3Sn2S2. Nat. Commun. 12, 4269 (2021)." href="/articles/s41535-024-00629-3#ref-CR8" id="ref-link-section-d105397969e758">8</a></sup>. The recently reported family AV<sub>3</sub>Sb<sub>5</sub> (A = K, Rb, Cs) presents an intriguing example of electronic instabilities on a kagome lattice driven by strong correlations<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Ortiz, B. R. et al. New kagome prototype materials: discovery of KV3Sb5, Rb3Sb5, and CsV3Sb5. Phys. Rev. Mater. 3, 094407 (2019)." href="#ref-CR9" id="ref-link-section-d105397969e767">9</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Ortiz, B. R. et al. CsV3Sb5: A Z2 topological kagome metal with a superconducting ground state. Phys. Rev. Lett. 125, 247002 (2020)." href="#ref-CR10" id="ref-link-section-d105397969e767_1">10</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Kang, M. et al. Twofold van Hove singularity and origin of charge order in topological kagome superconductor CsV3Sb5. Nat. Phys. 18, 301 (2022)." href="#ref-CR11" id="ref-link-section-d105397969e767_2">11</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Denner, M. M., Thomale, R. & Neupert, T. Analysis of charge order in the kagome metal AV3Sb5 (A = K, Rb, Cs). Phys. Rev. Lett. 127, 217601 (2021)." href="#ref-CR12" id="ref-link-section-d105397969e767_3">12</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Neupert, T., Denner, M. M., Yin, J.-X., Thomale, R. & Hasan, M. Z. Charge order and superconductivity in kagome materials. Nat. Phys. 18, 137 (2022)." href="#ref-CR13" id="ref-link-section-d105397969e767_4">13</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 14" title="Guo, C. et al. Correlated order at the tipping point in the kagome metal CsV3Sb5. Nat. Phys. https://www.nature.com/articles/s41567-023-02374-z (2023)." href="/articles/s41535-024-00629-3#ref-CR14" id="ref-link-section-d105397969e770">14</a></sup>. They all jointly undergo a charge order transition distorting the kagome lattice at <i>T</i><sub><i>C</i><i>D</i><i>W</i></sub> ~ 100 K. The main open question in this field concerns the types of broken symmetries within that ordered state, most prominently the fate of time-reversal and mirror symmetries. While a mirror symmetric structure appears in X-Ray diffraction<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 15" title="Chen, Q., Chen, D., Schnelle, W., Felser, C. & Gaulin, B. D. Charge density wave order and fluctuations above TCDW and below superconducting Tc in the kagome metal CsV3Sb5. Phys. Rev. Lett. 129, 056401 (2022)." href="/articles/s41535-024-00629-3#ref-CR15" id="ref-link-section-d105397969e784">15</a></sup>, experimental evidence for broken symmetries mounts, including electronic C2 anisotropy<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Xiang, Y. et al. Twofold symmetry of c-axis resistivity in topological kagome superconductor CsV3Sb5 with in-plane rotating magnetic field. Nat. Commun. 12, 6727 (2021)." href="#ref-CR16" id="ref-link-section-d105397969e788">16</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Nie, L. et al. Charge-density-wave-driven electronic nematicity in a kagome superconductor. Nature 604, 59 (2022)." href="#ref-CR17" id="ref-link-section-d105397969e788_1">17</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 18" title="Wulferding, D. et al. Emergent nematicity and intrinsic versus extrinsic electronic scattering processes in the kagome metal CsV3Sb5. Phys. Rev. Res. 4, 023215 (2022)." href="/articles/s41535-024-00629-3#ref-CR18" id="ref-link-section-d105397969e791">18</a></sup>, a chiral charge-density-wave state observed in STM experiments<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 19" title="Zhao, H. et al. Cascade of correlated electron states in a kagome superconductor CsV3Sb5. Nature 599, 216 (2021)." href="/articles/s41535-024-00629-3#ref-CR19" id="ref-link-section-d105397969e795">19</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 20" title="Jiang, Y.-X. et al. Unconventional chiral charge order in kagome superconductor KV3Sb5. Nat. Mat. 20, 1353 (2021)." href="/articles/s41535-024-00629-3#ref-CR20" id="ref-link-section-d105397969e798">20</a></sup> and three-state nematicity in the optical Kerr effect<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 21" title="Xu, Y. et al. Three-state nematicity and magneto-optical Kerr effect in the charge density waves in kagome superconductors. Nat. Phys. 18, 1470 (2022)." href="/articles/s41535-024-00629-3#ref-CR21" id="ref-link-section-d105397969e803">21</a></sup>. A further direct consequence of broken mirror symmetries in electric conductors is a current-direction dependent voltage response called electrical magneto-chiral anisotropy (eMChA)<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Rikken, G. L. J. A. & Avarvari, N. Strong electrical magnetochiral anisotropy in Tellurium. Phys. Rev. B 99, 245153 (2019)." href="#ref-CR22" id="ref-link-section-d105397969e807">22</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Rikken, G. L. J. A., Fölling, J. & Wyder, P. Electrical magnetochiral anisotropy. Phys. Rev. Lett. 87, 236602 (2001)." href="#ref-CR23" id="ref-link-section-d105397969e807_1">23</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Wei, J. et al. Magneto-chiral anisotropy in charge transport through single-walled carbon nanotubes. Phys. Rev. Lett. 95, 256601 (2005)." href="#ref-CR24" id="ref-link-section-d105397969e807_2">24</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Pop, F., Auban-Senzier, P., Canadell, E., Rikken, G. L. J. A. & Avarvari, N. Electrical magnetochiral anisotropy in a bulk chiral molecular conductor. Nat. Commun. 5, 3757 (2014)." href="#ref-CR25" id="ref-link-section-d105397969e807_3">25</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Aoki, R., Kousaka, Y. & Togawa, Y. Anomalous nonreciprocal electrical transport on chiral magnetic order. Phys. Rev. Lett. 122, 057206 (2019)." href="#ref-CR26" id="ref-link-section-d105397969e807_4">26</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 27" title="Yokouchi, T. et al. Electrical magnetochiral effect induced by chiral spin fluctuations. Nat. Commun. 8, 866 (2017)." href="/articles/s41535-024-00629-3#ref-CR27" id="ref-link-section-d105397969e810">27</a></sup>. This has been found recently in CsV<sub>3</sub>Sb<sub>5</sub>, which further demonstrates an electronic chirality within the charge order<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 28" title="Guo, C. et al. Switchable chiral transport in charge-ordered kagome metal CsV3Sb5. Nature 611, 461 (2022)." href="/articles/s41535-024-00629-3#ref-CR28" id="ref-link-section-d105397969e818">28</a></sup>. The direction of chiral transport is uniquely switchable by a magnetic field, which points to its origin in a mirror-symmetry-breaking correlated state rather than the common structural chirality found in diodes. Clearly, further experiments probing this dichotomy between electronic and structural chirality are called for.</p><p>A first key step concerns the generality of magneto-chiral transport among the AV<sub>3</sub>Sb<sub>5</sub> family of compounds. As an iso-structural analog to CsV<sub>3</sub>Sb<sub>5</sub>, KV<sub>3</sub>Sb<sub>5</sub> displays a similar charge order formation at high temperature as well as a superconducting ground state<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 29" title="Ortiz, B. R. et al. Superconductivity in the Z2 kagome metal KV3Sb5. Phys. Rev. Mater. 5, 034801 (2021)." href="/articles/s41535-024-00629-3#ref-CR29" id="ref-link-section-d105397969e838">29</a></sup>. Based on this similarity, its electronic chirality has also been explored. A rotational symmetry breaking chiral charge order is consistently observed yet contradictory conclusions have been made about whether its chirality can be controlled by the magnetic field<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 20" title="Jiang, Y.-X. et al. Unconventional chiral charge order in kagome superconductor KV3Sb5. Nat. Mat. 20, 1353 (2021)." href="/articles/s41535-024-00629-3#ref-CR20" id="ref-link-section-d105397969e842">20</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 30" title="Li, H. et al. Rotation symmetry breaking in the normal state of a kagome superconductor KV3Sb5. Nat. Phys. 18, 265 (2022)." href="/articles/s41535-024-00629-3#ref-CR30" id="ref-link-section-d105397969e845">30</a></sup>. Here, we examine the magneto-chiral transport properties of KV<sub>3</sub>Sb<sub>5</sub> with a side-by-side comparison to CsV<sub>3</sub>Sb<sub>5</sub>, offering a great opportunity for exploring the critical factors for the magneto-chiral transport among the AV<sub>3</sub>Sb<sub>5</sub> series of compounds and beyond.</p></div></div></section><section data-title="Results"><div class="c-article-section" id="Sec2-section"><h2 class="c-article-section__title js-section-title js-c-reading-companion-sections-item" id="Sec2">Results</h2><div class="c-article-section__content" id="Sec2-content"><h3 class="c-article__sub-heading" id="Sec3">Transport properties and electronic fermiology</h3><p>Experiments probing eMChA in CsV<sub>3</sub>Sb<sub>5</sub> have shown it to be extremely susceptible to external perturbations such as strain or magnetic field<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 14" title="Guo, C. et al. Correlated order at the tipping point in the kagome metal CsV3Sb5. Nat. Phys. https://www.nature.com/articles/s41567-023-02374-z (2023)." href="/articles/s41535-024-00629-3#ref-CR14" id="ref-link-section-d105397969e878">14</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 28" title="Guo, C. et al. Switchable chiral transport in charge-ordered kagome metal CsV3Sb5. Nature 611, 461 (2022)." href="/articles/s41535-024-00629-3#ref-CR28" id="ref-link-section-d105397969e881">28</a></sup>. A quantitative comparison of different AV<sub>3</sub>Sb<sub>5</sub> compounds requires to significantly reduce the uniaxial strain due to thermal contraction difference. We, therefore, decouple the crystalline sample mechanically as much as possible from the substrate by fabricating lithographic springs that act as ultra-soft mechanical support and electric contacts<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 28" title="Guo, C. et al. Switchable chiral transport in charge-ordered kagome metal CsV3Sb5. Nature 611, 461 (2022)." href="/articles/s41535-024-00629-3#ref-CR28" id="ref-link-section-d105397969e890">28</a></sup>. The central crystalline microstructure has been carved from a single crystal using focused-ion-beam (FIB) milling (Fig. <a data-track="click" data-track-label="link" data-track-action="figure anchor" href="/articles/s41535-024-00629-3#Fig1">1</a>). It features a Hall-bar device with six electric terminals. One of the current leads is fixed directly to the Si-substrate via FIB-assisted Pt-deposition to reduce the torque distortion at high magnetic field, and the other five electric contacts are supported only by soft gold-coated membrane springs (100 nm SiN<sub><i>x</i></sub> and 150 nm Au). This has been previously shown to reduce the forces on similar microstructures to below 50 bar<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 28" title="Guo, C. et al. Switchable chiral transport in charge-ordered kagome metal CsV3Sb5. Nature 611, 461 (2022)." href="/articles/s41535-024-00629-3#ref-CR28" id="ref-link-section-d105397969e901">28</a></sup>, a key prerequisite to observe eMChA in them.</p><div class="c-article-section__figure js-c-reading-companion-figures-item" data-test="figure" data-container-section="figure" id="figure-1" data-title="Temperature-dependence of resistivity."><figure><figcaption><b id="Fig1" class="c-article-section__figure-caption" data-test="figure-caption-text">Fig. 1: Temperature-dependence of resistivity.</b></figcaption><div class="c-article-section__figure-content"><div class="c-article-section__figure-item"><a class="c-article-section__figure-link" data-test="img-link" data-track="click" data-track-label="image" data-track-action="view figure" href="/articles/s41535-024-00629-3/figures/1" rel="nofollow"><picture><source type="image/webp" srcset="//media.springernature.com/lw685/springer-static/image/art%3A10.1038%2Fs41535-024-00629-3/MediaObjects/41535_2024_629_Fig1_HTML.png?as=webp"><img aria-describedby="Fig1" src="//media.springernature.com/lw685/springer-static/image/art%3A10.1038%2Fs41535-024-00629-3/MediaObjects/41535_2024_629_Fig1_HTML.png" alt="figure 1" loading="lazy" width="685" height="466"></picture></a></div><div class="c-article-section__figure-description" data-test="bottom-caption" id="figure-1-desc"><p><b>a</b> Temperature dependence of electric resistivity for CsV<sub>3</sub>Sb<sub>5</sub> and KV<sub>3</sub>Sb<sub>5</sub>. The inset displays the membrane-based microstructure, which features a Hall-bar geometry with long-axis along the c-direction, the legnth of scale bar stands for 20 μm. <b>b</b> Both materials display a clear resistivity jump due to the charge-density-wave (CDW) transition. The transition temperature <i>T</i><sub><i>C</i><i>D</i><i>W</i></sub> is 94 K and 76 K for CsV<sub>3</sub>Sb<sub>5</sub> and KV<sub>3</sub>Sb<sub>5,</sub> respectively. <b>c</b> Low temperature resistivity for both Cs and K compounds. No superconducting transition is found in KV<sub>3</sub>Sb<sub>5</sub> down to <i>T</i> = 2 K, and its residual resistivity is larger compared to CsV<sub>3</sub>Sb<sub>5</sub>.</p></div></div><div class="u-text-right u-hide-print"><a class="c-article__pill-button" data-test="article-link" data-track="click" data-track-label="button" data-track-action="view figure" href="/articles/s41535-024-00629-3/figures/1" data-track-dest="link:Figure1 Full size image" aria-label="Full size image figure 1" rel="nofollow"><span>Full size image</span><svg width="16" height="16" focusable="false" role="img" aria-hidden="true" class="u-icon"><use xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="#icon-eds-i-chevron-right-small"></use></svg></a></div></figure></div><p>With these low-strain devices, we firstly explore the electronic transport properties of both compounds within the linear response regime, which sets the basis for non-linear chiral transport. A clear anomaly in the temperature dependence of resistivity reveals the CDW transition temperatures at 94 K and 76 K for CsV<sub>3</sub>Sb<sub>5</sub> and KV<sub>3</sub>Sb<sub>5</sub> respectively, consistent with previous reports<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 9" title="Ortiz, B. R. et al. New kagome prototype materials: discovery of KV3Sb5, Rb3Sb5, and CsV3Sb5. Phys. Rev. Mater. 3, 094407 (2019)." href="/articles/s41535-024-00629-3#ref-CR9" id="ref-link-section-d105397969e983">9</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 10" title="Ortiz, B. R. et al. CsV3Sb5: A Z2 topological kagome metal with a superconducting ground state. Phys. Rev. Lett. 125, 247002 (2020)." href="/articles/s41535-024-00629-3#ref-CR10" id="ref-link-section-d105397969e986">10</a></sup> (Fig. <a data-track="click" data-track-label="link" data-track-action="figure anchor" href="/articles/s41535-024-00629-3#Fig1">1)</a>. The smaller lattice constant in KV<sub>3</sub>Sb<sub>5</sub> compared to CsV<sub>3</sub>Sb<sub>5</sub> could be considered as a positive chemical pressure effect, and this decrease of <i>T</i><sub><i>C</i><i>D</i><i>W</i></sub> indeed matches expectations from hydrostatic pressure experiments<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Du, F. et al. Pressure-induced double superconducting domes and charge instability in the kagome metal KV3Sb5. Phys. Rev. B 103, L220504 (2021)." href="#ref-CR31" id="ref-link-section-d105397969e1013">31</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Zhang, Z. et al. Pressure-induced reemergence of superconductivity in the topological kagome metal CsV3Sb5. Phys. Rev. B 103, 224513 (2021)." href="#ref-CR32" id="ref-link-section-d105397969e1013_1">32</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 33" title="Wang, Q. et al. Charge density wave orders and enhanced superconductivity under pressure in the kagome metal CsV3Sb5. Adv. Mat. 33, 2102813 (2021)." href="/articles/s41535-024-00629-3#ref-CR33" id="ref-link-section-d105397969e1016">33</a></sup>. However, the reported superconducting transition is suppressed down to <i>T</i><sub><i>c</i></sub> ≈ 0.7K in KV<sub>3</sub>Sb<sub>5</sub>, which is significantly lower than simple hydrostatic pressure arguments may explain<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 29" title="Ortiz, B. R. et al. Superconductivity in the Z2 kagome metal KV3Sb5. Phys. Rev. Mater. 5, 034801 (2021)." href="/articles/s41535-024-00629-3#ref-CR29" id="ref-link-section-d105397969e1031">29</a></sup>. Meanwhile, it displays a broader charge density wave transition with a less pronounced jump of resistivity, as well as a moderately larger residual resistivity at base temperature. It has been reported that <i>T</i><sub><i>c</i></sub> and K vacancies are closely related in this compound<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 29" title="Ortiz, B. R. et al. Superconductivity in the Z2 kagome metal KV3Sb5. Phys. Rev. Mater. 5, 034801 (2021)." href="/articles/s41535-024-00629-3#ref-CR29" id="ref-link-section-d105397969e1041">29</a></sup>, which implies lattice defects as a possible origin for the lower <i>T</i><sub><i>c</i></sub> and the increased residual resistivity in KV<sub>3</sub>Sb<sub>5</sub>.</p><p>To explore more quantitatively the differences between KV<sub>3</sub>Sb<sub>5</sub> and CsV<sub>3</sub>Sb<sub>5</sub>, we turn towards their electronic band structure studied both theoretically and experimentally. Ab-initio band structure calculations<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Giannozzi, P. et al. Advanced capabilities for materials modelling with QUANTUM ESPRESSO. J. Phys. Condens. Mat. 29, 465901 (2017)." href="#ref-CR34" id="ref-link-section-d105397969e1067">34</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Perdew, J. P., Burke, K. & Ernzerhof, M. Generalized gradient approximation made simple. Phys. Rev. Lett. 77, 3865 (1996)." href="#ref-CR35" id="ref-link-section-d105397969e1067_1">35</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 36" title="Dal Corso, A. Pseudopotentials periodic table: from H to Pu. Comp. Mat. Sci. 95, 337 (2014)." href="/articles/s41535-024-00629-3#ref-CR36" id="ref-link-section-d105397969e1070">36</a></sup> have been performed without taking the charge-order formation into account (Fig. <a data-track="click" data-track-label="link" data-track-action="figure anchor" href="/articles/s41535-024-00629-3#Fig2">2</a>). Since both KV<sub>3</sub>Sb<sub>5</sub> and CsV<sub>3</sub>Sb<sub>5</sub> crystallize in the P6/mmm space group with the kagome net formed by the V-atoms, it is not surprising that they share a clear similarity and slightly differ due to the unit cell change and the opening of the gap at the M point. This gap results in a reconstruction of the M pockets, as depicted in the Fermi Surface insets of Fig. <a data-track="click" data-track-label="link" data-track-action="figure anchor" href="/articles/s41535-024-00629-3#Fig2">2</a>. To confirm this similarity in the band structures, we have also examined its validity experimentally. The fermiology of KV<sub>3</sub>Sb<sub>5</sub> has rarely been studied in detail<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 37" title="Shrestha, K. et al. High quantum oscillation frequencies and nontrivial topology in kagome superconductor KV3Sb5 probed by torque magnetometry up to 45 T. Phys. Rev. B 107, 155128 (2023)." href="/articles/s41535-024-00629-3#ref-CR37" id="ref-link-section-d105397969e1094">37</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 38" title="Yang, S.-Y. et al. Giant, unconventional anomalous Hall effect in the metallic frustrated magnet candidate, KV3Sb5. Sci. Adv. 6, eabb6003 (2020)." href="/articles/s41535-024-00629-3#ref-CR38" id="ref-link-section-d105397969e1097">38</a></sup>, unlike CsV<sub>3</sub>Sb<sub>5</sub><sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Fu, Y. et al. Quantum transport evidence of topological band structures of kagome superconductor CsV3Sb5. Phys. Rev. Lett. 127, 207002 (2021)." href="#ref-CR39" id="ref-link-section-d105397969e1104">39</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Chen, D. et al. Anomalous thermoelectric effects and quantum oscillations in the kagome metal CsV3Sb5. Phys. Rev. B 105, L201109 (2022)." href="#ref-CR40" id="ref-link-section-d105397969e1104_1">40</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Zhang, W. et al. Emergence of large quantum oscillation frequencies in thin flakes of the kagome superconductor CsV3Sb5. Phys. Rev. B 106, 195103 (2022)." href="#ref-CR41" id="ref-link-section-d105397969e1104_2">41</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Ortiz, B. R. et al. Fermi surface mapping and the nature of charge density wave order in the kagome superconductor CsV3Sb5. Phys. Rev. X 11, 041030 (2021)." href="#ref-CR42" id="ref-link-section-d105397969e1104_3">42</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Chapai, R. et al. Magnetic breakdown and topology in the kagome superconductor CsV3Sb5 under high magnetic field. Phys. Rev. Lett. 130, 126401 (2023)." href="#ref-CR43" id="ref-link-section-d105397969e1104_4">43</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Broyles, C. et al. Effect of the interlayer ordering on the Fermi surface of kagome superconductor CsV3Sb5 revealed by quantum oscillations. Phys. Rev. Lett. 129, 157001 (2022)." href="#ref-CR44" id="ref-link-section-d105397969e1104_5">44</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 45" title="Huang, X. et al. Three-dimensional Fermi surfaces from charge order in layered CsV3Sb5. Phys. Rev. B 106, 064510 (2022)." href="/articles/s41535-024-00629-3#ref-CR45" id="ref-link-section-d105397969e1107">45</a></sup>. To directly contrast the Fermi surfaces of these two compounds, we have performed magneto-transport measurements of the membrane-based device elongated along the c-axis up to 35 T with a rotation of field direction from c to a’-axis for both materials (Supplementary Fig. <a data-track="click" data-track-label="link" data-track-action="supplementary material anchor" href="/articles/s41535-024-00629-3#MOESM1">S1</a>). A third-order polynomial fit for the field-dependence of magnetoresistance allows us to extract the Shubnikov-de-Haas oscillations.</p><div class="c-article-section__figure js-c-reading-companion-figures-item" data-test="figure" data-container-section="figure" id="figure-2" data-title="Electronic structure and fermiology."><figure><figcaption><b id="Fig2" class="c-article-section__figure-caption" data-test="figure-caption-text">Fig. 2: Electronic structure and fermiology.</b></figcaption><div class="c-article-section__figure-content"><div class="c-article-section__figure-item"><a class="c-article-section__figure-link" data-test="img-link" data-track="click" data-track-label="image" data-track-action="view figure" href="/articles/s41535-024-00629-3/figures/2" rel="nofollow"><picture><source type="image/webp" srcset="//media.springernature.com/lw685/springer-static/image/art%3A10.1038%2Fs41535-024-00629-3/MediaObjects/41535_2024_629_Fig2_HTML.png?as=webp"><img aria-describedby="Fig2" src="//media.springernature.com/lw685/springer-static/image/art%3A10.1038%2Fs41535-024-00629-3/MediaObjects/41535_2024_629_Fig2_HTML.png" alt="figure 2" loading="lazy" width="685" height="274"></picture></a></div><div class="c-article-section__figure-description" data-test="bottom-caption" id="figure-2-desc"><p><b>a</b> Electronic band structure of both CsV<sub>3</sub>Sb<sub>5</sub> and KV<sub>3</sub>Sb<sub>5</sub> calculated by density-functional theory (DFT). <b>b</b> Angular dependence of quantum oscillation frequency. A side-by-side comparison between CsV<sub>3</sub>Sb<sub>5</sub> and KV<sub>3</sub>Sb<sub>5</sub> suggest a qualitative similarity in fermiology, as also demonstrated by the DFT calculation displayed in the inset.</p></div></div><div class="u-text-right u-hide-print"><a class="c-article__pill-button" data-test="article-link" data-track="click" data-track-label="button" data-track-action="view figure" href="/articles/s41535-024-00629-3/figures/2" data-track-dest="link:Figure2 Full size image" aria-label="Full size image figure 2" rel="nofollow"><span>Full size image</span><svg width="16" height="16" focusable="false" role="img" aria-hidden="true" class="u-icon"><use xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="#icon-eds-i-chevron-right-small"></use></svg></a></div></figure></div><p>The quantum oscillation frequencies disperse in lockstep for both compounds, directly evidencing the similarity of their electronic structures. Multiple orbits are detected that show 2D and 3D characteristics. Several low frequency oscillations below 500 T consistently appear with field applied almost within the kagome plane (Supplementary Fig. <a data-track="click" data-track-label="link" data-track-action="supplementary material anchor" href="/articles/s41535-024-00629-3#MOESM1">S2)</a>, demonstrating the 3D nature of the corresponding Fermi surfaces, consistent with previous reports<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 45" title="Huang, X. et al. Three-dimensional Fermi surfaces from charge order in layered CsV3Sb5. Phys. Rev. B 106, 064510 (2022)." href="/articles/s41535-024-00629-3#ref-CR45" id="ref-link-section-d105397969e1163">45</a></sup>. The main high frequencies observed can be divided into two branches around 1700 T and 700 T. These frequencies are comparable with the Fermi surfaces located around A and H points obtained from ab-initio calculations<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 42" title="Ortiz, B. R. et al. Fermi surface mapping and the nature of charge density wave order in the kagome superconductor CsV3Sb5. Phys. Rev. X 11, 041030 (2021)." href="/articles/s41535-024-00629-3#ref-CR42" id="ref-link-section-d105397969e1167">42</a></sup>, while the Brillouin-zone-sized pocket around Γ point is not observed in our measurements. The angular dependences of the frequencies follow nicely the general description of a 2D Fermi surface (<i>F</i> <span class="stix">∝</span> 1/cos(<i>θ</i>)), suggesting the quasi-2D nature of these Fermi surfaces. The similarity in fermiology between these compounds results in the consistent electronic properties among the AV<sub>3</sub>Sb<sub>5</sub> family, such as the previously proposed orbital loop current and correlated charge order. In light of this similarity, the striking difference in eMChA between the compounds is puzzling, as will be shown next.</p><h3 class="c-article__sub-heading" id="Sec4">Significant suppression of eMChA in KV<sub>3</sub>Sb<sub>5</sub> </h3><p>The electrical magneto-chiral anisotropy, eMChA, can occur in the absence of mirror symmetries in the system. It results in a polarity-dependent resistance value as <i>R</i>(<b><i>B</i></b>, <b><i>I</i></b>) ≠ <i>R</i>(<b><i>B</i></b>, − <b><i>I</i></b>), which is usually detected by the second-harmonic voltage generation with low-frequency AC currents<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Rikken, G. L. J. A. & Avarvari, N. Strong electrical magnetochiral anisotropy in Tellurium. Phys. Rev. B 99, 245153 (2019)." href="#ref-CR22" id="ref-link-section-d105397969e1214">22</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Rikken, G. L. J. A., Fölling, J. & Wyder, P. Electrical magnetochiral anisotropy. Phys. Rev. Lett. 87, 236602 (2001)." href="#ref-CR23" id="ref-link-section-d105397969e1214_1">23</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Wei, J. et al. Magneto-chiral anisotropy in charge transport through single-walled carbon nanotubes. Phys. Rev. Lett. 95, 256601 (2005)." href="#ref-CR24" id="ref-link-section-d105397969e1214_2">24</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Pop, F., Auban-Senzier, P., Canadell, E., Rikken, G. L. J. A. & Avarvari, N. Electrical magnetochiral anisotropy in a bulk chiral molecular conductor. Nat. Commun. 5, 3757 (2014)." href="#ref-CR25" id="ref-link-section-d105397969e1214_3">25</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" title="Aoki, R., Kousaka, Y. & Togawa, Y. Anomalous nonreciprocal electrical transport on chiral magnetic order. Phys. Rev. Lett. 122, 057206 (2019)." href="#ref-CR26" id="ref-link-section-d105397969e1214_4">26</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 27" title="Yokouchi, T. et al. Electrical magnetochiral effect induced by chiral spin fluctuations. Nat. Commun. 8, 866 (2017)." href="/articles/s41535-024-00629-3#ref-CR27" id="ref-link-section-d105397969e1217">27</a></sup>. Recently, eMChA with a field-switchable forward direction has been reported<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 28" title="Guo, C. et al. Switchable chiral transport in charge-ordered kagome metal CsV3Sb5. Nature 611, 461 (2022)." href="/articles/s41535-024-00629-3#ref-CR28" id="ref-link-section-d105397969e1221">28</a></sup>, pointing to field-induced mirror symmetry breaking of the correlated order and setting the system apart from other structurally chiral conductors, in which the handedness is firmly imprinted during materials synthesis. Indeed, the sign of eMChA is controlled by a small out-of-plane field component <i>B</i><sub><i>c</i></sub>, demonstrating a field-switchable electronic chirality.</p><p>To further explore and compare the electronic chirality in CsV<sub>3</sub>Sb<sub>5</sub> and KV<sub>3</sub>Sb<sub>5</sub>, we have performed measurements of second harmonic voltage generation due to eMChA for both compounds up to 35 T (Fig. <a data-track="click" data-track-label="link" data-track-action="figure anchor" href="/articles/s41535-024-00629-3#Fig3">3</a>). A non-saturating, field-asymmetric <i>V</i><sub>2<i>ω</i></sub> signal is observed in CsV<sub>3</sub>Sb<sub>5</sub>, which increases beyond 4 μV at <i>B</i> = 35 T. Due to the equally non-saturating magnetoresistance, the second harmonic voltage displays a nearly <i>B</i><sup>3</sup> dependence throughout the entire field window, suggesting the electronic chirality is not affected by the in-plane magnetic field. As the lowest-order coupling between magnetic field and current, the chiral contribution to electrical conductance Δ<i>σ</i> is proportional to <span class="mathjax-tex">${V}_{2\omega }\,/\,{V}_{\omega }^{2}$</span> and displays a linear field-dependence. This naturally explains the nearly <i>B</i><sup>3</sup>-dependence of <i>V</i><sub>2<i>ω</i></sub><sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 28" title="Guo, C. et al. Switchable chiral transport in charge-ordered kagome metal CsV3Sb5. Nature 611, 461 (2022)." href="/articles/s41535-024-00629-3#ref-CR28" id="ref-link-section-d105397969e1335">28</a></sup>. Most importantly, the sign of Δ<i>σ</i> is reversed when the magnetic field rotates across the kagome plane, suggesting a direct correspondence between the handedness of electronic chirality and the direction of the out-of-plane field component, which is consistent with the previously constructed phenomenological model<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 28" title="Guo, C. et al. Switchable chiral transport in charge-ordered kagome metal CsV3Sb5. Nature 611, 461 (2022)." href="/articles/s41535-024-00629-3#ref-CR28" id="ref-link-section-d105397969e1343">28</a></sup>. Even in fields of 35 T, no saturation to the fast growth of the eMChA signal is observed, indicating that any putative crossover occurs at yet higher fields.</p><div class="c-article-section__figure js-c-reading-companion-figures-item" data-test="figure" data-container-section="figure" id="figure-3" data-title="Suppression of eMChA in KV3Sb5 and comparison to CsV3Sb5."><figure><figcaption><b id="Fig3" class="c-article-section__figure-caption" data-test="figure-caption-text">Fig. 3: Suppression of eMChA in KV<sub>3</sub>Sb<sub>5</sub> and comparison to CsV<sub>3</sub>Sb<sub>5</sub>.</b></figcaption><div class="c-article-section__figure-content"><div class="c-article-section__figure-item"><a class="c-article-section__figure-link" data-test="img-link" data-track="click" data-track-label="image" data-track-action="view figure" href="/articles/s41535-024-00629-3/figures/3" rel="nofollow"><picture><source type="image/webp" srcset="//media.springernature.com/lw685/springer-static/image/art%3A10.1038%2Fs41535-024-00629-3/MediaObjects/41535_2024_629_Fig3_HTML.png?as=webp"><img aria-describedby="Fig3" src="//media.springernature.com/lw685/springer-static/image/art%3A10.1038%2Fs41535-024-00629-3/MediaObjects/41535_2024_629_Fig3_HTML.png" alt="figure 3" loading="lazy" width="685" height="543"></picture></a></div><div class="c-article-section__figure-description" data-test="bottom-caption" id="figure-3-desc"><p><b>a</b> Field dependence of second harmonic voltage. A clear <i>B</i><sup>3</sup>-dependence is observed in CsV<sub>3</sub>Sb<sub>5</sub> as consistent with previous report<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 28" title="Guo, C. et al. Switchable chiral transport in charge-ordered kagome metal CsV3Sb5. Nature 611, 461 (2022)." href="/articles/s41535-024-00629-3#ref-CR28" id="ref-link-section-d105397969e1378">28</a></sup>. The magneto-chiral conductivity displays a clear field-linear dependence, as shown in (<b>b</b>), indicating robust magneto-chiral transport up to 35 T. On the other hand, the second harmonic voltage measured in KV<sub>3</sub>Sb<sub>5</sub> is about two orders of magnitude smaller compared to CsV<sub>3</sub>Sb<sub>5</sub>. Moreover, this tiny signal remains nearly unchanged with magnetic field rotated across the kagome plane (<b>c</b>), suggesting its non-switchable nature that is distinct from CsV<sub>3</sub>Sb<sub>5</sub>.</p></div></div><div class="u-text-right u-hide-print"><a class="c-article__pill-button" data-test="article-link" data-track="click" data-track-label="button" data-track-action="view figure" href="/articles/s41535-024-00629-3/figures/3" data-track-dest="link:Figure3 Full size image" aria-label="Full size image figure 3" rel="nofollow"><span>Full size image</span><svg width="16" height="16" focusable="false" role="img" aria-hidden="true" class="u-icon"><use xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="#icon-eds-i-chevron-right-small"></use></svg></a></div></figure></div><div class="c-article-section__figure js-c-reading-companion-figures-item" data-test="figure" data-container-section="figure" id="figure-4" data-title="In-plane spike of magnetoresistance."><figure><figcaption><b id="Fig4" class="c-article-section__figure-caption" data-test="figure-caption-text">Fig. 4: In-plane spike of magnetoresistance.</b></figcaption><div class="c-article-section__figure-content"><div class="c-article-section__figure-item"><a class="c-article-section__figure-link" data-test="img-link" data-track="click" data-track-label="image" data-track-action="view figure" href="/articles/s41535-024-00629-3/figures/4" rel="nofollow"><picture><source type="image/webp" srcset="//media.springernature.com/lw685/springer-static/image/art%3A10.1038%2Fs41535-024-00629-3/MediaObjects/41535_2024_629_Fig4_HTML.png?as=webp"><img aria-describedby="Fig4" src="//media.springernature.com/lw685/springer-static/image/art%3A10.1038%2Fs41535-024-00629-3/MediaObjects/41535_2024_629_Fig4_HTML.png" alt="figure 4" loading="lazy" width="685" height="486"></picture></a></div><div class="c-article-section__figure-description" data-test="bottom-caption" id="figure-4-desc"><p><b>a</b> The nearly in-plane magnetoresistance for KV<sub>3</sub>Sb<sub>5</sub> compared to CsV<sub>3</sub>Sb<sub>5</sub>. <b>b</b> Angular dependence of magnetoresistance further demonstrates the difference between the Cs- and K-compounds. A significant spike can be observed for CsV<sub>3</sub>Sb<sub>5</sub> when the magnetic field is applied within the kagome plane. On the other hand, the magnetoresistance is also maximized with the same field configuration for KV<sub>3</sub>Sb<sub>5</sub>, yet the magnitude of the spike is strongly reduced.</p></div></div><div class="u-text-right u-hide-print"><a class="c-article__pill-button" data-test="article-link" data-track="click" data-track-label="button" data-track-action="view figure" href="/articles/s41535-024-00629-3/figures/4" data-track-dest="link:Figure4 Full size image" aria-label="Full size image figure 4" rel="nofollow"><span>Full size image</span><svg width="16" height="16" focusable="false" role="img" aria-hidden="true" class="u-icon"><use xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="#icon-eds-i-chevron-right-small"></use></svg></a></div></figure></div><p>In absence of saturation, the sizable chiral contribution Δ<i>R</i>/<i>R</i> reaches 1.2% at 35 T. This value is substantial for a second-order correction term. It is clear, however, that this growth cannot continue much further. The eMChA signal is already appreciable, yet with a continued growth following a B<sup>3</sup> dependence, it may overtake the resistance itself, when Δ<i>R</i>/<i>R</i> = 1. A naive extrapolation places this transition at 150 T, and further high-field investigations of eMChA may be successful at detecting the incipient deviations.</p><p>On the contrary, KV<sub>3</sub>Sb<sub>5</sub> displays an almost negligible second-harmonic signal. At the same current density as CsV<sub>3</sub>Sb<sub>5</sub>, the second harmonic voltage stays below 30 nV up to 35 T, more than two orders of magnitude smaller. Furthermore, the sign of Δ<i>σ</i> cannot be switched by tilting the magnetic field through the kagome planes as in CsV<sub>3</sub>Sb<sub>5</sub> (Fig. <a data-track="click" data-track-label="link" data-track-action="figure anchor" href="/articles/s41535-024-00629-3#Fig3">3</a>). On both sides of the planes (<i>θ</i> = −1 and 2), the sign of the signal remains unchanged and stays negligible over a wide range of rotation angle (Supplementary Fig. <a data-track="click" data-track-label="link" data-track-action="supplementary material anchor" href="/articles/s41535-024-00629-3#MOESM1">3)</a>. As the second harmonic signal in KV<sub>3</sub>Sb<sub>5</sub> is so small, it is experimentally difficult to determine if at all any non-trivial eMChA exists in it. The main difficulty comes from asymmetric Joule heating due to accidentally imbalanced magnetoresistances at the contacts (Supplementary Fig. <a data-track="click" data-track-label="link" data-track-action="supplementary material anchor" href="/articles/s41535-024-00629-3#MOESM1">4</a>). The striking difference between these materials is clear already from the raw data.</p></div></div></section><section data-title="Discussion"><div class="c-article-section" id="Sec5-section"><h2 class="c-article-section__title js-section-title js-c-reading-companion-sections-item" id="Sec5">Discussion</h2><div class="c-article-section__content" id="Sec5-content"><p>It is difficult to reconcile the stark difference between their eMChA signals with the similarities of their single-particle spectrum, hence likely the key differences reside in interacting physics and differences in the electronic order. One structural difference is the higher density of vacancies in KV<sub>3</sub>Sb<sub>5</sub> compared to CsV<sub>3</sub>Sb<sub>5</sub>. This reflects in the higher residual resistivity, the lower magnetoresistance, comparatively weaker SdH oscillations and a reduced transport anisotropy at zero field. This scenario finds support in the angular dependence of the magnetoresistance. In CsV<sub>3</sub>Sb<sub>5</sub>, a pronounced spike is observed with field applied within the kagome plane (Fig. <a data-track="click" data-track-label="link" data-track-action="figure anchor" href="/articles/s41535-024-00629-3#Fig4">4</a>). This is a signature of coherent interlayer transport as despite the emergence of small 3D pockets due to charge-order formation<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 45" title="Huang, X. et al. Three-dimensional Fermi surfaces from charge order in layered CsV3Sb5. Phys. Rev. B 106, 064510 (2022)." href="/articles/s41535-024-00629-3#ref-CR45" id="ref-link-section-d105397969e1530">45</a></sup>, the Brillouin zone is still predominantly occupied by quasi-2D Fermi surfaces at low temperature. However this spike is strongly suppressed in KV<sub>3</sub>Sb<sub>5</sub>, consistent with enhanced decoherence scattering.</p><p>Depending on the origin of eMChA, such enhanced scattering in KV<sub>3</sub>Sb<sub>5</sub> influences the system in several possible ways. Firstly, since the temperature coefficients for transport remains metallic in all directions and the residual resistivity does not differ significantly (only by a factor of 2), it is hard to explain the huge difference in eMChA just by the smearing effect due to increased isotropic, achiral scattering sites. This suggests that the defining factor of eMChA in KV<sub>3</sub>Sb<sub>5</sub> may reside beyond just the band structure effect within the (chiral) ordered phase. Secondly, if eMChA originates in the scattering on chiral domains, the disorders/vacancies distort the kagome net formed by the V-atoms and can act as the pinning centers that imprint the electronic chiral domains to a fixed pattern. Since these point disorders are achiral, this fixed pattern is naturally balanced in chirality. Moreover, this fixed pattern is stable against the out-of-plane magnetic field and, therefore, does not have a minority/majority chirality. This means the chiral scattering process is always canceled out, which results in the strong suppression of eMChA. Last but not least, the possibility of an achiral bulk state cannot be ruled out. Despite the report of chiral or even switchable chiral state by STM measurements<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 19" title="Zhao, H. et al. Cascade of correlated electron states in a kagome superconductor CsV3Sb5. Nature 599, 216 (2021)." href="/articles/s41535-024-00629-3#ref-CR19" id="ref-link-section-d105397969e1549">19</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 20" title="Jiang, Y.-X. et al. Unconventional chiral charge order in kagome superconductor KV3Sb5. Nat. Mat. 20, 1353 (2021)." href="/articles/s41535-024-00629-3#ref-CR20" id="ref-link-section-d105397969e1552">20</a></sup>, the possibility still exists that such a state only appears at the surface. Previous studies demonstrate that CsV<sub>3</sub>Sb<sub>5</sub> is located at a tipping point between different correlated orders and the subtle differences in electronic structures we observed could drive KV<sub>3</sub>Sb<sub>5</sub> sufficiently deep in an achiral state, eliminating the origin of chiral transport observed in CsV<sub>3</sub>Sb<sub>5</sub>. Other origins of the possible achiral bulk state in KV<sub>3</sub>Sb<sub>5</sub>, such as the potential difference in phonon spectrum, should also be further examined.</p><p>All proposals suggest that the surprising suppression of eMChA in KV<sub>3</sub>Sb<sub>5</sub> relies on subtle electronic features. Therefore to differentiate these scenarios and identify the origin of the strong eMChA signal in CsV<sub>3</sub>Sb<sub>5</sub> it is of particular interest to revisit eMChA in AV<sub>3</sub>Sb<sub>5</sub> at slightly different aspects. The first thing to establish is the detailed relation between defect concentration and the strength of eMChA. This can be achieved via controlling the effective chemical substitution such as Sn-doping<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 46" title="Oey, Y. M. et al. Fermi level tuning and double-dome superconductivity in the kagome metal $${{{{\rm{CsV}}}}}_{3}{{{{\rm{Sb}}}}}_{5-x}{{{{\rm{Sn}}}}}_{x}$$ CsV 3 Sb 5 − x Sn x . Phys. Rev. Mater. 6, L041801 (2022)." href="/articles/s41535-024-00629-3#ref-CR46" id="ref-link-section-d105397969e1590">46</a></sup>, K-vacancies<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 29" title="Ortiz, B. R. et al. Superconductivity in the Z2 kagome metal KV3Sb5. Phys. Rev. Mater. 5, 034801 (2021)." href="/articles/s41535-024-00629-3#ref-CR29" id="ref-link-section-d105397969e1594">29</a></sup> or electron radiation<sup><a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 47" title="Sunko, V. et al. Controlled introduction of defects to delafossite metals by electron irradiation. Phys. Rev. X 10, 021018 (2020)." href="/articles/s41535-024-00629-3#ref-CR47" id="ref-link-section-d105397969e1598">47</a>,<a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 48" title="Putzke, C. et al. h/e oscillations in interlayer transport of delafossites. Science 368, 1234 (2020)." href="/articles/s41535-024-00629-3#ref-CR48" id="ref-link-section-d105397969e1601">48</a></sup>. If the K-vacancies can be reduced to a level, where the difference in scattering rate between KV<sub>3</sub>Sb<sub>5</sub> and CsV<sub>3</sub>Sb<sub>5</sub> becomes negligible, one can explore the possible intrinsic difference in (switchable) electronic chirality between them. Furthermore, for systematic doping studies, if the amplitude of eMChA is directly proportional to the defect concentration, the single-particle scenario is valid and the chiral transport is swamped by the increase of isotropic, achiral scattering sites. On the other hand, if the eMChA is dramatically suppressed only at a threshold of doping level, this would suggest that once a sufficient number of pinning centers is formed, the domain pattern is locked and, therefore, eMChA vanishes. Based on this scenario, it is also worth exploring whether a stronger magnetic field can overcome the pinning energy of the locked domain pattern near the critical doping level, which provides further evidence for the chiral domain scenario.</p><p>In summary, we have reported a distinct switching of chiral transport in the kagome metal KV<sub>3</sub>Sb<sub>5</sub> and CsV<sub>3</sub>Sb<sub>5</sub>. KV<sub>3</sub>Sb<sub>5</sub> displays a negligible electronic chiral transport signature compared to CsV<sub>3</sub>Sb<sub>5</sub>. Moreover, the direction of the chiral transport is no longer switchable by the magnetic field. The minor difference in electronic structure between these compounds apparently contrasts strongly with the massive difference in magneto-chiral transport. This is clearly beyond the simple description on the single-particle level, where the electronic correlation becomes significant. These results point towards exotic correlated states with extreme tunability/sensitivity in AV<sub>3</sub>Sb<sub>5</sub> compounds, calling for further attention.</p></div></div></section><section data-title="Methods"><div class="c-article-section" id="Sec6-section"><h2 class="c-article-section__title js-section-title js-c-reading-companion-sections-item" id="Sec6">Methods</h2><div class="c-article-section__content" id="Sec6-content"><h3 class="c-article__sub-heading" id="Sec7">Crystal synthesis</h3><p>CsV<sub>3</sub>Sb<sub>5</sub> crystallizes in the hexagonal structure with P6/mmm space group. Following the crystal growth procedure described in ref. <a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 10" title="Ortiz, B. R. et al. CsV3Sb5: A Z2 topological kagome metal with a superconducting ground state. Phys. Rev. Lett. 125, 247002 (2020)." href="/articles/s41535-024-00629-3#ref-CR10" id="ref-link-section-d105397969e1653">10</a>, we obtained plate-like single crystals with typical dimensions of 2 × 2 × 0.04 mm<sup>3</sup>. The crystals of KV<sub>3</sub>Sb<sub>5</sub> were grown by the self-flux method. K, V, and Sb with atomic ratio of 7: 3: 14 were loaded in an alumina crucible and then sealed in a tantalum tube. The sample was heated to 1000 °C, annealed for 20 h, and cooled down to 400 °C with a rate of 3 °C per hour. After that, the sample was naturally cooled down to room temperature by turning off the furnace. Hexagonal crystals of KV<sub>3</sub>Sb<sub>5</sub> were obtained by dissolving the flux with water.</p><h3 class="c-article__sub-heading" id="Sec8">Microstructure characterization</h3><p>The fabrication procedure of the membrane-based device is described in ref. <a data-track="click" data-track-action="reference anchor" data-track-label="link" data-test="citation-ref" aria-label="Reference 28" title="Guo, C. et al. Switchable chiral transport in charge-ordered kagome metal CsV3Sb5. Nature 611, 461 (2022)." href="/articles/s41535-024-00629-3#ref-CR28" id="ref-link-section-d105397969e1675">28</a>. The device is firstly calibrated in a commercial PPMS system with 9 T superconducting magnet for the temperature dependence of resistivity and the angular dependence of magnetoresistance.</p><h3 class="c-article__sub-heading" id="Sec9">High-field magnetotransport measurements</h3><p>High-field magnetotransport was performed inside a 35 T Bitter magnet at the High Field Magnet Laboratory. This was done using a probe with an in-situ rotatable stage equipped with the electrical connections for magnetotransport, which were read out via standard lock-in techniques (SR830 and SR860).</p></div></div></section> </div> <div class="u-mt-32"> <section data-title="Data availability"><div class="c-article-section" id="data-availability-section"><h2 class="c-article-section__title js-section-title js-c-reading-companion-sections-item" id="data-availability">Data availability</h2><div class="c-article-section__content" id="data-availability-content"> <p>Data that support the findings of this study is deposited to Zendo with the access link: <a href="https://doi.org/10.5281/zenodo.10138673">https://doi.org/10.5281/zenodo.10138673</a>.</p> </div></div></section><div id="MagazineFulltextArticleBodySuffix"><section aria-labelledby="Bib1" data-title="References"><div class="c-article-section" id="Bib1-section"><h2 class="c-article-section__title js-section-title js-c-reading-companion-sections-item" id="Bib1">References</h2><div class="c-article-section__content" id="Bib1-content"><div data-container-section="references"><ol class="c-article-references" data-track-component="outbound reference" data-track-context="references section"><li class="c-article-references__item js-c-reading-companion-references-item" data-counter="1."><p class="c-article-references__text" id="ref-CR1">Yin, J.-X., Lian, B. & Hasan, M. 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This project received funding by the Swiss National Science Foundation (Grants No. PP00P2_176789). This work was supported by HFML-RU/NWO-I, member of the European Magnetic Field Laboratory (EMFL). M.G.V., I.E. and M.G.A. acknowledge the Spanish Ministerio de Ciencia e Innovacion (grant PID2019-109905GB-C21). I.E. and M.G.-A. received funding from the Spanish Ministry of Science and Innovation (Grant No. PID2022-142861NA-I00). This work has been financially supported by the Ministry for Digital Transformation and of Civil Service of the Spanish Government through the QUANTUM ENIA project call - Quantum Spain project, and by the European Union through the Recovery, Transformation and Resilience Plan - NextGenerationEU within the framework of the Digital Spain 2026 Agenda. M.G.V., C.F., and T.N. acknowledge support from FOR 5249 (QUAST) lead by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation). M.G.V. acknowledges partial support to European Research Council grant agreement no. 101020833. This work has been supported in part by Basque Government grant IT979-16. This work was also supported by the European Research Council Advanced Grant (No. 742068) “TOPMAT”, the Deutsche Forschungsgemeinschaft (Project-ID No. 247310070) “SFB 1143”, and the DFG through the Würzburg-Dresden Cluster of Excellence on Complexity and Topology in Quantum Matter ct.qmat (EXC 2147, Project-ID No. 390858490). G.W. acknowledges funding from the University of Zurich postdoc grant FK-23-134.</p></div></div></section><section data-title="Funding"><div class="c-article-section" id="Fun-section"><h2 class="c-article-section__title js-section-title js-c-reading-companion-sections-item" id="Fun">Funding</h2><div class="c-article-section__content" id="Fun-content"><p>Open Access funding enabled and organized by Projekt DEAL.</p></div></div></section><section aria-labelledby="author-information" data-title="Author information"><div class="c-article-section" id="author-information-section"><h2 class="c-article-section__title js-section-title js-c-reading-companion-sections-item" id="author-information">Author information</h2><div class="c-article-section__content" id="author-information-content"><h3 class="c-article__sub-heading" id="affiliations">Authors and Affiliations</h3><ol class="c-article-author-affiliation__list"><li id="Aff1"><p class="c-article-author-affiliation__address">Max Planck Institute for the Structure and Dynamics of Matter, Hamburg, Germany</p><p class="c-article-author-affiliation__authors-list">Chunyu Guo, Carsten Putzke & Philip J. W. Moll</p></li><li id="Aff2"><p class="c-article-author-affiliation__address">High Field Magnet Laboratory (HFML—EMFL), Radboud University, Toernooiveld 7, 6525 ED, Nijmegen, the Netherlands</p><p class="c-article-author-affiliation__authors-list">Maarten R. van Delft & Steffen Wiedmann</p></li><li id="Aff3"><p class="c-article-author-affiliation__address">Institute for Molecules and Materials, Radboud University, Nijmegen, 6525 AJ, the Netherlands</p><p class="c-article-author-affiliation__authors-list">Maarten R. van Delft & Steffen Wiedmann</p></li><li id="Aff4"><p class="c-article-author-affiliation__address">Centro de Física de Materiales (CSIC-UPV/EHU), Donostia-San Sebastian, Spain</p><p class="c-article-author-affiliation__authors-list">Martin Gutierrez-Amigo & Ion Errea</p></li><li id="Aff5"><p class="c-article-author-affiliation__address">Department of Physics, University of the Basque Country (UPV/EHU), Bilbao, Spain</p><p class="c-article-author-affiliation__authors-list">Martin Gutierrez-Amigo</p></li><li id="Aff6"><p class="c-article-author-affiliation__address">Donostia International Physics Center, Donostia-San Sebastian, Spain</p><p class="c-article-author-affiliation__authors-list">Martin Gutierrez-Amigo, Ion Errea & Maia G. Vergniory</p></li><li id="Aff7"><p class="c-article-author-affiliation__address">Max Planck Institute for Chemical Physics of Solids, Dresden, Germany</p><p class="c-article-author-affiliation__authors-list">Dong Chen, Maia G. Vergniory & Claudia Felser</p></li><li id="Aff8"><p class="c-article-author-affiliation__address">College of Physics, Qingdao University, Qingdao, China</p><p class="c-article-author-affiliation__authors-list">Dong Chen</p></li><li id="Aff9"><p class="c-article-author-affiliation__address">Department of Physics, University of Zürich, Zürich, Switzerland</p><p class="c-article-author-affiliation__authors-list">Glenn Wagner, Mark H. Fischer & Titus Neupert</p></li><li id="Aff10"><p class="c-article-author-affiliation__address">Fisika Aplikatua Saila, Gipuzkoako Ingeniaritza Eskola, University of the Basque Country (UPV/EHU), Donostia-San Sebastian, Spain</p><p class="c-article-author-affiliation__authors-list">Ion Errea</p></li></ol><div class="u-js-hide u-hide-print" data-test="author-info"><span class="c-article__sub-heading">Authors</span><ol class="c-article-authors-search u-list-reset"><li id="auth-Chunyu-Guo-Aff1"><span class="c-article-authors-search__title u-h3 js-search-name">Chunyu Guo</span><div class="c-article-authors-search__list"><div class="c-article-authors-search__item c-article-authors-search__list-item--left"><a href="/search?author=Chunyu%20Guo" class="c-article-button" data-track="click" data-track-action="author link - publication" data-track-label="link" rel="nofollow">View author publications</a></div><div class="c-article-authors-search__item c-article-authors-search__list-item--right"><p class="search-in-title-js c-article-authors-search__text">You can also search for this author in <span class="c-article-identifiers"><a class="c-article-identifiers__item" href="http://www.ncbi.nlm.nih.gov/entrez/query.fcgi?cmd=search&term=Chunyu%20Guo" data-track="click" data-track-action="author link - 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W. Moll</span><div class="c-article-authors-search__list"><div class="c-article-authors-search__item c-article-authors-search__list-item--left"><a href="/search?author=Philip%20J.%20W.%20Moll" class="c-article-button" data-track="click" data-track-action="author link - publication" data-track-label="link" rel="nofollow">View author publications</a></div><div class="c-article-authors-search__item c-article-authors-search__list-item--right"><p class="search-in-title-js c-article-authors-search__text">You can also search for this author in <span class="c-article-identifiers"><a class="c-article-identifiers__item" href="http://www.ncbi.nlm.nih.gov/entrez/query.fcgi?cmd=search&term=Philip%20J.%20W.%20Moll" data-track="click" data-track-action="author link - pubmed" data-track-label="link" rel="nofollow">PubMed</a><span class="u-hide"> </span><a class="c-article-identifiers__item" href="http://scholar.google.co.uk/scholar?as_q=&num=10&btnG=Search+Scholar&as_epq=&as_oq=&as_eq=&as_occt=any&as_sauthors=%22Philip%20J.%20W.%20Moll%22&as_publication=&as_ylo=&as_yhi=&as_allsubj=all&hl=en" data-track="click" data-track-action="author link - scholar" data-track-label="link" rel="nofollow">Google Scholar</a></span></p></div></div></li></ol></div><h3 class="c-article__sub-heading" id="contributions">Contributions</h3><p>Crystals were synthesized and characterized by D.C. and C.F. The experiment design, FIB microstructuring and high-field magnetotransport measurements were performed by C.G., M.R.V.D., S.W., C.P., and P.J.W.M. Band structures were calculated by M.G.A., I.E. and M.G.V.; G.W., M.H.F., and T.N. developed the general theoretical framework for eMChA analysis, and the analysis of experimental results has been done by C.G., C.P., and P.J.W.M. All authors were involved in writing the paper.</p><h3 class="c-article__sub-heading" id="corresponding-author">Corresponding authors</h3><p id="corresponding-author-list">Correspondence to <a id="corresp-c1" href="mailto:chunyu.guo@mpsd.mpg.de">Chunyu Guo</a> or <a id="corresp-c2" href="mailto:philip.moll@mpsd.mpg.de">Philip J. W. 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id="citeas">Cite this article</h3><p class="c-bibliographic-information__citation">Guo, C., van Delft, M.R., Gutierrez-Amigo, M. <i>et al.</i> Distinct switching of chiral transport in the kagome metals KV<sub>3</sub>Sb<sub>5</sub> and CsV<sub>3</sub>Sb<sub>5</sub>. <i>npj Quantum Mater.</i> <b>9</b>, 20 (2024). https://doi.org/10.1038/s41535-024-00629-3</p><p class="c-bibliographic-information__download-citation u-hide-print"><a data-test="citation-link" data-track="click" data-track-action="download article citation" data-track-label="link" data-track-external="" rel="nofollow" href="https://citation-needed.springer.com/v2/references/10.1038/s41535-024-00629-3?format=refman&flavour=citation">Download citation<svg width="16" height="16" focusable="false" role="img" aria-hidden="true" class="u-icon"><use xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="#icon-eds-i-download-medium"></use></svg></a></p><ul class="c-bibliographic-information__list" data-test="publication-history"><li class="c-bibliographic-information__list-item"><p>Received<span class="u-hide">: </span><span class="c-bibliographic-information__value"><time datetime="2023-06-01">01 June 2023</time></span></p></li><li class="c-bibliographic-information__list-item"><p>Accepted<span class="u-hide">: </span><span class="c-bibliographic-information__value"><time datetime="2024-01-24">24 January 2024</time></span></p></li><li class="c-bibliographic-information__list-item"><p>Published<span class="u-hide">: </span><span class="c-bibliographic-information__value"><time datetime="2024-02-22">22 February 2024</time></span></p></li><li class="c-bibliographic-information__list-item c-bibliographic-information__list-item--full-width"><p><abbr title="Digital Object Identifier">DOI</abbr><span class="u-hide">: </span><span class="c-bibliographic-information__value">https://doi.org/10.1038/s41535-024-00629-3</span></p></li></ul><div data-component="share-box"><div 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class="print-link" data-track="click" data-track-action="view further reading article" data-track-label="link:Phonon collapse and anharmonic melting of the 3D charge-density wave in kagome metals" href="https://doi.org/10.1038/s43246-024-00676-0"> Phonon collapse and anharmonic melting of the 3D charge-density wave in kagome metals </a> </h3> <ul data-test="author-list" class="c-author-list c-author-list--compact c-author-list--truncated u-sans-serif u-mb-4 u-mt-auto"> <li>Martin Gutierrez-Amigo</li><li>Ðorđe Dangić</li><li>Ion Errea</li> </ul> <p class="c-article-further-reading__journal-title"><i>Communications Materials</i> (2024)</p> </li> </ul> </div> </div> </section> </div> </article> </main> <aside class="c-article-extras u-hide-print" aria-label="Article navigation" data-component-reading-companion data-container-type="reading-companion" data-track-component="reading companion"> <div class="js-context-bar-sticky-point-desktop" data-track-context="reading companion"> <div 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