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Influence of Selective Deposition of CeO2 and CuO on Surface MWCNTs Walls on the Activity, Selectivity and Stability in the PROX Reaction - Journal of Applied Catalysis & Chemical Engineering
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Activity, Selectivity and Stability in the PROX Reaction</h1> </header> <div class="entry-thumbnail"> <img width="260" height="146" src="https://jcatchem.com/wp-content/uploads/sites/12/2020/12/ACCE-004.jpg" class="attachment-content-single wp-post-image" alt="ACCE-004"/></div> <p class="entry-meta"> </p> <div class="entry-content clearfix"> <div class="italics"><i>Dayana Sánchez, Amanda Garcez, Fabio Souza Toniolo and Martin Schmal*</i></div> <div class="italics"></div> <div class="italics"></div> <div></div> <div> <br/> <strong>Abstract</strong></p> <p>In the present study, we synthesized catalysts based on CuO<sub>2</sub> and CeO<sub>2</sub> on pretreated MWCNT (Multi-Walled Carbon Nanotubes) support. The metallic oxides were selectively deposited (on internal and/or external surfaces of the MWCNT) by wet impregnation. The CeO<sub>2</sub>/CNT@CuO, CuO/CNT@CeO<sub>2</sub> and CuO-CeO<sub>2</sub>/CNT@CeO<sub>2</sub> catalysts (which means “external component”/CNT@“internal component”) were tested in the PROX reaction. We studied the selective introduction of the CuO and CeO<sub>2</sub> nanostructures in and outside the CNT (carbon nanotubes) walls and their influence on the activity, selectivity and stability in the PROX reaction. Characterizations showed that it was possible to drive selectively the deposition of the metallic oxides to one of the MWCNTs surface. Results showed that the activity does not depend whether metallic oxides are internally or externally located on the MWCNTs walls. There are no sintering or interaction of metal oxides. The catalysts reached high conversions 65-70% and are very stable for long time. The CNT contribute</p> <div></div> <p> <br/> <strong>Published on:</strong> January 06, 2021<br/> <strong>doi:</strong> <a href="https://doi.org/10.17756/acce.2020-004" onclick="__gaTracker('send', 'event', 'outbound-article', 'https://doi.org/10.17756/acce.2020-004', '10.17756/acce.2020-004');">10.17756/acce.2020-004</a><br/> <strong>Citation: </strong>Sánchez D, Garcez A, Toniolo FS, Schmal M. 2020. Influence of Selective Deposition of CeO2 and CuO on Surface MWCNTs Walls on the Activity, Selectivity and Stability in the PROX Reaction. <i>J Appl Cat Chem Eng </i>1(1): 17-28.</p> <div class="pdfdownloadlink"><img class="alignleft size-full wp-image-507" style="margin: 4px -5px 4px 5px;" src="http://jnanoworld.com/wp-content/uploads/2017/04/pdf-icon-24-e1509106685135-1.png" alt="" width="16" height="16"/><div class="sdm_download_link"><a href="https://jcatchem.com/?smd_process_download=1&download_id=284" class="sdm_download green" title="acce-004-dayana-sanchez.pdf" target="_self">PDF (Download Full text)</a></div></div> <div><div class="sdm_download_count"><span class="sdm_count_number"><strong>829</strong></span><br/><span class="sdm_count_string"> Downloads</span></div><span class="postviews_eachpost"><div class="post-views post-281 entry-meta"> <span class="post-views-label">Views </span> <span class="post-views-count">1,718</span> </div></span></div> </div> <script type="text/javascript">jQuery(document).ready(function($){$.post('https://jcatchem.com/wp-admin/admin-ajax.php',{action:'wpt_view_count',id:'281'});});</script><div class="addtoany_share_save_container addtoany_content_bottom"><div class="a2a_kit a2a_kit_size_32 addtoany_list" data-a2a-url="https://jcatchem.com/2021/01/06/influence-of-selective-deposition-of-ceo2-and-cuo-on-surface-mwcnts/" data-a2a-title="Influence of Selective Deposition of CeO2 and CuO on Surface MWCNTs Walls on the Activity, Selectivity and Stability in the PROX Reaction"><a href="https://www.addtoany.com/add_to/facebook?linkurl=https%3A%2F%2Fjcatchem.com%2F2021%2F01%2F06%2Finfluence-of-selective-deposition-of-ceo2-and-cuo-on-surface-mwcnts%2F&linkname=Influence%20of%20Selective%20Deposition%20of%20CeO2%20and%20CuO%20on%20Surface%20MWCNTs%20Walls%20on%20the%20Activity%2C%20Selectivity%20and%20Stability%20in%20the%20PROX%20Reaction" onclick="__gaTracker('send', 'event', 'outbound-article', 'https://www.addtoany.com/add_to/facebook?linkurl=https%3A%2F%2Fjcatchem.com%2F2021%2F01%2F06%2Finfluence-of-selective-deposition-of-ceo2-and-cuo-on-surface-mwcnts%2F&linkname=Influence%20of%20Selective%20Deposition%20of%20CeO2%20and%20CuO%20on%20Surface%20MWCNTs%20Walls%20on%20the%20Activity%2C%20Selectivity%20and%20Stability%20in%20the%20PROX%20Reaction', '');" class="a2a_button_facebook" title="Facebook" rel="nofollow noopener" target="_blank"></a><a href="https://www.addtoany.com/add_to/twitter?linkurl=https%3A%2F%2Fjcatchem.com%2F2021%2F01%2F06%2Finfluence-of-selective-deposition-of-ceo2-and-cuo-on-surface-mwcnts%2F&linkname=Influence%20of%20Selective%20Deposition%20of%20CeO2%20and%20CuO%20on%20Surface%20MWCNTs%20Walls%20on%20the%20Activity%2C%20Selectivity%20and%20Stability%20in%20the%20PROX%20Reaction" onclick="__gaTracker('send', 'event', 'outbound-article', 'https://www.addtoany.com/add_to/twitter?linkurl=https%3A%2F%2Fjcatchem.com%2F2021%2F01%2F06%2Finfluence-of-selective-deposition-of-ceo2-and-cuo-on-surface-mwcnts%2F&linkname=Influence%20of%20Selective%20Deposition%20of%20CeO2%20and%20CuO%20on%20Surface%20MWCNTs%20Walls%20on%20the%20Activity%2C%20Selectivity%20and%20Stability%20in%20the%20PROX%20Reaction', '');" class="a2a_button_twitter" title="Twitter" rel="nofollow noopener" target="_blank"></a><a href="https://www.addtoany.com/add_to/google_plus?linkurl=https%3A%2F%2Fjcatchem.com%2F2021%2F01%2F06%2Finfluence-of-selective-deposition-of-ceo2-and-cuo-on-surface-mwcnts%2F&linkname=Influence%20of%20Selective%20Deposition%20of%20CeO2%20and%20CuO%20on%20Surface%20MWCNTs%20Walls%20on%20the%20Activity%2C%20Selectivity%20and%20Stability%20in%20the%20PROX%20Reaction" onclick="__gaTracker('send', 'event', 'outbound-article', 'https://www.addtoany.com/add_to/google_plus?linkurl=https%3A%2F%2Fjcatchem.com%2F2021%2F01%2F06%2Finfluence-of-selective-deposition-of-ceo2-and-cuo-on-surface-mwcnts%2F&linkname=Influence%20of%20Selective%20Deposition%20of%20CeO2%20and%20CuO%20on%20Surface%20MWCNTs%20Walls%20on%20the%20Activity%2C%20Selectivity%20and%20Stability%20in%20the%20PROX%20Reaction', '');" class="a2a_button_google_plus" title="Google+" rel="nofollow noopener" target="_blank"></a><a href="https://www.addtoany.com/share" onclick="__gaTracker('send', 'event', 'outbound-article', 'https://www.addtoany.com/share', '');" class="a2a_dd addtoany_share_save"></a></div></div> </div> </article> </div> <aside class="mh-sidebar"> <div id="wp_editor_widget-8" class="sb-widget clearfix WP_Editor_Widget"><h4 class="widget-title"><span>Editorial Board Members</span></h4><div style="min-height: 180px;"><img class="size-full wp-image-204 alignleft" src="https://jcatchem.com/wp-content/uploads/sites/12/2020/12/Jacob-Moulijn.jpg" alt="" width="150" height="150"/><br/> <h4>Jacob A. 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